As mentioned in the previous chapter, many experiments on food irradiation in the 1950s were carried out with spent-fuel rods from nuclear reactors. Such fuel rods contain a mixture of many fission products, with greatly differing half-lives, emitting different types of radiation with different energies. The composition of fuel rods changes all the time because the radionuclides with short half-lives disappear quickly, whereas those with longer half-lives remain. Although fuel rods are primarily a source of gamma radiation (the less penetrating alpha and beta radiation are absorbed by the steel hull of the rods) they do give off some neutrons. Since the latter can produce radioactivity when they interact with matter such as food, fuel rods have not been used for irraditation of foods since the early 1960s. Because of their constantly varying composition, fuel rods also make dosimetry difficult, and this was another reason for abandoning their use. Individual constituents of spent fuel rods can be separated in reprocessing plants by chemical methods. One of the radionuclides obtainable in this way is Cs. With a half-life of 30 years and emission of gamma radiation (0.66 MeV) and beta radiation (0.51 MeV and 1.18 MeV), '^C s decays to stable '^B a (barium). After the ,37Cs is separated from the other constituents of the fission waste in the form of CsCl it is triply encapsulated in stainless steel containers because CsCl is soluble in water. If it leaked out it could cause contamination of the environment. As provided by the Waste Encapsulation and Storage Facility (WESF) at Hanford, Washington, the 137Cs capsule is 400 mm in active length (500 mm in total length) and 67 mm in diameter. There are only a few reprocessing plants in the world and the capacity for extracting ,37Cs from spent fuel rods is very limited. Plans for building several commercial reprocessing facilities in the United States were canceled by Presi dent Carter’s 1977 decision that the United States would not engage in commer cial reprocessing of spent nuclear fuel. As a consequence, not much ,37Cs is available and there are not many gamma radiation facilities which use ,Cs. No
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2001 ◽
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