scholarly journals Semiclassical approach for excitonic spectrum of Coulomb coupling between two Dirac particles

Author(s):  
Victor V. Zalipaev ◽  
Vladislav V. Kuidin

The properties of the energy spectrum of excitons in monolayer transition metal dichalcogenides are investigated using a multiband model. In the multiband model, we use the excitonic Hamiltonian in the product base of the Dirac single-particle states at the conduction and valence band edges. Following the separation of variables, we decouple the corresponding energy eigenvalue system of the first-order ODE radial equations rigorously and solve the resulting second-order ODE self-consistently, using the finite difference method, thus we determine the energy eigenvalues of the discrete excitonic spectrum and the corresponding wave functions. We also developed a WKB approach to solve the same spectral problem in semiclassical approximation for the resulting ODE. We compare the results for the energy spectrum and the corresponding eigen-function forms for WS 2 and WSe 2 obtained by means of both methods. We also compare our results for the energy spectrum with other theoretical works for excitons, and with available experimental data.

2021 ◽  
Vol 2015 (1) ◽  
pp. 012169
Author(s):  
V. Zalipaev ◽  
V. Kuidin

Abstract The properties of screening effect for energy spectrum of excitons in monolayer transition metal dichalcogenides are investigated using a multiband model. The excitonic hamiltonian in the product base of the Dirac single-particle is used. The corresponding energy eigenvalue system of the first order ODE (radial equations) was solved using the finite difference method. This enables to determine the energy eigenvalues of the discrete excitonic spectrum and the wave functions. We compare the results for the energy spectrum and the corresponding eigen-functions forms for WS 2 and WSe 2 computed for two different potentials: pure Coulomb and screened Coulomb (Keldysh potential). It is demonstrated that excitonic energy levels for unscreened potential lie dipper, and the corresponding eigen-functions’ forms differ from those obtained for screened one.


ACS Nano ◽  
2021 ◽  
Author(s):  
Miao Zhang ◽  
Martina Lihter ◽  
Tzu-Heng Chen ◽  
Michal Macha ◽  
Archith Rayabharam ◽  
...  

Author(s):  
Yoobeen Lee ◽  
Jin Won Jung ◽  
Jin Seok Lee

The reduction of intrinsic defects, including vacancies and grain boundaries, remains one of the greatest challenges to produce high-performance transition metal dichalcogenides (TMDCs) electronic systems. A deeper comprehension of the...


Nanoscale ◽  
2021 ◽  
Author(s):  
Thayer Walmsley ◽  
Yaqiong Xu

Group IVB transition metal dichalcogenides (TMDCs) have attracted significant attention due to their predicted high charge carrier mobility, large sheet current density, and enhanced thermoelectric power. Here, we investigate the...


Nanophotonics ◽  
2020 ◽  
Vol 9 (8) ◽  
pp. 2569-2576 ◽  
Author(s):  
Lu Li ◽  
Lihui Pang ◽  
Qiyi Zhao ◽  
Yao Wang ◽  
Wenjun Liu

AbstractTransition metal dichalcogenides have been widely utilized as nonlinear optical materials for laser pulse generation applications. Herein, we study the nonlinear optical properties of a VS2-based optical device and its application as a new saturable absorber (SA) for high-power pulse generation. Few-layer VS2 nanosheets are deposited on the tapered region of a microfiber to form an SA device, which shows a modulation depth of 40.52%. After incorporating the microfiber-VS2 SA into an Er-doped fiber laser cavity, passively Q-switched pulse trains could be obtained with repetition rates varying from 95 to 233 kHz. Under the pump power of 890 mW, the largest output power and shortest pulse duration are measured to be 43 mW and 854 ns, respectively. The high signal-to-noise ratio of 60 dB confirms the excellent stability of the Q-switching state. To the best of our knolowdge, this is the first illustration of using VS2 as an SA. Our experimental results demonstrate that VS2 nanomaterials have a large potential for nonlinear optics applications.


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