Long-Range Transport of Anthropogenically and Naturally Produced Particulate Matter in the Mediterranean and North Atlantic: Current State of Knowledge

2007 ◽  
Vol 46 (8) ◽  
pp. 1230-1251 ◽  
Author(s):  
George Kallos ◽  
Marina Astitha ◽  
Petros Katsafados ◽  
Chris Spyrou

Abstract During the past 20 years, organized experimental campaigns as well as continuous development and implementation of air-pollution modeling have led to significant gains in the understanding of the paths and scales of pollutant transport and transformation in the greater Mediterranean region (GMR). The work presented in this paper has two major objectives: 1) to summarize the existing knowledge on the transport paths of particulate matter (PM) in the GMR and 2) to illustrate some new findings related to the transport and transformation properties of PM in the GMR. Findings from previous studies indicate that anthropogenically produced air pollutants from European sources can be transported over long distances, reaching Africa, the Atlantic Ocean, and North America. The PM of natural origin, like Saharan dust, can be transported toward the Atlantic Ocean and North America mostly during the warm period of the year. Recent model simulations and studies in the area indicate that specific long-range transport patterns of aerosols, such as the transport from Asia and the Indian Ocean, central Africa, or America, have negligible or at best limited contribution to air-quality degradation in the GMR when compared with the other sources. Also, new findings from this work suggest that the imposed European Union limits on PM cannot be applicable for southern Europe unless the origin (natural or anthropogenic) of the PM is taken into account. The impacts of high PM levels in the GMR are not limited only to air quality, but also include serious implications for the water budget and the regional climate. These are issues that require extensive investigation because the processes involved are complex, and further model development is needed to include the relevant physicochemical processes properly.

2008 ◽  
Vol 8 (11) ◽  
pp. 2999-3014 ◽  
Author(s):  
A. van Donkelaar ◽  
R. V. Martin ◽  
W. R. Leaitch ◽  
A. M. Macdonald ◽  
T. W. Walker ◽  
...  

Abstract. We interpret a suite of satellite, aircraft, and ground-based measurements over the North Pacific Ocean and western North America during April–May 2006 as part of the Intercontinental Chemical Transport Experiment Phase B (INTEX-B) campaign to understand the implications of long-range transport of East Asian emissions to North America. The Canadian component of INTEX-B included 33 vertical profiles from a Cessna 207 aircraft equipped with an aerosol mass spectrometer. Long-range transport of organic aerosols was insignificant, contrary to expectations. Measured sulfate plumes in the free troposphere over British Columbia exceeded 2 μg/m3. We update the global anthropogenic emission inventory in a chemical transport model (GEOS-Chem) and use it to interpret the observations. Aerosol Optical Depth (AOD) retrieved from two satellite instruments (MISR and MODIS) for 2000–2006 are analyzed with GEOS-Chem to estimate an annual growth in Chinese sulfur emissions of 6.2% and 9.6%, respectively. Analysis of aircraft sulfate measurements from the NASA DC-8 over the central Pacific, the NSF C-130 over the east Pacific and the Cessna over British Columbia indicates most Asian sulfate over the ocean is in the lower free troposphere (800–600 hPa), with a decrease in pressure toward land due to orographic effects. We calculate that 56% of the measured sulfate between 500–900 hPa over British Columbia is due to East Asian sources. We find evidence of a 72–85% increase in the relative contribution of East Asian sulfate to the total burden in spring off the northwest coast of the United States since 1985. Campaign-average simulations indicate anthropogenic East Asian sulfur emissions increase mean springtime sulfate in Western Canada at the surface by 0.31 μg/m3 (~30%) and account for 50% of the overall regional sulfate burden between 1 and 5 km. Mean measured daily surface sulfate concentrations taken in the Vancouver area increase by 0.32 μg/m3 per 10% increase in the simulated fraction of Asian sulfate, and suggest current East Asian emissions episodically degrade local air quality by more than 1.5 μg/m3.


2018 ◽  
Vol 18 (7) ◽  
pp. 1734-1745 ◽  
Author(s):  
Leila Droprinchinski Martins ◽  
Ricardo Hallak ◽  
Rafaela Cruz Alves ◽  
Daniela S. de Almeida ◽  
Rafaela Squizzato ◽  
...  

2015 ◽  
Vol 15 (22) ◽  
pp. 32323-32365 ◽  
Author(s):  
G. Ancellet ◽  
J. Pelon ◽  
J. Totems ◽  
P. Chazette ◽  
A. Bazureau ◽  
...  

Abstract. Long range transport of biomass burning (BB) aerosols between North America and the Mediterranean region took place in June 2013. A large number of ground based and airborne lidar measurements were deployed in the Western Mediterranean during the Chemistry-AeRosol Mediterranean EXperiment (ChArMEx) intensive observation period. A detailed analysis of the potential North American aerosol sources is conducted including the assessment of their transport to Europe using forward simulations of the FLEXPART Lagrangian particle dispersion model initialized using satellite observations by MODIS and CALIOP. The three dimensional structure of the aerosol distribution in the ChArMEx domain observed by the ground-based lidars (Menorca, Barcelona and Lampedusa), a Falcon-20 aircraft flight and three CALIOP tracks, agree very well with the model simulation of the three major sources considered in this work: Canadian and Colorado fires, a dust storm from Western US and the contribution of Saharan dust streamers advected from the North Atlantic trade wind region into the Westerlies region. Four aerosol types were identified using the optical properties of the observed aerosol layers (aerosol depolarization ratio, lidar ratio) and the transport model analysis of the contribution of each aerosol source: (I) pure BB layer, (II) weakly dusty BB, (III) significant mixture of BB and dust transported from the trade wind region (IV) the outflow of Saharan dust by the subtropical jet and not mixed with BB aerosol. The contribution of the Canadian fires is the major aerosol source during this episode while mixing of dust and BB is only significant at altitude above 5 km. The mixing corresponds to a 20–30 % dust contribution in the total aerosol backscatter. The comparison with the MODIS AOD horizontal distribution during this episode over the Western Mediterranean sea shows that the Canadian fires contribution were as large as the direct northward dust outflow from Sahara.


2017 ◽  
Author(s):  
Zhe Jiang ◽  
Helen Worden ◽  
John R. Worden ◽  
Daven K. Henze ◽  
Dylan B. A. Jones ◽  
...  

Abstract. Decreases in surface emissions of nitrogen oxides (NOx = NO + NO2) in North America have led to substantial improvements in air-quality over the last several decades. Here we show that satellite observations of tropospheric nitrogen dioxide (NO2) columns over the contiguous United States (US) do not decrease after about 2009, while surface NO2 concentrations continue to decline through to the present. This divergence, if it continues, could have a substantial impact on surface air quality due to mixing of free-tropospheric air into the boundary layer. Our results show only limited contributions from local effects such as fossil fuel emissions, lightning, or instrument artifacts, but we do find a possible relationship of NO2 changes to decadal climate variability. Our analysis demonstrates that the intensity of transpacific transport is stronger in El Niño years and weaker in La Niña years, and consequently, that decadal-scale climate variability impacts the contribution of Asian emissions on North American atmospheric composition. Because of the short lifetime, it is usually believed that the direct contribution of long-range transport to tropospheric NOx distribution is limited. If our hypothesis about transported Asian emissions is correct, then this observed divergence between satellite and surface NOx could indicate mechanisms that allow for either NOx or its reservoir species to have a larger than expected effect on North American tropospheric composition. These results therefore suggest more aircraft and satellite studies to determine the possible missing processes in our understanding of the long-range transport of tropospheric NOx.


SOLA ◽  
2005 ◽  
Vol 1 ◽  
pp. 121-124 ◽  
Author(s):  
Chan Bong Park ◽  
Nobuo Sugimoto ◽  
Ichiro Matsui ◽  
Atsushi Shimizu ◽  
Boyan Tatarov ◽  
...  

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