A global perspective of ground level, 'ambient' carbon dioxide for assessing the response of plants to atmospheric CO2

2001 ◽  
Vol 7 (7) ◽  
pp. 789-796 ◽  
Author(s):  
L. H. Ziska ◽  
O. Ghannoum ◽  
J. T. Baker ◽  
J. Conroy ◽  
J. A. Bunce ◽  
...  
2001 ◽  
Vol 7 (7) ◽  
pp. 789-796 ◽  
Author(s):  
L. H. Ziska ◽  
O. Ghannoum ◽  
J. T. Baker ◽  
J. Conroy ◽  
J. A. Bunce ◽  
...  

2014 ◽  
Vol 7 (2) ◽  
pp. 521-610 ◽  
Author(s):  
C. Le Quéré ◽  
R. Moriarty ◽  
R. M. Andrew ◽  
G. P. Peters ◽  
P. Ciais ◽  
...  

Abstract. Accurate assessment of anthropogenic carbon dioxide (CO2) emissions and their redistribution among the atmosphere, ocean, and terrestrial biosphere is important to better understand the global carbon cycle, support the development of climate policies, and project future climate change. Here we describe datasets and a methodology to quantify all major components of the global carbon budget, including their uncertainties, based on the combination of a range of data, algorithms, statistics and model estimates and their interpretation by a broad scientific community. We discuss changes compared to previous estimates, consistency within and among components, alongside methodology and data limitations. CO2 emissions from fossil fuel combustion and cement production (EFF) are based on energy statistics and cement production data, respectively, while emissions from Land-Use Change (ELUC), mainly deforestation, are based on combined evidence from land-cover change data, fire activity associated with deforestation, and models. The global atmospheric CO2 concentration is measured directly and its rate of growth (GATM) is computed from the annual changes in concentration. The mean ocean CO2 sink (SOCEAN) is based on observations from the 1990s, while the annual anomalies and trends are estimated with ocean models. The variability in SOCEAN is evaluated with data products based on surveys of ocean CO2 measurements. The global residual terrestrial CO2 sink (SLAND) is estimated by the difference of the other terms of the global carbon budget and compared to results of independent Dynamic Global Vegetation Models forced by observed climate, CO2 and land cover change (some including nitrogen-carbon interactions). We compare the variability and mean land and ocean fluxes to estimates from three atmospheric inverse methods for three broad latitude bands. All uncertainties are reported as ±1σ, reflecting the current capacity to characterise the annual estimates of each component of the global carbon budget. For the last decade available (2004–2013), EFF was 8.9 ± 0.4 GtC yr−1, ELUC 0.9 ± 0.5 GtC yr−1, GATM 4.3 ± 0.1 GtC yr−1, SOCEAN 2.6 ± 0.5 GtC yr−1, and SLAND 2.9 ± 0.8 GtC yr−1. For year 2013 alone, EFF grew to 9.9 ± 0.5 GtC yr−1, 2.3% above 2012, contining the growth trend in these emissions. ELUC was 0.9 ± 0.5 GtC yr−1, GATM was 5.4 ± 0.2 GtC yr−1, SOCEAN was 2.9 ± 0.5 GtC yr−1 and SLAND was 2.5 ± 0.9 GtC yr−1. GATM was high in 2013 reflecting a steady increase in EFF and smaller and opposite changes between SOCEAN and SLAND compared to the past decade (2004–2013). The global atmospheric CO2 concentration reached 395.31 ± 0.10 ppm averaged over 2013. We estimate that EFF will increase by 2.5% (1.3–3.5%) to 10.1 ± 0.6 GtC in 2014 (37.0 ± 2.2 GtCO2 yr−1), 65% above emissions in 1990, based on projections of World Gross Domestic Product and recent changes in the carbon intensity of the economy. From this projection of EFF and assumed constant ELUC for 2014, cumulative emissions of CO2 will reach about 545 ± 55 GtC (2000 ± 200 GtCO2) for 1870–2014, about 75% from EFF and 25% from ELUC. This paper documents changes in the methods and datasets used in this new carbon budget compared with previous publications of this living dataset (Le Quéré et al., 2013, 2014). All observations presented here can be downloaded from the Carbon Dioxide Information Analysis Center (doi:10.3334/CDIAC/GCP_2014). Italic font highlights significant methodological changes and results compared to the Le Quéré et al. (2014) manuscript that accompanies the previous version of this living data.


2018 ◽  
Vol 176 ◽  
pp. 05045 ◽  
Author(s):  
Erwan Cadiou ◽  
Jean-Baptiste Dherbecourt ◽  
Guillaume Gorju ◽  
Jean-Michel Melkonian ◽  
Antoine Godard ◽  
...  

We report on ground-based atmospheric concentration measurements of carbon dioxide, using a pulsed direct detection differential absorption lidar operating at 2051 nm. The transmitter is based on a tunable parametric source emitting 10-mJ energy, 10-ns duration Fourier-limited pulses. Range resolved concentration measurements have been carried out on the aerosol back-scattered signal. Cloud signals have been used to get long range integrated-path measurements.


2005 ◽  
Vol 2 (1) ◽  
pp. 3 ◽  
Author(s):  
Roger J. Francey

Environmental Context.Excessive levels of carbon dioxide are accumulating in the atmosphere, principally from burning fossil fuels. The gas is linked to the enhanced greenhouse effect and climate change, and is thus monitored carefully, along with other trace gases that reflect human activity.The rate of growth of carbon dioxide has increased gradually over the past century, and more rapidly in the last decade. Teasing out fossil emissions from changes due to wildfires and to natural exchange with plants and oceans guide global attempts in reducing emissions.


2014 ◽  
Vol 11 (22) ◽  
pp. 6293-6305 ◽  
Author(s):  
L. Xue ◽  
W. Yu ◽  
H. Wang ◽  
L.-Q. Jiang ◽  
L. Feng ◽  
...  

Abstract. Information on changes in the oceanic carbon dioxide (CO2) concentration and air–sea CO2 flux as well as on ocean acidification in the Indian Ocean is very limited. In this study, temporal changes of the inorganic carbon system in the eastern equatorial Indian Ocean (EIO, 5° N–5° S, 90–95° E) are examined using partial pressure of carbon dioxide (pCO2) data collected in May 2012, historical pCO2 data since 1962, and total alkalinity (TA) data calculated from salinity. Results show that sea surface pCO2 in the equatorial belt (2° N–2° S, 90–95° E) increased from ∼307 μatm in April 1963 to ∼373 μatm in May 1999, ∼381 μatm in April 2007, and ∼385 μatm in May 2012. The mean rate of pCO2 increase in this area (∼1.56 μatm yr−1) was close to that in the atmosphere (∼1.46 μatm yr−1). Despite the steady pCO2 increase in this region, no significant change in air–sea CO2 fluxes was detected during this period. Ocean acidification as indicated by pH and saturation states for carbonate minerals has indeed taken place in this region. Surface water pH (total hydrogen scale) and saturation state for aragonite (Ωarag), calculated from pCO2 and TA, decreased significantly at rates of −0.0016 ± 0.0001 and −0.0095 ± 0.0005 yr−1, respectively. The respective contributions of temperature, salinity, TA, and dissolved inorganic carbon (DIC) to the increase in surface pCO2 and the decreases in pH and Ωarag are quantified. We find that the increase in DIC dominated these changes, while contributions from temperature, salinity, and TA were insignificant. The increase in DIC was most likely associated with the increasing atmospheric CO2 concentration, and the transport of accumulated anthropogenic CO2 from a CO2 sink region via basin-scale ocean circulations. These two processes may combine to drive oceanic DIC to follow atmospheric CO2 increase.


2009 ◽  
Vol 66 (7) ◽  
pp. 1538-1546 ◽  
Author(s):  
Ferial Louanchi ◽  
Meriem Boudjakdji ◽  
Lamri Nacef

Abstract Louanchi, F., Boudjakdji, M, and Nacef, L. 2009. Decadal changes in surface carbon dioxide and related variables in the Mediterranean Sea as inferred from a coupled data-diagnostic model approach. – ICES Journal of Marine Science, 66: 1538–1546. A coupled approach based on available datasets of temperature, salinity, oxygen, nutrients, and chlorophyll, and a surface layer box model previously developed and modified for the present study, allowed us to reconstruct dissolved inorganic carbon (DIC), total alkalinity, and carbon dioxide fugacity (fCO2) mixed-layer fields for the Mediterranean Sea, from the 1960s to the 1990s. The approach used in this study resulted in a 7% relative error on reconstructed surface fCO2 fields. The Mediterranean Sea transformed from a source of 0.62 Tg C year−1 for atmospheric CO2 in the 1960s, to a net sink of −1.98 Tg C year−1 in the 1990s. The annual cycle in surface fCO2 was driven mainly by temperature variations in the Mediterranean Sea, whereas its decadal variations resulted from a balance between primary production and the thermal effect. According to our model results, the atmospheric CO2 increase of ∼40 µatm over the period of our investigation induced an increase in DIC of ∼30 µmol l−1 in surface waters. A 50% reduction in the magnitude of seasonal variations in surface temperature occurred during the 1990s relative to the earlier decades. Therefore, surface fCO2 only increased by 24 µatm from the 1960s to the 1990s. Changes in pH were not significant over this period.


2015 ◽  
Vol 12 (3) ◽  
pp. 653-679 ◽  
Author(s):  
S. Sitch ◽  
P. Friedlingstein ◽  
N. Gruber ◽  
S. D. Jones ◽  
G. Murray-Tortarolo ◽  
...  

Abstract. The land and ocean absorb on average just over half of the anthropogenic emissions of carbon dioxide (CO2) every year. These CO2 "sinks" are modulated by climate change and variability. Here we use a suite of nine dynamic global vegetation models (DGVMs) and four ocean biogeochemical general circulation models (OBGCMs) to estimate trends driven by global and regional climate and atmospheric CO2 in land and oceanic CO2 exchanges with the atmosphere over the period 1990–2009, to attribute these trends to underlying processes in the models, and to quantify the uncertainty and level of inter-model agreement. The models were forced with reconstructed climate fields and observed global atmospheric CO2; land use and land cover changes are not included for the DGVMs. Over the period 1990–2009, the DGVMs simulate a mean global land carbon sink of −2.4 ± 0.7 Pg C yr−1 with a small significant trend of −0.06 ± 0.03 Pg C yr−2 (increasing sink). Over the more limited period 1990–2004, the ocean models simulate a mean ocean sink of −2.2 ± 0.2 Pg C yr−1 with a trend in the net C uptake that is indistinguishable from zero (−0.01 ± 0.02 Pg C yr−2). The two ocean models that extended the simulations until 2009 suggest a slightly stronger, but still small, trend of −0.02 ± 0.01 Pg C yr−2. Trends from land and ocean models compare favourably to the land greenness trends from remote sensing, atmospheric inversion results, and the residual land sink required to close the global carbon budget. Trends in the land sink are driven by increasing net primary production (NPP), whose statistically significant trend of 0.22 ± 0.08 Pg C yr−2 exceeds a significant trend in heterotrophic respiration of 0.16 ± 0.05 Pg C yr−2 – primarily as a consequence of widespread CO2 fertilisation of plant production. Most of the land-based trend in simulated net carbon uptake originates from natural ecosystems in the tropics (−0.04 ± 0.01 Pg C yr−2), with almost no trend over the northern land region, where recent warming and reduced rainfall offsets the positive impact of elevated atmospheric CO2 and changes in growing season length on carbon storage. The small uptake trend in the ocean models emerges because climate variability and change, and in particular increasing sea surface temperatures, tend to counter\\-act the trend in ocean uptake driven by the increase in atmospheric CO2. Large uncertainty remains in the magnitude and sign of modelled carbon trends in several regions, as well as regarding the influence of land use and land cover changes on regional trends.


2016 ◽  
Author(s):  
Craig A. Emmerton ◽  
Vincent L. St. Louis ◽  
Igor Lehnherr ◽  
Jennifer A. Graydon ◽  
Jane L. Kirk ◽  
...  

Abstract. A warming climate is rapidly changing the distribution and exchanges of carbon within high Arctic ecosystems. Few data exist, however, which quantify exchange of both carbon dioxide (CO2) and methane (CH4) between the atmosphere and freshwater systems, or estimate freshwater contributions to total catchment exchange of these gases, in the high Arctic. During the summers of 2005 and 2007–2012, we quantified CO2 and CH4 concentrations in, and atmospheric exchange with, common freshwater systems in the high Arctic watershed of Lake Hazen, Nunavut, Canada. We identified four types of biogeochemically-distinct freshwater systems in the watershed, however mean CO2 concentrations (21–28 μmol L−1) and atmospheric exchange (−0.013–0.046 g C-CO2 m−2 d−1) were similar between these systems. Seasonal flooding of ponds bordering Lake Hazen generated considerable CH4 emissions to the atmosphere (0.008 g C-CH4 m−2 d−1), while all other freshwater systems were minimal emitters of this gas (< 0.001 g C-CH4 m−2 d−1). Measurements made on terrestrial landscapes in the same watershed between 2008–2012 determined that the near-barren polar semidesert was a very weak consumer of atmospheric CO2 (−0.004 g C-CO2 m−2 d−1), but an important consumer of atmospheric CH4 (−0.001 g C-CH4 m−2 d−1). Alternatively, meadow wetlands were very productive consumers of atmospheric CO2 (−0.96 g C-CO2 m−2 d−1) but relatively weak emitters of CH4 to the atmosphere (0.001 g C-CH4m−2 d−1). When using ecosystem-cover classification mapping, we found that freshwaters were unimportant contributors to total watershed carbon exchange, in part because they covered less than 10 % of total cover in the watershed. High Arctic watersheds are experiencing warmer and wetter climates than in the past, which may have implications for the net uptake of carbon greenhouse gases by currently underproductive polar semidesert and freshwater systems.


2014 ◽  
Vol 11 (3) ◽  
pp. 4251-4299 ◽  
Author(s):  
E. M. Thaysen ◽  
D. Jacques ◽  
S. Jessen ◽  
C. E. Andersen ◽  
E. Laloy ◽  
...  

Abstract. The efflux of carbon dioxide (CO2) from soils influences atmospheric CO2 concentrations and thereby climate change. The partitioning of inorganic carbon fluxes in the vadose zone between emission to the atmosphere and to the groundwater was investigated. Carbon dioxide partial pressure in the soil gas (pCO2), alkalinity, soil moisture and temperature were measured over depth and time in unplanted and planted (barley) mesocosms. The dissolved inorganic carbon (DIC) percolation flux was calculated from the pCO2, alkalinity and the water flux at the mesocosm bottom. Carbon dioxide exchange between the soil surface and the atmosphere was measured at regular intervals. The soil diffusivity was determined from soil radon-222 (222Rn) emanation rates and soil air Rn concentration profiles, and was used in conjunction with measured pCO2 gradients to calculate the soil CO2 production. Carbon dioxide fluxes were modelled using the HP1 module of the Hydrus 1-D software. The average CO2 effluxes to the atmosphere from unplanted and planted mesocosm ecosystems during 78 days of experiment were 0.1 ± 0.07 and 4.9 ± 0.07 μmol carbon (C) m−2 s−1, respectively, and largely exceeded the corresponding DIC percolation fluxes of 0.01 ± 0.004 and 0.06 ± 0.03 μmol C m−2 s−1. Post-harvest soil respiration (Rs) was only 10% of the Rs during plant growth, while the post-harvest DIC percolation flux was more than one third of the flux during growth. The Rs was controlled by production and diffusivity of CO2 in the soil. The DIC percolation flux was largely controlled by the pCO2 and the drainage flux due to low solution pH. Plant biomass and soil pCO2 were high in the mesocosms as compared to a standard field situation. Our results indicate no change of the cropland C balance under elevated atmospheric CO2 in a warmer future climate, in which plant biomass and soil pCO2 are expected to increase.


2007 ◽  
Vol 3 (2) ◽  
Author(s):  
Peter Read

This paper focuses on policy instruments designed to drive the preferential adoption of two technology types – involving carbon-conservative processing of the products of the land commercially as food, fibre and fuel (biofuel) – whilst, through tradability, generating the cash flow needed to finance the necessary capital investments. These are technologies for getting carbon dioxide (CO2) out of the atmosphere, and technologies for stocking it (or carbonaceous material derived from atmospheric CO2 somewhere other than in the atmosphere.


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