scholarly journals Retrieval of ice-nucleating particle concentrations from lidar observations and comparison with UAV in situ measurements

2019 ◽  
Vol 19 (17) ◽  
pp. 11315-11342 ◽  
Author(s):  
Eleni Marinou ◽  
Matthias Tesche ◽  
Athanasios Nenes ◽  
Albert Ansmann ◽  
Jann Schrod ◽  
...  

Abstract. Aerosols that are efficient ice-nucleating particles (INPs) are crucial for the formation of cloud ice via heterogeneous nucleation in the atmosphere. The distribution of INPs on a large spatial scale and as a function of height determines their impact on clouds and climate. However, in situ measurements of INPs provide sparse coverage over space and time. A promising approach to address this gap is to retrieve INP concentration profiles by combining particle concentration profiles derived by lidar measurements with INP efficiency parameterizations for different freezing mechanisms (immersion freezing, deposition nucleation). Here, we assess the feasibility of this new method for both ground-based and spaceborne lidar measurements, using in situ observations collected with unmanned aerial vehicles (UAVs) and subsequently analyzed with the FRIDGE (FRankfurt Ice nucleation Deposition freezinG Experiment) INP counter from an experimental campaign at Cyprus in April 2016. Analyzing five case studies we calculated the cloud-relevant particle number concentrations using lidar measurements (n250,dry with an uncertainty of 20 % to 40 % and Sdry with an uncertainty of 30 % to 50 %), and we assessed the suitability of the different INP parameterizations with respect to the temperature range and the type of particles considered. Specifically, our analysis suggests that our calculations using the parameterization of Ullrich et al. (2017) (applicable for the temperature range −50 to −33 ∘C) agree within 1 order of magnitude with the in situ observations of nINP; thus, the parameterization of Ullrich et al. (2017) can efficiently address the deposition nucleation pathway in dust-dominated environments. Additionally, our calculations using the combination of the parameterizations of DeMott et al. (2015, 2010) (applicable for the temperature range −35 to −9 ∘C) agree within 2 orders of magnitude with the in situ observations of INP concentrations (nINP) and can thus efficiently address the immersion/condensation pathway of dust and nondust particles. The same conclusion is derived from the compilation of the parameterizations of DeMott et al. (2015) for dust and Ullrich et al. (2017) for soot. Furthermore, we applied this methodology to estimate the INP concentration profiles before and after a cloud formation, indicating the seeding role of the particles and their subsequent impact on cloud formation and characteristics. More synergistic datasets are expected to become available in the future from EARLINET (European Aerosol Research Lidar Network) and in the frame of the European ACTRIS-RI (Aerosols, Clouds, and Trace gases Research Infrastructure). Our analysis shows that the developed techniques, when applied on CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations) spaceborne lidar observations, are in agreement with the in situ measurements. This study gives us confidence for the production of global 3-D products of cloud-relevant particle number concentrations (n250,dry, Sdry and nINP) using the CALIPSO 13-year dataset. This could provide valuable insight into the global height-resolved distribution of INP concentrations related to mineral dust, as well as possibly other aerosol types.

2018 ◽  
Author(s):  
Eleni Marinou ◽  
Matthias Tesche ◽  
Athanasios Nenes ◽  
Albert Ansmann ◽  
Jann Schrod ◽  
...  

Abstract. Aerosols that are efficient ice nucleating particles (INPs) are crucial for the formation of cloud ice via heterogeneous nucleation in the atmosphere. The distribution of INPs on a large spatial scale and as a function of height determines their impact on clouds and climate. However, in-situ measurements of INPs provide sparse coverage over space and time. A promising approach to address this gap is to retrieve INP concentration profiles by combining particle concentration profiles derived by lidar measurements with INP efficiency parametrization for different freezing mechanisms (immersion freezing, deposition nucleation). Here, we assess the feasibility of this new method for both ground-based and space-borne lidar measurements, using airborne in-situ observations from an experimental campaign at Cyprus in April 2016. Analyzing five case studies we calculated the particle number concentrations using lidar measurements (with an uncertainty of 20 to 100 %) and we assessed the suitability of the different INP parameterizations with respect to the temperature range and the type of particles considered. Specifically, our analysis suggests that the parametrization of Ullrich et al. (2017) (applicable for the temperature range −50 °C to −33 °C) agree within 1 order of magnitude with the in-situ observations of nINP and can efficiently address the deposition nucleation pathway in dust-dominated environments. Additionally, the combination of the parameterizations of DeMott et al. (2015) and DeMott et al. (2010) (applicable 15 for the temperature range −35 °C to −9 °C) agree within 2 orders of magnitude with the in-situ observations of nINP and can efficiently address the immersion/condensation pathway of dust and continental/anthropogenic particles. The same conclusion is derived from the compilation of the parameterizations of DeMott et al. (2015) for dust and Ullrich et al. (2017) for soot. Furthermore, we applied this methodology to estimate the INP concentration profiles before and after a cloud formation, indicating the seeding role of the particles and their subsequent impact on cloud formation and characteristics. More synergistic data-sets are expected to become available in the future from EARLINET (European Aerosol Research Lidar NETwork) and in the frame of the European ACTRIS-RI (Aerosols, Clouds and Trace gases Research Infrastructure). Our analysis shown that the developed techniques, when applied on CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations) space-born lidar observations, are in very good agreement with the in-situ measurements. This study give us confidence for the production of global 3D products of n250,dry, Sdry and nINP using the CALIPSO 13-yrs dataset. This could provide valuable insight into global height-resolved distribution of INP concentrations related to mineral dust, and possibly other aerosol types.


2019 ◽  
Author(s):  
Moritz Haarig ◽  
Adrian Walser ◽  
Albert Ansmann ◽  
Maximilian Dollner ◽  
Dietrich Althausen ◽  
...  

Abstract. The present study aims to validate lidar retrievals of cloud-relevant aerosol properties by using polarization lidar and coincident airborne in situ measurements in the Saharan Air Layer over the Barbados region. Vertical profiles of the number concentration of cloud condensation nuclei (CCN), large particles (diameter d > 500 nm), surface area, and ice nucleating particles (INP) are estimated from the lidar measurements and compared with CCN concentrations and the INP-relevant aerosol properties in situ measured with aircraft in the framework of the Saharan Aerosol Long-range Transport and Aerosol–Cloudinteraction Experiment (SALTRACE) in summer 2013. The CCN number concentrations derived from lidar observations were up to a factor of two higher than the ones measured in situ on board the research aircraft Falcon. However, a reasonable agreement was obtained when taking the lidar uncertainty into account. The number concentration of particles with dry radius > 250 nm and the surface area concentration obtained from the lidar observations and used as input for the INP parameterizations agreed well (


2019 ◽  
Vol 99 ◽  
pp. 04002
Author(s):  
Moritz Haarig ◽  
Albert Ansmann ◽  
Adrian Walser ◽  
Holger Baars ◽  
Claudia Urbanneck ◽  
...  

Vertical profiles of number concentrations of dust particles relevant for ice nucleation in clouds are derived from lidar measurements. The results are compared to coincidental airborne in-situ measurements of particle number and surface area concentrations in the dust layer. The observations were performed in long- range transported Saharan dust at Barbados and Asian dust at Cyprus. The Asian dust data analysis is ongoing. A comparison of Asian and Saharan dust will be given at the conference. Concentrations of ice nucleating particles in the order of 10 to 1000 per cm-3 in the dust layer are derived for a temperature of -25°C at Barbados. The method can be used to continuously monitor the concentration of ice nucleating dust particles vertically resolved from lidar measurements.


2014 ◽  
Vol 7 (9) ◽  
pp. 3095-3112 ◽  
Author(s):  
P. Sawamura ◽  
D. Müller ◽  
R. M. Hoff ◽  
C. A. Hostetler ◽  
R. A. Ferrare ◽  
...  

Abstract. Retrievals of aerosol microphysical properties (effective radius, volume and surface-area concentrations) and aerosol optical properties (complex index of refraction and single-scattering albedo) were obtained from a hybrid multiwavelength lidar data set for the first time. In July 2011, in the Baltimore–Washington DC region, synergistic profiling of optical and microphysical properties of aerosols with both airborne (in situ and remote sensing) and ground-based remote sensing systems was performed during the first deployment of DISCOVER-AQ. The hybrid multiwavelength lidar data set combines ground-based elastic backscatter lidar measurements at 355 nm with airborne High-Spectral-Resolution Lidar (HSRL) measurements at 532 nm and elastic backscatter lidar measurements at 1064 nm that were obtained less than 5 km apart from each other. This was the first study in which optical and microphysical retrievals from lidar were obtained during the day and directly compared to AERONET and in situ measurements for 11 cases. Good agreement was observed between lidar and AERONET retrievals. Larger discrepancies were observed between lidar retrievals and in situ measurements obtained by the aircraft and aerosol hygroscopic effects are believed to be the main factor in such discrepancies.


2017 ◽  
Author(s):  
Sebastian Düsing ◽  
Birgit Wehner ◽  
Patric Seifert ◽  
Albert Ansmann ◽  
Holger Baars ◽  
...  

Abstract. This study presents vertical profiles up to a height of 2300 m a.s.l. of aerosol microphysical and optical properties and cloud condensation nuclei (CCN). Corresponding data have been measured during a field campaign as part of the High-Definition Clouds and Precipitation for Advancing Climate Prediction (HD(CP)2) Observational Prototype Experiments (HOPE), which took place at Melpitz, Germany from September 9 to 29, 2013. The helicopter-borne payload ACTOS (Airborne Cloud and Turbulence Observation System) was used to determine the aerosol particle number size distribution (PNSD), the number concentrations of aerosol particles (PNC) and cloud condensation nuclei (CCN) (CCN-NC), the ambient relative humidity (RH), and temperature (T). Simultaneous measurements on ground provided a holistic view on aerosol microphysical properties such as the PNSD, the chemical composition and the CCN-NC. Additional measurements of a 3 + 2 wavelength polarization lidar system (PollyXT) provided profiles of the aerosol particle light backscatter coefficient (σbsc) for three wavelengths (355, 532 and 1064 nm). From profiles of σbsc profiles of the aerosol particle light extinction coefficient (σext) were determined using the extinction-to-backscatter ratio. Furthermore, CCN-NC profiles were estimated on basis of the lidar-measurements. Ambient state optical properties of aerosol particles were derived on the basis of airborne in situ measurements of ACTOS (PNSD) and in situ measurements on ground (chemical aerosol characterization) using Mie-theory. On the basis of ground-based and airborne measurements, this work investigates the representativeness of ground-based aerosol microphysical properties for the boundary layer for two case-studies. The PNSD measurements on ground showed a good agreement with the measurements provided with ACTOS for lower altitudes. The ground-based measurements of PNC and CCN-NC are representative for the PBL when the PBL is well mixed. Locally isolated new particle formation events on ground or at the top of the PBL led to vertical variability in the here presented cases and ground-based measurements are not representative for the PBL. Furthermore, the lidar-based estimates of CCN-NC profiles were compared with the airborne in situ measurements of ACTOS. This comparison showed good agreements within the uncertainty range. Finally, this work provides a closure study between the optical aerosol particle properties in ambient state based on the airborne ACTOS measurements and derived with the lidar measurements. The investigation of the optical properties shows for 14 measurement-points that the airborne-based particle light backscatter coefficient is for 1064 nm 50 % smaller than the measurements of the lidar system, 27.6 % smaller for 532 nm and 29.9 % smaller for 355 nm. These results are quite promising, since in-situ measurement based Mie-calculations of the particle light backscattering are scarce and the modelling is quite challenging. In contradiction for the particle light extinction coefficient retrieved from the airborne in situ measurements were found a good agreement. The airborne-based particle light extinction coefficient was just 7.9 % larger for 532 nm and 3.5 % smaller for 355 nm, for an assumed lidar ratio (LR) of 55 sr. The particle light extinction coefficient for 1064 nm was derived with a LR of 30 sr. For this wavelength, the airborne-based particle light extinction coefficient is 5.2 % smaller than the lidar-measurements. Also, the correlation for the particle light extinction coefficient in combination with Mie-based LR's are in agreement for typical LR's of European background aerosol.


2018 ◽  
Vol 18 (2) ◽  
pp. 1263-1290 ◽  
Author(s):  
Sebastian Düsing ◽  
Birgit Wehner ◽  
Patric Seifert ◽  
Albert Ansmann ◽  
Holger Baars ◽  
...  

Abstract. This paper examines the representativeness of ground-based in situ measurements for the planetary boundary layer (PBL) and conducts a closure study between airborne in situ and ground-based lidar measurements up to an altitude of 2300 m. The related measurements were carried out in a field campaign within the framework of the High-Definition Clouds and Precipitation for Advancing Climate Prediction (HD(CP)2) Observational Prototype Experiment (HOPE) in September 2013 in a rural background area of central Europe.The helicopter-borne probe ACTOS (Airborne Cloud and Turbulence Observation System) provided measurements of the aerosol particle number size distribution (PNSD), the aerosol particle number concentration (PNC), the number concentration of cloud condensation nuclei (CCN-NC), and meteorological atmospheric parameters (e.g., temperature and relative humidity). These measurements were supported by the ground-based 3+2 wavelength polarization lidar system PollyXT, which provided profiles of the particle backscatter coefficient (σbsc) for three wavelengths (355, 532, and 1064 nm). Particle extinction coefficient (σext) profiles were obtained by using a fixed backscatter-to-extinction ratio (also lidar ratio, LR). A new approach was used to determine profiles of CCN-NC for continental aerosol. The results of this new approach were consistent with the airborne in situ measurements within the uncertainties.In terms of representativeness, the PNSD measurements on the ground showed a good agreement with the measurements provided with ACTOS for lower altitudes. The ground-based measurements of PNC and CCN-NC are representative of the PBL when the PBL is well mixed. Locally isolated new particle formation events on the ground or at the top of the PBL led to vertical variability in the cases presented here and ground-based measurements are not entirely representative of the PBL. Based on Mie theory (Mie, 1908), optical aerosol properties under ambient conditions for different altitudes were determined using the airborne in situ measurements and were compared with the lidar measurements. The investigation of the optical properties shows that on average the airborne-based particle light backscatter coefficient is 50.1 % smaller for 1064 nm, 27.4 % smaller for 532 nm, and 29.5 % smaller for 355 nm than the measurements of the lidar system. These results are quite promising, since in situ measurement-based Mie calculations of the particle light backscattering are scarce and the modeling is quite challenging. In contrast, for the particle light extinction coefficient we found a good agreement. The airborne-based particle light extinction coefficient was just 8.2 % larger for 532 nm and 3 % smaller for 355 nm, for an assumed LR of 55 sr. The particle light extinction coefficient for 1064 nm was derived with a LR of 30 sr. For this wavelength, the airborne-based particle light extinction coefficient is 5.2 % smaller than the lidar measurements. For the first time, the lidar ratio of 30 sr for 1064 nm was determined on the basis of in situ measurements and the LR of 55 sr for 355 and 532 nm wavelength was reproduced for European continental aerosol on the basis of this comparison. Lidar observations and the in situ based aerosol optical properties agree within the uncertainties. However, our observations indicate that a determination of the PNSD for a large size range is important for a reliable modeling of aerosol particle backscattering.


2007 ◽  
Vol 7 (3) ◽  
pp. 815-838 ◽  
Author(s):  
B. Sauvage ◽  
R. V. Martin ◽  
A. van Donkelaar ◽  
X. Liu ◽  
K. Chance ◽  
...  

Abstract. We use a global chemical transport model (GEOS-Chem) to evaluate the consistency of satellite measurements of lightning flashes and ozone precursors with in situ measurements of tropical tropospheric ozone. The measurements are tropospheric O3, NO2, and HCHO columns from the GOME satellite instrument, lightning flashes from the OTD and LIS satellite instruments, profiles of O3, CO, and relative humidity from the MOZAIC aircraft program, and profiles of O3 from the SHADOZ ozonesonde network. We interpret these multiple data sources with our model to better understand what controls tropical tropospheric ozone. Tropical tropospheric ozone is mainly affected by lightning NOx and convection in the upper troposphere and by surface emissions in the lower troposphere. Scaling the spatial distribution of lightning in the model to the observed flashes improves the simulation of O3 in the upper troposphere by 5–20 ppbv versus in situ observations and by 1–4 Dobson Units versus GOME retrievals of tropospheric O3 columns. A lightning source strength of 6±2 Tg N/yr best represents in situ observations from aircraft and ozonesonde. Tropospheric NO2 and HCHO columns from GOME are applied to provide top-down constraints on emission inventories of NOx (biomass burning and soils) and VOCs (biomass burning). The top-down biomass burning inventory is larger than the bottom-up inventory by a factor of 2 for HCHO and alkenes, and by a factor of 2.6 for NOx over northern equatorial Africa. These emissions increase lower tropospheric O3 by 5–20 ppbv, improving the simulation versus aircraft observations, and by 4 Dobson Units versus GOME observations of tropospheric O3 columns. Emission factors in the a posteriori inventory are more consistent with a recent compilation from in situ measurements. The ozone simulation using two different dynamical schemes (GEOS-3 and GEOS-4) is evaluated versus observations; GEOS-4 better represents O3 observations by 5–15 ppbv, reflecting enhanced convective detrainment in the upper troposphere. Heterogeneous uptake of HNO3 on aerosols reduces simulated O3 by 5–7 ppbv, reducing a model bias versus in situ observations over and downwind of deserts. Exclusion of HO2 uptake on aerosols increases O3 by 5 ppbv in biomass burning regions, reducing a model bias versus MOZAIC aircraft measurements.


2011 ◽  
Vol 11 (20) ◽  
pp. 10705-10726 ◽  
Author(s):  
P. Royer ◽  
P. Chazette ◽  
K. Sartelet ◽  
Q. J. Zhang ◽  
M. Beekmann ◽  
...  

Abstract. An innovative approach using mobile lidar measurements was implemented to test the performances of chemistry-transport models in simulating mass concentrations (PM10) predicted by chemistry-transport models. A ground-based mobile lidar (GBML) was deployed around Paris onboard a van during the MEGAPOLI (Megacities: Emissions, urban, regional and Global Atmospheric POLlution and climate effects, and Integrated tools for assessment and mitigation) summer experiment in July 2009. The measurements performed with this Rayleigh-Mie lidar are converted into PM10 profiles using optical-to-mass relationships previously established from in situ measurements performed around Paris for urban and peri-urban aerosols. The method is described here and applied to the 10 measurements days (MD). MD of 1, 15, 16 and 26 July 2009, corresponding to different levels of pollution and atmospheric conditions, are analyzed here in more details. Lidar-derived PM10 are compared with results of simulations from POLYPHEMUS and CHIMERE chemistry-transport models (CTM) and with ground-based observations from the AIRPARIF network. GBML-derived and AIRPARIF in situ measurements have been found to be in good agreement with a mean Root Mean Square Error RMSE (and a Mean Absolute Percentage Error MAPE) of 7.2 μg m−3 (26.0%) and 8.8 μg m−3 (25.2%) with relationships assuming peri-urban and urban-type particles, respectively. The comparisons between CTMs and lidar at ~200 m height have shown that CTMs tend to underestimate wet PM10 concentrations as revealed by the mean wet PM10 observed during the 10 MD of 22.4, 20.0 and 17.5 μg m−3 for lidar with peri-urban relationship, and POLYPHEMUS and CHIMERE models, respectively. This leads to a RMSE (and a MAPE) of 6.4 μg m−3 (29.6%) and 6.4 μg m−3 (27.6%) when considering POLYPHEMUS and CHIMERE CTMs, respectively. Wet integrated PM10 computed (between the ground and 1 km above the ground level) from lidar, POLYPHEMUS and CHIMERE results have been compared and have shown similar results with a RMSE (and MAPE) of 6.3 mg m−2 (30.1%) and 5.2 mg m−2 (22.3%) with POLYPHEMUS and CHIMERE when comparing with lidar-derived PM10 with periurban relationship. The values are of the same order of magnitude than other comparisons realized in previous studies. The discrepancies observed between models and measured PM10 can be explained by difficulties to accurately model the background conditions, the positions and strengths of the plume, the vertical turbulent diffusion (as well as the limited vertical model resolutions) and chemical processes as the formation of secondary aerosols. The major advantage of using vertically resolved lidar observations in addition to surface concentrations is to overcome the problem of limited spatial representativity of surface measurements. Even for the case of a well-mixed boundary layer, vertical mixing is not complete, especially in the surface layer and near source regions. Also a bad estimation of the mixing layer height would introduce errors in simulated surface concentrations, which can be detected using lidar measurements. In addition, horizontal spatial representativity is larger for altitude integrated measurements than for surface measurements, because horizontal inhomogeneities occurring near surface sources are dampened.


2009 ◽  
Vol 48 (6) ◽  
pp. 1199-1216 ◽  
Author(s):  
Otto Hyvärinen ◽  
Kalle Eerola ◽  
Niilo Siljamo ◽  
Jarkko Koskinen

Abstract Snow cover has a strong effect on the surface and lower atmosphere in NWP models. Because the progress of in situ observations has stalled, satellite-based snow analyses are becoming increasingly important. Currently, there exist several products that operationally map global or continental snow cover. In this study, satellite-based snow cover analyses from NOAA, NASA, and the European Organisation for the Exploitation of Meteorological Satellites (EUMETSAT), and NWP snow analyses from the High-Resolution Limited-Area Model (HIRLAM) and ECMWF, were compared using data from January to June 2006. Because no analyses were independent and since available in situ measurements were already used in the NWP analyses, no independent ground truth was available and only the consistency between analyses could be compared. Snow analyses from NOAA, NASA, and ECMWF were similar, but the analysis from NASA was greatly hampered by clouds. HIRLAM and EUMETSAT deviated most from other analyses. Even though the analysis schemes of HIRLAM and ECMWF were quite similar, the resulting snow analyses were quite dissimilar, because ECMWF used the satellite information of snow cover in the form of NOAA analyses, while HIRLAM used none. The differences are especially prominent in areas around the snow edge where few in situ observations are available. This suggests that NWP snow analyses based only on in situ measurements would greatly benefit from inclusion of satellite-based snow cover information.


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