atmospheric particulate
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2021 ◽  
Vol 2139 (1) ◽  
pp. 012003
Author(s):  
A D Pinzón-Hassan ◽  
V Tique-Ortiz ◽  
C A Zafra-Mejía

Abstract The objective of this paper is to show the development of Box-Jenkins stochastic models to study the behavior of air pollutants concentrations in the megacity of Bogotá, Colombia. Information was collected from 10 stations in the city’s air quality monitoring network over a ten-year period. The temporal relationship between air pollutants, their spatial variation, and the occurrence of extreme pollution episodes was studied using Box-Jenkins models. The results showed that the moving average term of the models developed was the main indicator of spatial distribution for the daily pollutant concentrations. In the case of atmospheric particulate matter < 10 μm, the following spatial distribution was identified in the megacity: northwestern, center-southwest, and southeast. For atmospheric particulate matter < 2.5 μm: north, center, and southwest. For ozone: northwest, center, and south. Maximum hourly particulate matter concentrations were observed between 6-10 a.m., and between 11 a.m. - 4 p.m. for ozone. Monthly, the highest particulate matter concentrations were observed in February (14.1%), January (13.5%), and March (12.2%). In the context of atmospheric physics, this study was relevant for the following findings: The usefulness of Box-Jenkins models in simulating the temporal behavior of air pollutants, and for their adequate performance in detecting urban spatial trends.


Author(s):  
Joel Sánchez-Piñero ◽  
Paula Gómez-Meijide ◽  
Estefanía Concha-Graña ◽  
Jorge Moreda-Piñeiro ◽  
Soledad Muniategui-Lorenzo ◽  
...  

AbstractPolycyclic aromatic hydrocarbons (PAHs) in atmospheric particulate matter have adverse effects on human health, yet total PAH concentrations should overestimate the toxicity compared to the bioavailable amount of PAHs. To explore this hypothesis, we measured PAHs oral bioavailability in vitro in particulate matter with aerodynamic diameter lower than 10 µm (PM10) using a test that mimics the human digestive system. This assay combines the use of simulated gastrointestinal fluids and a dialysis membrane to simulate intestinal absorption. Results show that oral PAH bioavailability was below 5%, with fluorene, anthracene, acenaphthene and phenanthrene as the most bioavailable PAHs. Data suggest no carcinogenic risk of oral bioavailable PM10-bound PAHs following a health risk assessment via inhalation-ingestion by using benzo(a)pyrene-equivalent carcinogenic concentration and hazard indexes. To our best knowledge, this is the first research study of in vitro oral bioavailability estimation of PM10-associated PAHs.


2021 ◽  
Author(s):  
Adam Matthew Brighty ◽  
Véronique Jacob ◽  
Gaëlle Uzu ◽  
Lucille Borlaza ◽  
Sebastien Conil ◽  
...  

2021 ◽  
Author(s):  
Karuna Singh ◽  
Dhananjay Tripathi

This chapter provides an introduction to particulate matter by discussing various ways of categorisation, characterisation and their health effects. The natural and anthropogenic sources of atmospheric particulate matter are discussed. The chapter also introduces qualitatively some aerosol concepts, such as their chemical composition and size distribution. Some examples are provided to illustrate how particulate matter, despite being microscopic particles, can manifest themselves in the atmosphere. Finally, the various pathways by which particulate matter impacts the health system are reviewed along with their interactions to understand concept behind the PM-associated health effects.


Atmosphere ◽  
2021 ◽  
Vol 12 (11) ◽  
pp. 1467
Author(s):  
Kai Xiao ◽  
Yichun Lin ◽  
Qingyue Wang ◽  
Senlin Lu ◽  
Weiqian Wang ◽  
...  

Environmentally persistent free radicals (EPFRs) were previously considered an unrecognized composition of air pollutants and might help explain the long-standing medical mystery of why non-smokers develop tobacco-related diseases such as lung cancer. However, there is no investigated on EPFRs in Xuanwei rural areas, especially in high prevalence of lung cancer areas. In this study, we selected six types of coal and three types of biomass in Xuanwei, then conducted simulated combustion, and six group of atmospheric particulate matters (APMs) to explore the content and particle size distribution pattern of EPFRs and a new health risk assessment method to evaluate the risk of EPFRs in PM for adults and children. Our results show that the contribution of EPFRs for biomass combustion, coal combustion and APMs were mainly distributed in the size range of <1.1 μm, which accounted for 76.15 ± 4.14%, 74.85 ± 10.76%, and 75.23 ± 8.18% of PM3.3. The mean g factors and ΔHp-p indicated that the EPFRs were mainly oxygen-centered radicals in PM in Xuanwei. The results suggest that the health risk of EPFRs is significantly increased when the particle size distribution of EPFRs is taken into account, and coal combustion particulate matter (174.70 ± 37.86 cigarettes for an adult, 66.39 ± 14.39 cigarettes per person per year for a child) is more hazardous to humans than biomass combustion particulate matter (69.41 ± 4.83 cigarettes for an adult, 26.37 ± 1.84 cigarettes per person per year for), followed by APMs (102.88 ± 39.99 cigarettes for an adult, 39.10 ±15.20 cigarettes per person per year for) in PM3.3. Our results provides a new perspective and evidence for revealing the reason for the high incidence of lung cancer in Xuanwei, China.


Atmosphere ◽  
2021 ◽  
Vol 12 (11) ◽  
pp. 1393
Author(s):  
Qianjun Mao ◽  
Fangyuan Cheng ◽  
Min Chen

Air pollution has a significant impact on the use of solar energy. On the one hand, the polluted environment directly reduces the intensity of solar radiation, on the other hand, pollution of the environment will also reduce the life of the equipment. Therefore, mastering the dynamic characteristics of the atmospheric environment has certain guiding significance for the efficient utilization of solar energy. In this study, the concentrations of particulate matter, CO, SO2 and NO2 from Tianyun big data website are analyzed to obtain the general characteristics of particulate pollution in Wuhan. At the same time, a long-period sampling atmospheric particulate matter sampler in the Huangjiahu area of Wuhan has been used, and experimental analysis of the physical and chemical characteristics of the samples has been obtained. The results show that both PM2.5 and PM10 show obvious seasonal changes, and the concentration of the four anions during the sampling period is SO42− > NO3− > Cl− > F−. During the sampling period, atmospheric particulate matter is mainly composed of organic matter, inorganic anions and oxides of more than 20 elements. The results of the enrichment factor analysis show that elements such as Br, Pb, Sb and Zn are the main enriched elements during the sampling period. The enrichment factors of these elements are 246.43 ± 168.81, 133.28 ± 115.03, 403.305 ± 396.18 and 90.67 ± 67.01, respectively. The high enrichment of these elements also reflects the contribution of motor vehicle exhaust emission during the sampling period. Traffic source is the main emission source in the Huangjiahu area of Wuhan. This research has a certain guiding significance for many industries such as energy utilization, environmental monitoring, health care, transportation and so on.


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