The Critical Volume for Nucleation

2010 ◽  
Vol 660-661 ◽  
pp. 279-283 ◽  
Author(s):  
Marcos Flavio de Campos ◽  
José Adilson de Castro

In magnets based in phases with high magnetocrystalline anisotropy like Nd2Fe14B or SmCo5 there is a competition between magnetostatic energy and domain wall energies. If the grain size is large, the formation of domain walls is energetically favorable. When the formation of domain walls is an unfavorable process, coercivity is larger. A better comprehension of this phenomenon is possible if the energy necessary for the first domain wall formation is properly evaluated. To address this problem, the magnetostatic energy of a sphere magnetized in two opposite directions, separated by a domain wall, is calculated using Legendre Polynomials. The data allow the determination of the reversible volume for nucleation. It is predicted a “recoil effect”, the magnetization may be reversible until a given volume of reverse magnetization.

2001 ◽  
Vol 674 ◽  
Author(s):  
M.I. Rosales ◽  
H. Montiel ◽  
R. Valenzuela

ABSTRACTAn investigation of the frequency behavior of polycrystalline ferrites is presented. It is shown that the low frequency dispersion (f < 10 MHz) of permeability is associated with the bulging of pinned domain walls, and has a mixed resonance-relaxation character, closer to the latter. It is also shown that there is a linear relationship between the magnetocrystalline anisotropy constant, K1, and the relaxation frequency. The slope of this correlation depends on the grain size. Such a relationship could allow the determination of this basic parameter from polycrystalline samples.


1987 ◽  
Vol 96 ◽  
Author(s):  
F. E. Pinkerton

ABSTRACTInitial magnetization and demagnetization data are reported for three forms of rapidly solidified Nd-Fe-B permanent magnet materials: melt-spun ribbons, hot pressed magnets, and die upset magnets. In all three materials the results are consistent with domain wall pinning at grain boundary phases as the coercivity mechanism. Optimally quenched ribbons are comprised of randomly oriented single domain Nd2Fe14B grains, and both initial magnetization and demagnetization are controlled by strong domain wall pinning at grain boundaries. Maximum coercivity is accompanied by a low initial permeability. Coercivity is reduced in overquenched ribbons by partial retention of a magnetically soft amorphous or very finely crystalline microstructure. Coercivity decreases in underquenched ribbons because wall pinning weakens as the grain size increases above optimum. Correlation of magnetization and demagnetization behaviors suggests that maximum coercivity in ribbons is largely determined by the resistance to domain wall formation in grains smaller than the single domain particle limit. Grain size is much less important in the aligned die upset magnets. Domain walls are initially free to move until they become strongly pinned at grain edges, and complete magnetization requires an applied field greater than the coercive field. Hot pressed magnets show a mixture of ribbon and die upset behavior.


2012 ◽  
Vol 727-728 ◽  
pp. 157-162 ◽  
Author(s):  
Marcos Flavio de Campos

The effect of crystalline imperfections (as for instance, grain size, inclusions and dislocations) on the coercivity of soft magnetic materials is additive. This only can be explained by an Energy Balance Model. By another hand, the angular dependence of the coercivity only can be explained with a Force Balance Model. Thus both models, Energy Balance and Force Balance have to be invoked for the construction of a general model. The effect of dislocations on the coercivity can be treated as short range magnetostrictive effect. The effect of inclusions needs the consideration of the global magnetostatic energy of the system. The dependence of the coercivity with the grain size can also be explained analyzing the magnetostatic energy. The idea of pinning of domain walls by crystalline defects is reformulated, and it is shown that the coercivity increase due to crystalline defects is principally caused by variations of the magnetostatic energy in the system.


2012 ◽  
Vol 2012 ◽  
pp. 1-21 ◽  
Author(s):  
Eduardo Martinez

The current-induced domain wall motion along thin ferromagnetic strips with high perpendicular magnetocrystalline anisotropy is studied by means of full micromagnetic simulations and the extended one-dimensional model, taking into account thermal effects and edge roughness. A slow creep regime, where the motion is controlled by wall pinning and thermal activation, and a flow regime with linear variation of the DW velocity, are observed. In asymmetric stacks, where the Rashba spin-orbit field stabilizes the domain wall against turbulent transformations, the steady linear regime is extended to higher currents, leading to higher velocities than in single-layer or symmetric stacks. The pinning and depinning at and from a local constriction were also studied. The results indicate that engineering pinning sites in these strips provide an efficient pathway to achieve both high stability against thermal fluctuations and low-current depinning avoiding Joule heating. Finally, the current-driven dynamics of a pinned domain wall is examined, and both the direct and the alternating contributions to the induced voltage signal induced are characterized. It was confirmed that the direct contribution to the voltage signal can be linearly enhanced with the number of pinned walls, an observation which could be useful to develop domain-wall-based nano-oscillators.


Author(s):  
B. B. Narod

Abstract. 6-81.3 Mo permalloy, developed in the 1960s for use in high performance ring-core fluxgate sensors, remains the state-of-the-art for permalloy-cored fluxgate magnetometers. The magnetic properties of 6-81.3, namely magnetocrystalline and magnetoelastic anisotropies and saturation induction are all optimum in the Fe–Ni–Mo system. In such polycrystalline permalloy fluxgate sensors a single phenomenon may cause both fluxgate noise and magnetic hysteresis, explain Barkhausen jumps, remanence and coercivity, and avoid domain denucleation. The phenomenon, domain wall reconnection, is presented as part of a theoretical model. In the unmagnetized state a coarse-grain high-quality permalloy foil ideally forms stripe domains, which present at the free surface as parallel, uniformly spaced domain walls that cross the entire thickness of the foil. Leakage flux "in" and "out" of alternating domains is a requirement of the random orientation, grain-by-grain, of magnetic easy axes' angles with respect to the foil free surface. Its magnetostatic energy together with domain wall energy determines an energy budget to be minimized. Throughout the magnetization cycle the free surface domain pattern remains essentially unchanged, due to the magnetostatic energy cost such a change would elicit. Thus domain walls are "pinned" to free surfaces. Driven to saturation, domain walls first bulge then reconnect via Barkhausen jumps to form a new domain configuration this author has called "channel domains", that are attached to free surfaces. The approach to saturation now continues as reversible channel domain compression. Driving the permalloy deeper into saturation compresses the channel domains to arbitrarily small thickness, but will not cause them to denucleate. Returning from saturation the channel domain structure will survive through zero H, thus explaining remanence. The Barkhausen jumps being irreversible exothermic events are sources of fluxgate noise, powered by the energy available from domain wall reconnection. A simplified domain energy model can then provide a predictive relation between ring core magnetic properties and fluxgate sensor noise power. Four properties are predicted to affect noise power, two of which, are well known: saturation total magnetic flux density and magnetic anisotropy. The two additional properties are easy axes alignment and foil thickness. Flux density and magnetic anisotropy are primary magnetic properties determined by an alloy's chemistry and crystalline lattice properties. Easy axes alignment and foil thickness are secondary, geometrical properties related to an alloy's polycrystalline fabric and manufacture. Improvements to fluxgate noise performance can in principle be achieved by optimizing any of these four properties in such a way as to minimize magnetostatic energy. Fluxgate signal power is proportional to B–H loop curvature (d2B/dH2). The degree to which Barkhausen jumps coincide with loop curvature is a measure of noise that accompanies fluxgate signal. B–H loops with significant curvature beyond the open hysteresis loop may be used to advantage to acquire fluxgate signal with reduced noise.


2015 ◽  
Vol 820 ◽  
pp. 199-204 ◽  
Author(s):  
Marcos Flavio de Campos ◽  
Fernanda A. Sampaio da Silva

The applicability of micromagnetics for phases with high magnetocrystalline anisotropy as barium ferrite Ba2Fe12O19and Nd2Fe14B is discussed. The Stoner-Wohlfarth model is very suitable for such phases, and also for PtFe and PtCo. It was discussed how to take into account the total energy of the system for grain size above the single domain particle size. For this situation of large grain size, the net magnetostatic energy of the system cannot be neglected. From energy considerations, it follows that the coercive force should decrease with the inverse of the square root of the grain size.


2012 ◽  
Vol 727-728 ◽  
pp. 140-145 ◽  
Author(s):  
Marcos Flavio de Campos ◽  
José Adilson de Castro

The high uniaxial magnetic anisotropy makes phases like Nd2Fe14B, Sm2Co17, SmCo5or BaFe12O19are very suitable as hard permanent magnetic materials. In the case of ferromagnetic materials, the global magnetostatic energy changes, according to the domain wall configuration. The simplest case to be studied is that of spherical grain with only one domain wall, in phases with uniaxial symmetry. The magnetostic energy in this system is calculated by means of Legendre polynomials. Studying the maximums and minimums of energy in this system, a simple hysteresis model can be developed. The model provides insight about the dependence of the coercive force on the grain size.


2014 ◽  
Vol 3 (2) ◽  
pp. 201-210 ◽  
Author(s):  
B. B. Narod

Abstract. Developed in the 1960s for use in high-performance ring-core fluxgate sensors, 6–81.3 Mo permalloy remains the state of the art for permalloy-cored fluxgate magnetometers. The magnetic properties of 6–81.3, namely magnetocrystalline and magnetoelastic anisotropies and saturation induction, are all optimum in the Fe–Ni–Mo system. In such polycrystalline permalloy fluxgate sensors, a single phenomenon may cause both fluxgate noise and magnetic hysteresis; explain Barkhausen jumps, remanence and coercivity; and avoid domain denucleation. This phenomenon, domain wall reconnection, is presented as part of a theoretical model. In the unmagnetized state a coarse-grain high-quality permalloy foil ideally forms stripe domains, which present at the free surface as parallel, uniformly spaced domain walls that cross the entire thickness of the foil. Leakage flux "in" and "out" of alternating domains is a requirement of the random orientation, grain by grain, of magnetic easy axes' angles with respect to the foil free surface. Its magnetostatic energy together with domain wall energy determines an energy budget to be minimized. Throughout the magnetization cycle the free-surface domain pattern remains essentially unchanged, due to the magnetostatic energy cost such a change would elicit. Thus domain walls are "pinned" to free surfaces. Driven to saturation, domain walls first bulge then reconnect via Barkhausen jumps to form a new domain configuration that I have called "channel domains", which are attached to free surfaces. The approach to saturation now continues as reversible channel domain compression. Driving the permalloy deeper into saturation compresses the channel domains to arbitrarily small thickness, but will not cause them to denucleate. Returning from saturation the channel domain structure will survive through zero H, thus explaining remanence. The Barkhausen jumps, being irreversible exothermic events, are sources of fluxgate noise powered by the energy available from domain wall reconnection. A simplified domain energy model can then provide a predictive relation between ring-core magnetic properties and fluxgate sensor noise power. Four properties are predicted to affect noise power, two of which are well known: saturation total magnetic flux density and magnetic anisotropy. The two additional properties are easy axes alignment and foil thickness. Flux density and magnetic anisotropy are primary magnetic properties determined by an alloy's chemistry and crystalline lattice properties. Easy axes alignment and foil thickness are secondary, geometrical properties related to an alloy's polycrystalline fabric and manufacture. Improvements to fluxgate noise performance can in principle be achieved by optimizing any of these four properties in such a way as to minimize magnetostatic energy. Fluxgate signal power is proportional to B − H loop curvature [d2B/dH2]. The degree to which Barkhausen jumps coincide with loop curvature is a measure of noise that accompanies the fluxgate signal. B − H loops with significant curvature beyond the open hysteresis loop may be used to advantage to acquire the fluxgate signal with reduced noise.


Author(s):  
J.N. Chapman ◽  
P.E. Batson ◽  
E.M. Waddell ◽  
R.P. Ferrier

By far the most commonly used mode of Lorentz microscopy in the examination of ferromagnetic thin films is the Fresnel or defocus mode. Use of this mode in the conventional transmission electron microscope (CTEM) is straightforward and immediately reveals the existence of all domain walls present. However, if such quantitative information as the domain wall profile is required, the technique suffers from several disadvantages. These include the inability to directly observe fine image detail on the viewing screen because of the stringent illumination coherence requirements, the difficulty of accurately translating part of a photographic plate into quantitative electron intensity data, and, perhaps most severe, the difficulty of interpreting this data. One solution to the first-named problem is to use a CTEM equipped with a field emission gun (FEG) (Inoue, Harada and Yamamoto 1977) whilst a second is to use the equivalent mode of image formation in a scanning transmission electron microscope (STEM) (Chapman, Batson, Waddell, Ferrier and Craven 1977), a technique which largely overcomes the second-named problem as well.


Author(s):  
Wenwu Cao

Domain structures play a key role in determining the physical properties of ferroelectric materials. The formation of these ferroelectric domains and domain walls are determined by the intrinsic nonlinearity and the nonlocal coupling of the polarization. Analogous to soliton excitations, domain walls can have high mobility when the domain wall energy is high. The domain wall can be describes by a continuum theory owning to the long range nature of the dipole-dipole interactions in ferroelectrics. The simplest form for the Landau energy is the so called ϕ model which can be used to describe a second order phase transition from a cubic prototype,where Pi (i =1, 2, 3) are the components of polarization vector, α's are the linear and nonlinear dielectric constants. In order to take into account the nonlocal coupling, a gradient energy should be included, for cubic symmetry the gradient energy is given by,


Sign in / Sign up

Export Citation Format

Share Document