scholarly journals NO<sub>x</sub> production by lightning in Hector: first airborne measurements during SCOUT-O3/ACTIVE

2009 ◽  
Vol 9 (4) ◽  
pp. 14361-14451 ◽  
Author(s):  
H. Huntrieser ◽  
H. Schlager ◽  
M. Lichtenstern ◽  
A. Roiger ◽  
P. Stock ◽  
...  

Abstract. During the SCOUT-O3/ACTIVE field phase in November–December 2005 airborne in situ measurements were performed inside and in the vicinity of thunderstorms over northern Australia with several research aircraft (German Falcon, Russian M55 Geophysica, and British Dornier-228). Here a case study from 19 November is presented in large detail on the basis of airborne trace gas measurements (NO, NOy, CO, O3) and stroke measurements from the German LIghtning Location NETwork (LINET), set up in the vicinity of Darwin during the field campaign. The anvil outflow from three different types of thunderstorms was probed by the Falcon aircraft: 1) a continental thunderstorm developing in a tropical airmass near Darwin, 2) a mesoscale convective system (MCS) developing within the tropical maritime continent (Tiwi Islands) known as Hector, and 3) a continental thunderstorm developing in a subtropical airmass ~200 km south of Darwin. For the first time detailed measurements of NO were performed in the Hector outflow. The highest NO mixing ratios were observed in Hector with peaks up to 7 nmol mol−1 in the main anvil outflow at ~11.5–12.5 km altitude. The mean NOx (=NO+NO2) mixing ratios during these penetrations (~100 km width) varied between 2.2 and 2.5 nmol mol−1. The NOx contribution from the boundary layer (BL), transported upward with the convection, to total anvil-NOx was found to be minor (<10%). On the basis of Falcon measurements, the mass flux of lightning-produced NOx (LNOx) in the well-developed Hector system was estimated to 0.6–0.7 kg(N) s−1. The highest average stroke rate of the probed thunderstorms was observed in the Hector system with 0.2 strokes s−1 (here only strokes with peak currents ≥10 kA contributing to LNOx were considered). The LNOx mass flux and the stroke rate were combined to estimate the LNOx production rate in the different thunderstorm types. For a better comparison with other studies, LINET strokes were scaled with Lightning Imaging Sensor (LIS) flashes. The LNOx production rate per LIS flash was estimated to 4.1–4.8 kg(N) for the well-developed Hector system, and to 5.4 and 1.7 kg(N) for the continental thunderstorms developing in subtropical and tropical airmasses, respectively. If we assume, that these different types of thunderstorms are typical thunderstorms globally (LIS flash rate ~44 s−1), the annual global LNOx production rate based on Hector would be ~5.7–6.6 Tg(N) a−1 and based on the continental thunderstorms developing in subtropical and tropical airmasses ~7.6 and ~2.4 Tg(N) a−1, respectively. The latter thunderstorm type produced much less LNOx per flash compared to the subtropical and Hector thunderstorms, which may be caused by the shorter mean flash component length observed in this storm. It is suggested that the vertical wind shear influences the horizontal extension of the charged layers, which seems to play an important role for the flash lengths that may originate. In addition, the horizontal dimension of the anvil outflow and the cell organisation within the thunderstorm system are probably important parameters influencing flash length and hence LNOx production per flash.

2009 ◽  
Vol 9 (21) ◽  
pp. 8377-8412 ◽  
Author(s):  
H. Huntrieser ◽  
H. Schlager ◽  
M. Lichtenstern ◽  
A. Roiger ◽  
P. Stock ◽  
...  

Abstract. During the SCOUT-O3/ACTIVE field phase in November–December 2005, airborne in situ measurements were performed inside and in the vicinity of thunderstorms over northern Australia with several research aircraft (German Falcon, Russian M55 Geophysica, and British Dornier-228. Here a case study from 19 November is presented in detail on the basis of airborne trace gas measurements (NO, NOy, CO, O3) and stroke measurements from the German LIghtning Location NETwork (LINET), set up in the vicinity of Darwin during the field campaign. The anvil outflow from three different types of thunderstorms was probed by the Falcon aircraft: (1) a continental thunderstorm developing in a tropical airmass near Darwin, (2) a mesoscale convective system (MCS), known as Hector, developing within the tropical maritime continent (Tiwi Islands), and (3) a continental thunderstorm developing in a subtropical airmass ~200 km south of Darwin. For the first time detailed measurements of NO were performed in the Hector outflow. The highest NO mixing ratios were observed in Hector with peaks up to 7 nmol mol−1 in the main anvil outflow at ~11.5–12.5 km altitude. The mean NOx (=NO+NO2) mixing ratios during these penetrations (~100 km width) varied between 2.2 and 2.5 nmol mol−1. The NOx contribution from the boundary layer (BL), transported upward with the convection, to total anvil-NOx was found to be minor (<10%). On the basis of Falcon measurements, the mass flux of lightning-produced NOx (LNOx) in the well-developed Hector system was estimated to 0.6–0.7 kg(N) s−1. The highest average stroke rate of the probed thunderstorms was observed in the Hector system with 0.2 strokes s−1 (here only strokes with peak currents ≥10 kA contributing to LNOx were considered). The LNOx mass flux and the stroke rate were combined to estimate the LNOx production rate in the different thunderstorm types. For a better comparison with other studies, LINET strokes were scaled with Lightning Imaging Sensor (LIS) flashes. The LNOx production rate per LIS flash was estimated to 4.1–4.8 kg(N) for the well-developed Hector system, and to 5.4 and 1.7 kg(N) for the continental thunderstorms developing in subtropical and tropical airmasses, respectively. If we assume, that these different types of thunderstorms are typical thunderstorms globally (LIS flash rate ~44 s−1), the annual global LNOx production rate based on Hector would be ~5.7–6.6 Tg(N) a−1 and based on the continental thunderstorms developing in subtropical and tropical airmasses ~7.6 and ~2.4 Tg(N) a−1, respectively. The latter thunderstorm type produced much less LNOx per flash compared to the subtropical and Hector thunderstorms, which may be caused by the shorter mean flash component length observed in this storm. It is suggested that the vertical wind shear influences the horizontal extension of the charged layers, which seems to play an important role for the flash lengths that may originate. In addition, the horizontal dimension of the anvil outflow and the cell organisation within the thunderstorm system are probably important parameters influencing flash length and hence LNOx production per flash.


2010 ◽  
Vol 10 (10) ◽  
pp. 22765-22853
Author(s):  
H. Huntrieser ◽  
H. Schlager ◽  
M. Lichtenstern ◽  
P. Stock ◽  
T. Hamburger ◽  
...  

Abstract. During the "African Monsoon Multidisciplinary Analysis" (AMMA) field phase in August 2006, a variety of measurements focusing on deep convection were performed over West Africa. The German research aircraft Falcon based in Ouagadougou (Burkina Faso) investigated the chemical composition in the outflow of large mesoscale convective systems (MCS). Here we analyse two different types of MCS originating north and south of the intertropical convergence zone (ITCZ, ~10° N), respectively. In addition to the airborne trace gas measurements, stroke measurements from the Lightning Location Network (LINET), set up in Northern Benin, are analysed. The main focus of the present study is 1) to analyse the trace gas composition (CO, O3, NO, NOx, NOy, and HCHO) in the convective outflow as a function of distance from the convective core, 2) to investigate how different trace gas compositions in the boundary layer (BL) and ambient air may influence the O3 concentration in the convective outflow, and 3) to estimate the rate of lightning-produced nitrogen oxides per flash in selected thunderstorms and compare it to our previous results for the tropics. The MCS outflow was probed at different altitudes (~10–12 km) and distances from the convective core (<500 km). Trace gas signatures similar to the conditions in the MCS inflow region were observed in the outflow close to the convective core, due to efficient vertical transport. In the fresh MCS outflow, low O3 mixing ratios in the range of 35–40 nmol mol−1 were observed. Further downwind, O3 mixing ratios in the outflow rapidly increased with distance, due to mixing with the ambient O3-rich air. After 2–3 h, O3 mixing ratios in the range of ~65 nmol mol−1 were observed in the aged outflow. Within the fresh MCS outflow, mean NOx (=NO+NO2) mixing ratios were in the range of ~0.3–0.4 nmol mol−1 (peaks ~1 nmol mol−1) and only slightly enhanced compared to the background. Both lightning-produced NOx (LNOx) and NOx transported upward from the BL contributed about equally to this enhancement. On the basis of Falcon measurements, the mass flux of LNOx in the investigated MCS was estimated to be ~100 g(N) s−1. The average stroke rate of the probed thunderstorms was 0.04–0.07 strokes s−1 (here only strokes with peak currents ≥10 kA contributing to LNOx were considered). The LNOx mass flux and the stroke rate were combined to estimate the LNOx production rate. For a better comparison with other published results, LNOx estimates per LINET stroke were scaled to Lightning Imaging Sensor (LIS) flashes. The LNOx production rate per LIS flash was estimated to 1.0 and 2.5 kg(N) for the MCS located south and north of the ITCZ, respectively. If we assume, that these different types of MCS are typical thunderstorms occurring globally (LIS flash rate ~44 s−1), the annual global LNOx production rate was estimated to be ~1.4 and 3.5 Tg(N) a−1.


2011 ◽  
Vol 11 (6) ◽  
pp. 2503-2536 ◽  
Author(s):  
H. Huntrieser ◽  
H. Schlager ◽  
M. Lichtenstern ◽  
P. Stock ◽  
T. Hamburger ◽  
...  

Abstract. During the "African Monsoon Multidisciplinary Analysis" (AMMA) field phase in August 2006, a variety of measurements focusing on deep convection were performed over West Africa. The German research aircraft Falcon based in Ouagadougou (Burkina Faso) investigated the chemical composition in the outflow of large mesoscale convective systems (MCS). Here we analyse two different types of MCS originating north and south of the intertropical convergence zone (ITCZ, ~10° N), respectively. In addition to the airborne trace gas measurements, stroke measurements from the Lightning Location Network (LINET), set up in Northern Benin, are analysed. The main focus of the present study is (1) to analyse the trace gas composition (CO, O3, NO, NOx, NOy, and HCHO) in the convective outflow as a function of distance from the convective core, (2) to investigate how different trace gas compositions in the boundary layer (BL) and ambient air may influence the O3 concentration in the convective outflow, and (3) to estimate the rate of lightning-produced nitrogen oxides per flash in selected thunderstorms and compare it to our previous results for the tropics. The MCS outflow was probed at different altitudes (~10–12 km) and distances from the convective core (<500 km). Trace gas signatures similar to the conditions in the MCS inflow region were observed in the outflow close to the convective core, due to efficient vertical transport. In the fresh MCS outflow, low O3 mixing ratios in the range of 35–40 nmol mol−1 were observed. Further downwind, O3 mixing ratios in the outflow rapidly increased with distance, due to mixing with the ambient O3-rich air. After 2–3 h, O3 mixing ratios in the range of ~65 nmol mol−1 were observed in the aged outflow. Within the fresh MCS outflow, mean NOx (=NO+NO2) mixing ratios were in the range of ~0.3–0.4 nmol mol−1 (peaks ~1 nmol mol−1) and only slightly enhanced compared to the background. Both lightning-produced NOx (LNOx) and NOx transported upward from the BL contributed about equally to this enhancement. On the basis of Falcon measurements, the mass flux of LNOx in the investigated MCS was estimated to be ~100 g(N) s−1. The average stroke rate of the probed thunderstorms was 0.04–0.07 strokes s−1 (here only strokes with peak currents ≥10 kA contributing to LNOx were considered). The LNOx mass flux and the stroke rate were combined to estimate the LNOx production rate. For a better comparison with other published results, LNOx estimates per LINET stroke were scaled to Lightning Imaging Sensor (LIS) flashes. The LNOx production rate per LIS flash was estimated to 1.0 and 2.5 kg(N) for the MCS located south and north of the ITCZ, respectively. If we assume, that these different types of MCS are typical thunderstorms occurring globally (LIS flash rate ~44 s−1), the annual global LNOx production rate was estimated to be ~1.4 and 3.5 Tg(N) a−1.


2007 ◽  
Vol 7 (5) ◽  
pp. 14813-14894 ◽  
Author(s):  
H. Huntrieser ◽  
U. Schumann ◽  
H. Schlager ◽  
H. Höller ◽  
A. Giez ◽  
...  

Abstract. During the TROCCINOX field experiment in January and February 2005, the contribution of lightning-induced nitrogen oxides (LNOx) from tropical and subtropical thunderstorms in Southern Brazil was investigated. Airborne trace gas measurements (NO, NOy, CO and O3) were performed up to 12.5 km with the German research aircraft Falcon. During anvil penetrations in selected tropical and subtropical thunderstorms of 4 and 18 February, NOx mixing ratios were on average enhanced by 0.7–1.2 and 0.2–0.8 nmol mol−1 totally, respectively. The relative contributions of boundary layer NOx (BL-NOx) and LNOx to anvil-NOx were derived from the NOx-CO correlations. On average ~80–90% of the anvil-NOx was attributed to LNOx. A Lightning Location Network (LINET) was set up to monitor the local distribution of cloud-to-ground (CG) and intra-cloud (IC) radiation sources (here called "strokes") and compared with lightning data from the operational Brazilian network RINDAT (Rede Integrada Nacional de Detecção de Descargas Atmosféricas). The horizontal LNOx mass flux out of the anvil was determined from the mean LNOx mixing ratio, the horizontal outflow velocity and the size of the vertical cross-section of the anvil, and related to the number of strokes contributing to LNOx. The values of these parameters were derived from the airborne measurements, from lightning and radar observations, and from a trajectory analysis. The amount of LNOx produced per LINET stroke depending on measured peak current was determined. The results were scaled up with the Lightning Imaging Sensor (LIS) flash rate (44 flashes s−1) to obtain an estimate of the global LNOx production rate. The final results gave ~1 and ~2–3 kg(N) per LIS flash based on measurements in three tropical and one subtropical Brazilian thunderstorms, respectively, suggesting that tropical flashes may be less productive than subtropical ones. The equivalent mean annual global LNOx nitrogen mass production rate was estimated to be 1.6 and 3.1 Tg a−1, respectively. By use of LINET observations in Germany in July 2005, a comparison with the lightning activity in mid-latitude thunderstorms was also performed. In general, the same frequency distribution of stroke peak currents as for tropical thunderstorms over Brazil was found. The different LNOx production rates per stroke in tropical thunderstorms compared with subtropical and mid-latitude thunderstorms seem to be related to the different stroke lengths (inferred from comparison with laboratory data and observed lengths). In comparison, the impact of other lightning parameters as stroke peak current and stroke release height was assessed to be minor. The results from TROCCINOX suggest that the different vertical wind shear may be responsible for the different stroke lengths.


2008 ◽  
Vol 8 (4) ◽  
pp. 921-953 ◽  
Author(s):  
H. Huntrieser ◽  
U. Schumann ◽  
H. Schlager ◽  
H. Höller ◽  
A. Giez ◽  
...  

Abstract. During the TROCCINOX field experiment in January and February 2005, the contribution of lightning-induced nitrogen oxides (LNOx) from tropical and subtropical thunderstorms in Southern Brazil was investigated. Airborne trace gas measurements (NO, NOy, CO and O3) were performed up to 12.5 km with the German research aircraft Falcon. During anvil penetrations in selected tropical and subtropical thunderstorms of 4 and 18 February, NOx mixing ratios were on average enhanced by 0.7–1.2 and 0.2–0.8 nmol mol−1 totally, respectively. The relative contributions of boundary layer NOx (BL-NOx) and LNOx to anvil-NOx were derived from the NOx-CO correlations. On average ~80–90% of the anvil-NOx was attributed to LNOx. A Lightning Location Network (LINET) was set up to monitor the local distribution of cloud-to-ground (CG) and intra-cloud (IC) radiation sources (here called "strokes") and compared with lightning data from the operational Brazilian network RINDAT (Rede Integrada Nacional de Detecção de Descargas Atmosféricas). The horizontal LNOx mass flux out of the anvil was determined from the mean LNOx mixing ratio, the horizontal outflow velocity and the size of the vertical cross-section of the anvil, and related to the number of strokes contributing to LNOx. The values of these parameters were derived from the airborne measurements, from lightning and radar observations, and from a trajectory analysis. The amount of LNOx produced per LINET stroke depending on measured peak current was determined. The results were scaled up with the Lightning Imaging Sensor (LIS) flash rate (44 flashes s−1) to obtain an estimate of the global LNOx production rate. The final results gave ~1 and ~2–3 kg(N) per LIS flash based on measurements in three tropical and one subtropical Brazilian thunderstorms, respectively, suggesting that tropical flashes may be less productive than subtropical ones. The equivalent mean annual global LNOx nitrogen mass production rate was estimated to be 1.6 and 3.1 Tg a−1, respectively. By use of LINET observations in Germany in July 2005, a comparison with the lightning activity in mid-latitude thunderstorms was also performed. In general, the same frequency distribution of stroke peak currents as for tropical thunderstorms over Brazil was found. The different LNOx production rates per stroke in tropical thunderstorms compared with subtropical and mid-latitude thunderstorms seem to be related to the different stroke lengths (inferred from comparison with laboratory data and observed lengths). In comparison, the impact of other lightning parameters as stroke peak current and stroke release height was assessed to be minor. The results from TROCCINOX suggest that the different vertical wind shear may be responsible for the different stroke lengths.


2015 ◽  
Vol 72 (5) ◽  
pp. 1945-1962 ◽  
Author(s):  
Agnieszka A. Mrowiec ◽  
O. M. Pauluis ◽  
A. M. Fridlind ◽  
A. S. Ackerman

Abstract Application of an isentropic analysis of convective motions to a simulated mesoscale convective system is presented. The approach discriminates the vertical mass transport in terms of equivalent potential temperature. The scheme separates rising air at high entropy from subsiding air at low entropy. This also filters out oscillatory motions associated with gravity waves and isolates the overturning motions associated with convection and mesoscale circulation. The mesoscale convective system is additionally partitioned into stratiform and convective regions based on the radar reflectivity field. For each of the subregions, the mass transport derived in terms of height and an isentropic invariant of the flow is analyzed. The difference between the Eulerian mass flux and the isentropic counterpart is a significant and symmetric contribution of the buoyant oscillations to the upward and downward mass fluxes. Filtering out these oscillations results in substantial reduction of the diagnosed downward-to-upward convective mass flux ratio. The analysis is also applied to graupel and snow mixing ratios and number concentrations, illustrating the relationship of the particle formation process to the updrafts.


2019 ◽  
Vol 147 (2) ◽  
pp. 495-517 ◽  
Author(s):  
Christopher A. Kerr ◽  
David J. Stensrud ◽  
Xuguang Wang

AbstractConvection intensity and longevity is highly dependent on the surrounding environment. Ensemble sensitivity analysis (ESA), which quantitatively and qualitatively interprets impacts of initial conditions on forecasts, is applied to very short-term (1–2 h) convective-scale forecasts for three cases during the Mesoscale Predictability Experiment (MPEX) in 2013. The ESA technique reveals several dependencies of individual convective storm evolution on their nearby environments. The three MPEX cases are simulated using a previously verified 36-member convection-allowing model (Δx = 3 km) ensemble created via the Weather Research and Forecasting (WRF) Model. Radar and other conventional observations are assimilated using an ensemble adjustment Kalman filter. The three cases include a mesoscale convective system (MCS) and both nontornadic and tornadic supercells. Of the many ESAs applied in this study, one of the most notable is the positive sensitivity of supercell updraft helicity to increases in both storm inflow region deep and shallow vertical wind shear. This result suggests that larger values of vertical wind shear within the storm inflow yield higher values of storm updraft helicity. Results further show that the supercell storms quickly enhance the environmental vertical wind shear within the storm inflow region. Application of ESA shows that these storm-induced perturbations then affect further storm evolution, suggesting the presence of storm–environment feedback cycles where perturbations affect future mesocyclone strength. Overall, ESA can provide insight into convection dependencies on the near-storm environment.


2019 ◽  
Vol 19 (5) ◽  
pp. 1023-1040 ◽  
Author(s):  
Luca Mathias ◽  
Patrick Ludwig ◽  
Joaquim G. Pinto

Abstract. A major linear mesoscale convective system caused severe weather over northern France, Belgium, the Netherlands and northwestern Germany on 3 January 2014. The storm was classified as a cold-season derecho with widespread wind gusts exceeding 25 m s−1. While such derechos occasionally develop along cold fronts of extratropical cyclones, this system formed in a postfrontal air mass along a baroclinic surface pressure trough and was favoured by a strong large-scale air ascent induced by an intense mid-level jet. The lower-tropospheric environment was characterised by weak latent instability and strong vertical wind shear. Given the poor operational forecast of the storm, we analyse the role of initial and lateral boundary conditions to the storm's development by performing convection-resolving limited-area simulations with operational analysis and reanalysis datasets. The storm is best represented in simulations with high temporally and spatially resolved initial and lateral boundary conditions derived from ERA5, which provide the most realistic development of the essential surface pressure trough. Moreover, simulations at convection-resolving resolution enable a better representation of the observed derecho intensity. This case study is testimony to the usefulness of ensembles of convection-resolving simulations in overcoming the current shortcomings of forecasting cold-season convective storms, particularly for cases not associated with a cold front.


2009 ◽  
Vol 66 (3) ◽  
pp. 686-704 ◽  
Author(s):  
Christopher A. Davis ◽  
Thomas J. Galarneau

Abstract Simulations of two cases of developing mesoscale convective vortices (MCVs) are examined to determine the dynamics governing the origin and vertical structure of these features. Although one case evolves in strong vertical wind shear and the other evolves in modest shear, the evolutions are remarkably similar. In addition to the well-known mesoscale convergence that spins up vorticity in the midtroposphere, the generation of vorticity in the lower troposphere occurs along the convergent outflow boundary of the parent mesoscale convective system (MCS). Lateral transport of this vorticity from the convective region back beneath the midtropospheric vorticity center is important for obtaining a deep column of cyclonic vorticity. However, this behavior would be only transient without a secondary phase of vorticity growth in the lower troposphere that results from a radical change in the divergence profile favoring lower-tropospheric convergence. Following the decay of the nocturnal MCS, subsequent convection occurs in a condition of greater relative humidity through the lower troposphere and small conditional instability. Vorticity and potential vorticity are efficiently produced near the top of the boundary layer and a cyclonic circulation appears at the surface.


2011 ◽  
Vol 139 (8) ◽  
pp. 2367-2385 ◽  
Author(s):  
Hsiao-Wei Lai ◽  
Christopher A. Davis ◽  
Ben Jong-Dao Jou

AbstractThis study examines a subtropical oceanic mesoscale convective vortex (MCV) that occurred from 1800 UTC 4 June to 1200 UTC 6 June 2008 during intensive observing period (IOP) 6 of the Southwest Monsoon Experiment (SoWMEX) and the Terrain-influenced Monsoon Rainfall Experiment (TiMREX). A dissipating mesoscale convective system reorganized within a nearly barotropic vorticity strip, which formed as a southwesterly low-level jet developed to the south of subsiding easterly flow over the southern Taiwan Strait. A cyclonic circulation was revealed on the northern edge of the mesoscale rainband with a horizontal scale of 200 km. An inner subvortex, on a scale of 25–30 km with maximum shear vorticity of 3 × 10−3 s−1, was embedded in the stronger convection. The vortex-relative southerly flow helped create local potential instability favorable for downshear convection enhancement. Strong low-level convergence suggests that stretching occurred within the MCV. Higher θe air, associated with significant potential and conditional instability, and high reflectivity signatures near the vortex center suggest that deep moist convection was responsible for the vortex stretching. Dry rear inflow penetrated into the MCV and suppressed convection in the upshear direction. A mesolow was also roughly observed within the larger vortex. The presence of intense vertical wind shear in the higher troposphere limited the vortex vertical extent to about 6 km.


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