scholarly journals Total ozone column retrieval from OMPS-NM measurements

2021 ◽  
Author(s):  
Andrea Orfanoz-Cheuquelaf ◽  
Alexei Rozanov ◽  
Mark Weber ◽  
Carlo Arosio ◽  
Annette Ladstätter-Weißenmayer ◽  
...  
Keyword(s):  
Total Ozone ◽  
Weighting Function ◽  
Optical Absorption Spectroscopy ◽  
Retrieval Algorithm ◽  
Polar Regions ◽  
Total Ozone Column ◽  
Function Fitting ◽  
Ozone Column ◽  
Good Agreement ◽  
Column Product

Abstract. A scientific total ozone column product from the Ozone Mapping and Profiler Suite Nadir Mapper (OMPS-NM) observations and its retrieval algorithm are presented. The retrieval employs the Weighting Function Fitting Approach (WFFA), a modification of the Weighting Function Differential Optical Absorption Spectroscopy (WFDOAS) technique. The total ozone columns retrieved with WFFA are in very good agreement with other datasets. A mean difference of 0.6 % with respect to ground-based Brewer and Dobson measurements is observed. Seasonal and latitudinal variations are well represented and in agreement with other satellite datasets. The comparison of our product with the scientific product of OMPS-NM indicate a mean bias of around 0.1 %. The comparison with the Tropospheric Monitoring Instrument products (S5P/TROPOMI) OFFL and WFDOAS, shows a persistent negative bias of about −0.5 % for OFFL and –2 % for WFDOAS. Larger differences are only observed in the polar regions. This data product is intended to be used for trend analysis and the retrieval of tropospheric ozone combined with the OMPS limb profiler data.

scholarly journals Total ozone column from Ozone Mapping and Profiler Suite Nadir Mapper (OMPS-NM) measurements using the broadband weighting function fitting approach (WFFA)

2021 ◽  
Vol 14 (8) ◽  
pp. 5771-5789
Author(s):  
Andrea Orfanoz-Cheuquelaf ◽  
Alexei Rozanov ◽  
Mark Weber ◽  
Carlo Arosio ◽  
Annette Ladstätter-Weißenmayer ◽  
...  
Keyword(s):  
Total Ozone ◽  
Weighting Function ◽  
Optical Absorption Spectroscopy ◽  
Retrieval Algorithm ◽  
Polar Regions ◽  
Total Ozone Column ◽  
Function Fitting ◽  
Ozone Column ◽  
Good Agreement ◽  
Column Product

Abstract. A scientific total ozone column product from Ozone Mapping and Profiler Suite Nadir Mapper (OMPS-NM) observations and the retrieval algorithm are presented. The retrieval employs the weighting function fitting approach (WFFA), a modification of the weighting function differential optical absorption spectroscopy (WFDOAS) technique. The total ozone columns retrieved with WFFA are in very good agreement with other datasets. A mean difference of 0.3 % with respect to ground-based Brewer and Dobson measurements is observed. Seasonal and latitudinal variations are well represented and in agreement with other satellite datasets. The comparison of our product with the operational product of OMPS-NM indicates a mean bias of around zero. The comparison with the Tropospheric Monitoring Instrument products (S5P/TROPOMI) OFFL and WFDOAS shows a persistent negative bias of about −0.6 % for OFFL and −2.5 % for WFDOAS. Larger differences are only observed in the polar regions. This data product is intended to be used for trend analysis and the retrieval of tropospheric ozone combined with the OMPS limb profiler data.

scholarly journals Seasonal impact of biogenic VSL bromine on the evolution of mid-latitude lowermost stratospheric ozone during the 21<sup>st</sup> century

2020 ◽  
Author(s):  
Javer A. Barrera ◽  
Rafael P. Fernandez ◽  
Fernando Iglesias-Suarez ◽  
Carlos A. Cuevas ◽  
Jean-Francois Lamarque ◽  
...  
Keyword(s):  
21St Century ◽  
Total Ozone ◽  
Stratospheric Ozone ◽  
Polar Regions ◽  
Total Ozone Column ◽  
Seasonal Impact ◽  
The Tropics ◽  
The Impact ◽  
Ozone Column ◽  
Modelling Study

Abstract. Biogenic very short-lived bromine (VSLBr) represents, nowadays, ~ 25 % of the total stratospheric bromine loading. Owing to their much shorter lifetime compared to anthropogenic long-lived bromine (LLBr, e.g., halons) and chlorine (LLCl, e.g., chlorofluorocarbons) substances, the impact of VSLBr on ozone peaks at the extratropical lowermost stratosphere, a key climatic and radiative atmospheric region. Here we present a modelling study of the evolution of stratospheric ozone and its chemical losses in extra-polar regions during the 21st century, under two different scenarios: considering and neglecting the additional stratospheric injection of 5 ppt biogenic VSLBr naturally released from the ocean. Our analysis shows that the inclusion of VSLBr result in a realistic stratospheric bromine loading and improves the quantitative 1980–2015 model-satellite agreement of total ozone column (TOC) in the mid-latitudes. We show that the overall ozone response to VSLBr within the mid-latitudes follows the stratospheric abundances evolution of long-lived inorganic chlorine and bromine throughout the 21st century. Additional ozone losses due to VSLBr are maximised during the present-day period (1990–2010), with TOC differences of −8 DU (−3 %) and −5.5 DU (−2 %) for the southern (SH-ML) and northern (NH-ML) mid-latitudes, respectively. Moreover, the projected TOC differences at the end of the 21st century are at least half of the values found for the present-day period. In the tropics, a small (

scholarly journals Total ozone column intercomparison of Brewers, Dobsons, and BTS-Solar at Hohenpeißenberg and Davos in 2019/2020

2021 ◽  
Vol 14 (7) ◽  
pp. 4915-4928
Author(s):  
Ralf Zuber ◽  
Ulf Köhler ◽  
Luca Egli ◽  
Mario Ribnitzky ◽  
Wolfgang Steinbrecht ◽  
...  
Keyword(s):  
Seasonal Variation ◽  
Standard Deviation ◽  
Total Ozone ◽  
Retrieval Algorithm ◽  
Measurement Campaign ◽  
Total Ozone Column ◽  
Stratospheric Temperature ◽  
Retrieval Algorithms ◽  
Double Monochromator ◽  
Ozone Column

Abstract. During the 2019/2020 measurement campaign at Hohenpeißenberg (Germany) and Davos (Switzerland) we compared the well-established Dobson and Brewer spectrometers (single- and double-monochromator Brewer) with newer BTS array-spectroradiometer-based systems in terms of total ozone column (TOC) determination. The aim of this study is to validate the BTS performance in a longer-term TOC analysis over more than 1 year with seasonal and weather influences. Two different BTS setups have been used – a fibre-coupled entrance optic version by PMOD/WRC called Koherent and a diffusor optic version from Gigahertz Optik GmbH called BTS-Solar, which proved to be simpler in terms of calibration. The array-spectrometer-based BTS systems have been calibrated with traceability to NMI, and both versions of TOC retrieval algorithms are based on spectral measurements in the range of 305 to 350 nm instead of single-wavelength or wavelength pair measurements as per Brewer or Dobson. The two BTS-based systems, however, used fundamentally different retrieval algorithms for the TOC assessment, whereby the retrieval of the BTS-Solar turned out to achieve significantly smaller seasonal drifts. The intercomparison showed a difference of the BTS-Solar to Brewers of < 0.1 % with an expanded standard deviation (k=2) of < 1.5 % over the whole measurement campaign. Koherent showed a difference of 1.7 % with an expanded standard deviation (k=2) of 2.7 % mostly caused by a significant seasonal variation. To summarize, the BTS-Solar performed at the level of Brewers in the comparison in Hohenpeißenberg. The BTS-Solar showed very small dependence on the slant path column compared to the double-monochromator Brewer and performed better than the single-monochromator Brewer. Koherent showed a strong seasonal variation in Davos due to the sensitivity of its ozone retrieval algorithm to stratospheric temperature.

scholarly journals Pole-to-pole validation of GOME WFDOAS total ozone with groundbased data

2005 ◽  
Vol 5 (5) ◽  
pp. 1341-1355 ◽  
Author(s):  
M. Weber ◽  
L. N. Lamsal ◽  
M. Coldewey-Egbers ◽  
K. Bramstedt ◽  
J. P. Burrows
Keyword(s):  
Total Ozone ◽  
Weighting Function ◽  
Stratospheric Ozone ◽  
Extended Period ◽  
Companion Paper ◽  
Temperature Correction ◽  
Global Network ◽  
Optical Absorption Spectroscopy ◽  
Polar Regions ◽  
Data Processor

Abstract. This paper summarises the validation of GOME total ozone retrieved using the Weighting Function Differential Optical Absorption Spectroscopy (WFDOAS) algorithm Version 1.0. This algorithm has been described in detail in a companion paper by Coldewey-Egbers et al. (2005). Compared to the operational GDP (GOME Data Processor) V3, several improvements to the total ozone retrieval have been introduced that account for the varying ozone dependent contribution to rotational Raman scattering, includes a new cloud scheme, and uses the GOME measured effective albedo in the retrieval. In this paper the WFDOAS results have been compared with selected ground-based measurements from the WOUDC (World Ozone and UV Radiation Data Centre) that collects total ozone measurements from a global network of stations covering all seasons. From the global validation excellent agreement between WFDOAS and ground data was observed. The agreement lies within ±1%, and very little seasonal variations in the differences are found. In the polar regions and at high solar zenith angles, however, a positive bias varying between 5 and 8% is found near the polar night period. As a function of solar zenith angle as well as of the retrieved total ozone, the WFDOAS differences to ground polar data, however, show a much weaker dependence as compared to the operational GOME Data Processor Version 3 of GOME that represents a significant improvement. Very few stations carry out simultaneous measurements by Brewer and Dobson spectrometers over an extended period (three years or more). Simultaneous Brewer and Dobson measurements from Hradec Kralove, Czech Republic (50.2N, 15.8E) and Hohenpeissenberg, Germany (47.8N, 11.0E) covering the period 1996-1999 have been compared with our GOME results. Agreement with Brewers are generally better than with the simultaneous Dobson measurements and this may be explained by the neglect of stratospheric (ozone) temperature correction in the standard ozone retrieval from the ground.

scholarly journals Synergy of Using Nadir and Limb Instruments for Tropospheric Ozone Monitoring

2021 ◽  
Author(s):  
Viktoria F. Sofieva ◽  
Risto Hänninen ◽  
Mikhail Sofiev ◽  
Monika Szelag ◽  
Hei Shing Lee ◽  
...  
Keyword(s):  
Satellite Data ◽  
Tropospheric Ozone ◽  
Total Ozone ◽  
Stratospheric Ozone ◽  
Intermediate Step ◽  
Residual Method ◽  
Total Ozone Column ◽  
Clear Sky ◽  
Ozone Column ◽  
Good Agreement

Abstract. The satellite measurements in nadir and limb viewing geometry provide a complementary view of the atmosphere. An effective combination of the limb and nadir measurements can provide a new information about atmospheric composition. In this work, we present tropospheric ozone column datasets that have been created using combination of total ozone column from OMI and TROPOMI with stratospheric ozone column dataset from several available limb-viewing instruments (MLS, OSIRIS, MIPAS, SCIAMACHY, OMPS-LP, GOMOS). We have developed further the methodological aspects of assessment of tropospheric ozone using the residual method using simulations with the chemistry-transport model SILAM. It has been shown that the accurate assessment of ozone in the upper troposphere and the lower stratosphere (UTLS) is of high importance for detecting the ground-level ozone patterns. The stratospheric ozone column is derived from a combination of ozone profiles from several satellite instruments in limb-viewing geometry. We developed a method for the data homogenization, which includes the removal of biases and a-posteriori estimation (validation) of random uncertainties, thus making the data from different instruments compatible with each other. The high horizontal and vertical resolution dataset of ozone profiles is created via interpolation of the limb profiles from each day to 1° × 1° horizonal grid. A new kriging-type interpolation method, which takes into account data uncertainties and the information about natural ozone variations from the SILAM-adjusted ozone field, has been developed. To mitigate the limited accuracy and coverage of the limb profile data in the UTLS, a smooth transition to the model data is applied below the tropopause. This allows estimation of stratospheric ozone column with full coverage of the UTLS. The derived ozone profiles are in very good agreement with collocated ozonesonde measurements. The residual method was successfully applied to OMI and TROPOMI clear-sky total ozone data in combination with the stratospheric ozone column from the high-resolution limb profile dataset. The resulting tropospheric ozone column is in very good agreement with other satellite data. The global distributions of tropospheric ozone exhibit enhancements associated with the regions of high tropospheric ozone production. The main created datasets are (i) monthly 1° × 1° global tropospheric ozone column dataset using OMI and limb instruments, (ii) monthly 1° × 1° global tropospheric ozone column dataset using TROPOMI and limb instruments and (iii) daily 1° × 1° interpolated stratospheric ozone column from limb instruments. Other datasets, which are created as an intermediate step of creating the tropospheric ozone column data, are: (i) daily 1° × 1° clear sky and total ozone column from OMI and TROPOMI (ii) Daily 1° × 1° homogenized and interpolated dataset of ozone profiles and (iii) daily 1° × 1° dataset of ozone profiles from SILAM simulations with adjustment to satellite data. These datasets can be used in various studies related to ozone distributions, variability and trends, both in the troposphere and the stratosphere.

scholarly journals Comparison of OMI-DOAS total ozone column with ground-based measurements in Argentina

2020 ◽  
pp. 13
Author(s):  
P. F. Orte ◽  
E. Luccini ◽  
E. Wolfram ◽  
F. Nollas ◽  
J. Pallotta ◽  
...  
Keyword(s):  
Linear Regression ◽  
Optical Absorption ◽  
Southern Hemisphere ◽  
Total Ozone ◽  
Buenos Aires ◽  
Optical Absorption Spectroscopy ◽  
Ozone Monitoring Instrument ◽  
Total Ozone Column ◽  
Ozone Monitoring ◽  
Ozone Column

<p>Total ozone column (TOC) measurements through the Ozone Monitoring Instrument (OMI/NASA EOSAura) are compared with ground-based observations made using Dobson and SAOZ instruments for the period 2004–2019 and 2008–02/2020, respectively. The OMI data were inverted using the Differential Optical Absorption Spectroscopy algorithm (overpass OMI-DOAS). The four ground-based sites used for the analysis are located in subpolar and subtropical latitudes spanning from 34°S to 54°S in the Southern Hemisphere, in the Argentine cities of Buenos Aires (34.58°S, 58.36°W; 25 m a.s.l.), Comodoro Rivadavia (45.86°S, 67.50°W; 46 m a.s.l.), Río Gallegos (51.60°S, 69.30°W; 72 m a.s.l.) and Ushuaia (54.80°S, 68.30°W; 14 m a.s.l.). The linear regression analyzes showed correlation values greater than 0.90 for all sites. The OMI measurements revealed an overestimation of less than 4 % with respect to the Dobson instruments, while the comparison with the SAOZ instrument presented a very low underestimation of less than 1 %.</p>

scholarly journals TROPOMI/S5P total ozone column data: global ground-based validation and consistency with other satellite missions

2019 ◽  
Vol 12 (10) ◽  
pp. 5263-5287 ◽  
Author(s):  
Katerina Garane ◽  
Maria-Elissavet Koukouli ◽  
Tijl Verhoelst ◽  
Christophe Lerot ◽  
Klaus-Peter Heue ◽  
...  
Keyword(s):  
Standard Deviation ◽  
Spatial Resolution ◽  
Total Ozone ◽  
Optical Absorption Spectroscopy ◽  
Total Ozone Column ◽  
Global Comparison ◽  
The Mean ◽  
Ozone Monitoring ◽  
Ozone Column

Abstract. In October 2017, the Sentinel-5 Precursor (S5P) mission was launched, carrying the TROPOspheric Monitoring Instrument (TROPOMI), which provides a daily global coverage at a spatial resolution as high as 7 km × 3.5 km and is expected to extend the European atmospheric composition record initiated with GOME/ERS-2 in 1995, enhancing our scientific knowledge of atmospheric processes with its unprecedented spatial resolution. Due to the ongoing need to understand and monitor the recovery of the ozone layer, as well as the evolution of tropospheric pollution, total ozone remains one of the leading species of interest during this mission. In this work, the TROPOMI near real time (NRTI) and offline (OFFL) total ozone column (TOC) products are presented and compared to daily ground-based quality-assured Brewer and Dobson TOC measurements deposited in the World Ozone and Ultraviolet Radiation Data Centre (WOUDC). Additional comparisons to individual Brewer measurements from the Canadian Brewer Network and the European Brewer Network (Eubrewnet) are performed. Furthermore, twilight zenith-sky measurements obtained with ZSL-DOAS (Zenith Scattered Light Differential Optical Absorption Spectroscopy) instruments, which form part of the SAOZ network (Système d'Analyse par Observation Zénitale), are used for the validation. The quality of the TROPOMI TOC data is evaluated in terms of the influence of location, solar zenith angle, viewing angle, season, effective temperature, surface albedo and clouds. For this purpose, globally distributed ground-based measurements have been utilized as the background truth. The overall statistical analysis of the global comparison shows that the mean bias and the mean standard deviation of the percentage difference between TROPOMI and ground-based TOC is within 0 –1.5 % and 2.5 %–4.5 %, respectively. The mean bias that results from the comparisons is well within the S5P product requirements, while the mean standard deviation is very close to those limits, especially considering that the statistics shown here originate both from the satellite and the ground-based measurements. Additionally, the TROPOMI OFFL and NRTI products are evaluated against already known spaceborne sensors, namely, the Ozone Mapping Profiler Suite, on board the Suomi National Polar-orbiting Partnership (OMPS/Suomi-NPP), NASA v2 TOCs, and the Global Ozone Monitoring Experiment 2 (GOME-2), on board the Metop-A (GOME-2/Metop-A) and Metop-B (GOME-2/Metop-B) satellites. This analysis shows a very good agreement for both TROPOMI products with well-established instruments, with the absolute differences in mean bias and mean standard deviation being below +0.7 % and 1 %, respectively. These results assure the scientific community of the good quality of the TROPOMI TOC products during its first year of operation and enhance the already prevalent expectation that TROPOMI/S5P will play a very significant role in the continuity of ozone monitoring from space.

scholarly journals 2.5 years of TROPOMI S5P total ozone column data: geophysical global ground-based validation and inter-comparison with other satellite missions

2020 ◽  
Author(s):  
Katerina Garane ◽  
Maria-Elissavet Koukouli ◽  
Tijl Verhoelst ◽  
Christophe Lerot ◽  
Klaus-Peter Heue ◽  
...  
Keyword(s):  
Standard Deviation ◽  
Total Ozone ◽  
Scattered Light ◽  
Atmospheric Composition ◽  
Optical Absorption Spectroscopy ◽  
Total Ozone Column ◽  
Global Comparison ◽  
Percentage Difference ◽  
The Mean ◽  
Ozone Column

&lt;p&gt;The Sentinel-5 Precursor (S5P) mission, launched in October 2017, carries the TROPOspheric Monitoring Instrument (TROPOMI), which provides a daily global coverage at a spatial resolution as high as 5.5 km x 3.5 km and will extend the European atmospheric composition record initiated with GOME/ERS-2 in 1995. Due to the ongoing need to understand and monitor the recovery of the ozone layer, as well as the evolution of tropospheric pollution, ozone remains one of the leading species of interest during this mission.&lt;/p&gt;&lt;p&gt;In this work, two and a half years of TROPOMI near real time (NRTI) and offline (OFFL) total ozone column (TOC) products are presented and compared to daily and individual, globally distributed, ground-based quality assured Brewer and Dobson TOC measurements. The daily ground-based ozone measurements used here are deposited in the World Ozone and Ultraviolet Radiation Data Centre (WOUDC). The individual Brewer measurements are made available by the European Brewer Network (Eubrewnet). Furthermore, twilight zenith-sky measurements obtained with ZSL-DOAS (Zenith Scattered Light Differential Optical Absorption Spectroscopy) instruments, which form part of the SAOZ network (Syst&amp;#232;me d&amp;#8217;Analyse par Observation Z&amp;#233;nitale), are used for the validation.&lt;/p&gt;&lt;p&gt;The quality of the TROPOMI TOC data is evaluated in terms of the influence of various geophysical quantities such as location, solar zenith angle, viewing angle, season, effective temperature, surface albedo and clouds. The overall statistical analysis of the global comparison shows that the mean bias and the mean standard deviation of the percentage difference between TROPOMI and ground-based TOC is within 0 &amp;#8211;1.5% and 2.5 %&amp;#8211;4.5 %, respectively. Moreover, based on the full available dataset, a first attempt is made for a drift investigation.&lt;/p&gt;&lt;p&gt;Additionally, the TROPOMI OFFL and NRTI products are evaluated against already known spaceborne sensors, namely, the Ozone Mapping Profiler Suite, on board the Suomi National Polar-orbiting Partnership (OMPS/Suomi-NPP), NASA, and the Global Ozone Monitoring Experiment 2 (GOME-2), on board the Metop-A (GOME-2/Metop-A) and Metop-B (GOME-2/Metop-B) satellites. This analysis shows a very good agreement for both TROPOMI products with well-established instruments, with the absolute differences in mean bias and mean standard deviation being below +0.7% and 1%, respectively.&lt;/p&gt;

scholarly journals Symptoms of total ozone recovery inside the Antarctic vortex during Austral spring

2017 ◽  
Author(s):  
Andrea Pazmino ◽  
Sophie Godin-Beekmann ◽  
Alain Hauchecorne ◽  
Chantal Claud ◽  
Sergey Khaykin ◽  
...  
Keyword(s):  
Total Ozone ◽  
Ozone Hole ◽  
Polar Regions ◽  
Multilinear Regression ◽  
Austral Spring ◽  
Quasi Biennial Oscillation ◽  
Total Ozone Column ◽  
The Antarctic ◽  
Ozone Column ◽  
Mlr Model

Abstract. The long-term evolution of total ozone column inside the Antarctic polar vortex is investigated over the 1980–2016 period. Trend analyses are performed using a multilinear regression (MLR) model based on various proxies (heat flux, Quasi-Biennial Oscillation, solar flux, Antarctic Oscillation and aerosols). Annual total ozone column corresponding to the mean monthly values inside the vortex in September and during the period of maximum ozone depletion from September 15th to October 15th are used. Total ozone columns from combined SBUV, TOMS and OMI satellite datasets and the Multi-Sensor Reanalysis (MSR-2) dataset are considered in the study. Ozone trends are computed by a piecewise trend model (PWT) before and after the turnaround in 2001. In order to evaluate total ozone within the vortex, two classification methods are used, based on the potential vorticity gradient as a function of equivalent latitude. The first standard one considers this gradient at a single isentropic level (475 K or 550 K), while the second one uses a range of isentropic levels between 400 K and 600 K. The regression model includes a new proxy that represents the stability of the vortex during the studied month period. The determination coefficient (R2) between observations and modeled values increases by ~ 0.05 when this proxy is included in the MLR model. The higher R2 (0.93–0.95) and the minimum residuals are observed for the second classification method for both datasets and months periods. Trends in September are statistically significant at 2 sigma level over 2001–2016 period with values ranging between 1.85 and 2.67 DU yr−1 depending on the methods and data sets. This result confirms the recent studies of Antarctic ozone healing during that month. Trends after 2001 are 2 to 3 times lower than before the turnaround year as expected from the response to the slowly ozone-depleting substances decrease in Polar regions. Estimated trends in the 15 Sept–15 Oct period are smaller than in September. They vary from 1.15 to 1.78 DU yr−1 and are hardly significant at 2σ level. Ozone recovery is also confirmed by a steady decrease of the relative area of total ozone values lower than 150 DU within the vortex in the 15 Sept–15 Oct period since 2010. Comparison of the evolution of the ozone hole area in September and October shows a decrease in September, confirming the later formation of the ozone hole during that month.

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