scholarly journals Aerosol Single Scattering Albedo retrieval in the UV range: an application to OMI satellite validation

2010 ◽  
Vol 10 (2) ◽  
pp. 331-340 ◽  
Author(s):  
I. Ialongo ◽  
V. Buchard ◽  
C. Brogniez ◽  
G. R. Casale ◽  
A. M. Siani
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Single Scattering ◽  
Single Scattering Albedo ◽  
Spectral Irradiance ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Ozone Monitoring Instrument ◽  
Mean Values ◽  
Absorbing Aerosols

Abstract. The aerosol Single Scattering Albedo (SSA) and Absorbing Aerosol Optical Depth (AAOD) at 320.1 nm are derived at Rome site by the comparison between Brewer and modelled spectra. The UVSPEC radiative transfer model is used to calculate the UV irradiances for different SSA values, taking into account as input data total ozone and Aerosol Optical Depth (AOD) obtained from Brewer spectral measurements. The accuracy in determining SSA depends on the aerosol amount and on Solar Zenith Angle (SZA) value: SSA uncertainty increases when AOD and SZA decrease. The monthly mean values of SSA and AAOD during the period January 2005–June 2008 are analysed, showing a monthly and seasonal variability. It is found that the SSA and AAOD averages are 0.80±0.08 and 0.056±0.028, respectively. AAOD retrievals are also used to quantify the error in the Ozone Monitoring Instrument (OMI) surface UV products due to absorbing aerosols, not included in the current OMI UV algorithm. OMI and Brewer UV irradiances at 324.1 nm and Erythemal Dose Rates (EDRs) under clear sky conditions, are compared as a function of AAOD. Three methods are considered to investigate on the applicability of an absorbing aerosol correction on OMI UV data at Rome site. Depending on the correction methodology, the bias value decreases from 18% to 2% for spectral irradiance at 324.1 nm and from 25% to 8% for EDR.

scholarly journals Aerosol Single Scattering Albedo retrieval in the UV range: an application to OMI satellite validation

2009 ◽  
Vol 9 (5) ◽  
pp. 19009-19033 ◽  
Author(s):  
I. Ialongo ◽  
V. Buchard ◽  
C. Brogniez ◽  
G. R. Casale ◽  
A. M. Siani
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Single Scattering ◽  
Single Scattering Albedo ◽  
Spectral Irradiance ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Ozone Monitoring Instrument ◽  
Mean Values ◽  
Absorbing Aerosols

Abstract. The aerosol Single Scattering Albedo (SSA) and Absorbing Aerosol Optical Depth (AAOD) at 320.1 nm are derived at Rome site by the comparison between Brewer and modelled spectra. The UVSPEC radiative transfer model is used to calculate the UV irradiances for different SSA values, taking into account as input data total ozone and Aerosol Optical Depth (AOD) obtained from Brewer spectral measurements. The accuracy in determining SSA depends on the aerosol amount and on Solar Zenith Angle (SZA) value: SSA uncertainty increases when AOD and SZA decrease. The monthly mean values of SSA and AAOD during the period January 2005–June 2008 are analysed, showing a monthly and seasonal variability. It is found that the SSA and AAOD averages are 0.80±0.08 and 0.056±0.028, respectively. AAOD retrievals are also used to quantify the error in the Ozone Monitoring Instrument (OMI) surface UV products due to absorbing aerosols, not included in the current OMI UV algorithm. OMI and Brewer UV irradiances at 324.1 nm and Erythemal Dose Rates (EDRs) under clear sky conditions, are compared as a function of AAOD. Three methods are considered to investigate on the applicability of an absorbing aerosol correction on OMI UV data at Rome site. Depending on the correction methodology, the bias value decreases from 18% to 2% for spectral irradiance at 324.1 nm and from 25% to 8% for EDR.

scholarly journals Comparison of UV-RSS spectral measurements and TUV model runs for clear skies for the May 2003 ARM aerosol intensive observation period

2007 ◽  
Vol 7 (6) ◽  
pp. 17401-17427
Author(s):  
J. J. Michalsky ◽  
P. W. Kiedron
Keyword(s):  
Radiative Transfer ◽  
Single Scattering ◽  
Single Scattering Albedo ◽  
Spectral Irradiance ◽  
Radiative Transfer Model ◽  
Visible Range ◽  
Transfer Model ◽  
Intensive Observation ◽  
Aerosol Properties ◽  
Observation Period

Abstract. The first successful deployment of the fully-operational ultraviolet rotating shadow-band spectroradiometer occurred during the May 2003 U.S. Department of Energy's Atmospheric Radiation Measurement program's Aerosol Intensive Observation Period. The aerosol properties in the visible range were characterized using redundant measurements with several instruments to determine the column aerosol optical depth, the single scattering albedo, and the asymmetry parameter needed as input for radiative transfer calculations of the downwelling direct normal and diffuse horizontal solar irradiance in clear-sky conditions. The Tropospheric Ultraviolet and Visible (TUV) radiative transfer model developed by Madronich and his colleagues at the U.S. National Center for Atmospheric Research was used for the calculations of the spectral irradiance between 300–360 nm. Since there are few ultraviolet measurements of aerosol properties, most of the input aerosol data for the radiative transfer model are based on the assumption that UV input parameters can be extrapolated from the visible portion of the spectrum. Disagreements between available extraterrestrial spectra, which are discussed briefly, suggested that instead of comparing irradiances that measured and modeled spectral transmittances between 300–360 nm should be compared for the seven cases studied. These cases included low to moderate aerosol loads and low to high solar-zenith angles. A procedure for retrieving single scattering albedo in the ultraviolet based on the comparisons of direct and diffuse transmittance is outlined.

scholarly journals Aerosol forcing efficiency in the UVA region from spectral solar irradiance measurements at an urban environment

2009 ◽  
Vol 27 (6) ◽  
pp. 2515-2522 ◽  
Author(s):  
S. Kazadzis ◽  
N. Kouremeti ◽  
A. Bais ◽  
A. Kazantzidis ◽  
C. Meleti
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Model Calculations ◽  
Aerosol Forcing ◽  
Aerosol Absorption ◽  
Absorbing Aerosols ◽  
Spectral Solar Irradiance ◽  
The City

Abstract. Spectral Ultraviolet (UV) measurements using a Brewer MKIII double spectroradiometer were used for the determination of the aerosol forcing efficiency (RFE) under cloud free conditions at Thessaloniki, Greece for the period 1998–2006. Using measured spectral UVA irradiance in combination with synchronous aerosol optical depth (AOD) measurements at 340 nm, we calculated the seasonal and the percent RFE changes with the help of radiative transfer model calculations used for cloud and aerosol free conditions reference. The calculated RFE for the 325–340 nm wavelength integral was found to be −0.71±0.30 W m−2/τs340 nm and corresponds to a mean calculated RFE% value of −15.2%±3.8% (2 σ) per unit of τs340 nm, for the whole period. This indicates a mean reduction of 15.2% of the 325–340 nm irradiance for a unit of aerosol optical depth slant column increase. Lower RFE% was found during summertime, which is a possible indication of lower absorbing aerosols. Mean AOD slant at 340 nm for the city of Thessaloniki were processed in combination with RFE% and a mean monthly UVA attenuation of ~10% for the whole period was revealed. The nine years' analysis results showed a reduction in RFE%, which provides a possible indication of the changes in the optical properties over the city area. If such changes are only due to changes in the aerosol absorbing properties, the above finding suggests a 2% per decade increase in UVA due to changes in the aerosol absorption properties, in addition to the calculated increase by 4.2%, which is attributed only to AOD decrease at Thessaloniki area over the 1998–2006 period.

scholarly journals Comparison of Columnar, Surface, and UAS Profiles of Absorbing Aerosol Optical Depth and Single-Scattering Albedo in South-East Poland

Atmosphere ◽  
2019 ◽  
Vol 10 (8) ◽  
pp. 446 ◽  
Author(s):  
Michał T. Chiliński ◽  
Krzysztof M. Markowicz ◽  
Olga Zawadzka ◽  
Iwona S. Stachlewska ◽  
Justyna Lisok ◽  
...  
Keyword(s):  
Absorption Coefficient ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Measurement Data ◽  
Single Scattering ◽  
Single Scattering Albedo ◽  
Height Distribution ◽  
Vertical Profiles ◽  
Absorbing Aerosols ◽  
The Impact

The impact of absorbing aerosols on climate is complex, with their potential positive or negative forcing, depending on many factors, including their height distribution and reflective properties of the underlying background. Measurement data is very limited, due to insufficient remote sensing methods dedicated to the retrieval of their vertical distribution. Columnar values of absorbing aerosol optical depth (AAOD) and single scattering albedo (SSA) are retrieved by the Aerosol Robotic Network (AERONET). However, the number of available results is low due to sky condition and aerosol optical depth (AOD) limitation. Presented research describes results of field campaigns in Strzyżów (South-East Poland, Eastern Europe) dedicated to the comparison of the absorption coefficient and SSA measurements performed with on-ground in-situ devices (aethalomter, nephelometer), small unmanned aerial system (UAS) carrying micro-aethalometer, as well as with lidar/ceilometer. An important aspect is the comparison of measurement results with those delivered by AERONET. Correlation of absorption to scattering coefficients measured on ground (0.79) and correlation of extinction on ground to AOD measured by AERONET (0.77) was visibly higher than correlation between AOD and AAOD retrieved by AERONET (0.56). Columnar SSA was weakly correlated with ground SSA (higher values of columnar SSA), which were mainly explained by hygroscopic effects, increasing scattering coefficient in ambient (wet conditions), and partly high uncertainty of SSA retrieval. AAOD derived with the use of profiles from UAS up to PBL height, was estimated to contribute in average to 37% of the total AAOD. A method of AAOD estimation, in the whole troposphere, with use of measured vertical profiles of absorption coefficient and extinction coefficient profiles from lidars was proposed. AAOD measured with this method has poor correlation with AERONET data, however for some measurements, within PBL, AAOD was higher than reported by AERONET, suggesting potential underestimation in photometric measurement under particular conditions. Correlation of absorption coefficient in profile to on ground measurements decrease with altitude. Measurements of SSA from drones agree well with ground measurements and are lower than results from AERONET, which suggests a larger contribution of absorbing aerosols. As an alternative for AAOD estimation in case of lack of AERONET AAOD data simple models are proposed, which base on AOD scaling with SSA measured with different methods. Proposed solution increase potential of absorption coefficient measurements in vertical profiles and columns of the atmosphere. Presented solutions make measurements of absorption coefficients in vertical profiles more affordable and allow rough estimation of columnar values for the whole atmosphere.

scholarly journals Quantifying the single-scattering albedo for the January 2017 Chile wildfires from simulations of the OMI absorbing aerosol index

2018 ◽  
Vol 11 (9) ◽  
pp. 5261-5277 ◽  
Author(s):  
Jiyunting Sun ◽  
J. Pepijn Veefkind ◽  
Peter van Velthoven ◽  
Pieternel F. Levelt
Keyword(s):  
Radiative Transfer ◽  
Single Scattering ◽  
Single Scattering Albedo ◽  
Radiative Transfer Model ◽  
Orthogonal Polarization ◽  
Satellite Measurement ◽  
Transfer Model ◽  
Backscatter Coefficient ◽  
Ozone Monitoring Instrument ◽  
Aerosol Index

Abstract. The absorbing aerosol index (AAI) is a qualitative parameter directly calculated from satellite-measured reflectance. Its sensitivity to absorbing aerosols in combination with a long-term data record since 1978 makes it an important parameter for climate research. In this study, we attempt to quantify aerosol absorption by retrieving the single-scattering albedo (ω0) at 550 nm from the satellite-measured AAI. In the first part of this study, AAI sensitivity studies are presented exclusively for biomass-burning aerosols. Later on, we employ a radiative transfer model (DISAMAR) to simulate the AAI measured by the Ozone Monitoring Instrument (OMI) in order to derive ω0 at 550 nm. Inputs for the radiative transfer calculations include satellite measurement geometry and surface conditions from OMI, aerosol optical thickness (τ) from the Moderate Resolution Imaging Spectroradiometer (MODIS) and aerosol microphysical parameters from the AErosol RObotic NETwork (AERONET), respectively. This approach is applied to the Chile wildfires for the period from 26 to 30 January 2017, when the OMI-observed AAI of this event reached its peak. The Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) overpasses missed the evolution of the smoke plume over the research region; therefore the aerosol profile is parameterized. The simulated plume is at an altitude of 4.5–4.9 km, which is in good agreement with available CALIOP backscatter coefficient measurements. The data may contain pixels outside the plume, so an outlier detection criterion is applied. The results show that the AAI simulated by DISAMAR is consistent with satellite observations. The correlation coefficients fall into the range between 0.85 and 0.95. The retrieved mean ω0 at 550 nm for the entire plume over the research period from 26 to 30 January 2017 varies from 0.81 to 0.87, whereas the nearest AERONET station reported ω0 between 0.89 and 0.92. The difference in geolocation between the AERONET site and the plume, the assumption of homogeneous plume properties, the lack of the aerosol profile information and the uncertainties in the inputs for radiative transfer calculation are primarily responsible for this discrepancy in ω0.

scholarly journals Comparison of UV-RSS spectral measurements and TUV model runs for clear skies for the May 2003 ARM aerosol intensive observation period

2008 ◽  
Vol 8 (6) ◽  
pp. 1813-1821 ◽  
Author(s):  
J. J. Michalsky ◽  
P. W. Kiedron
Keyword(s):  
Radiative Transfer ◽  
Single Scattering ◽  
Single Scattering Albedo ◽  
Spectral Irradiance ◽  
Radiative Transfer Model ◽  
Visible Range ◽  
Transfer Model ◽  
Intensive Observation ◽  
Aerosol Properties ◽  
Observation Period

Abstract. The first successful deployment of the fully-operational ultraviolet rotating shadow-band spectroradiometer occurred during the May 2003 US Department of Energy's Atmospheric Radiation Measurement program's Aerosol Intensive Observation Period. The aerosol properties in the visible range were characterized using redundant measurements with several instruments to determine the column aerosol optical depth, the single scattering albedo, and the asymmetry parameter needed as input for radiative transfer calculations of the downwelling direct normal and diffuse horizontal solar irradiance in clear-sky conditions. The Tropospheric Ultraviolet and Visible (TUV) radiative transfer model developed by Madronich and his colleagues at the US National Center for Atmospheric Research was used for the calculations of the spectral irradiance between 300–360 nm. Since there are few ultraviolet measurements of aerosol properties, most of the input aerosol data for the radiative transfer model are based on the assumption that UV input parameters can be extrapolated from the visible portion of the spectrum. Disagreements among available extraterrestrial spectra, which are discussed briefly, suggested that instead of comparing irradiances, measured and modeled spectral transmittances between 300–360 nm should be compared for the seven cases studied. Transmittance was calculated by taking the ratios of the measured irradiances to the Langley-derived, top-of-the-atmosphere irradiances. The cases studied included low to moderate aerosol loads and low to high solar-zenith angles. A procedure for retrieving single scattering albedo in the ultraviolet based on the comparisons of direct and diffuse transmittance is outlined.

scholarly journals Retrieval of aerosol absorption properties using the AATSR satellite instrument: a case study of wildfires over Russia 2010

2014 ◽  
Vol 7 (9) ◽  
pp. 9839-9868 ◽  
Author(s):  
E. Rodríguez ◽  
P. Kolmonen ◽  
T. H. Virtanen ◽  
L. Sogacheva ◽  
A.-M. Sundström ◽  
...  
Keyword(s):  
Optical Depth ◽  
Complex Refractive Index ◽  
Single Scattering ◽  
Radiative Transfer Model ◽  
Retrieval Algorithm ◽  
Transfer Model ◽  
Ozone Monitoring Instrument ◽  
Aerosol Model ◽  
Definition Of ◽  
Aerosol Properties

Abstract. The retrieval of aerosol properties from satellite data is based on the optimized fit of simulated and measured radiances at the top of the atmosphere (TOA). The simulations are made using a radiative transfer model with a variety of representative aerosol properties.The optimum fit is obtained for a certain combination of aerosol components, which are externally mixed to provide the aerosol model which in turn is used to calculate the aerosol optical depth (AOD). However, other aerosol properties could be provided. In the aerosol retrieval algorithm (ADV) applied to data from the Advanced Along Track Scanning Radiometer (AATSR), four aerosol components are used, each of which is defined by their (lognormal) size distribution and a complex refractive index. The fine mode fraction is a continuous mixture of weakly and strongly absorbing components which allows for the definition of any absorbing aerosol model within the specified limits. Hence, assuming that the correct aerosol model is selected during the retrieval process, also the single scattering albedo (SSA) should correctly be retrieved. In this paper we present the SSA retrieval using the ADV algorithm by application to wildfires over Russia in the summer of 2010. Together with the AOD, the SSA provides the aerosol absorbing optical depth (AAOD). The results are compared with AERONET data, i.e. AOD level 2.0 and SSA and AAOD inversion products. The RMSE is 0.03 for SSA and 0.02 for AAOD. The SSA is further evaluated by comparison with the SSA retrieved from the Ozone Monitoring Instrument (OMI). The SSA retrieved from both instruments show similar features, but the AATSR-retrieved SSA values over areas affected by wildfires are lower.

scholarly journals Retrieval of aerosol single-scattering albedo and polarized phase function from polarized sun-photometer measurements for Zanjan's atmosphere

2013 ◽  
Vol 6 (10) ◽  
pp. 2659-2669 ◽  
Author(s):  
A. Bayat ◽  
H. R. Khalesifard ◽  
A. Masoumi
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Atmospheric Aerosols ◽  
Phase Function ◽  
Single Scattering ◽  
Single Scattering Albedo ◽  
Angstrom Exponent ◽  
Ångström Exponent ◽  
Sun Photometer ◽  
Ångstrom Exponent

Abstract. The polarized phase function of atmospheric aerosols has been investigated for the atmosphere of Zanjan, a city in northwest Iran. To do this, aerosol optical depth, Ångström exponent, single-scattering albedo, and polarized phase function have been retrieved from the measurements of a Cimel CE 318-2 polarized sun-photometer from February 2010 to December 2012. The results show that the maximum value of aerosol polarized phase function as well as the polarized phase function retrieved for a specific scattering angle (i.e., 60°) are strongly correlated (R = 0.95 and 0.95, respectively) with the Ångström exponent. The latter has a meaningful variation with respect to the changes in the complex refractive index of the atmospheric aerosols. Furthermore the polarized phase function shows a moderate negative correlation with respect to the atmospheric aerosol optical depth and single-scattering albedo (R = −0.76 and −0.33, respectively). Therefore the polarized phase function can be regarded as a key parameter to characterize the atmospheric particles of the region – a populated city in the semi-arid area and surrounded by some dust sources of the Earth's dust belt.

scholarly journals Study of the effect of different type of aerosols on UV-B radiation from measurements during EARLINET

2003 ◽  
Vol 3 (5) ◽  
pp. 4671-4700
Author(s):  
D. S. Balis ◽  
V. Amiridis ◽  
C. Zerefos ◽  
A. Kazantzidis ◽  
S. Kazadzis ◽  
...  
Keyword(s):  
Total Ozone ◽  
Single Scattering ◽  
Single Scattering Albedo ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Combined Use ◽  
Lidar Measurements ◽  
The Vertical Distribution ◽  
Aerosol Type

Abstract. Routine lidar measurements of the vertical distribution of the aerosol extinction coefficient and the extinction-to-backscatter ratio have been performed at Thessaloniki, Greece using a Raman lidar system in the frame of the EARLINET project since 2000. Spectral and broadband UV-B irradiance measurements, as well as total ozone observations, were available whenever lidar measurements were obtained. From the available measurements several cases could be identified that allowed the study of the effect of different types of aerosol on the levels of the UV-B solar irradiance at the Earth's surface. The TUV radiative transfer model has been used to simulate the irradiance measurements, using total ozone and the lidar aerosol data as input. From the comparison of the model results with the measured spectra the effective single scattering albedo was determined using an iterative procedure, which has been verified against results from the 1998 Lindenberg Aerosol Characterization Experiment. It is shown that the same aerosol optical depth and same total ozone values can show differences up to 10% in the UV-B irradiance at the Earth's surface, which can be attributed to differences in the aerosol type. It is shown that the combined use of the estimated single scattering albedo and the measured extinction-to-backscatter ratio leads to a better characterization of the aerosol type probed.

scholarly journals Continental pollution in the Western Mediterranean basin: large variability of the aerosol single scattering albedo and influence on the direct shortwave radiative effect

2016 ◽  
Author(s):  
C. Di Biagio ◽  
P. Formenti ◽  
L. Doppler ◽  
C. Gaimoz ◽  
N. Grand ◽  
...  
Keyword(s):  
Mediterranean Basin ◽  
Single Scattering ◽  
Western Mediterranean ◽  
Single Scattering Albedo ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Radiative Effect ◽  
Large Variability ◽  
Western Mediterranean Basin ◽  
Study Results

Abstract. Pollution aerosols strongly influence the composition of the Western Mediterranean basin, but at present little is known on their optical properties. We report in this study in situ observations of the single scattering albedo (ω) of pollution aerosol plumes measured over the Western Mediterranean basin during the TRAQA (TRansport and Air QuAlity) airborne campaign in summer 2012. Cases of pollution export from different source regions around the basin and at different altitudes between ~160 and 3500 m above sea level have been sampled during the flights. Data from this study show a large variability of ω, with values between 0.84–0.98 at 370 nm and 0.70–0.99 at 950 nm. The single scattering albedo generally decreases with the wavelength, with some exception associated to the mixing of pollution with sea spray over the sea surface. Lowest values of ω (0.84–0.70 between 370 and 950 nm) are measured in correspondence of a fresh plume possibly linked to ship emissions over the basin. The range of variability of ω observed in this study seems to be independent of the source region around the basin, as well as of the altitude and ageing time of the plumes. The observed variability of ω reflects in a large variability for the complex refractive index of pollution aerosols, which is estimated to span in the large range 1.41–1.75 and 0.002–0.068 for the real and the imaginary parts, respectively, between 370 and 950 nm. Radiative calculations in clear-sky conditions have been performed with the GAME radiative transfer model to test the sensitivity of the aerosol shortwave Direct Radiative Effect (DRE) to the variability of ω as observed in this study. Results from the calculations suggest up to a 50 % and 30 % change of the forcing efficiency (FE), i.e. the DRE per unit of optical depth, at the surface (−160÷−235 Wm−2 τ−1 at 60° solar zenith angle) and at the Top-Of-Atmosphere (−137÷−92 5 Wm−2 τ−1) for ω varying between its maximum and minimum value. This induces a change of up to an order of magnitude (+23÷+143 Wm−2 τ−1) for the radiative effect within the atmosphere.

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