scholarly journals Implications of sea-ice biogeochemistry for oceanic production and emissions of dimethylsulfide in the Arctic

2016 ◽  
Author(s):  
Hakase Hayashida ◽  
Nadja Steiner ◽  
Adam Monahan ◽  
Virginie Galindo ◽  
Martine Lizotte ◽  
...  

Abstract. Sea ice represents an additional oceanic source of the climatically active gas dimethylsulfide (DMS) for the Arctic atmosphere. To what extent this source contributes to the dynamics of summertime Arctic clouds is however not known due to scarcity of field measurements. In this study, we developed a coupled sea ice-ocean ecosystem-sulfur cycle model to investigate the potential impact of bottom-ice DMS and its precursor dimethylsulfoniopropionate (DMSP) on the oceanic production and emission of DMS in the Arctic. The result of the 1-D model simulation was compared with field data collected during May and June of 2010 in Resolute Passage. Our result reproduced the accumulation of DMS and DMSP in the bottom ice during the development of an ice algal bloom. The flushing of these sulfur species took place predominantly during the earlier phase of the melt period, resulting in an increase of DMS and DMSP in the underlying water column prior to the onset of an under-ice phytoplankton bloom. Processes that dominated the budgets of bottom- and under-ice DMS and DMSP were identified through an analysis of production and removal rates of processes considered in the model. When openings in the ice were taken into account, the simulated sea-air DMS flux during the melt period was dominated by episodic spikes of up to 5.6 μmol m−2 d−1. Further model simulations were conducted to assess the effects of the incorporation of sea-ice biogeochemistry on DMS production and emissions, as well as the sensitivity of our results to changes of uncertain model parameters of the sea-ice sulfur cycle. The results highlight the importance of taking into account both the sea-ice sulfur cycle and ecosystem in the flux estimates of oceanic DMS near the ice margins and identify key uncertainties in processes and rates that would be better constrained by new observations.

2017 ◽  
Vol 14 (12) ◽  
pp. 3129-3155 ◽  
Author(s):  
Hakase Hayashida ◽  
Nadja Steiner ◽  
Adam Monahan ◽  
Virginie Galindo ◽  
Martine Lizotte ◽  
...  

Abstract. Sea ice represents an additional oceanic source of the climatically active gas dimethyl sulfide (DMS) for the Arctic atmosphere. To what extent this source contributes to the dynamics of summertime Arctic clouds is, however, not known due to scarcity of field measurements. In this study, we developed a coupled sea ice–ocean ecosystem–sulfur cycle model to investigate the potential impact of bottom-ice DMS and its precursor dimethylsulfoniopropionate (DMSP) on the oceanic production and emissions of DMS in the Arctic. The results of the 1-D model simulation were compared with field data collected during May and June of 2010 in Resolute Passage. Our results reproduced the accumulation of DMS and DMSP in the bottom ice during the development of an ice algal bloom. The release of these sulfur species took place predominantly during the earlier phase of the melt period, resulting in an increase of DMS and DMSP in the underlying water column prior to the onset of an under-ice phytoplankton bloom. Production and removal rates of processes considered in the model are analyzed to identify the processes dominating the budgets of DMS and DMSP both in the bottom ice and the underlying water column. When openings in the ice were taken into account, the simulated sea–air DMS flux during the melt period was dominated by episodic spikes of up to 8.1 µmol m−2 d−1. Further model simulations were conducted to assess the effects of the incorporation of sea-ice biogeochemistry on DMS production and emissions, as well as the sensitivity of our results to changes of uncertain model parameters of the sea-ice sulfur cycle. The results highlight the importance of taking into account both the sea-ice sulfur cycle and ecosystem in the flux estimates of oceanic DMS near the ice margins and identify key uncertainties in processes and rates that should be better constrained by new observations.


2008 ◽  
Vol 21 (5) ◽  
pp. 866-882 ◽  
Author(s):  
Irina V. Gorodetskaya ◽  
L-Bruno Tremblay ◽  
Beate Liepert ◽  
Mark A. Cane ◽  
Richard I. Cullather

Abstract The impact of Arctic sea ice concentrations, surface albedo, cloud fraction, and cloud ice and liquid water paths on the surface shortwave (SW) radiation budget is analyzed in the twentieth-century simulations of three coupled models participating in the Intergovernmental Panel on Climate Change Fourth Assessment Report. The models are the Goddard Institute for Space Studies Model E-R (GISS-ER), the Met Office Third Hadley Centre Coupled Ocean–Atmosphere GCM (UKMO HadCM3), and the National Center for Atmosphere Research Community Climate System Model, version 3 (NCAR CCSM3). In agreement with observations, the models all have high Arctic mean cloud fractions in summer; however, large differences are found in the cloud ice and liquid water contents. The simulated Arctic clouds of CCSM3 have the highest liquid water content, greatly exceeding the values observed during the Surface Heat Budget of the Arctic Ocean (SHEBA) campaign. Both GISS-ER and HadCM3 lack liquid water and have excessive ice amounts in Arctic clouds compared to SHEBA observations. In CCSM3, the high surface albedo and strong cloud SW radiative forcing both significantly decrease the amount of SW radiation absorbed by the Arctic Ocean surface during the summer. In the GISS-ER and HadCM3 models, the surface and cloud effects compensate one another: GISS-ER has both a higher summer surface albedo and a larger surface incoming SW flux when compared to HadCM3. Because of the differences in the models’ cloud and surface properties, the Arctic Ocean surface gains about 20% and 40% more solar energy during the melt period in the GISS-ER and HadCM3 models, respectively, compared to CCSM3. In twenty-first-century climate runs, discrepancies in the surface net SW flux partly explain the range in the models’ sea ice area changes. Substantial decrease in sea ice area simulated during the twenty-first century in CCSM3 is associated with a large drop in surface albedo that is only partly compensated by increased cloud SW forcing. In this model, an initially high cloud liquid water content reduces the effect of the increase in cloud fraction and cloud liquid water on the cloud optical thickness, limiting the ability of clouds to compensate for the large surface albedo decrease. In HadCM3 and GISS-ER, the compensation of the surface albedo and cloud SW forcing results in negligible changes in the net SW flux and is one of the factors explaining moderate future sea ice area trends. Thus, model representations of cloud properties for today’s climate determine the ability of clouds to compensate for the effect of surface albedo decrease on the future shortwave radiative budget of the Arctic Ocean and, as a consequence, the sea ice mass balance.


2007 ◽  
Vol 34 (17) ◽  
Author(s):  
E. Sokolova ◽  
K. Dethloff ◽  
A. Rinke ◽  
A. Benkel

2014 ◽  
Vol 14 (21) ◽  
pp. 28949-28972 ◽  
Author(s):  
J. D. Allan ◽  
P. I. Williams ◽  
J. Najera ◽  
J. D. Whitehead ◽  
M. J. Flynn ◽  
...  

Abstract. Accurately accounting for new particle formation (NPF) is crucial to our ability to predict aerosol number concentrations and thus cloud properties, which is in turn vital in simulating radiative transfer and climate. Here we present an analysis of NPF events observed in the Greenland Sea during the summertime as part of the Aerosol-Cloud Coupling And Climate Interactions in the Arctic (ACCACIA) project. While NPF events have been reported in the Arctic before, we were able, for the first time, to detect iodine in the growing particles using an Aerosol Mass Spectrometer (AMS) during a persistent event in the region of the coastal sea ice near Greenland. Given the potency of iodine as a nucleation precursor, the results imply that iodine was responsible for the initial NPF, a phenomenon that has been reported at lower latitudes and associated with molecular iodine emissions from coastal macroalgae. The initial source of iodine in this instance is not clear, but it was associated with air originating approximately 1 day previously over melting coastal sea ice. These results show that atmospheric models must consider iodine as a source of new particles in addition to established precursors such as sulphur compounds.


2017 ◽  
Author(s):  
Ki-Tae Park ◽  
Sehyun Jang ◽  
Kitack Lee ◽  
Young Jun Yoon ◽  
Min-Seob Kim ◽  
...  

Abstract. The connection between marine biogenic dimethyl sulfide (DMS) and the formation of aerosol particles in the Arctic atmosphere was evaluated by analyzing atmospheric DMS mixing ratios, aerosol particle size distributions and aerosol chemical composition data that were concurrently collected at Ny-Ålesund, Svalbard (78.5° N, 11.8° E) during April and May 2015. Measurements of aerosol sulfur (S) compounds showed distinct patterns during periods of Arctic haze (April) and phytoplankton blooms (May). Specifically, during the phytoplankton bloom period the contribution of DMS-derived SO42− to the total aerosol SO42− increased by 7-fold compared with that during the proceeding Arctic haze period, accounting for up to 70 % of fine SO42− particles (


2019 ◽  
Vol 53 (11) ◽  
pp. 7113-7130
Author(s):  
Takahiro Toyoda ◽  
Katsushi Iwamoto ◽  
L. Shogo Urakawa ◽  
Hiroyuki Tsujino ◽  
Hideyuki Nakano ◽  
...  

Abstract The presence of thin sea ice is indicative of active freezing conditions in the polar ocean. We propose a simple yet effective method to incorporate information of thin-ice category into coupled ocean–sea-ice model simulations. In our approach, the thin-ice distribution restricts thick-ice extent and constrains atmosphere–ocean heat exchange through the sea ice. Our model simulation with the incorporation of satellite-derived thin-ice data for the Arctic Ocean showed much improved representation of sea-ice and upper-ocean fields, including sea-ice thickness in the Canadian Archipelago and the region north of Greenland, mixed-layer depth over the Central Arctic, and surface-layer salinity over the open ocean. Enhanced sea-ice production by the thin-ice data constraint increased the total sea-ice volume of the Arctic Ocean by $$5 \times 10^{3}$$ 5 × 10 3 –$$10 \times 10^{3}$$ 10 × 10 3  km3. Subsequent sea-ice melting was also enhanced, leading to the greater amplitude of the seasonal cycle by approximately $$2 \times 10^{3}$$ 2 × 10 3  km3 (15% of the baseline value from the experiment without the thin-ice data incorporation). Overall, our results demonstrate that the incorporation of satellite-derived information on thin sea ice has great potential for the improvement of coupled ocean–sea-ice simulations.


1984 ◽  
Vol 5 ◽  
pp. 170-176 ◽  
Author(s):  
John E. Walsh ◽  
William D. Hibler ◽  
Becky Ross

A dynamic-thermodynamic sea-ice model (Hibler 1979) is used to simulate northern hemisphere sea ice for a 20-year period, 1961 to 1980. The model is driven by daily atmospheric grids of sea-level pressure (geo-strophic wind) and by temperatures derived from the Russian surface temperature data set. Among the modifications to earlier formulations are the inclusion of snow cover and a multilevel ice-thickness distribution in the thermodynamic computations.The time series of the simulated anomalies show relatively large amounts of ice during the early 1960s and middle 1970s, and relatively small amounts during the late 1960s and early 1970s. The fluctuations of ice mass, both in the entire domain and in individual regions, are more persistent than are the fluctuations of ice-covered area. The ice dynamics tend to introduce more high-frequency variability into the regional (and total) amounts of ice mass. The simulated annual ice export from the Arctic Basin into the East Greenland Sea varies interannually by factors of 3 to 4.


2016 ◽  
Vol 97 (11) ◽  
pp. 2163-2176 ◽  
Author(s):  
Abhay Devasthale ◽  
Joseph Sedlar ◽  
Brian H. Kahn ◽  
Michael Tjernström ◽  
Eric J. Fetzer ◽  
...  

Abstract Arctic sea ice is declining rapidly and its annual ice extent minima reached record lows twice during the last decade. Large environmental and socioeconomic implications related to sea ice reduction in a warming world necessitate realistic simulations of the Arctic climate system, not least to formulate relevant environmental policies on an international scale. However, despite considerable progress in the last few decades, future climate projections from numerical models still exhibit the largest uncertainties over the polar regions. The lack of sufficient observations of essential climate variables is partly to blame for the poor representation of key atmospheric processes, and their coupling to the surface, in climate models. Observations from the hyperspectral Atmospheric Infrared Sounder (AIRS) instrument on board the National Aeronautics and Space Administration (NASA)’s Aqua satellite are contributing toward improved understanding of the vertical structure of the atmosphere over the poles since 2002, including the lower troposphere. This part of the atmosphere is especially important in the Arctic, as it directly impacts sea ice and its short-term variability. Although in situ measurements provide invaluable ground truth, they are spatially and temporally inhomogeneous and sporadic over the Arctic. A growing number of studies are exploiting AIRS data to investigate the thermodynamic structure of the Arctic atmosphere, with applications ranging from understanding processes to deriving climatologies—all of which are also useful to test and improve parameterizations in climate models. As the AIRS data record now extends more than a decade, a select few of many such noteworthy applications of AIRS data over this challenging and rapidly changing landscape are highlighted here.


1990 ◽  
Vol 14 ◽  
pp. 339-339
Author(s):  
W.D Hibler ◽  
Peter Ranelli

Sea-ice drift and dynamics can significantly affect the exchanges of heat between the atmosphere and ocean and salt fluxes into the ocean. The ice drift and dynamics, in turn, can be modified by the ocean circulation. This is especially true of the ice margin location whose seasonal characteristics are largely controlled by the substantial oceanic heat flux in the Greenland Sea due to convective overturning.A useful framework to analyze the interannual variability of ice–ocean interaction effects relevant to climatic change is the diagnostic ice–ocean model developed by Hibler and Bryan (1987). In this model, the oceanic temperature and salinity is weakly relaxed (except in the upper layer of the ocean which is essentially driven by the ice dynamic-thermodynamic sea-ice model) to climatological temperature and salinity data. This procedure allows seasonal and interannual variability to be simulated while still preventing the baroclinic characteristics of the ocean circulation from gradually drifting off into a total model defined state. However, in the work of Hibler and Bryan only the seasonal equilibrium characteristics of this model with the same forcing repeated year after year have been considered.In order to begin to examine the interannual behavior of this model, we have carried out a three-year simulation for the Arctic Greenland and Norwegian seas over the time period 1981–83. (The geographical region is essentially the same as used by Hibler and Bryan.) This three year simulation is carried out after an initial two year spin up using the 1981 atmospheric forcing data. For comparison purposes, an ice model simulation with only a fixed depth mixed layer was also carried out over this time interval.The results of these two simulations are analyzed with special attention to the ice margin characteristics in the Greenland and Norwegian seas to determine the role of ocean circulation on the variability there. The ice margin results are also compared to the variability in the northward transports of heat through the Faero-Shetland passage which in the fully-coupled model are calculated rather than specified.


2010 ◽  
Vol 10 (11) ◽  
pp. 28859-28908 ◽  
Author(s):  
H. Struthers ◽  
A. M. L. Ekman ◽  
P. Glantz ◽  
T. Iversen ◽  
A. Kirkevåg ◽  
...  

Abstract. Understanding Arctic climate change requires knowledge of both the external and the local drivers of Arctic climate as well as local feedbacks within the system. An Arctic feedback mechanism relating changes in sea ice extent to an alteration of the emission of sea salt aerosol and the consequent change in radiative balance is examined. A set of idealized climate model simulations were performed to quantify the radiative effects of changes in sea salt aerosol emissions induced by prescribed changes in sea ice extent. The model was forced using sea ice concentrations consistent with present day conditions and projections of sea ice extent for 2100. Sea salt aerosol emissions increase in response to a decrease in sea ice, the model results showing an annual average increase in number emission over the polar cap (70–90° N) of 86×106 m−2 s−1 (mass emission increase of 23 μg m−2 s−1). This in turn leads to an increase in the natural aerosol optical depth of approximately 23%. In response to changes in aerosol optical depth, the natural component of the aerosol direct forcing over the Arctic polar cap is estimated to be between −0.2 and −0.4 W m−2 for the summer months, which results in a negative feedback on the system. The model predicts that the change in first indirect aerosol effect (cloud albedo effect) is approximately a factor of ten greater than the change in direct aerosol forcing although this result is highly uncertain due to the crude representation of Arctic clouds and aerosol-cloud interactions in the model. This study shows that both the natural aerosol direct and first indirect effects are strongly dependent on the surface albedo, highlighting the strong coupling between sea ice, aerosols, Arctic clouds and their radiative effects.


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