scholarly journals Shipborne lidar measurements showing the progression of the tropical reservoir of volcanic aerosol after the June 1991 Pinatubo eruption

2020 ◽  
Vol 12 (4) ◽  
pp. 2843-2851
Author(s):  
Juan-Carlos Antuña-Marrero ◽  
Graham W. Mann ◽  
Philippe Keckhut ◽  
Sergey Avdyushin ◽  
Bruno Nardi ◽  
...  
Keyword(s):  
Lower Layer ◽  
Extinction Ratio ◽  
Stratospheric Aerosol ◽  
Aerosol Extinction ◽  
Volcanic Aerosol ◽  
Tropical Reservoir ◽  
Aerosol Cloud ◽  
Pinatubo Eruption ◽  
The Tropics ◽  
Aerosol Backscatter

Abstract. A key limitation of volcanic forcing datasets for the Pinatubo period is the large uncertainty that remains with respect to the extent of the optical depth of the Pinatubo aerosol cloud in the first year after the eruption, the saturation of the SAGE-II instrument restricting it to only be able to measure the upper part of the aerosol cloud in the tropics. Here we report the recovery of stratospheric aerosol measurements from two shipborne lidars, both of which measured the tropical reservoir of volcanic aerosol produced by the June 1991 Mount Pinatubo eruption. The lidars were on board two Soviet vessels, each ship crossing the Atlantic, their measurement datasets providing unique observational transects of the Pinatubo cloud across the tropics from Europe to the Caribbean (∼ 40 to 8∘ N) from July to September 1991 (the Professor Zubov ship) and from Europe to south of the Equator (∼ 40∘ N to 8∘ S) between January and February 1992 (the Professor Vize ship). Our philosophy with the data recovery is to follow the same algorithms and parameters that appear in the two peer-reviewed articles that presented these datasets in the same issue of GRL in 1993, and here we provide all 48 lidar soundings made from the Professor Zubov and 11 of the 20 conducted from the Professor Vize, ensuring we have reproduced the aerosol backscatter and extinction values in the figures of those two papers. These original approaches used thermodynamic properties from the CIRA-86 standard atmosphere to derive the molecular backscattering, vertically and temporally constant values applied for the aerosol backscatter-to-extinction ratio, and the correction factor of the aerosol backscatter wavelength dependence. We demonstrate this initial validation of the recovered stratospheric aerosol extinction profiles, providing full details of each dataset in this paper's Supplement S1, the original profiles of backscatter ratio, and the calculated profiles of aerosol backscatter and extinction. We anticipate these datasets will provide potentially important new observational case studies for modelling analyses, including a 1-week series of consecutive soundings (in September 1991) at the same location showing the progression of the entrainment of part of the Pinatubo plume into the upper troposphere and the formation of an associated cirrus cloud. The Zubov lidar dataset illustrates how the tropically confined Pinatubo aerosol cloud transformed from a highly heterogeneous vertical structure in August 1991, maximum aerosol extinction values around 19 km for the lower layer and 23–24 for the upper layer, to a more homogeneous and deeper reservoir of volcanic aerosol in September 1991. We encourage modelling groups to consider new analyses of the Pinatubo cloud, comparing the recovered datasets, with the potential to increase our understanding of the evolution of the Pinatubo aerosol cloud and its effects. Data described in this work are available at https://doi.org/10.1594/PANGAEA.912770 (Antuña-Marrero et al., 2020).

scholarly journals Ship-borne lidar measurements showing the progression of the tropical reservoir of volcanic aerosol after the June 1991 Pinatubo eruption

2020 ◽  
Author(s):  
Juan-Carlos Antuña-Marrero ◽  
Graham W. Mann ◽  
Philippe Keckhut ◽  
Sergey Avdyushin ◽  
Bruno Nardi ◽  
...  
Keyword(s):  
Lower Layer ◽  
Extinction Ratio ◽  
Stratospheric Aerosol ◽  
Original Text ◽  
Aerosol Extinction ◽  
Volcanic Aerosol ◽  
Tropical Reservoir ◽  
Aerosol Cloud ◽  
Pinatubo Eruption ◽  
The Tropics

Abstract. A key limitation of volcanic forcing datasets for the Pinatubo period, is the large uncertainty that remains with respect to the extent of the optical depth of the Pinatubo aerosol cloud in the first year after the eruption, the saturation of the SAGE-II instrument restricting it to only be able to measure the upper part of the aerosol cloud in the tropics. Here we report the recovery of stratospheric aerosol measurements from two ship-borne lidars, both of which measured the tropical reservoir of volcanic aerosol produced by the June 1991 Mount Pinatubo eruption. The lidars were on-board two Soviet vessels, each ship crossing the Atlantic, their measurement datasets providing unique observational transects of the Pinatubo cloud across the tropics from Europe to the Caribbean (~ 40° N to 8° N) from July to September 1991 (the Prof Zubov ship) and from Europe to south of the Equator (8° S to ~ 40° N) between January and February 1992 (the Prof Vize ship). Our philosophy with the data recovery is to follow the same algorithms and parameters appearing in the two peer-reviewed articles that presented these datasets in the same issue of GRL in 1993, and here we provide all 48 lidar soundings made from the Prof. Zubov, and 11 of the 20 conducted from the Prof. Vize, ensuring we have reproduced the aerosols backscatter and extinction values in the Figures of those two papers. These original approaches used thermodynamic properties from the CIRA-86 standard atmosphere to derive the molecular backscattering, vertically and temporally constant values applied for the aerosol backscatter to extinction ratio and the correction factor of the aerosols backscattering wavelength dependence. We demonstrate this initial validation of the recovered stratospheric aerosol extinction profiles, providing full details of each dataset in this paper's Supplement S1, the original text files of the backscatter ratio, the calculated aerosols backscatter and extinction profiles. We anticipate the data providing potential new observational case studies for modelling analyses, including a 1-week series of consecutive soundings (in September 1991) at the same location showing the progression of the entrainment of part of the Pinatubo plume into the upper troposphere and the formation of an associated cirrus cloud. The Zubov lidar dataset illustrates how the tropically confined Pinatubo aerosol cloud transformed from a highly heterogeneous vertical structure in August 1991, maximum aerosol extinction values around 19 km for the lower layer and 23–24 for the upper layer, to a more homogeneous and deeper reservoir of volcanic aerosol in September 1991. We encourage modelling groups to consider new analyses of the Pinatubo cloud, comparing to the recovered datasets, with the potential to increase our understanding of the evolution of the Pinatubo aerosol cloud and its effects. Data described in this work are available at https://doi.pangaea.de/10.1594/PANGAEA.912770 (Antuña-Marrero et al., 2020).

Interactive Stratospheric Aerosol models response to different sulfur injection amount and altitude distribution during volcanic eruption

2021 ◽  
Author(s):  
Ilaria Quaglia ◽  
Christoph Brühl ◽  
Sandip Dhomse ◽  
Henning Franke ◽  
Anton Laakso ◽  
...  
Keyword(s):  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Climate Modelling ◽  
Aerosol Layer ◽  
Volcanic Aerosol ◽  
Surface Cooling ◽  
Altitude Distribution ◽  
Aerosol Cloud ◽  
Modelling Studies ◽  
Intercomparison Project

<p>Large magnitude tropical volcanic eruptions emit sulphur dioxide and other gases directly into the stratosphere, creating a long-lived volcanic aerosol cloud which scatter incoming solar radiation, absorbs outgoing terrestrial radiation, and can strongly affect the composition of the stratosphere.</p><p>Such major volcanic enhancements of the stratospheric aerosol layer have strong “direct effects” on climate via these influences on radiative transfer, primarily surface cooling via the reduced insolation, but also have a range of indirect effects, due to the volcanic aerosol cloud’s effects on stratospheric circulation, dynamics and chemistry.</p><p>In this study, we investigate the 3 largest volcanic enhancements to the stratospheric aerosol layer in the last 100 years (Mt Agung 1963; Mt El Chichón 1982; Mt Pinatubo 1991), comparing co-ordinated simulations within the so-called HErSEA experiments (Historical Eruptions SO2 Emission Assessment) several national climate modelling centres carried out for the model intercomparison project ISA-MIP.</p><p>The HErSEA experiment saw participating models performing interactive stratospheric aerosol simulations of each of the volcanic aerosol clouds with common upper-, mid- and lower-estimate amounts and injection heights of sulfur dioxide, in order to better understand known differences among modelling studies for which initial emission gives best agreement with observations. </p><p>First, we compare results of several models HErSEA simulations with a range of observations, with the aim to find where there is agreement between the models and where there are differences, at the different initial sulfur injection amount and altitude distribution.</p><p>In this way, we could understand the differences and limitations in the mechanisms that controls the dynamical, microphysical and chemical processes of stratospheric aerosol layer.</p>

scholarly journals Evaluation of a method for converting Stratospheric Aerosol and Gas Experiment (SAGE) extinction coefficients to backscatter coefficients for intercomparison with lidar observations

2020 ◽  
Vol 13 (8) ◽  
pp. 4261-4276
Author(s):  
Travis N. Knepp ◽  
Larry Thomason ◽  
Marilee Roell ◽  
Robert Damadeo ◽  
Kevin Leavor ◽  
...  
Keyword(s):  
Stratospheric Aerosol ◽  
Aerosol Extinction ◽  
Extinction Coefficients ◽  
Mauna Loa ◽  
Quiescent Period ◽  
Table Mountain ◽  
Ground Based Lidar ◽  
Aerosol Backscatter ◽  
Lidar Observations ◽  
Major Eruption

Abstract. Aerosol backscatter coefficients were calculated using multiwavelength aerosol extinction products from the SAGE II and III/ISS instruments (SAGE: Stratospheric Aerosol and Gas Experiment). The conversion methodology is presented, followed by an evaluation of the conversion algorithm's robustness. The SAGE-based backscatter products were compared to backscatter coefficients derived from ground-based lidar at three sites (Table Mountain Facility, Mauna Loa, and Observatoire de Haute-Provence). Further, the SAGE-derived lidar ratios were compared to values from previous balloon and theoretical studies. This evaluation includes the major eruption of Mt. Pinatubo in 1991, followed by the atmospherically quiescent period beginning in the late 1990s. Recommendations are made regarding the use of this method for evaluation of aerosol extinction profiles collected using the occultation method.

scholarly journals Impact of the eruption of Mt Pinatubo on the chemical composition of the stratosphere

2020 ◽  
Vol 20 (20) ◽  
pp. 11697-11715
Author(s):  
Markus Kilian ◽  
Sabine Brinkop ◽  
Patrick Jöckel
Keyword(s):  
Chemical Composition ◽  
Atmospheric Chemistry ◽  
Chemical Effect ◽  
Heterogeneous Chemistry ◽  
Volcanic Aerosol ◽  
Heating Effect ◽  
Subsequent Decrease ◽  
Pinatubo Eruption ◽  
The Tropics ◽  
Ozone Column

Abstract. This article describes the volcanic effect of the Mt Pinatubo eruption in June 1991 on the ozone (O3) and methane (CH4) distribution in the stratosphere, as simulated with the chemistry–climate model EMAC (ECHAM/MESSy Atmospheric Chemistry: ECHAM5, version 5.3.02; MESSy, version 2.51). In this study, the effects of volcanic heating and heterogeneous chemistry on the chemical composition, caused by the volcanic aerosol, are separated. Global model simulations over the relevant period of the eruption from 1989 to 1997 with EMAC in T42L90MA resolution with specified dynamics and interactive chemistry were performed. The first simulation (VOL) contains the volcanic perturbation as an additional aerosol load and thus simulates the interaction of the aerosol with the chemistry and the radiation. The second simulation (NOVOL) neglects the eruption and represents the undisturbed atmosphere. In the third simulation (CVOL) the volcanic aerosol only interacts with the heterogeneous chemistry, such that volcanic heating is omitted. The differences between the simulation results VOL−NOVOL describe the total effect of the Mt Pinatubo eruption on the chemical composition, VOL−CVOL the stratospheric heating effect, and CVOL−NOVOL the chemical effect of the aerosol on the heterogeneous chemistry. The post-volcanic stratosphere shows a decrease in the O3 column in the tropics and an increase in the midlatitudes and polar regions, lasting roughly 1 year. This change in the ozone column is solely a result of the heating effect. The subsequent decrease in the ozone column is related to the chemical effect. The contribution of the catalytic loss cycles (NOx, HOx, ClOx, and BrOx) on the depletion of O3 is analysed in detail. In the tropics, CH4 increases in the upper stratosphere because of stronger vertical transport.

Long-lived ultra-fine ash particles within the Pinatubo volcanic aerosol cloud and their potential impact on its global dispersion and radiative forcings

2021 ◽  
Author(s):  
Sarah Shallcross ◽  
Graham Mann ◽  
Anja Schmidt ◽  
Jim Haywood ◽  
Frances Beckett ◽  
...  
Keyword(s):  
Vertical Profile ◽  
Climate Model ◽  
Airborne Lidar ◽  
Radiative Heating ◽  
Volcanic Plume ◽  
Volcanic Aerosol ◽  
Mount Pinatubo ◽  
Aerosol Cloud ◽  
Pinatubo Eruption ◽  
Volcanic Cloud

<p>Volcanic aerosol simulations with interactive stratospheric aerosol models mostly neglect ash particles, due to a general assumption they sediment out of the volcanic plume within the first few weeks and have limited impacts on the progression of the volcanic aerosol cloud (Niemeier et al., 2009). </p> <p>However, observations, such as ground-based and airborne lidar (Vaughan et al., 1994; Browell et al., 1993), along with impactor measurements (Pueschel et al., 1994) in the months after the Mount Pinatubo eruption suggest the base of the aerosol cloud contained ash particles coated in sulphuric acid for around 9 months after the eruption occurred.  Impactor measurements from flights following the 1963 Agung and 1982 El Chichon eruptions also show ash remained present for many months after the eruption (Mossop, 1964; Gooding et al., 1983).  <br /><br />More recently, satellite, in situ and optical particle counter measurements after the 2014 Mount Kelud eruption showed ash particles ~0.3 µm in size accounting for 20-28% of the volcanic cloud AOD 3 months following the eruption (Vernier et al., 2016; Deshler, 2016).  This evidence suggests that sub-micron ash particles may persist for longer in the atmosphere than is often assumed. </p> <p>We explore how the presence of these sub-micron ash particles affects the progression of a major tropical volcanic aerosol cloud, showing results from simulations with a new configuration of the composition-climate model UM-UKCA, adapted to co-emit fine-ash alongside SO2.   In the UM-UKCA simulations, internally mixed ash-sulphuric particles are transported within the existing coarse-insoluble mode of the GLOMAP-mode aerosol scheme. <br /><br />Size fractions of 0.1, 0.316 and 1 µm diameter ash were tested for the 1991 Mount Pinatubo eruption with an ultra-fine ash mass co-emission of 0.05 and 0.5 Tg, based on 0.1% and 1% of an assumed fine ash emission of 50Tg.  Whereas the 0.316 and 1 µm sized particles sedimented out of the stratosphere within the first 90 days after the eruption, the 0.1 µm persisted within the lower portion of volcanic cloud for ~9 months,  retaining over half its original mass (0.035 Tg) February 1992. </p> <p>We investigate model experiments with different injection heights for the co-emitted SO2 and ash, analysing the vertical profile of the ultra-fine ash compared to the sulphate aerosol, and explore the effects on the volcanic aerosol cloud in terms of its overall optical depth and vertical profile of extinction.</p> <p>The analysis demonstrates that although fine-ash is more persistent than previous modelling studies suggest, these particles have only modest impacts with the radiative heating effect the dominant pathway, with the sub-micron particles not scavenging sufficiently.  </p> <p>Future work will explore simulations with a further adapted UM-UKCA model with an additional “super-coarse” insoluble mode resolving the super-micron ash, then both components of the fine-ash resolved to test the magnitude of sulfate scavenging effect. </p>

scholarly journals CALIPSO observations of stratospheric aerosols: a preliminary assessment

2007 ◽  
Vol 7 (20) ◽  
pp. 5283-5290 ◽  
Author(s):  
L. W. Thomason ◽  
M. C. Pitts ◽  
D. M. Winker
Keyword(s):  
Stratospheric Aerosol ◽  
Backscatter Coefficient ◽  
Volcanic Plumes ◽  
Aerosol Distribution ◽  
The Difference ◽  
The Tropics ◽  
Lidar Calibration ◽  
Aerosol Backscatter ◽  
532 Nm ◽  
2006 Eruption

Abstract. We have examined the 532-nm aerosol backscatter coefficient measurements by the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) for their use in the monitoring of stratospheric aerosol. CALIPSO makes observations that span from 82° S to 82° N each day and, for each profile, backscatter coefficient values reported up to ~40 km. The possibility of using CALIPSO for stratospheric aerosol monitoring is demonstrated by the clear observation of the 20 May 2006 eruption of Montserrat in the earliest CALIPSO data in early June as well as by observations showing the 7 October 2006 eruption of Tavurvur (Rabaul). However, the very low aerosol loading within the stratosphere makes routine observations of the stratospheric aerosol far more difficult than relatively dense volcanic plumes. Nonetheless, we found that averaging a complete days worth of nighttime-only data into 5-deg latitude by 1-km vertical bins yields a stratospheric aerosol distribution that is fairly consistent with past measurements by spaceborne instruments. Based on comparisons with 2004 data from the Stratospheric Aerosol and Gas Experiment, the derived values are close to expectation except in the tropics where they are larger by about a factor of 2. The cause of the difference in the tropics is not readily apparent but is most likely related to difficulties in the lidar calibration process currently found in the CALIOP data at tropical latitudes.

scholarly journals Comparison of aerosol extinction between lidar and SAGE II over Gadanki, a tropical station in India

2015 ◽  
Vol 33 (3) ◽  
pp. 351-362 ◽  
Author(s):  
P. Kulkarni ◽  
S. Ramachandran
Keyword(s):  
Meteorological Parameters ◽  
Lower Stratosphere ◽  
Stratospheric Aerosol ◽  
Lidar Measurement ◽  
Aerosol Extinction ◽  
Upper Troposphere ◽  
Measurement Site ◽  
Space And Time ◽  
The Tropics ◽  
Tropical Station

Abstract. An extensive comparison of aerosol extinction has been performed using lidar and Stratospheric Aerosol and Gas Experiment (SAGE) II data over Gadanki (13.5° N, 79.2° E), a tropical station in India, following coincident criteria during volcanically quiescent conditions from 1998 to 2005. The aerosol extinctions derived from lidar are higher than SAGE II during all seasons in the upper troposphere (UT), while in the lower-stratosphere (LS) values are closer. The seasonal mean percent differences between lidar and SAGE II aerosol extinctions are > 100% in the UT and < 50% above 25 km. Different techniques (point and limb observations) played the major role in producing the observed differences. SAGE II aerosol extinction in the UT increases as the longitudinal coverage is increased as the spatial aerosol extent increases, while similar extinction values in LS confirm the zonal homogeneity of LS aerosols. The study strongly emphasized that the best meteorological parameters close to the lidar measurement site in terms of space and time and Ba (sr−1), the ratio between aerosol backscattering and extinction, are needed for the tropics for a more accurate derivation of aerosol extinction.

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