scholarly journals Enhanced responsivity and detectivity of fast WSe2 phototransistor using electrostatically tunable in-plane lateral p-n homojunction

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Sayantan Ghosh ◽  
Abin Varghese ◽  
Kartikey Thakar ◽  
Sushovan Dhara ◽  
Saurabh Lodha

AbstractLayered transition metal dichalcogenides have shown tremendous potential for photodetection due to their non-zero direct bandgaps, high light absorption coefficients and carrier mobilities, and ability to form atomically sharp and defect-free heterointerfaces. A critical and fundamental bottleneck in the realization of high performance detectors is their trap-dependent photoresponse that trades off responsivity with speed. This work demonstrates a facile method of attenuating this trade-off by nearly 2x through integration of a lateral, in-plane, electrostatically tunable p-n homojunction with a conventional WSe2 phototransistor. The tunable p-n junction allows modulation of the photocarrier population and width of the conducting channel independently from the phototransistor. Increased illumination current with the lateral p-n junction helps achieve responsivity enhancement upto 2.4x at nearly the same switching speed (14–16 µs) over a wide range of laser power (300 pW–33 nW). The added benefit of reduced dark current enhances specific detectivity (D*) by nearly 25x to yield a maximum measured flicker noise-limited D* of 1.1×1012 Jones. High responsivity of 170 A/W at 300 pW laser power along with the ability to detect sub-1 pW laser switching are demonstrated.

Author(s):  
Manoj K. Jana ◽  
C. N. R. Rao

The discovery of graphene marks a major event in the physics and chemistry of materials. The amazing properties of this two-dimensional (2D) material have prompted research on other 2D layered materials, of which layered transition metal dichalcogenides (TMDCs) are important members. Single-layer and few-layer TMDCs have been synthesized and characterized. They possess a wide range of properties many of which have not been known hitherto. A typical example of such materials is MoS 2 . In this article, we briefly present various aspects of layered analogues of graphene as exemplified by TMDCs. The discussion includes not only synthesis and characterization, but also various properties and phenomena exhibited by the TMDCs. This article is part of the themed issue ‘Fullerenes: past, present and future, celebrating the 30th anniversary of Buckminster Fullerene’.


2021 ◽  
Vol 11 (1) ◽  
Author(s):  
Chunrui Han ◽  
Yu Wang ◽  
Weihu Zhou ◽  
Minpeng Liang ◽  
Jianting Ye

AbstractLayered transition metal dichalcogenides (TMDCs) have shown great potential for a wide range of applications in photonics and optoelectronics. Nevertheless, valley decoherence severely randomizes its polarization which is important to a light emitter. Plasmonic metasurface with a unique way to manipulate the light-matter interaction may provide an effective and practical solution. Here by integrating TMDCs with plasmonic nanowire arrays, we demonstrate strong anisotropic enhancement of the excitonic emission at different spectral positions. For the indirect bandgap transition in bilayer WS2, multifold enhancement can be achieved with the photoluminescence (PL) polarization either perpendicular or parallel to the long axis of nanowires, which arises from the coupling of WS2 with localized or guided plasmon modes, respectively. Moreover, PL of high linearity is obtained in the direct bandgap transition benefiting from, in addition to the plasmonic enhancement, the directional diffraction scattering of nanowire arrays. Our method with enhanced PL intensity contrasts to the conventional form-birefringence based on the aspect ratio of nanowire arrays where the intensity loss is remarkable. Our results provide a prototypical plasmon-exciton hybrid system for anisotropic enhancement of the PL at the nanoscale, enabling simultaneous control of the intensity, polarization and wavelength toward practical ultrathin photonic devices based on TMDCs.


2020 ◽  
Author(s):  
Chunrui Han ◽  
Yu Wang ◽  
Weihu Zhou ◽  
Jianting Ye

Abstract Layered transition metal dichalcogenides (TMDCs) have shown great potential for a wide range of applications in photonics and optoelectronics. Nevertheless, valley decoherence severely randomizes its polarization which is important to a light emitter. Plasmonic metasurface with a unique way to manipulate the light-matter interaction may provide an effective and practical solution. Here by integrating TMDCs with plasmonic nanowire arrays, we demonstrate strong anisotropic enhancement of the excitonic emission at different spectral positions. For the indirect bandgap transition in bilayer WS2, multifold enhancement can be achieved with the PL polarization either perpendicular or parallel to the long axis of nanowires, which arises from the coupling of WS2 with localized or guided plasmon modes, respectively. Moreover, PL of a high linearity is obtained in the direct bandgap transition benefiting from, in addition to the plasmonic enhancement, the directional diffraction scattering of nanowire arrays. Our method with enhanced PL intensity contrasts to the conventional form-birefringence based on the aspect ratio of nanowire arrays where the intensity loss is remarkable. Our results provide a prototypical plasmon-exciton hybrid system for anisotropic enhancement of the PL at the nanoscale, enabling simultaneous control of intensity, polarization and wavelength toward practical ultrathin photonic devices based on TMDCs.


RSC Advances ◽  
2017 ◽  
Vol 7 (43) ◽  
pp. 26665-26672 ◽  
Author(s):  
Chao Zhao ◽  
Tien Khee Ng ◽  
Chien-Chih Tseng ◽  
Jun Li ◽  
Yumeng Shi ◽  
...  

High-quality nitride nanowires on large-area layered transition metal dichalcogenides are first reported, which yielded light-emitting diodes (LEDs) with superior performance.


Author(s):  
Yoobeen Lee ◽  
Jin Won Jung ◽  
Jin Seok Lee

The reduction of intrinsic defects, including vacancies and grain boundaries, remains one of the greatest challenges to produce high-performance transition metal dichalcogenides (TMDCs) electronic systems. A deeper comprehension of the...


Author(s):  
Alwin Daus ◽  
Sam Vaziri ◽  
Victoria Chen ◽  
Çağıl Köroğlu ◽  
Ryan W. Grady ◽  
...  

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