A High-Resolution Record of Atmospheric Dust Composition and Variability since a.d. 1650 from a Mount Everest Ice Core

2009 ◽  
Vol 22 (14) ◽  
pp. 3910-3925 ◽  
Author(s):  
S. Kaspari ◽  
P. A. Mayewski ◽  
M. Handley ◽  
S. Kang ◽  
S. Hou ◽  
...  
Keyword(s):  
High Resolution ◽  
Anthropogenic Activities ◽  
Ice Core ◽  
Major And Trace Elements ◽  
Back Trajectory ◽  
Mount Everest ◽  
Atmospheric Dust ◽  
Back Trajectory Analysis ◽  
Anthropogenic Inputs ◽  
Dust Generation

Abstract A Mount Everest ice core analyzed at high resolution for major and trace elements (Sr, Cs, Ba, La, Ce, Pr, Nd, Sm, Eu, Tb, Dy, Ho, Er, Tm, Yb, Lu, Bi, U, Tl, Al, S, Ca, Ti, V, Cr, Mn, Fe, Co) and spanning the period a.d. 1650–2002 is used to investigate the sources of and variations in atmospheric dust through time. The chemical composition of dust varies seasonally, and peak dust concentrations occur during the winter–spring months. Significant correlations between the Everest dust record and dust observations at stations suggest that the Everest record is representative of regional variations in atmospheric dust loading. Back-trajectory analysis in addition to a significant correlation of Everest dust concentrations and the Total Ozone Mapping Spectrometer (TOMS) aerosol index indicates that the dominant winter sources of dust are the Arabian Peninsula, Thar Desert, and northern Sahara. Factors that contribute to dust generation at the surface include soil moisture and temperature, and the long-range transport of dust aerosols appears to be sensitive to the strength of 500-mb zonal winds. There are periods of high dust concentration throughout the 350-yr Mount Everest dust record; however, there is an increase in these periods since the early 1800s. The record was examined for recent increases in dust emissions associated with anthropogenic activities, but no recent dust variations can be conclusively attributed to anthropogenic inputs of dust.

A High-Resolution Record of Atmospheric Dust Composition and Variability Since 1650 AD from a Mt. Everest Ice Core

2007 ◽  
Vol preprint (2008) ◽  
pp. 1
Author(s):  
S. Kaspari ◽  
P. A. Mayewski ◽  
M. Handley ◽  
S. Kang ◽  
S. Hou ◽  
...  
Keyword(s):  
High Resolution ◽  
Ice Core ◽  
Atmospheric Dust ◽  
Dust Composition

scholarly journals Heavy Metals in PM10 Aerosols Over an Urban Industrial City

2019 ◽  
Vol 9 (1) ◽  
pp. 1402-1408
Keyword(s):  
Heavy Metal ◽  
Anthropogenic Activities ◽  
Winter Season ◽  
Principal Component ◽  
Heavy Metal Concentration ◽  
Back Trajectory ◽  
Air Masses ◽  
Back Trajectory Analysis ◽  
Source Correlation ◽  
Heavy Metal Determination

PM10 aerosols were monitored and analyzed for heavy metal concentration at Raipur city Chhattisgarh, India for possible source identification of pollutants. Sampling of PM10 aerosols was carried out by using respirable dust sampler during the year 2016. Daily PM10 average concentrations varied between 122.033 and 197.854 µg/m3, 91.350 and 133.950 µg/m3 and 112.770 and 480.170 µg/m3 in summer, monsoon and winter respectively. Chemical analysis of PM10 samples was carried out for heavy metal determination. Heavy metal (Fe, Mn, Ni and Pb) were analyzed with the help of atomic absorption spectroscopy (AAS) and found in the range of 2.713-36.862, 0.131-9.129. 0.880-4.195 and 0.015-0.321 µg/m3 for Fe, Mn, Pb and Ni respectively. PM10 concentrations shows distinct seasonal variation being twice in winter season than in summer; winter (mean: 241.820 ± 33.912 µg/m3) > summer (mean: 159.512 ± 14.360 µg/m3) > monsoon (mean: 107.480 ± 9.213 µg/m3). The concentration of heavy metal was different in all the seasons depending on their sources. Identification of possible sources was done by principal component analysis (PCA) illustrating industrial activities, soil (crustal) dust and biomass burning as the major sources in the region. The back trajectory analysis of the air masses depicts that the local anthropogenic activities affect the concentration of pollutants at the source. Correlation analysis between the heavy metal concentrations agreed the results obtained by PCA. The work helped in observing the seasonal trend of particulate matter concentrations and in identification of major sources of air pollution in the city.

scholarly journals Preliminary Evidence for the Role Played by South Westerly Wind Strength on the Marine Diatom Content of an Antarctic Peninsula Ice Core (1980–2010)

Geosciences ◽  
2020 ◽  
Vol 10 (3) ◽  
pp. 87
Author(s):  
Claire S. Allen ◽  
Elizabeth R. Thomas ◽  
Hilary Blagbrough ◽  
Dieter R. Tetzner ◽  
Richard A. Warren ◽  
...  
Keyword(s):  
Antarctic Peninsula ◽  
Ice Core ◽  
Preliminary Evidence ◽  
Marine Diatom ◽  
Back Trajectory ◽  
Westerly Wind ◽  
Ice Shelves ◽  
Air Masses ◽  
Back Trajectory Analysis ◽  
New Evidence

Winds in the Southern Ocean drive exchanges of heat and carbon dioxide between the ocean and atmosphere. Wind dynamics also explain the dominant patterns of both basal and surface melting of glaciers and ice shelves in the Amundsen and Bellingshausen Seas. Long records of past wind strength and atmospheric circulation are needed to assess the significance of these recent changes. Here we present evidence for a novel proxy of past south westerly wind (SWW) strength over the Amundsen and Bellingshausen Seas, based on diatoms preserved in an Antarctic Peninsula ice core. Ecological affinities of the identified diatom taxa indicate an almost exclusively marine assemblage, dominated by open ocean taxa from the Northern Antarctic Zone (NAZ). Back-trajectory analysis shows the routes of air masses reaching the ice core site and reveals that many trajectories involve contact with surface waters in the NAZ of the Amundsen and Bellingshausen Seas. Correlation analyses between ice core diatom abundance and various wind vectors yield positive and robust coefficients for the 1980–2010 period, with average annual SWW speeds exhibiting the strongest match. Collectively, the data presented here provide new evidence that diatoms preserved in an Antarctic Peninsula ice core offer genuine potential as a new proxy for SWW strength.

A high‐resolution atmospheric dust record for 1810–2004 A.D. derived from an ice core in eastern Tien Shan, central Asia

2017 ◽  
Vol 122 (14) ◽  
pp. 7505-7518 ◽  
Author(s):  
Wangbin Zhang ◽  
Shugui Hou ◽  
Yaping Liu ◽  
Shuangye Wu ◽  
Wenling An ◽  
...  
Keyword(s):  
High Resolution ◽  
Central Asia ◽  
Ice Core ◽  
Tien Shan ◽  
Atmospheric Dust

scholarly journals One-Year Measurements of Equivalent Black Carbon, Optical Properties, and Sources in the Urumqi River Valley, Tien Shan, China

Atmosphere ◽  
2020 ◽  
Vol 11 (5) ◽  
pp. 478 ◽  
Author(s):  
Xin Zhang ◽  
Zhongqin Li ◽  
Jing Ming ◽  
Feiteng Wang
Keyword(s):  
Central Asia ◽  
Black Carbon ◽  
Anthropogenic Activities ◽  
River Valley ◽  
Tien Shan ◽  
Back Trajectory ◽  
Long Distance ◽  
Boundary Layer Height ◽  
Back Trajectory Analysis ◽  
Moderate Resolution Imaging Spectroradiometer

Equivalent black carbon (EBC) was measured with a seven-wavelength Aethalometer (AE-31) in the Urumqi River Valley, eastern Tien Shan, China. This is the first high-resolution, online measurement of EBC conducted in the eastern Tien Shan allowing analysis of the seasonal and hourly variations of the light absorption properties of EBC. Results showed that the highest concentrations of EBC were in autumn, followed by those in summer. The hourly variations of EBC showed two plateaus during 8:00–9:00 h local time (LT) and 16:00–19:00 h LT, respectively. The contribution of biomass burning to EBC in winter and spring was higher than in summer and autumn. The planetary boundary layer height (PBLH) showed an inverse relationship with EBC concentrations, suggesting that the reduction of the PBLH leads to enhanced EBC. The aerosol optical depths (AOD) over the Urumqi River Valley, derived from the Moderate Resolution Imaging Spectroradiometer (MODIS) data and back trajectory analysis, showed that the pollution from Central Asia was more likely to affect the atmosphere of Tien Shan in summer and autumn. This suggests that long-distance transported pollutants from Central Asia could also be potential contributors to EBC concentrations in the Urumqi River Valley, the same as local anthropogenic activities.

scholarly journals A comparison of annual layer thickness model estimates with observational measurements using the Berkner Island ice core, Antarctica

2017 ◽  
Vol 29 (4) ◽  
pp. 382-393
Author(s):  
A. Massam ◽  
S.B. Sneed ◽  
G.P. Lee ◽  
R.R. Tuckwell ◽  
R. Mulvaney ◽  
...  
Keyword(s):  
High Resolution ◽  
Layer Thickness ◽  
Inductively Coupled Plasma ◽  
Ice Core ◽  
Ultra Violet ◽  
Analytical Techniques ◽  
Inductively Coupled ◽  
Annual Layer ◽  
Icp Ms ◽  
Chemical Profiles

AbstractA model to estimate the annual layer thickness of deposited snowfall at a deep ice core site, compacted by vertical strain with respect to depth, is assessed using ultra-high-resolution laboratory analytical techniques. A recently established technique of high-resolution direct chemical analysis of ice using ultra-violet laser ablation inductively-coupled plasma mass spectrometry (LA ICP-MS) has been applied to ice from the Berkner Island ice core, and compared with results from lower resolution techniques conducted on parallel sections of ice. The results from both techniques have been analysed in order to assess the capability of each technique to recover seasonal cycles from deep Antarctic ice. Results do not agree with the annual layer thickness estimates from the age–depth model for individual samples <1 m long as the model cannot reconstruct the natural variability present in annual accumulation. However, when compared with sections >4 m long, the deviation between the modelled and observational layer thicknesses is minimized to within two standard deviations. This confirms that the model is capable of successfully estimating mean annual layer thicknesses around analysed sections. Furthermore, our results confirm that the LA ICP-MS technique can reliably recover seasonal chemical profiles beyond standard analytical resolution.

scholarly journals Quantification of southwest China rainfall during the 8.2 ka BP event with response to North Atlantic cooling

2016 ◽  
Vol 12 (7) ◽  
pp. 1583-1590 ◽  
Author(s):  
Yuhui Liu ◽  
Chaoyong Hu
Keyword(s):  
High Resolution ◽  
Southwest China ◽  
East Asian Monsoon ◽  
Moving Average ◽  
Ice Core ◽  
Scale Model ◽  
Annual Rainfall ◽  
Transport Pathway ◽  
Mean Annual Rainfall ◽  
Monsoon Area

Abstract. The 8.2 ka BP event could provide important information for predicting abrupt climate change in the future. Although published records show that the East Asian monsoon area responded to the 8.2 ka BP event, there is no high-resolution quantitative reconstructed climate record in this area. In this study, a reconstructed 10-year moving average annual rainfall record in southwest China during the 8.2 ka BP event is presented by comparing two high-resolution stalagmite δ18O records from Dongge cave and Heshang cave. This decade-scale rainfall reconstruction is based on a central-scale model and is confirmed by inter-annual monitoring records, which show a significant positive correlation between the regional mean annual rainfall and the drip water annual average δ18O difference from two caves along the same monsoon moisture transport pathway from May 2011 to April 2014. Similar trends between the reconstructed rainfall and the stalagmite Mg ∕ Ca record, another proxy of rainfall, during the 8.2 ka BP period further increase the confidence of the quantification of the rainfall record. The reconstructed record shows that the mean annual rainfall in southwest China during the central 8.2 ka BP event is less than that of present (1950–1990) by  ∼  200 mm and decreased by  ∼  350 mm in  ∼  70 years experiencing an extreme drying period lasting for  ∼  50 years. Comparison of the reconstructed rainfall record in southwest China with Greenland ice core δ18O and δ15N records suggests that the reduced rainfall in southwest China during the 8.2 ka BP period was coupled with Greenland cooling with a possible response rate of 110 ± 30 mm °C−1.

scholarly journals A 60-year ice-core record of regional climate from Adélie Land, coastal Antarctica

2017 ◽  
Vol 11 (1) ◽  
pp. 343-362 ◽  
Author(s):  
Sentia Goursaud ◽  
Valérie Masson-Delmotte ◽  
Vincent Favier ◽  
Susanne Preunkert ◽  
Michel Fily ◽  
...  
Keyword(s):  
High Resolution ◽  
Sea Ice ◽  
Interannual Variability ◽  
Ice Core ◽  
Ice Sheet ◽  
Sea Ice Extent ◽  
Antarctic Ice Sheet ◽  
Ice Core Record ◽  
Decadal Variations ◽  
The Mean

Abstract. A 22.4 m-long shallow firn core was extracted during the 2006/2007 field season from coastal Adélie Land. Annual layer counting based on subannual analyses of δ18O and major chemical components was combined with 5 reference years associated with nuclear tests and non-retreat of summer sea ice to build the initial ice-core chronology (1946–2006), stressing uncertain counting for 8 years. We focus here on the resulting δ18O and accumulation records. With an average value of 21.8 ± 6.9 cm w.e. yr−1, local accumulation shows multi-decadal variations peaking in the 1980s, but no long-term trend. Similar results are obtained for δ18O, also characterised by a remarkably low and variable amplitude of the seasonal cycle. The ice-core records are compared with regional records of temperature, stake area accumulation measurements and variations in sea-ice extent, and outputs from two models nudged to ERA (European Reanalysis) atmospheric reanalyses: the high-resolution atmospheric general circulation model (AGCM), including stable water isotopes ECHAM5-wiso (European Centre Hamburg model), and the regional atmospheric model Modèle Atmosphérique Régional (AR). A significant linear correlation is identified between decadal variations in δ18O and regional temperature. No significant relationship appears with regional sea-ice extent. A weak and significant correlation appears with Dumont d'Urville wind speed, increasing after 1979. The model-data comparison highlights the inadequacy of ECHAM5-wiso simulations prior to 1979, possibly due to the lack of data assimilation to constrain atmospheric reanalyses. Systematic biases are identified in the ECHAM5-wiso simulation, such as an overestimation of the mean accumulation rate and its interannual variability, a strong cold bias and an underestimation of the mean δ18O value and its interannual variability. As a result, relationships between simulated δ18O and temperature are weaker than observed. Such systematic precipitation and temperature biases are not displayed by MAR, suggesting that the model resolution plays a key role along the Antarctic ice sheet coastal topography. Interannual variations in ECHAM5-wiso temperature and precipitation accurately capture signals from meteorological data and stake observations and are used to refine the initial ice-core chronology within 2 years. After this adjustment, remarkable positive (negative) δ18O anomalies are identified in the ice-core record and the ECHAM5-wiso simulation in 1986 and 2002 (1998–1999), respectively. Despite uncertainties associated with post-deposition processes and signal-to-noise issues, in one single coastal ice-core record, we conclude that the S1C1 core can correctly capture major annual anomalies in δ18O as well as multi-decadal variations. These findings highlight the importance of improving the network of coastal high-resolution ice-core records, and stress the skills and limitations of atmospheric models for accumulation and δ18O in coastal Antarctic areas. This is particularly important for the overall East Antarctic ice sheet mass balance.

scholarly journals High-resolution glacial and deglacial record of atmospheric methane by continuous-flow and laser spectrometer analysis along the NEEM ice core

2013 ◽  
Vol 9 (6) ◽  
pp. 2579-2593 ◽  
Author(s):  
J. Chappellaz ◽  
C. Stowasser ◽  
T. Blunier ◽  
D. Baslev-Clausen ◽  
E. J. Brook ◽  
...  
Keyword(s):  
High Resolution ◽  
Continuous Flow ◽  
Ice Core ◽  
Rate Of Change ◽  
Atmospheric Methane ◽  
Data Set ◽  
Rate Of Increase ◽  
Concentration Changes ◽  
Cross Dating ◽  
Laser Spectroscopic

Abstract. The Greenland NEEM (North Greenland Eemian Ice Drilling) operation in 2010 provided the first opportunity to combine trace-gas measurements by laser spectroscopic instruments and continuous-flow analysis along a freshly drilled ice core in a field-based setting. We present the resulting atmospheric methane (CH4) record covering the time period from 107.7 to 9.5 ka b2k (thousand years before 2000 AD). Companion discrete CH4 measurements are required to transfer the laser spectroscopic data from a relative to an absolute scale. However, even on a relative scale, the high-resolution CH4 data set significantly improves our knowledge of past atmospheric methane concentration changes. New significant sub-millennial-scale features appear during interstadials and stadials, generally associated with similar changes in water isotopic ratios of the ice, a proxy for local temperature. In addition to the midpoint of Dansgaard–Oeschger (D/O) CH4 transitions usually used for cross-dating, sharp definition of the start and end of these events brings precise depth markers (with ±20 cm uncertainty) for further cross-dating with other palaeo- or ice core records, e.g. speleothems. The method also provides an estimate of CH4 rates of change. The onsets of D/O events in the methane signal show a more rapid rate of change than their endings. The rate of CH4 increase associated with the onsets of D/O events progressively declines from 1.7 to 0.6 ppbv yr−1 in the course of marine isotope stage 3. The largest observed rate of increase takes place at the onset of D/O event #21 and reaches 2.5 ppbv yr−1.

scholarly journals Use of Low-Cost Ambient Particulate Sensors in Nablus, Palestine with Application to the Assessment of Regional Dust Storms

Atmosphere ◽  
2019 ◽  
Vol 10 (9) ◽  
pp. 539
Author(s):  
Abdelhaleem Khader ◽  
Randal S. Martin
Keyword(s):  
Low Cost ◽  
Dust Storms ◽  
Air Pollutant ◽  
World Health ◽  
Back Trajectory ◽  
Hysplit Model ◽  
Air Masses ◽  
Palestinian Territories ◽  
Back Trajectory Analysis ◽  
Lower Elevation

Few air pollutant studies within the Palestinian territories have been reported in the literature. In March–April and May–June of 2018, three low-cost, locally calibrated particulate monitors (AirU’s) were deployed at different elevations and source areas throughout the city of Nablus in Northern West Bank, Palestine. During each of the three-week periods, high but site-to-site similar particulate matter less than 2.5 µm in aerodynamic diameter (PM2.5) and less than 10 µm (PM10) concentrations were observed. The PM2.5 concentrations at the three sampling locations and during both sampling periods averaged 38.2 ± 3.6 µg/m3, well above the World Health Organization’s (WHO) 24 h guidelines. Likewise, the PM10 concentrations exceeded or were just below the WHO’s 24 h guidelines, averaging 48.5 ± 4.3 µg/m3. During both periods, short episodes were identified in which the particulate levels at all three sites increased substantially (≈2×) above the regional baseline. Air mass back trajectory analyses using U.S. National Oceanic and Atmospheric Administration’s (NOAA) Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model suggested that, during these peak episodes, the arriving air masses spent recent days over desert areas (e.g., the Saharan Desert in North Africa). On days with regionally low PM2.5 concentrations (≈20 µg/m3), back trajectory analysis showed that air masses were directed in from the Mediterranean Sea area. Further, the lower elevation (downtown) site often recorded markedly higher particulate levels than the valley wall sites. This would suggest locally derived particulate sources are significant and may be beneficial in the identification of potential remediation options.

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