scholarly journals Quasi-one-dimensional metallic conduction channels in exotic ferroelectric topological defects

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Wenda Yang ◽  
Guo Tian ◽  
Yang Zhang ◽  
Fei Xue ◽  
Dongfeng Zheng ◽  
...  

AbstractFerroelectric topological objects provide a fertile ground for exploring emerging physical properties that could potentially be utilized in future nanoelectronic devices. Here, we demonstrate quasi-one-dimensional metallic high conduction channels associated with the topological cores of quadrant vortex domain and center domain (monopole-like) states confined in high quality BiFeO3 nanoislands, abbreviated as the vortex core and the center core. We unveil via the phase-field simulation that the superfine metallic conduction channels along the center cores arise from the screening charge carriers confined at the core region, whereas the high conductance of vortex cores results from a field-induced twisted state. These conducting channels can be reversibly created and deleted by manipulating the two topological states via electric field, leading to an apparent electroresistance effect with an on/off ratio higher than 103. These results open up the possibility of utilizing these functional one-dimensional topological objects in high-density nanoelectronic devices, e.g. nonvolatile memory.

2020 ◽  
Vol 11 (16) ◽  
pp. 6757-6762
Author(s):  
Johnpaul K. Pious ◽  
Manasa G. Basavarajappa ◽  
Chinnadurai Muthu ◽  
Nayana Krishna ◽  
Ryosuke Nishikubo ◽  
...  

2020 ◽  
Vol 6 (19) ◽  
pp. eaat9488 ◽  
Author(s):  
C.-C. Hsu ◽  
M. L. Teague ◽  
J.-Q. Wang ◽  
N.-C. Yeh

The existence of nontrivial Berry phases associated with two inequivalent valleys in graphene provides interesting opportunities for investigating the valley-projected topological states. Examples of such studies include observation of anomalous quantum Hall effect in monolayer graphene, demonstration of topological zero modes in “molecular graphene” assembled by scanning tunneling microscopy, and detection of topological valley transport either in graphene superlattices or at bilayer graphene domain walls. However, all aforementioned experiments involved nonscalable approaches of either mechanically exfoliated flakes or atom-by-atom constructions. Here, we report an approach to manipulating the topological states in monolayer graphene via nanoscale strain engineering at room temperature. By placing strain-free monolayer graphene on architected nanostructures to induce global inversion symmetry breaking, we demonstrate the development of giant pseudo-magnetic fields (up to ~800 T), valley polarization, and periodic one-dimensional topological channels for protected propagation of chiral modes in strained graphene, thus paving a pathway toward scalable graphene-based valleytronics.


Catalysts ◽  
2019 ◽  
Vol 9 (10) ◽  
pp. 787 ◽  
Author(s):  
Yun Yeol Ryu ◽  
Taekyung Kim ◽  
HyukSu Han

Zinc oxide (ZnO) has attractive photocatalytic properties. However, the high recombination rate of the photo-excited charge carriers on this material often restricts application. Here, we report that hybridization of one dimensional (1D) carbon nanotubes (CNT) on two dimensional (2D) porous ZnO nanosheets (NS) can be a promising strategy to overcome some of the challenges of ZnO. Specifically, a pulsed laser ablation technique was utilized to hybridize 1D CNT with 2D porous ZnO NS in environmentally friendly as well as super-economic (short time, less than 10 min) conditions. The synthesized ZnO NS-CNT hybrids show a significantly enhanced photocatalytic activity for water splitting relative to their counterpart ZnO NS.


Nanoscale ◽  
2018 ◽  
Vol 10 (43) ◽  
pp. 20256-20265 ◽  
Author(s):  
Donghyung Kim ◽  
Zhuo Zhang ◽  
Kijung Yong

One-dimensional heterojunction nanorods are highly attractive as photoanodes for developing efficient photoelectrochemical (PEC) systems for the effective photogeneration of charge carriers and transport.


2020 ◽  
Vol 12 (8) ◽  
pp. 1109-1115
Author(s):  
Xiaojiao Yang ◽  
Jun Li ◽  
Ying Liu

One-dimensional gold nanofibers are good candidates for next generation nanoelectronic devices. Here, gold nanofibers were synthesized via electrospinning with subsequent in-situ thermal reduction. The thermal behavior of the precursor nanofibers was investigated by thermogravimetric/differential thermal analysis and fourier transform infrared. The polymer parts are decomposed and removed step by step, meanwhile, gold salt is decomposed and in-situ reduced to form gold nanoparticles in air without any reducing agent or gas due to its strong oxidation ability. The effects of gold content, polymers type (PVP, PVA, PAN), calcination atmospheres (Air, H2, H2/Ar) and temperatures (200 °C to 500 °C) on the morphology and structures of gold nanofibers were characterized by XRD, SEM, and TEM. The results shows that PVP is the optimal polymer with the gold content of 6:1 (PVP:Au) to fabricate the continuous gold nanofibers with good morphology and structures. The final gold nanofibers with average diameter of 60 nm and several hundred micrometers long, were fabricated after calcined at 500 °C in air for 2 hours. It was composed of gold nanoparticles that ranged from 5 to 30 nm.


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