Interactive comment on “Transport, mixing, and feedback of dust, biomass burning and anthropogenic pollutants in eastern Asia: A case study” by Derong Zhou et al.

2018 ◽  
Author(s):  
Anonymous
Keyword(s):  
Biomass Burning ◽  
Eastern Asia ◽  
Anthropogenic Pollutants

scholarly journals Transport, mixing and feedback of dust, biomass burning and anthropogenic pollutants in eastern Asia: a case study

2018 ◽  
Vol 18 (22) ◽  
pp. 16345-16361 ◽  
Author(s):  
Derong Zhou ◽  
Ke Ding ◽  
Xin Huang ◽  
Lixia Liu ◽  
Qiang Liu ◽  
...  
Keyword(s):  
Air Pollution ◽  
Biomass Burning ◽  
Southern China ◽  
Eastern China ◽  
Measurement Data ◽  
Lower Troposphere ◽  
Climate Impacts ◽  
Eastern Asia ◽  
Pollution Episode ◽  
The Yrd

Abstract. Anthropogenic fossil fuel (FF) combustion, biomass burning (BB) and desert dust are the main sources of air pollutants around the globe but are particularly intensive and important for air quality in Asia in spring. In this study, we investigate the vertical distribution, transport characteristics, source contribution and meteorological feedback of these aerosols in a unique pollution episode that occurred in eastern Asia based on various measurement data and modeling methods. In this episode, the Yangtze River Delta (YRD) in eastern China experienced persistent air pollution, dramatically changing from secondary fine particulate pollution to dust pollution in late March 2015. The Eulerian and Lagrangian models were conducted to investigate the vertical structure, transport characteristics and mechanisms of the multi-scale, multisource and multiday air pollution episode. The regional polluted continental aerosols mainly accumulated near the surface, mixed with dust aerosol downwash from the upper planetary boundary layer (PBL) and middle–lower troposphere (MLT), and further transported by large-scale cold fronts and warm conveyor belts. BB smoke from Southeast Asia was transported by westerlies around the altitude of 3 km from southern China, was further mixed with dust and FF aerosols in eastern China and experienced long-range transport over the Pacific. These pollutants could all be transported to the YRD region and cause a structure of multilayer pollution there. These pollutants could also cause significant feedback with MLT meteorology and then enhance local anthropogenic pollution. This study highlights the importance of intensive vertical measurement in eastern China and the downwind Pacific Ocean and raises the need for quantitative understanding of environmental and climate impacts of these pollution sources.

The contributions of biomass burning to primary and secondary organics: A case study in Pearl River Delta (PRD), China

2016 ◽  
Vol 569-570 ◽  
pp. 548-556 ◽  
Author(s):  
BaoLin Wang ◽  
Ying Liu ◽  
Min Shao ◽  
SiHua Lu ◽  
Ming Wang ◽  
...  
Keyword(s):  
Biomass Burning ◽  
Pearl River Delta ◽  
River Delta ◽  
Pearl River

scholarly journals A model tool for assessing real-time mixing of mineral and anthropogenic pollutants in East Asia: a case study of April 2005

2008 ◽  
Vol 8 (13) ◽  
pp. 3603-3622 ◽  
Author(s):  
F. Lasserre ◽  
G. Cautenet ◽  
C. Bouet ◽  
X. Dong ◽  
Y. J. Kim ◽  
...  
Keyword(s):  
East Asia ◽  
Real Time ◽  
Anthropogenic Pollution ◽  
Atmospheric Modeling ◽  
Time Step ◽  
Anthropogenic Pollutants ◽  
Vertical Distributions ◽  
Dust Events ◽  
Horizontal And Vertical Distributions

Abstract. In order to assess the complex mixing of atmospheric anthropogenic and natural pollutants over the East Asian region, we present a modelling tool which takes into account the main aerosols which are to be found simultaneously over China, Korea and Japan during springtime. Using the mesoscale RAMS (Regional Atmospheric Modeling System) tool, we present a simulation of natural (desert) dust events along with some of the most critical anthropogenic pollutants over East Asia, sulphur elements (SO2 and SO2-4) and Black Carbon (BC). As regards a one-week case study of dust events which occurred during late April 2005 over an area extending from the Gobi deserts to the Japan surroundings, we satisfactorily model the behaviours of the different aerosol plumes. We focus on possible dust mixing with the anthropogenic pollutants from megacities. For both natural and anthropogenic pollution, the model results are in fairly good agreement with the horizontal and vertical distributions of concentrations as measured by in situ LIDAR, and as observed in remote data, PM10 data and literature. In particular, we show that a simplified chemistry approach of this complex issue is sufficient to model this event, with a real-time step of 3 h. The model reproduces the main patterns and orders of magnitude for Aerosol Optical Thickness (AOT) and species contributions (via the Angström Exponent) when compared with the AErosol RObotic NETwork (AERONET) data.

scholarly journals Transformation and aging of biomass burning carbonaceous aerosol over tropical South America from aircraft in-situ measurements during SAMBBA

2019 ◽  
Author(s):  
William T. Morgan ◽  
James D. Allan ◽  
Stéphane Bauguitte ◽  
Eoghan Darbyshire ◽  
Michael J. Flynn ◽  
...  
Keyword(s):  
South America ◽  
Biomass Burning ◽  
Chemical Properties ◽  
Carbonaceous Aerosol ◽  
Air Masses ◽  
Atmospheric Aging ◽  
Primary Driver ◽  
Tropical South America

Abstract. We present a range of airborne in-situ observations of biomass burning carbonaceous aerosol over tropical South America, including a case study of a large tropical forest wildfire and a series of regional survey flights across the Brazilian Amazon and Cerrado. The study forms part of the South American Biomass Burning Analysis (SAMBBA) Project, which was conducted during September and October 2012. We find limited evidence for net increases in aerosol mass through atmospheric aging combined with substantial changes in the chemical properties of organic aerosol (OA). Oxidation of the OA increases significantly and rapidly on the scale of 2.5–3 hours based on our case study analysis and is consistent with secondary organic aerosol production. The observations of limited net enhancement in OA coupled with such changes in chemical composition, imply that evaporation of OA is also occurring to balance these changes. We observe significant coatings on black carbon particles at source, but with limited changes with aging in both particle core size and coating thickness. We quantify variability in the ratio of OA to carbon monoxide across our study as a key parameter representing both initial fire conditions and an indicator of net aerosol production with atmospheric aging. We observe ratios of 0.075–0.13 μg sm−3 ppbv−1 in the west of our study region over the Amazon tropical forest in air masses less influenced by precipitation and a value of 0.095 μg sm−3 ppbv−1 over the Cerrado environment in the east. Such values are consistent with emission factors used by numerical models to represent biomass burning OA emissions. Black carbon particle core sizes typically range from 250–290 nm, while coating thicknesses range from 40–110 nm in air masses less influenced by precipitation. The primary driver of the variability we observe appears to be related to changes at the initial fire source. A key lesson from our study is that the complex nature of the regional aerosol and its drivers precludes aggregating our observations as a function of atmospheric aging due to the many conflating and competing factors present. Our study explores and quantifies key uncertainties in the evolution of biomass burning aerosol at both nearfield and regional scales. Our results suggest that the initial conditions of the fire are the primary driver of carbonaceous aerosol physical and chemical properties over tropical South America, aside from significant oxidation of OA during atmospheric aging. Such findings imply that uncertainties in the magnitude of the aerosol burden and its impact on weather, climate, health and natural ecosystems most likely lie in quantifying emission sources, alongside atmospheric dispersion, transport and removal rather than chemical enhancements in mass.

scholarly journals Case Study of Potential Vorticity Tower in Three Explosive Cyclones over Eastern Asia

2017 ◽  
Vol 74 (5) ◽  
pp. 1445-1454 ◽  
Author(s):  
Huaji Pang ◽  
Gang Fu
Keyword(s):  
Potential Vorticity ◽  
Morphological Characteristics ◽  
Lower Troposphere ◽  
Static Stability ◽  
Relative Vorticity ◽  
Eastern Asia ◽  
The North ◽  
Surface Cyclone ◽  
Explosive Cyclones

AbstractThree cases of explosively developing extratropical cyclones over eastern Asia are analyzed using ERA-Interim data. The morphological characteristics of the upper-tropospheric potential vorticity (PV) were examined. The common feature of all of these three cases is a hook-shaped high-PV streamer wrapping counterclockwise around the center of surface cyclones on the southern and eastern sides and an arch-shaped low-PV tongue that wrapped the high-PV hook head from the north. The hook-shaped high-PV tongue overlaps with the maximum centers of both the relative vorticity and static stability parameter, indicating the stratospheric nature of the PV source inside the hook-shaped high-PV tongue.The analysis indicates that there existed a deep tower of high PV above the surface cyclone at the time when these cyclones underwent explosive cyclogenesis. The high PV in the upper troposphere originates from the polar stratospheric PV reservoir associated with the tropopause-folding process. The high PV in the lower troposphere, however, is associated with the latent heat release, as nearly 70%–90% of the high-PV values in the lower troposphere reside in the region where the rainfall is the heaviest.

Modeling study of biomass burning plumes and their impact on urban air quality; a case study of Santiago de Chile

2017 ◽  
Vol 166 ◽  
pp. 79-91 ◽  
Author(s):  
G.C. Cuchiara ◽  
B. Rappenglück ◽  
M.A. Rubio ◽  
E. Lissi ◽  
E. Gramsch ◽  
...  
Keyword(s):  
Air Quality ◽  
Biomass Burning ◽  
Urban Air Quality ◽  
Urban Air ◽  
Santiago De Chile ◽  
Modeling Study
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