scholarly journals Compositional changes of present-day transatlantic Saharan dust deposition

2016 ◽  
Author(s):  
Laura F. Korte ◽  
Geert-Jan Brummer ◽  
Michèlle van der Does ◽  
Catarina V. Guerreiro ◽  
Rick Hennekam ◽  
...  

Abstract. Massive amounts of Saharan dust are blown from the African coast across the Atlantic Ocean towards the Americas each year. This dust has, depending on its chemistry, direct and indirect effects on global climate including reflection and absorption of solar radiation as well as transport and deposition of nutrients and metals fertilizing both ocean and land. To determine the temporal and spatial variability of Saharan dust transport and deposition and their marine environmental effects across the equatorial North Atlantic Ocean, we have set up a monitoring experiment using deep-ocean sediment traps as well as land-based dust collectors. The sediment traps were deployed at five ocean sites along a transatlantic transect between northwest Africa and the Caribbean along 12⁰ N, in a down-wind extension of the land-based dust collectors placed at 19⁰ N on the Mauritanian coast in Iwik. In this paper, we lay out the setup of the monitoring experiment and present the particle fluxes from sediment trap sampling over 24 continuous and synchronised intervals from October 2012 through to November 2013. We establish the temporal distribution of the particle fluxes deposited in the Atlantic and compare chemical compositions with the land-based dust collectors propagating to the down-wind sediment trap sites, and with satellite observations of Saharan dust outbreaks. First-year results show that the total mass fluxes in the ocean are highest at the sampling sites in the east and west, closest to the African continent and the Caribbean, respectively. Element ratios reveal that the lithogenic particles deposited nearest to Africa are most similar in composition to the Saharan dust collected in Iwik. Down-wind increasing Al, Fe and K contents suggest a downwind change in the mineralogical composition of Saharan dust and indicate an increasing contribution of clay minerals towards the west. In the westernmost Atlantic, admixture of re-suspended clay-sized sediments advected towards the deep sediment trap cannot be excluded. Seasonality is most prominent near both continents but generally weak, with mass fluxes dominated by calcium carbonate and clear seasonal maxima of biogenic silica towards the west. The monitoring experiment is now extended with autonomous dust sampling buoys for better quantification Saharan dust transport and deposition from source to sink and its impact on fertilization and carbon export to the deep ocean.

2017 ◽  
Vol 17 (9) ◽  
pp. 6023-6040 ◽  
Author(s):  
Laura F. Korte ◽  
Geert-Jan A. Brummer ◽  
Michèlle van der Does ◽  
Catarina V. Guerreiro ◽  
Rick Hennekam ◽  
...  

Abstract. Massive amounts of Saharan dust are blown from the coast of northern Africa across the Atlantic Ocean towards the Americas each year. This dust has, depending on its chemistry, direct and indirect effects on global climate which include reflection and absorption of solar radiation as well as transport and deposition of nutrients and metals fertilizing both ocean and land. To determine the temporal and spatial variability of Saharan dust transport and deposition and their marine environmental effects across the equatorial North Atlantic Ocean, we have set up a monitoring experiment using deep-ocean sediment traps as well as land-based dust collectors. The sediment traps were deployed at five ocean sites along a transatlantic transect between north-west Africa and the Caribbean along 12° N, in a downwind extension of the land-based dust collectors placed at 19° N on the Mauritanian coast in Iouîk. In this paper, we lay out the setup of the monitoring experiment and present the particle fluxes from sediment trap sampling over 24 continuous and synchronized intervals from October 2012 through to November 2013. We establish the temporal distribution of the particle fluxes deposited in the Atlantic and compare chemical compositions with the land-based dust collectors propagating to the downwind sediment trap sites, and with satellite observations of Saharan dust outbreaks. First-year results show that the total mass fluxes in the ocean are highest at the sampling sites in the east and west, closest to the African continent and the Caribbean, respectively. Element ratios reveal that the lithogenic particles deposited nearest to Africa are most similar in composition to the Saharan dust collected in Iouîk. Downwind increasing Al, Fe and K contents suggest a downwind change in the mineralogical composition of Saharan dust and indicate an increasing contribution of clay minerals towards the west. In the westernmost Atlantic Ocean, admixture of re-suspended clay-sized sediments advected towards the deep sediment trap cannot be excluded. Seasonality is most prominent near both continents but generally weak, with mass fluxes dominated by calcium carbonate and clear seasonal maxima of biogenic silica towards the west. The monitoring experiment is now extended, with autonomous dust sampling buoys for better quantification of Saharan dust transport and deposition from source to sink and their impact on fertilization and carbon export to the deep ocean.


2016 ◽  
Author(s):  
Michèlle van der Does ◽  
Laura F. Korte ◽  
Chris I. Munday ◽  
Geert-Jan A. Brummer ◽  
Jan-Berend W. Stuut

Abstract. Mineral dust has a large impact on regional and global climate, depending on its particle size. Especially in the Atlantic Ocean downwind of the Sahara, the largest dust source on earth, the effects can be substantial but are poorly understood. This study focuses on seasonal and spatial variations in particle size of Saharan dust deposition across the Atlantic Ocean, using an array of submarine sediment traps moored along a transect at 12˚ N. We show that the particle size decreases downwind with increased distance from the Saharan source, due to higher gravitational settling velocities of coarse particles in the atmosphere. Modal grain sizes vary between 4 and 33 μm throughout the different seasons and at five locations along the transect. This is much coarser than previously suggested and incorporated into climate models. In addition, seasonal changes are prominent, with coarser dust in summer, and finer dust in winter and spring. Such seasonal changes are caused by transport at higher altitudes and at greater wind velocities during summer than in winter. Also the latitudinal migration of the dust cloud, associated with the Intertropical Convergence Zone, causes seasonal differences in deposition as the summer dust cloud is located more to the north, and more directly above the sampled transect. Furthermore, increased precipitation and more frequent dust storms in summer coincide with coarser dust deposition. Our findings contribute to understanding Saharan dust transport and deposition relevant for the interpretation of sedimentary records for climate reconstructions, as well as for global and regional models for improved prediction of future climate.


2016 ◽  
Vol 16 (21) ◽  
pp. 13697-13710 ◽  
Author(s):  
Michèlle van der Does ◽  
Laura F. Korte ◽  
Chris I. Munday ◽  
Geert-Jan A. Brummer ◽  
Jan-Berend W. Stuut

Abstract. Mineral dust has a large impact on regional and global climate, depending on its particle size. Especially in the Atlantic Ocean downwind of the Sahara, the largest dust source on earth, the effects can be substantial but are poorly understood. This study focuses on seasonal and spatial variations in particle size of Saharan dust deposition across the Atlantic Ocean, using an array of submarine sediment traps moored along a transect at 12° N. We show that the particle size decreases downwind with increased distance from the Saharan source, due to higher gravitational settling velocities of coarse particles in the atmosphere. Modal grain sizes vary between 4 and 32 µm throughout the different seasons and at five locations along the transect. This is much coarser than previously suggested and incorporated into climate models. In addition, seasonal changes are prominent, with coarser dust in summer and finer dust in winter and spring. Such seasonal changes are caused by transport at higher altitudes and at greater wind velocities during summer than in winter. Also, the latitudinal migration of the dust cloud, associated with the Intertropical Convergence Zone, causes seasonal differences in deposition as the summer dust cloud is located more to the north and more directly above the sampled transect. Furthermore, increased precipitation and more frequent dust storms in summer coincide with coarser dust deposition. Our findings contribute to understanding Saharan dust transport and deposition relevant for the interpretation of sedimentary records for climate reconstructions, as well as for global and regional models for improved prediction of future climate.


2021 ◽  
Author(s):  
Guangyao Dai ◽  
Kangwen Sun ◽  
Xiaoye Wang ◽  
Songhua Wu ◽  
Xiangying E ◽  
...  

Abstract. In this paper, a long-term large-scale Sahara dust transport event occurred during 14 June and 27 June 2020 is tracked with the spaceborne lidars ALADIN and CALIOP observations and the models ECMWF and HYSPLIT analysis. We evaluate the performance of the ALADIN and CALIOP on the observations of dust optical properties and wind fields and explore the capability in tracking the dust events and in calculating the dust horizontal mass fluxes with the combination of measurement data from ALADIN and CALIOP coupled with the products from ECMWF and HYSPLIT. Compared with the traditional assessments based on the data from CALIOP and models, the complement of Aeolus-produced aerosol optical properties and wind data will significantly improve the accuracy of dust horizontal flux estimations. The dust plumes are identified with AIRS/Aqua Dust Score Index and with the Vertical Feature Mask products from CALIPSO. The emission, dispersion, transport and deposition of the dust event are monitored using the data from HYSPLIT, CALIPSO and AIRS/Aqua. With the quasi-synchronization observations by ALADIN and CALIOP, combining the wind vectors and relative humidity, the dust horizontal fluxes are calculated. From this study, it is found that the dust event generated on 14 and 15 June 2020 from Sahara Desert in North Africa, and then dispersed and transported westward over the Atlantic Ocean, and finally deposited in the Atlantic Ocean, the Americas and the Caribbean Sea. During the transport and deposition processes, the dust plumes are trapped in the Northeasterly Trade-wind zone between the latitudes of 5° N and 30° N and altitudes of 0 km and 6 km (in this paper we name this space area as “Saharan dust eastward transport tunnel”). From the measurement results on 19 June 2020, influenced by the hygroscopic effect and mixing with other types aerosols, the backscatter coefficients of dust plumes are increasing along the transport routes, with 3.88 × 10−6 ± 2.59 × 10−6 m−1 sr−1 in “dust portion during emission phase”, 7.09 × 10−6 ± 3.34 × 10−6 m−1 sr−1 in “dust portion during development phase” and 7.76 × 10−6 ± 3.74 × 10−6 m−1 sr−1 in “dust portion during deposition phase”. Finally, the horizontal fluxes at different dust parts and heights on 19 June and on entire transport routine during transportation are computed. On 19 June, the dust horizontal fluxes are about 2.17 ± 1.83 mg m−2 s−1 in dust portion during emission phase, 2.72 ± 1.89 mg m−2 s−1 in dust portion during development phase and 3.01 ± 2.77 mg m−2 s−1 in dust portion during deposition phase. In the whole life-time of the dust event, the dust horizontal fluxes are about 1.30 ± 1.07 mg m−2 s−1 on 15 June 2020, 2.62 ± 1.88 mg m−2 s−1 on 16 June 2020, 2.72 ± 1.89 mg m−2 s−1 on 19 June 2020, 1.98 ± 1.41 mg m−2 s−1 on 24 June 2020 and 2.11 ± 1.74 mg m−2 s−1 on 27 June 2020. From this study, it is found that the minimum of the fluxes appears when the dust event is initially generated on 15 June. During the dust development stage, the horizontal fluxes gradually increase and reach to the maximum value on 19 June with the enhancement of the dust event. Then, the horizontal fluxes gradually decrease since most of the dust deposited in the Atlantic Ocean, the Americas and the Caribbean Sea. Combining the Chlorophyll concentrations data provided by MODIS-Aqua, the Saharan Dust is found transported across the oligotrophic regions Atlantic Ocean towards the Americas and Caribbean Sea, which are also oligotrophic regions. The mineral dust delivers micronutrients including soluble Fe and P to the deposition zones and has the potential to fertilizing the ocean and increase the primary productivity in the Atlantic Ocean and Caribbean Sea.


2009 ◽  
Vol 6 (1) ◽  
pp. 85-102 ◽  
Author(s):  
G. Fischer ◽  
G. Karakaş

Abstract. The flux of materials to the deep sea is dominated by larger, organic-rich particles with sinking rates varying between a few meters and several hundred meters per day. Mineral ballast may regulate the transfer of organic matter and other components by determining the sinking rates, e.g. via particle density. We calculated particle sinking rates from mass flux patterns and alkenone measurements applying the results of sediment trap experiments from the Atlantic Ocean. We have indication for higher particle sinking rates in carbonate-dominated production systems when considering both regional and seasonal data. During a summer coccolithophorid bloom in the Cape Blanc coastal upwelling off Mauritania, particle sinking rates reached almost 570 m per day, most probably due the fast sedimentation of densely packed zooplankton fecal pellets, which transport high amounts of organic carbon associated with coccoliths to the deep ocean despite rather low production. During the recurring winter-spring blooms off NW Africa and in opal-rich production systems of the Southern Ocean, sinking rates of larger particles, most probably diatom aggregates, showed a tendency to lower values. However, there is no straightforward relationship between carbonate content and particle sinking rates. This could be due to the unknown composition of carbonate and/or the influence of particle size and shape on sinking rates. It also remains noticeable that the highest sinking rates occurred in dust-rich ocean regions off NW Africa, but this issue deserves further detailed field and laboratory investigations. We obtained increasing sinking rates with depth. By using a seven-compartment biogeochemical model, it was shown that the deep ocean organic carbon flux at a mesotrophic sediment trap site off Cape Blanc can be captured fairly well using seasonal variable particle sinking rates. Our model provides a total organic carbon flux of 0.29 Tg per year down to 3000 m off the NW African upwelling region between 5 and 35° N. Simple parameterisations of remineralisation and sinking rates in such models, however, limit their capability in reproducing the flux variation in the water column.


2011 ◽  
Vol 11 (16) ◽  
pp. 8415-8431 ◽  
Author(s):  
E. Nowottnick ◽  
P. Colarco ◽  
A. da Silva ◽  
D. Hlavka ◽  
M. McGill

Abstract. Saharan dust was observed over the Caribbean basin during the summer 2007 NASA Tropical Composition, Cloud, and Climate Coupling (TC4) field experiment. Airborne Cloud Physics Lidar (CPL) and satellite observations from MODIS suggest a barrier to dust transport across Central America into the eastern Pacific. We use the NASA GEOS-5 atmospheric transport model with online aerosol tracers to perform simulations of the TC4 time period in order to understand the nature of this barrier. Our simulations are driven by the Modern Era Retrospective-Analysis for Research and Applications (MERRA) meteorological analyses. Compared to observations from MODIS and CALIOP, GEOS-5 reproduces the observed location and magnitude of observed dust events, but our baseline simulation does not develop as strong a barrier to dust transport across Central America as observations suggest. Analysis of the dust transport dynamics and loss processes suggest that while both mechanisms play a role in defining the dust transport barrier, loss processes by wet removal of dust are about twice as important as transport. Sensitivity analyses with our model showed that the dust barrier would not exist without convective scavenging over the Caribbean. The best agreement between our model and the observations was obtained when dust wet removal was parameterized to be more aggressive, treating the dust as we do hydrophilic aerosols.


2021 ◽  
Author(s):  
Jan-Berend Stuut ◽  
Catarina Guerreiro ◽  
Geert-Jan Brummer ◽  
Michèlle van der Does

<p>Mineral dust plays an important role in the ocean’s carbon cycle through the input of nutrients and metals which potentially fertilise phytoplankton, and by ballasting organic matter from the surface ocean to the sea floor. However, time series and records of open-ocean dust deposition fluxes are sparse. Here, we present a multi-year time series of Saharan dust collected by dust-collecting buoys that are monitoring dust in the equatorial North Atlantic Ocean as well as by moored sediment traps at the buoys' positions at ~21°N/21°W and ~11°N/23°W. We present dust-flux data as well as particle-size distribution data, and make a comparison of the dust collected from the atmosphere at the ocean surface with the dust settling through the ocean and intercepted by the submarine sediment traps. See: www.nioz.nl/dust</p>


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