photon ionization
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Author(s):  
Simon Ranecky ◽  
G. Barratt Park ◽  
Peter C Samartzis ◽  
Ioannis C. Giannakidis ◽  
Dirk Schwarzer ◽  
...  

We report chirality detection of structural isomers in a gas phase mixture using nanosecond photoelectron circular dichroism (PECD). Combining pulsed molecular beams with high-resolution resonance enhanced multi-photon ionization (REMPI) allows...



2021 ◽  
Vol 104 (5) ◽  
Author(s):  
B. P. Acharya ◽  
M. Dodson ◽  
S. Dubey ◽  
K. L. Romans ◽  
A. H. N. C. De Silva ◽  
...  


2021 ◽  
Vol 4 (10) ◽  
pp. e2127042
Author(s):  
Qi Huang ◽  
Shaodong Wang ◽  
Qingyun Li ◽  
Peiyu Wang ◽  
Jianfeng Li ◽  
...  


Atoms ◽  
2021 ◽  
Vol 9 (3) ◽  
pp. 68
Author(s):  
Aleksandr Gomonai ◽  
Eugene Remeta ◽  
Anna Gomonai

Within the framework of a three-level model, the process of three-photon ionization with one-photon resonance between two excited levels (with the lower one being initially unpopulated) is considered using the density matrix method. It is shown that such resonance can result in the appearance of a maximum in the three-photon ionization spectrum when detuning between the resonance wavenumber and the wavenumber of the transition responsible for the lower excited level being populated exceeds the laser radiation linewidth by more than three orders of magnitude.







Optica ◽  
2021 ◽  
Author(s):  
Takuya Matsubara ◽  
Shinichi Fukahori ◽  
Erik Lotstedt ◽  
Yasuo Nabekawa ◽  
Kaoru Yamanouchi ◽  
...  
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2021 ◽  
Vol 75 (7) ◽  
Author(s):  
Severin Meister ◽  
Aaron Bondy ◽  
Kirsten Schnorr ◽  
Sven Augustin ◽  
Hannes Lindenblatt ◽  
...  

Abstract Ionization of laser-dressed atomic helium is investigated with focus on photoelectron angular distributions stemming from two-color multi-photon excited states. The experiment combines extreme ultraviolet (XUV) with infrared (IR) radiation, while the relative polarization and the temporal delay between the pulses can be varied. By means of an XUV photon energy scan over several electronvolts, we get access to excited states in the dressed atom exhibiting various binding energies, angular momenta, and magnetic quantum numbers. Furthermore, varying the relative polarization is employed as a handle to switch on and off the population of certain states that are only accessible by two-photon excitation. In this way, photoemission can be suppressed for specific XUV photon energies. Additionally, we investigate the dependence of the photoelectron angular distributions on the IR laser intensity. At our higher IR intensities, we start leaving the simple multi-photon ionization regime. The interpretation of the experimental results is supported by numerically solving the time-dependent Schrödinger equation in a single-active-electron approximation. Graphic abstract



2021 ◽  
Author(s):  
Dakota Merriles ◽  
Michael Morse ◽  
Erick Tieu ◽  
Christopher Nielson ◽  
Kimberly Tomchak


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