scholarly journals The representation of solar cycle signals in stratospheric ozone – Part 1: A comparison of recently updated satellite observations

2016 ◽  
Vol 16 (15) ◽  
pp. 10021-10043 ◽  
Author(s):  
Amanda C. Maycock ◽  
Katja Matthes ◽  
Susann Tegtmeier ◽  
Rémi Thiéblemont ◽  
Lon Hood

Abstract. Changes in incoming solar ultraviolet radiation over the 11-year solar cycle affect stratospheric ozone abundances. It is important to quantify the magnitude, structure, and seasonality of the associated solar-ozone response (SOR) to understand the impact of the 11-year solar cycle on climate. Part 1 of this two-part study uses multiple linear regression analysis to extract the SOR in a number of recently updated satellite ozone datasets covering different periods within the epoch 1970 to 2013. The annual mean SOR in the updated version 7.0 (v7.0) Stratospheric Aerosol and Gas Experiment (SAGE) II number density dataset (1984–2004) is very consistent with that found in the previous v6.2. In contrast, we find a substantial decrease in the magnitude of the SOR in the tropical upper stratosphere in the SAGE II v7.0 mixing ratio dataset (∼ 1 %) compared to the v6.2 (∼ 4 %). This difference is shown to be largely attributable to the change in the independent stratospheric temperature dataset used to convert SAGE II ozone number densities to mixing ratios. Since these temperature records contain substantial uncertainties, we suggest that datasets based on SAGE II number densities are currently most reliable for evaluating the SOR. We further analyse three extended ozone datasets that combine SAGE II v7.0 number densities with more recent GOMOS (Global Ozone Monitoring by Occultation of Stars) or OSIRIS (Optical Spectrograph and Infrared Imager System) measurements. The extended SAGE–OSIRIS dataset (1984–2013) shows a smaller and less statistically significant SOR across much of the tropical upper stratosphere compared to the SAGE II data alone. In contrast, the two SAGE–GOMOS datasets (1984–2011) show SORs that are in closer agreement with the original SAGE II data and therefore appear to provide a more reliable estimate of the SOR. We also analyse the SOR in the recent Solar Backscatter Ultraviolet Instrument (SBUV) Merged Ozone Dataset (SBUVMOD) version 8.6 (VN8.6) (1970–2012) and SBUV Merged Cohesive VN8.6 (1978–2012) datasets and compare them to the previous SBUVMOD VN8.0 (1970–2009). Over their full lengths, the three records generally agree in terms of the broad magnitude and structure of the annual mean SOR. The main difference is that SBUVMOD VN8.6 shows a smaller and less significant SOR in the tropical upper stratosphere and therefore more closely resembles the SAGE II v7.0 mixing ratio data than does the SBUV Merged Cohesive VN8.6, which has a more continuous SOR of ∼ 2 % in this region. The sparse spatial and temporal sampling of limb satellite instruments prohibits the extraction of sub-annual variations in the SOR from SAGE-based datasets. However, the SBUVMOD VN8.6 dataset suggests substantial month-to-month variations in the SOR, particularly in the winter extratropics, which may be important for the proposed high-latitude dynamical response to the solar cycle. Overall, the results highlight substantial uncertainties in the magnitude and structure of the observed SOR from different satellite records. The implications of these uncertainties for understanding and modelling the effects of solar variability on climate should be explored.

2016 ◽  
Author(s):  
A. Maycock ◽  
K. Matthes ◽  
S. Tegtmeier ◽  
R. Thiéblemont ◽  
L. Hood

Abstract. The impact of changes in incoming solar ultraviolet irradiance on stratospheric ozone forms an important part of the climate response to solar variability. To realistically simulate the climate response to solar variability using climate models, a minimum requirement is that they should include a solar cycle ozone component that has a realistic amplitude and structure, and which varies with season. For climate models that do not include interactive ozone chemistry, this component must be derived from observations and/or chemistry–climate model simulations and included in an externally prescribed ozone database that also includes the effects of all major external forcings. Part 1 of this two part study presents the solar-ozone responses in a number of updated satellite datasets for the period 1984–2004, including the Stratospheric Aerosol and Gas Experiment (SAGE) II version 6.2 and version 7.0 data, and the Solar Backscatter Ultraviolet Instrument (SBUV) version 8.0 and version 8.6 data. A number of combined datasets, which have extended SAGE II using more recent satellite measurements, are also analysed for the period 1984–2011. It is shown that SAGE II derived solar-ozone signals are sensitive to the independent temperature measurements used to convert ozone number density to mixing ratio units. A change in these temperature measurements in the recent SAGE II v7.0 data leads to substantial differences in the mixing ratio solar-ozone response compared to the previous v6.2, particularly in the tropical upper stratosphere. We also show that alternate satellite ozone datasets have issues (e.g., sparse spatial and temporal sampling, low vertical resolution, and shortness of measurement record), and that the methods of accounting for instrument offsets and drifts in merged satellite datasets can have a substantial impact on the solar cycle signal in ozone. For example, the magnitude of the solar-ozone response varies by around a factor of two across different versions of the SBUV VN8.6 record, which appears to be due to the methods used to combine the separate SBUV timeseries. These factors make it difficult to extract more than an annual-mean solar-ozone response from the available satellite observations. It is therefore unlikely that satellite ozone measurements alone can be applied to estimate the necessary solar cycle ozone component of the prescribed ozone database for future coupled model intercomparison projects (e.g., CMIP6).


2017 ◽  
Author(s):  
Amanda C. Maycock ◽  
Katja Matthes ◽  
Susann Tegtmeier ◽  
Hauke Schmidt ◽  
Rémi Thiéblemont ◽  
...  

Abstract. The impact of changes in incoming solar irradiance on stratospheric ozone abundances should be included in climate model simulations to fully capture the atmospheric response to solar variability. This study presents the first systematic comparison of the solar-ozone response (SOR) during the 11 year solar cycle amongst different chemistry-climate models (CCMs) and ozone databases specified in climate models that do not include chemistry. We analyse the SOR in eight CCMs from the WCRP/SPARC Chemistry-Climate Model Initiative (CCMI-1) and compare these with three ozone databases: the Bodeker Scientific database, the SPARC/AC&C database for CMIP5, and the SPARC/CCMI database for CMIP6. The results reveal substantial differences in the representation of the SOR between the CMIP5 and CMIP6 ozone databases. The peak amplitude of theSOR in the upper stratosphere (1–5 hPa) decreases from 5 % to 2 % between the CMIP5 and CMIP6 databases. This difference is because the CMIP5 database was constructed from a regression model fit to satellite observations, whereas the CMIP6 database is constructed from CCM simulations, which use a spectral solar irradiance (SSI) dataset with relatively weak UV forcing. The SOR in the CMIP6 ozone database is therefore implicitly more similar to the SOR in the CCMI-1 models than to the CMIP5 ozone database, which shows a greater resemblance in amplitude and structure to the SOR in the Bodeker database. The latitudinal structure of the annual mean SOR in the CMIP6 ozone database and CCMI-1 models is considerably smoother than in the CMIP5 database, which shows strong gradients in the SOR across the midlatitudes owing to the paucity of observations at high latitudes. The SORs in the CMIP6 ozone database and in the CCMI-1 models show a strong seasonal dependence, including large meridional gradients at mid to high latitudes during winter; such seasonal variations in the SOR are not included in the CMIP5 ozone database. Sensitivity experiments with a global atmospheric model without chemistry (ECHAM6.3) are performed to assess the impact of changes in the representation of the SOR and SSI forcing between CMIP5 and CMIP6. The experiments show that the smaller amplitude of the SOR in the CMIP6 ozone database compared to CMIP5 causes a decrease in the modelled tropical stratospheric temperature response over the solar cycle of up to 0.6 K, or around 50 % of the total amplitude. The changes in the SOR explain most of the difference in the amplitude of the tropical stratospheric temperature response in the case with combined changes in SOR and SSI between CMIP5 and CMIP6. The results emphasise the importance of adequately representing the SOR in climate models to capture the impact of solar variability on the atmosphere. Since a number of limitations in the representation of the SOR in the CMIP5 ozone database have been identified, CMIP6 models without chemistry are encouraged to use the CMIP6 ozone database to capture the climate impacts of solar variability.


2015 ◽  
Vol 15 (10) ◽  
pp. 14275-14314 ◽  
Author(s):  
S. Muthers ◽  
F. Arfeuille ◽  
C. C. Raible ◽  
E. Rozanov

Abstract. After strong volcanic eruptions stratospheric ozone changes are modulated by heterogeneous chemical reactions (HET) and dynamical perturbations related to the radiative heating in the lower stratosphere (RAD). Here, we assess the relative importance of both processes as well as the effect of the resulting ozone changes on the dynamics using ensemble simulations with the atmosphere–ocean–chemistry–climate model (AOCCM) SOCOL-MPIOM forced by eruptions with different strength. The simulations are performed under present day and preindustrial conditions to investigate changes in the response behaviour. The results show that the HET effect is only relevant under present day conditions and causes a pronounced global reduction of column ozone. These ozone changes further lead to a slight weakening of the Northern Hemisphere (NH) polar vortex during mid-winter. Independent from the climate state the RAD mechanism changes the column ozone pattern with negative anomalies in the tropics and positive anomalies in the mid-latitudes. The influence of the climate state on the RAD mechanism significantly differs in the polar latitudes, where an amplified ozone depletion during the winter months is simulated under present day conditions. This is in contrast to the preindustrial state showing a positive column ozone response also in the polar area. The dynamical response of the stratosphere is clearly dominated by the RAD mechanism showing an intensification of the NH polar vortex in winter. Still under present day conditions ozone changes due to the RAD mechanism slightly reduce the response of the polar vortex after the eruption.


2013 ◽  
Vol 13 (11) ◽  
pp. 29447-29481
Author(s):  
W. Wang ◽  
W. Tian ◽  
S. Dhomse ◽  
F. Xie ◽  
J. Shu

Abstract. We have investigated the impact of assumed nitrous oxide (N2O) increases on stratospheric chemistry and dynamics by a series of idealized simulations. In a future cooler stratosphere the net yield of NOy from a changed N2O is known to decrease, but NOy can still be significantly increased by the increase of N2O. Results with a coupled chemistry-climate model (CCM) show that increases in N2O of 50%/100% between 2001 and 2050 result in more ozone destruction, causing a reduction in ozone mixing ratios of maximally 6%/10% in the middle stratosphere at around 10 hPa. This enhanced destruction could cause an ozone decline in the second half of this century in the middle stratosphere. However, the total ozone column still shows an increase in future decades, though the increase of 50%/100% in N2O caused a 2%/6% decrease in TCO compared with the reference simulation. N2O increases have significant effects on ozone trends at 20–10 hPa in the tropics and at northern high latitude, but have no significant effect on ozone trends in the Antarctic stratosphere. The ozone depletion potential for N2O in a future climate depends both on stratospheric temperature changes and tropospheric N2O changes, which have reversed effects on ozone in the middle and upper stratosphere. A 50% CO2 increase in conjunction with a 50% N2O increase cause significant ozone depletion in the middle stratosphere and lead to an increase of ozone in the upper stratosphere. Based on the multiple linear regression analysis and a series of sensitivity simulations, we find that the chemical effect of N2O increases dominates the ozone changes in the stratosphere while the dynamical and radiative effects of N2O increases are insignificant on average. However, the dynamical effect of N2O increases may cause large local changes in ozone mixing ratios, particularly, in the Southern Hemisphere lower stratosphere.


2018 ◽  
Vol 18 (15) ◽  
pp. 11323-11343 ◽  
Author(s):  
Amanda C. Maycock ◽  
Katja Matthes ◽  
Susann Tegtmeier ◽  
Hauke Schmidt ◽  
Rémi Thiéblemont ◽  
...  

Abstract. The impact of changes in incoming solar irradiance on stratospheric ozone abundances should be included in climate simulations to aid in capturing the atmospheric response to solar cycle variability. This study presents the first systematic comparison of the representation of the 11-year solar cycle ozone response (SOR) in chemistry–climate models (CCMs) and in pre-calculated ozone databases specified in climate models that do not include chemistry, with a special focus on comparing the recommended protocols for the Coupled Model Intercomparison Project Phase 5 and Phase 6 (CMIP5 and CMIP6). We analyse the SOR in eight CCMs from the Chemistry–Climate Model Initiative (CCMI-1) and compare these with results from three ozone databases for climate models: the Bodeker Scientific ozone database, the SPARC/Atmospheric Chemistry and Climate (AC&C) ozone database for CMIP5 and the SPARC/CCMI ozone database for CMIP6. The peak amplitude of the annual mean SOR in the tropical upper stratosphere (1–5 hPa) decreases by more than a factor of 2, from around 5 to 2 %, between the CMIP5 and CMIP6 ozone databases. This substantial decrease can be traced to the CMIP5 ozone database being constructed from a regression model fit to satellite and ozonesonde measurements, while the CMIP6 database is constructed from CCM simulations. The SOR in the CMIP6 ozone database therefore implicitly resembles the SOR in the CCMI-1 models. The structure in latitude of the SOR in the CMIP6 ozone database and CCMI-1 models is considerably smoother than in the CMIP5 database, which shows unrealistic sharp gradients in the SOR across the middle latitudes owing to the paucity of long-term ozone measurements in polar regions. The SORs in the CMIP6 ozone database and the CCMI-1 models show a seasonal dependence with enhanced meridional gradients at mid- to high latitudes in the winter hemisphere. The CMIP5 ozone database does not account for seasonal variations in the SOR, which is unrealistic. Sensitivity experiments with a global atmospheric model without chemistry (ECHAM6.3) are performed to assess the atmospheric impacts of changes in the representation of the SOR and solar spectral irradiance (SSI) forcing between CMIP5 and CMIP6. The larger amplitude of the SOR in the CMIP5 ozone database compared to CMIP6 causes a likely overestimation of the modelled tropical stratospheric temperature response between 11-year solar cycle minimum and maximum by up to 0.55 K, or around 80 % of the total amplitude. This effect is substantially larger than the change in temperature response due to differences in SSI forcing between CMIP5 and CMIP6. The results emphasize the importance of adequately representing the SOR in global models to capture the impact of the 11-year solar cycle on the atmosphere. Since a number of limitations in the representation of the SOR in the CMIP5 ozone database have been identified, we recommend that CMIP6 models without chemistry use the CMIP6 ozone database and the CMIP6 SSI dataset to better capture the climate impacts of solar variability. The SOR coefficients from the CMIP6 ozone database are published with this paper.


2009 ◽  
Vol 22 (2) ◽  
pp. 429-445 ◽  
Author(s):  
Seok-Woo Son ◽  
Lorenzo M. Polvani ◽  
Darryn W. Waugh ◽  
Thomas Birner ◽  
Hideharu Akiyoshi ◽  
...  

Abstract The evolution of the tropopause in the past, present, and future climate is examined by analyzing a set of long-term integrations with stratosphere-resolving chemistry climate models (CCMs). These CCMs have high vertical resolution near the tropopause, a model top located in the mesosphere or above, and, most important, fully interactive stratospheric chemistry. Using such CCM integrations, it is found that the tropopause pressure (height) will continue to decrease (increase) in the future, but with a trend weaker than that in the recent past. The reduction in the future tropopause trend is shown to be directly associated with stratospheric ozone recovery. A significant ozone recovery occurs in the Southern Hemisphere lower stratosphere of the CCMs, and this leads to a relative warming there that reduces the tropopause trend in the twenty-first century. The future tropopause trends predicted by the CCMs are considerably smaller than those predicted by the Intergovernmental Panel on Climate Change Fourth Assessment Report (AR4) models, especially in the southern high latitudes. This difference persists even when the CCMs are compared with the subset of the AR4 model integrations for which stratospheric ozone recovery was prescribed. These results suggest that a realistic representation of the stratospheric processes might be important for a reliable estimate of tropopause trends. The implications of these finding for the Southern Hemisphere climate change are also discussed.


2016 ◽  
Vol 3 (2) ◽  
pp. 150320 ◽  
Author(s):  
Benjamin A. Laken ◽  
Frode Stordal

The Hess Brezowsky Großwetterlagen (HBGWL) European weather classification system, accumulated over a long period (more than 130 years), provides a rare opportunity to examine the impact of various factors on regional atmospheric flow. We have used these data to examine changes in the frequency (days/month) of given weather systems direction (WSD) during peak phases in the North Atlantic Oscillation (NAO), El Niño Southern Oscillation (ENSO), solar cycle (SC) and peaks in stratospheric aerosol optical depth (AOD) with superposed epoch analysis and Monte Carlo significance testing. We found highly significant responses to the NAO consistent with expectations: this signal confirmed the utility of the HBGWL data for this type of analysis and provided a benchmark of a clear response. WSD changes associated with ENSO, SC and AOD were generally within the ranges expected from random samples. When seasonal restrictions were added the results were similar, however, we found one clearly significant result: an increase in southerly flow of 2.6±0.8 days/month ( p =1.9×10 −4 ) during boreal summertime in association with El Niño. This result supports the existence of a robust teleconnection between the ENSO and European weather.


2020 ◽  
Vol 20 (11) ◽  
pp. 6821-6839 ◽  
Author(s):  
Fernando Chouza ◽  
Thierry Leblanc ◽  
John Barnes ◽  
Mark Brewer ◽  
Patrick Wang ◽  
...  

Abstract. As part of the Network for the Detection of Atmospheric Composition Change (NDACC), ground-based measurements obtained from the Jet Propulsion Laboratory (JPL) stratospheric ozone lidar and the NOAA stratospheric aerosol lidar at Mauna Loa, Hawaii, over the past 2 decades were used to investigate the impact of volcanic eruptions and pyrocumulonimbus (PyroCb) smoke plumes on the stratospheric aerosol load above Hawaii since 1999. Measurements at 355 and 532 nm conducted by these two lidars revealed a color ratio of 0.5 for background aerosols and small volcanic plumes and 0.8 for a PyroCb plume recorded on September 2017. Measurements of the Nabro plume by the JPL lidar in 2011–2012 showed a lidar ratio of (64±12.7) sr at 355 nm around the center of the plume. The new Global Space-based Stratospheric Aerosol Climatology (GloSSAC), Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) Level 3 and Stratospheric Aerosol and Gas Experiment III on the International Space Station (SAGE III-ISS) stratospheric aerosol datasets were compared to the ground-based lidar datasets. The intercomparison revealed a generally good agreement, with vertical profiles of extinction coefficient within 50 % discrepancy between 17 and 23 km above sea level (a.s.l.) and 25 % above 23 km a.s.l. The stratospheric aerosol depth derived from all of these datasets shows good agreement, with the largest discrepancy (20 %) being observed between the new CALIOP Level 3 and the other datasets. All datasets consistently reveal a relatively quiescent period between 1999 and 2006, followed by an active period of multiple eruptions (e.g., Nabro) until early 2012. Another quiescent period, with slightly higher aerosol background, lasted until mid-2017, when a combination of extensive wildfires and multiple volcanic eruptions caused a significant increase in stratospheric aerosol loading. This loading maximized at the very end of the time period considered (fall 2019) as a result of the Raikoke eruption, the plume of which ascended to 26 km altitude in less than 3 months.


2017 ◽  
Author(s):  
Thibaut Lurton ◽  
Fabrice Jégou ◽  
Gwenaël Berthet ◽  
Jean-Baptiste Renard ◽  
Lieven Clarisse ◽  
...  

Abstract. Volcanic eruptions impact climate through the injection of sulfur dioxide (SO2), which is oxidized to form sulfuric acid aerosol particles that can enhance the stratospheric aerosol optical depth (SAOD). Besides large-magnitude eruptions, moderate-magnitude eruptions such as Kasatochi in 2008 and Sarychev Peak in 2009 can have a significant impact on stratospheric aerosol and hence climate. However, uncertainties remain in quantifying the atmospheric and climatic impacts of the 2009 Sarychev Peak eruption due to limitations in previous model representations of volcanic aerosol microphysics and particle size, whilst biases have been identified in satellite estimates of post-eruption SAOD. In addition, the 2009 Sarychev Peak eruption co-injected hydrogen chloride (HCl) alongside SO2, whose potential stratospheric chemistry impacts have not been investigated to date. We present a study of the stratospheric SO2-particle-HCl processing and impacts following Sarychev Peak eruption, using the CESM1(WACCM)-CARMA sectional aerosol microphysics model (with no a priori assumption on particle size). The Sarychev Peak 2009 eruption injected 0.9 Tg of SO2 into the upper troposphere and lower stratosphere (UTLS), enhancing the aerosol load in the Northern hemisphere. The post-eruption evolution of the volcanic SO2 in space and time are well reproduced by the model when compared to IASI (Infrared Atmospheric Sounding Interferometer) satellite data. Co-injection of 27 Gg HCl causes a lengthening of the SO2 lifetime and a slight delay in the formation of aerosols, and acts to enhance the destruction of stratospheric ozone and mono-nitrogen oxides (NOx) compared to the simulation with volcanic SO2 only. We therefore highlight the need to account for volcanic halogen chemistry when simulating the impact of eruptions such as Sarychev on stratospheric chemistry. The model-simulated evolution of effective radius (reff), reflects new particle formation followed by particle growth that enhances reff to reach up to 0.2 µm on zonal average. Comparisons of the model-simulated particle number and size-distributions to balloon-borne in-situ stratospheric observations over Kiruna, Sweden, in August and September 2009, and over Laramie, U.S.A., in June and November 2009 show good agreement and quantitatively confirms the post-eruption particle enhancement. We show that the model-simulated SAOD is consistent with that derived from OSIRIS (Optical Spectrograph and InfraRed Imager System) when both the saturation bias of OSIRIS and the fact that extinction profiles may terminate well above the tropopause are taken into account. Previous modelling studies (involving assumptions on particle size) that reported agreement to (biased) post-eruption estimates of SAOD derived from OSIRIS likely underestimated the climate impact of the 2009 Sarychev Peak eruption.


2014 ◽  
Vol 27 (14) ◽  
pp. 5538-5559 ◽  
Author(s):  
Edwin P. Gerber ◽  
Seok-Woo Son

Abstract The impact of anthropogenic forcing on the summertime austral circulation is assessed across three climate model datasets: the Chemistry–Climate Model Validation activity 2 and phases 3 and 5 of the Coupled Model Intercomparison Project. Changes in stratospheric ozone and greenhouse gases impact the Southern Hemisphere in this season, and a simple framework based on temperature trends in the lower polar stratosphere and upper tropical troposphere is developed to separate their effects. It suggests that shifts in the jet stream and Hadley cell are driven by changes in the upper-troposphere–lower-stratosphere temperature gradient. The mean response is comparable in the three datasets; ozone has chiefly caused the poleward shift observed in recent decades, while ozone and greenhouse gases largely offset each other in the future. The multimodel mean perspective, however, masks considerable spread in individual models’ circulation projections. Spread resulting from differences in temperature trends is separated from differences in the circulation response to a given temperature change; both contribute equally to uncertainty in future circulation trends. Spread in temperature trends is most associated with differences in polar stratospheric temperatures, and could be narrowed by reducing uncertainty in future ozone changes. Differences in tropical temperatures are also important, and arise from both uncertainty in future emissions and differences in models’ climate sensitivity. Differences in climate sensitivity, however, only matter significantly in a high emissions future. Even if temperature trends were known, however, differences in the dynamical response to temperature changes must be addressed to substantially narrow spread in circulation projections.


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