ATR-FTIR Spectroscopic Study of Functional Groups in Aerosols: The Contribution of a Saharan Dust Transport to Urban Atmosphere in Istanbul, Turkey

2014 ◽  
Vol 225 (3) ◽  
Author(s):  
Ismail Anıl ◽  
Kurtulus Golcuk ◽  
Ferhat Karaca
Keyword(s):  
Spectroscopic Study ◽  
Functional Groups ◽  
Urban Atmosphere ◽  
Saharan Dust ◽  
Dust Transport

scholarly journals Interpreting elevated space-borne HCHO columns over the Mediterranean Sea using the OMI sensor

2011 ◽  
Vol 11 (24) ◽  
pp. 12787-12798 ◽  
Author(s):  
A. Sabolis ◽  
N. Meskhidze ◽  
G. Curci ◽  
P. I. Palmer ◽  
B. Gantt
Keyword(s):  
Mediterranean Sea ◽  
Hot Spot ◽  
Urban Atmosphere ◽  
Saharan Dust ◽  
Ozone Monitoring Instrument ◽  
Remotely Sensed Data ◽  
Vertical Column ◽  
Dust Transport ◽  
Wide Range ◽  
The Mediterranean

Abstract. Formaldehyde (HCHO) is an oxidation product of a wide range of volatile organic compounds (VOCs) and important atmospheric constituent found in both the polluted urban atmosphere and remote background sites. In this study, remotely sensed data of HCHO vertical column densities are analyzed over the Mediterranean Sea using the Ozone Monitoring Instrument (OMI). Data analysis indicates a marked seasonal cycle with a summer maximum and winter minimum confined to the marine environment during a three year period (2005–2007) examined. A possible retrieval artifact associated with Saharan dust transport over the region is explored by changing intensity of Saharan dust sources in GEOS-Chem following the recommendation of Generoso et al. (2008). Recalculated air mass factors (AMF), based on the new values of aerosol loadings, lead to a reduction of the summertime "hot spot" in OMI retrieval of HCHO vertical columns over the Mediterranean Sea; however, even after the correction, enhanced values are still present in this region. To explain these values, marine biogenic sources of VOCs are examined. Calculations indicate that emission of phytoplankton-produced isoprene is not likely to explain the enhanced HCHO vertical columns over the Mediterranean Sea. Model simulations in conjunction with measurements studies may be required to fully explore the complex mechanism of HCHO formation over the Mediterranean and its implications for the air quality in the region.

scholarly journals Saharan dust and giant quartz particle transport towards Iceland

2021 ◽  
Vol 11 (1) ◽  
Author(s):  
György Varga ◽  
Pavla Dagsson-Walhauserová ◽  
Fruzsina Gresina ◽  
Agusta Helgadottir
Keyword(s):  
Numerical Models ◽  
Saharan Dust ◽  
Atmospheric Environment ◽  
The Arctic ◽  
Dust Particles ◽  
Atmospheric Flow ◽  
Dust Transport ◽  
Strong Winds ◽  
Dust Events ◽  
Local Dust

AbstractMineral dust emissions from Saharan sources have an impact on the atmospheric environment and sedimentary units in distant regions. Here, we present the first systematic observations of long-range Saharan dust transport towards Iceland. Fifteen Saharan dust episodes were identified to have occurred between 2008 and 2020 based on aerosol optical depth data, backward trajectories and numerical models. Icelandic samples from the local dust sources were compared with deposited dust from two severe Saharan dust events in terms of their granulometric and mineralogical characteristics. The episodes were associated with enhanced meridional atmospheric flow patterns driven by unusual meandering jets. Strong winds were able to carry large Saharan quartz particles (> 100 µm) towards Iceland. Our results confirm the atmospheric pathways of Saharan dust towards the Arctic, and identify new northward meridional long-ranged transport of giant dust particles from the Sahara, including the first evidence of their deposition in Iceland as previously predicted by models.

A Lagrangian method to descripe Saharan dust transport towards Europe

1997 ◽  
Vol 28 ◽  
pp. S461-S462
Author(s):  
S. Külzer ◽  
R. Ries ◽  
L. Schütz
Keyword(s):  
Lagrangian Method ◽  
Saharan Dust ◽  
Dust Transport

scholarly journals Three-dimensional evolution of Saharan dust transport towards Europe based on a 9-year EARLINET-optimized CALIPSO dataset

2017 ◽  
Vol 17 (9) ◽  
pp. 5893-5919 ◽  
Author(s):  
Eleni Marinou ◽  
Vassilis Amiridis ◽  
Ioannis Binietoglou ◽  
Athanasios Tsikerdekis ◽  
Stavros Solomos ◽  
...  
Keyword(s):  
Cloud Condensation Nuclei ◽  
Three Dimensional ◽  
Satellite Observation ◽  
Saharan Dust ◽  
Winter Period ◽  
Dust Transport ◽  
The Balkans ◽  
Potential Applications ◽  
The Mediterranean ◽  
Dust Evolution

Abstract. In this study we use a new dust product developed using CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) observations and EARLINET (European Aerosol Research Lidar Network) measurements and methods to provide a 3-D multiyear analysis on the evolution of Saharan dust over North Africa and Europe. The product uses a CALIPSO L2 backscatter product corrected with a depolarization-based method to separate pure dust in external aerosol mixtures and a Saharan dust lidar ratio (LR) based on long-term EARLINET measurements to calculate the dust extinction profiles. The methodology is applied on a 9-year CALIPSO dataset (2007–2015) and the results are analyzed here to reveal for the first time the 3-D dust evolution and the seasonal patterns of dust over its transportation paths from the Sahara towards the Mediterranean and Continental Europe. During spring, the spatial distribution of dust shows a uniform pattern over the Sahara desert. The dust transport over the Mediterranean Sea results in mean dust optical depth (DOD) values up to 0.1. During summer, the dust activity is mostly shifted to the western part of the desert where mean DOD near the source is up to 0.6. Elevated dust plumes with mean extinction values between 10 and 75 Mm−1 are observed throughout the year at various heights between 2 and 6 km, extending up to latitudes of 40° N. Dust advection is identified even at latitudes of about 60° N, but this is due to rare events of episodic nature. Dust plumes of high DOD are also observed above the Balkans during the winter period and above northwest Europe during autumn at heights between 2 and 4 km, reaching mean extinction values up to 50 Mm−1. The dataset is considered unique with respect to its potential applications, including the evaluation of dust transport models and the estimation of cloud condensation nuclei (CCN) and ice nuclei (IN) concentration profiles. Finally, the product can be used to study dust dynamics during transportation, since it is capable of revealing even fine dynamical features such as the particle uplifting and deposition on European mountainous ridges such as the Alps and Carpathian Mountains.

scholarly journals Synergetic monitoring of Saharan dust plumes and potential impact on surface: a case study of dust transport from Canary Islands to Iberian Peninsula

2011 ◽  
Vol 11 (7) ◽  
pp. 3067-3091 ◽  
Author(s):  
C. Córdoba-Jabonero ◽  
M. Sorribas ◽  
J. L. Guerrero-Rascado ◽  
J. A. Adame ◽  
Y. Hernández ◽  
...  
Keyword(s):  
Iberian Peninsula ◽  
Particle Deposition ◽  
Ground Level ◽  
In Situ Measurements ◽  
Saharan Dust ◽  
Dust Transport ◽  
Air Masses ◽  
Potential Impact

Abstract. The synergetic use of meteorological information, remote sensing both ground-based active (lidar) and passive (sun-photometry) techniques together with backtrajectory analysis and in-situ measurements is devoted to the characterization of dust intrusions. A case study of air masses advected from the Saharan region to the Canary Islands and the Iberian Peninsula, located relatively close and far away from the dust sources, respectively, was considered for this purpose. The observations were performed over three Spanish geographically strategic stations within the dust-influenced area along a common dust plume pathway monitored from 11 to 19 of March 2008. A 4-day long dust event (13–16 March) over the Santa Cruz de Tenerife Observatory (SCO), and a linked short 1-day dust episode (14 March) in the Southern Iberian Peninsula over the Atmospheric Sounding Station "El Arenosillo" (ARN) and the Granada station (GRA) were detected. Meteorological conditions favoured the dust plume transport over the area under study. Backtrajectory analysis clearly revealed the Saharan region as the source of the dust intrusion. Under the Saharan air masses influence, AERONET Aerosol Optical Depth at 500 nm (AOD500) ranged from 0.3 to 0.6 and Ångström Exponent at 440/675 nm wavelength pair (AE440/675) was lower than 0.5, indicating a high loading and predominance of coarse particles during those dusty events. Lidar observations characterized their vertical layering structure, identifying different aerosol contributions depending on altitude. In particular, the 3-km height dust layer transported from the Saharan region and observed over SCO site was later on detected at ARN and GRA stations. No significant differences were found in the lidar (extinction-to-backscatter) ratio (LR) estimation for that dust plume over all stations when a suitable aerosol scenario for lidar data retrieval is selected. Lidar-retrieved LR values of 60–70 sr were obtained during the main dust episodes. These similar LR values found in all the stations suggest that dust properties were kept nearly unchanged in the course of its medium-range transport. In addition, the potential impact on surface of that Saharan dust intrusion over the Iberian Peninsula was evaluated by means of ground-level in-situ measurements for particle deposition assessment together with backtrajectory analysis. However, no connection between those dust plumes and the particle sedimentation registered at ground level is found. Differences on particle deposition processes observed in both Southern Iberian Peninsula sites are due to the particular dust transport pattern occurred over each station. Discrepancies between columnar-integrated and ground-level in-situ measurements show a clear dependence on height of the dust particle size distribution. Then, further vertical size-resolved observations are needed for evaluation of the impact on surface of the Saharan dust arrival to the Iberian Peninsula.

scholarly journals Saharan dust levels in Greece and received inhalation doses

2008 ◽  
Vol 8 (3) ◽  
pp. 11967-11996 ◽  
Author(s):  
C. Mitsakou ◽  
G. Kallos ◽  
N. Papantoniou ◽  
C. Spyrou ◽  
S. Solomos ◽  
...  
Keyword(s):  
Urban Areas ◽  
Particle Deposition ◽  
Mineral Dust ◽  
Weather Conditions ◽  
Pm10 Concentration ◽  
Saharan Dust ◽  
Dust Particles ◽  
Annual Number ◽  
Human Respiratory Tract ◽  
Dust Transport

Abstract. The desert of Sahara is one of the major sources of mineral dust on Earth, producing around 2×108 tons/yr. Under certain weather conditions, dust particles from Saharan desert get transported over the Mediterranean Sea and most of Europe. The limiting values set by the directive EC/30/1999 of European Union can easily be exceeded by the transport of desert dust particles in all south European areas and especially urban. In this study, the effects of dust transport on air quality in several Greek urban areas are quantified. PM10 concentration values from stationary monitoring stations are compared to dust concentrations for the 4-year period 2003–2006. The dust concentration values in the Greek areas were estimated by the SKIRON modelling system coupled with embedded algorithms describing the dust cycle. The mean annual dust contribution to daily-averaged PM10 concentration values was found to be around or even greater than 10% in the urban areas throughout the years examined. Natural dust transport may contribute by much more than 20% to the annual number of exceedances – PM10 values greater than EU limits – depending on the specific monitoring location. In a second stage of the study, the inhaled lung dose received by the residents in various Greek locations is calculated. The particle deposition efficiency of mineral dust at the different parts of the human respiratory tract is determined by applying a lung dosimetry numerical model, which incorporates inhalation dynamics and aerosol physical processes. The inhalation dose from mineral dust particles was greater in the upper respiratory system (extrathoracic region) and less significant in the lungs, especially in the sensitive alveolar region. However, in cases of dust episodes, the amounts of mineral dust deposited along the human lung are comparable to those received during exposure in heavily polluted urban or smoking areas.

scholarly journals Coarse and giant particles are ubiquitous in Saharan dust export regions and are radiatively significant over the Sahara

2020 ◽  
Author(s):  
Claire Ryder ◽  
Eleanor Highwood ◽  
Adrian Walser ◽  
Petra Walser ◽  
Anne Philipp ◽  
...  
Keyword(s):  
Mass Concentration ◽  
Size Range ◽  
State Of The Art ◽  
Chem Phys ◽  
Saharan Dust ◽  
Dust Particles ◽  
Field Campaign ◽  
Dust Transport ◽  
Coarse Mode ◽  
Significant Underestimation

<p>Mineral dust is an important component of the climate system, interacting with radiation, clouds, and biogeochemical systems and impacting atmospheric circulation, air quality, aviation, and solar energy generation. These impacts are sensitive to dust particle size distribution (PSD), yet models struggle or even fail to represent coarse (diameter (<span><em>d</em></span>) <span>>2.5</span> <span>µ</span>m) and giant (<span><em>d</em>>20</span> <span>µ</span>m) dust particles and the evolution of the PSD with transport. Here we examine three state-of-the-art airborne observational datasets, all of which measured the full size range of dust (<span><em>d</em>=0.1</span> to <span>>100</span> <span>µ</span>m) at different stages during transport with consistent instrumentation. We quantify the presence and evolution of coarse and giant particles and their contribution to optical properties using airborne observations over the Sahara (from the Fennec field campaign) and in the Saharan Air Layer (SAL) over the tropical eastern Atlantic (from the AER-D field campaign).</p><p>Observations show significantly more abundant coarse and giant dust particles over the Sahara compared to the SAL: effective diameters of up to 20 <span>µ</span>m were observed over the Sahara compared to 4 <span>µ</span>m in the SAL. Excluding giant particles over the Sahara results in significant underestimation of mass concentration (40 %), as well as underestimates of both shortwave and longwave extinction (18 % and 26 %, respectively, from scattering calculations), while the effects in the SAL are smaller but non-negligible. The larger impact on longwave extinction compared to shortwave implies a bias towards a radiative cooling effect in dust models, which typically exclude giant particles and underestimate coarse-mode concentrations.</p><p>A compilation of the new and published effective diameters against dust age since uplift time suggests that two regimes of dust transport exist. During the initial 1.5 d, both coarse and giant particles are rapidly deposited. During the subsequent 1.5 to 10 d, PSD barely changes with transport, and the coarse mode is retained to a much greater degree than expected from estimates of gravitational sedimentation alone. The reasons for this are unclear and warrant further investigation in order to improve dust transport schemes and the associated radiative effects of coarse and giant particles in models.</p><p>This work has been recently published in ACP (Ryder, C. L., Highwood, E. J., Walser, A., Seibert, P., Philipp, A., and Weinzierl, B.: Coarse and giant particles are ubiquitous in Saharan dust export regions and are radiatively significant over the Sahara, Atmos. Chem. Phys., 19, 15353–15376, https://doi.org/10.5194/acp-19-15353-2019, 2019).</p>

scholarly journals Lidar Measuremnt on Dust Transport from the Saharan Desert to the Iran Plateau

2020 ◽  
Vol 237 ◽  
pp. 02020
Author(s):  
Hossein Panahifar ◽  
Ruhollah Moradhaseli ◽  
Hadi Bourzoie ◽  
Mahdi Gholami ◽  
Hamid Reza Khalesifard
Keyword(s):  
Trajectory Analysis ◽  
Saharan Dust ◽  
Dust Particles ◽  
Raman Lidar ◽  
Dust Layer ◽  
Mean Values ◽  
Dust Transport ◽  
Lidar Ratio ◽  
532 Nm ◽  
Iran Plateau

Optical properties of long-range Saharan dust particles transported to the Iran Plateau have been investigated. The results were derived from the measurements of a dual-wavelength Depolarized backscatter/Raman lidar and a Cimel CE318-2 sunphotometer. Observations were performed in Zanjan, Northwest Iran. The backward trajectory analysis show that the lofted dust plumes come from the Saharan desert and travel along Mediterranean Sea and Turkey toward Iran. The lidar ratio within the lofted dust layer has been found with mean values of 50 sr at 532 nm. For the depolarization ratio, mean values of 25% have been found.

scholarly journals The fate of saharan dust across the atlantic and implications for a central american dust barrier

2011 ◽  
Vol 11 (16) ◽  
pp. 8415-8431 ◽  
Author(s):  
E. Nowottnick ◽  
P. Colarco ◽  
A. da Silva ◽  
D. Hlavka ◽  
M. McGill
Keyword(s):  
Central America ◽  
Transport Model ◽  
Atmospheric Transport ◽  
Saharan Dust ◽  
Sensitivity Analyses ◽  
Transport Barrier ◽  
Dust Transport ◽  
Transport Dynamics ◽  
The Caribbean ◽  
Wet Removal

Abstract. Saharan dust was observed over the Caribbean basin during the summer 2007 NASA Tropical Composition, Cloud, and Climate Coupling (TC4) field experiment. Airborne Cloud Physics Lidar (CPL) and satellite observations from MODIS suggest a barrier to dust transport across Central America into the eastern Pacific. We use the NASA GEOS-5 atmospheric transport model with online aerosol tracers to perform simulations of the TC4 time period in order to understand the nature of this barrier. Our simulations are driven by the Modern Era Retrospective-Analysis for Research and Applications (MERRA) meteorological analyses. Compared to observations from MODIS and CALIOP, GEOS-5 reproduces the observed location and magnitude of observed dust events, but our baseline simulation does not develop as strong a barrier to dust transport across Central America as observations suggest. Analysis of the dust transport dynamics and loss processes suggest that while both mechanisms play a role in defining the dust transport barrier, loss processes by wet removal of dust are about twice as important as transport. Sensitivity analyses with our model showed that the dust barrier would not exist without convective scavenging over the Caribbean. The best agreement between our model and the observations was obtained when dust wet removal was parameterized to be more aggressive, treating the dust as we do hydrophilic aerosols.

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