scholarly journals Organic molecular tracers in the atmospheric aerosols from Lumbini, Nepal, in the northern Indo-Gangetic Plain: influence of biomass burning

2017 ◽  
Vol 17 (14) ◽  
pp. 8867-8885 ◽  
Author(s):  
Xin Wan ◽  
Shichang Kang ◽  
Quanlian Li ◽  
Dipesh Rupakheti ◽  
Qianggong Zhang ◽  
...  

Abstract. To better understand the characteristics of biomass burning in the northern Indo-Gangetic Plain (IGP), total suspended particles were collected in a rural site, Lumbini, Nepal, during April 2013 to March 2014 and analyzed for the biomass burning tracers (i.e., levoglucosan, mannosan, vanillic acid). The annual average concentration of levoglucosan was 734 ± 1043 ng m−3 with the maximum seasonal mean concentration during post-monsoon season (2206 ± 1753 ng m−3), followed by winter (1161 ± 1347 ng m−3), pre-monsoon (771 ± 524 ng m−3) and minimum concentration during monsoon season (212 ± 279 ng m−3). The other biomass burning tracers (mannosan, galactosan, p-hydroxybenzoic acid, vanillic acid, syringic acid and dehydroabietic acid) also showed the similar seasonal variations. There were good correlations among levoglucosan, organic carbon (OC) and elemental carbon (EC), indicating significant impact of biomass burning activities on carbonaceous aerosol loading throughout the year in Lumbini area. According to the characteristic ratios, levoglucosan ∕ mannosan (lev ∕ man) and syringic acid ∕ vanillic acid (syr ∕ van), we deduced that the high abundances of biomass burning products during non-monsoon seasons were mainly caused by the burning of crop residues and hardwood while the softwood had less contribution. Based on the diagnostic tracer ratio (i.e., lev ∕ OC), the OC derived from biomass burning constituted large fraction of total OC, especially during post-monsoon season. By analyzing the MODIS fire spot product and 5-day air-mass back trajectories, we further demonstrated that organic aerosol composition was not only related to the local agricultural activities and residential biomass usage but also impacted by the regional emissions. During the post-monsoon season, the emissions from rice residue burning in western India and eastern Pakistan could impact particulate air pollution in Lumbini and surrounding regions in southern Nepal. Therefore, our finding is meaningful and has a great importance for adopting the appropriate mitigation measures, not only at the local level but also by involving different regions and nations, to reduce the biomass burning emissions in the broader IGP region nations.

2017 ◽  
Author(s):  
Xin Wan ◽  
Shichang Kang ◽  
Quanlian Li ◽  
Dipesh Rupakheti ◽  
Qianggong Zhang ◽  
...  

Abstract. To better understand the characteristics of biomass burning in the northern Indo-Gangetic Plain (IGP), total suspended particles were collected in a rural site, Lumbini, Nepal during April 2013 to March 2014 and analyzed for the biomass burning tracers (i.e., levoglucosan, mannosan, vanillic acid, etc.). The annual average concentration of levoglucosan was 734 ± 1043 ng m−3 with the maximum seasonal mean concentration during post-monsoon season (2206 ± 1753 ng m−3), followed by winter (1161 ± 1347 ng m−3), pre-monsoon (771 ± 524 ng m−3) and minimum concentration during monsoon season (212 ± 279 ng m−3). The other biomass burning tracers (mannosan, galactosan, p-hydroxybenzoic acid, vanillic acid, syringic acid, and dehydroabietic acid) also showed the similar seasonal variations. There were good correlations among levoglucosan, organic carbon (OC) and elemental carbon (EC), indicating significant impact of biomass burning activities on carbonaceous aerosol loading throughout the year in Lumbini area. According to the characteristic ratios: levoglucosan / mannosan (Lev / Man) and syringic acid / vanillic acid (Syr / Van), we deduced that the high abundances of biomass burning products during non-monsoon seasons were mainly caused by the burning of crop residues and hardwood while the softwood had less contribution. Based on the diagnostic tracer ratio (i.e., Lev / OC), the OC derived from biomass burning constituted large fraction of total OC, especially during post-monsoon season. By analyzing the MODIS fire spot product and five-day air-mass back trajectories, we further demonstrated that organic aerosol composition was not only related to the local agricultural activities and residential biomass usage, but was also impacted by the regional emissions. During the post-monsoon season, the emissions from rice residue burning in western India and eastern Pakistan could impact particulate air pollution in Lumbini and surrounding regions in southern Nepal. Therefore, our finding is meaningful and has a great importance for adopting the appropriate mitigation measures, not only at the local level but also by involving different regions and nations, to reduce the biomass burning emissions in the broader IGP region nations.


2021 ◽  
Vol 21 (14) ◽  
pp. 10881-10909
Author(s):  
Caterina Mogno ◽  
Paul I. Palmer ◽  
Christoph Knote ◽  
Fei Yao ◽  
Timothy J. Wallington

Abstract. The Indo-Gangetic Plain (IGP) is home to 9 % of the global population and is responsible for a large fraction of agricultural crop production in Pakistan, India, and Bangladesh. Levels of fine particulate matter (mean diameter <2.5 µm, PM2.5) across the IGP often exceed human health recommendations, making cities across the IGP among the most polluted in the world. Seasonal changes in the physical environment over the IGP are dominated by the large-scale south Asian monsoon system that dictates the timing of agricultural planting and harvesting. We use the WRF-Chem model to study the seasonal anthropogenic, pyrogenic, and biogenic influences on fine particulate matter and its constituent organic aerosol (OA) over the IGP that straddles Pakistan, India, and Bangladesh during 2017–2018. We find that surface air quality during pre-monsoon (March–May) and monsoon (June–September) seasons is better than during post-monsoon (October–December) and winter (January–February) seasons, but all seasonal mean values of PM2.5 still exceed the recommended levels, so that air pollution is a year-round problem. Anthropogenic emissions influence the magnitude and distribution of PM2.5 and OA throughout the year, especially over urban sites, while pyrogenic emissions result in localised contributions over the central and upper parts of IGP in all non-monsoonal seasons, with the highest impact during post-monsoon seasons that correspond to the post-harvest season in the agricultural calendar. Biogenic emissions play an important role in the magnitude and distribution of PM2.5 and OA during the monsoon season, and they show a substantial contribution to secondary OA (SOA), particularly over the lower IGP. We find that the OA contribution to PM2.5 is significant in all four seasons (17 %–30 %), with primary OA generally representing the larger fractional contribution. We find that the volatility distribution of SOA is driven mainly by the mean total OA loading and the washout of aerosols and gas-phase aerosol precursors that result in SOA being less volatile during the pre-monsoon and monsoon season than during the post-monsoon and winter seasons.


2021 ◽  
Vol 3 ◽  
Author(s):  
Vaibhav Bangar ◽  
Amit Kumar Mishra ◽  
Manish Jangid ◽  
Prashant Rajput

In this study, we have coupled measurements, modeling, and remote sensing techniques to better delineate the source characteristics and variability of air pollutants in Delhi primarily during the post-monsoon season in 2019. We show a comparison of ambient PM2.5 (particulate matter having aerodynamic diameter ≤2.5 μm) levels and associated elements during the post-monsoon with those during a relatively clean season of monsoon (experiencing frequent wet precipitation). Air-mass back trajectories from Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model have been used to infer the possible source pathways of PM2.5 impacting at the receptor site in Delhi. The average concentrations of PM2.5 during monsoon (June–July) and post-monsoon (October–November) were 42.2 ± 15.5 μg m−3 (range: 22–73 μg m−3) and 121.4 ± 53.6 μg m−3 (range: 46–298 μg m−3), respectively. The PM2.5 samples were analyzed for heavy and trace elements (Si, S, Na, Mg, Al, Cl, Ca, K, Ti, V, Cr, Mn, Fe, Ni, Cu, Br, Rb, Zr, and Pb) using an Energy Dispersive X-ray Fluorescence (ED-XRF) technique and their concentrations have been used to carry out the source-apportionment utilizing principal component analysis (PCA) tool. The PCA analysis has identified three major sources of fine aerosols including contributions from the sources viz. vehicular emission, biomass burning, coal combustion, secondary aerosols formation, soil dust, solid-waste burning and industrial emission. The source involving biomass burning contributed largely to the PM2.5 in post-monsoon season through long-range transport of large-scale agriculture-residue burning emissions (occurring in the states of Punjab, Haryana, and western part of Uttar Pradesh). The industrial emissions include primarily, medium- and small-scale metal processing industries (e.g. steel sheet rolling) in Delhi-National Capital Region. Traces of emission from coal based thermal power plants and waste incineration have also been observed in this study.


2021 ◽  
Author(s):  
Manish Jangid ◽  
Amit Mishra

&lt;p&gt;Atmospheric brown clouds (ABCs) are a dense and extensive pollution layer and have significant implications on air quality, agriculture, water cycle, and regional climate. The objective of the present study is to observe seasonal and spatial variations in the occurrence of ABCs and its radiative effects. The Indo-Gangetic plain (IGP) is the most populated region of India, which is an extended region in the foothills of the Himalayas. The IGP is one of the ABCs hotspots over the globe. The frequency of ABCs occurrences and radiative forcing were calculated using data from seven ground-based remote sensors situated across the IGP. We have used total ~ 5000 days of Level-2 aerosol measurements from seven AERosol Robotic NETwork (AERONET) stations (Karachi, Lahore, Jaipur, New Delhi, Kanpur, Gandhi college and Dhaka University) for three seasons (Pre-monsoon, Post-monsoon, and Winter) during 2000-2019. An algorithm based on the optical properties of aerosols is used to defined extreme pollution events (ABCs days) for each site. Our results show more frequent occurrences of ABCs over the region in the pre-monsoon out of all three seasons. However, spatial variation is found in all seasons, like maximum frequency of ABCs over western IGP region in post-monsoon and minimum is at eastern IGP region in the winter season. Further, we have used the Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART) model to calculate radiative forcing during ABCs days on all sites of study. Aerosol optical depth (AOD) and absorption optical depth (AAOD) was used to calculate radiative forcing over the IGP region. Radiative forcing of ABCs is negative at both the surface (SRF) and top of the atmosphere (TOA), whereas it is positive in the atmosphere (ATM). In magnitude, it was found minimum in the pre-monsoon season at TOA. However, other seasons have specific features over specific locations, for example, in the winter season, radiative forcing is maximum over Kolkata at TOA, SRF, and ATM, which are -13.81 W/m&lt;sup&gt;2&lt;/sup&gt;, -50.90 W/m&lt;sup&gt;2&lt;/sup&gt;, and +37.09 W/m&lt;sup&gt;2&lt;/sup&gt; respectively. In the pre-monsoon season, radiative forcing is maximum at Delhi (-9.59 W/m&lt;sup&gt;2&lt;/sup&gt;) at TOA. In post-monsoon season radiative forcing maximum at Gandhi-college (-11.30 W/m&lt;sup&gt;2&lt;/sup&gt;) at TOA. This ground observation is also compared with Modern Era Retrospective analysis and Research and Applications-2 (MEERA 2) modal data. These results indicate the cooling effect of ABCs at the surface and TOA over the IGP region throughout the period.&lt;/p&gt;


Water ◽  
2021 ◽  
Vol 13 (15) ◽  
pp. 2117
Author(s):  
Su-mi Kim ◽  
Hyun-su Kim

The variations in water quality parameters and trophic status of a multipurpose reservoir in response to changing intensity of monsoon rain was investigated by applying a trophic state index deviation (TSID) analysis and an empirical regression model to the data collected in two periods from 2014 to 2017. The reservoir in general maintained mesotrophic conditions, and Carlson’s trophic state index (TSIc) was affected most by TSITP. Nutrient concentrations, particularly phosphorus, did not show strong correlations with precipitation, particularly in the period with weak monsoon, and a significant increase in total phosphorus (TP) was observed in Spring 2015, indicating the possibility of internal phosphorus loading under decreased depth and stability of water body due to a lack of precipitation. TSIChl was higher than TSISD in most data in period 1 when a negligible increase in precipitation was observed in the monsoon season while a significant fraction in period 2 showed the opposite trend. Phytoplankton growth was not limited by nutrient limitation although nutrient ratios (N/P) of most samples were significantly higher than 20, indicating phosphorus-limited condition. TSID and regression analysis indicated that phytoplankton growth was limited by zooplankton grazing in the Spring, and that cell concentrations and community structure in the monsoon and post-monsoon season were controlled by the changing intensity of the monsoon, as evidenced by the positive and negative relationships between community size and cyanobacterial population with the amount of precipitation in the Summer, respectively. The possibility of contribution from internal loading and an increase in cyanobacterial population associated with weak monsoon, in addition to potential for nutrient enrichment in the post-monsoon season, implies a need for the application of more stringent water quality management in the reservoir that can handle all potential scenarios of eutrophication.


2016 ◽  
Vol 43 (23) ◽  
pp. 12,102-12,112 ◽  
Author(s):  
Vimal Mishra ◽  
Saran Aadhar ◽  
Akarsh Asoka ◽  
Sivananda Pai ◽  
Rohini Kumar

Healthline ◽  
2020 ◽  
Vol 11 (2) ◽  
pp. 100-107
Author(s):  
Arti Agrawal ◽  
Vikas Kumar ◽  
Sanjeev Kumar ◽  
Neha K Mani

Introduction: Dengue virus infection is a major public health issue prevalent in tropical and sub-tropical countries all over the world mostly in urban and semi-urban areas. WHO estimates about 50-100 million dengue infections worldwide every year. The present study is aimed to assess the prevalence and seasonal distribution of dengue disease during three consecutive years from 2016-2018 at a tertiary care centre of North India. Method: This is an observational retrospective study conducted on total 6,481 clinical suspected cases referred from indoor and outdoor departments of Medicine and Pediatrics of one of the medical colleges of Agra during the period from 1st January 2016 to 31st December 2018. Results: The maximum positivity was recorded in the year 2016 (16.66%), followed by 2017 (14.07%) and 2018(13.56%).Our study shows male preponderance with maximum cases in the year 2018 was recorded in the month of October (22.75%) whereas the lowest in the month of May (1.96%). Most of the cases were in the age group 0-30 years with a male preponderance. The outbreak occurred during the months of August to November indicating vector transmission in the monsoon and post-monsoon season. Conclusion: From the analysis, this study reflects that the numbers of dengue cases in 2016 were maximum and outnumbered the dengue cases among three consecutive years from 2016 to 2018. The peak in dengue positivity was observed during September to October. As this disease affects the population in the monsoon and post monsoon months therefore continuous monitoring of dengue infection is important during the post-monsoon season.


2021 ◽  
Vol 21 (21) ◽  
pp. 16427-16452
Author(s):  
Shohei Nomura ◽  
Manish Naja ◽  
M. Kawser Ahmed ◽  
Hitoshi Mukai ◽  
Yukio Terao ◽  
...  

Abstract. Emissions of greenhouse gases (GHGs) from the Indian subcontinent have increased during the last 20 years along with rapid economic growth; however, there remains a paucity of GHG measurements for policy-relevant research. In northern India and Bangladesh, agricultural activities are considered to play an important role in GHG concentrations in the atmosphere. We performed weekly air sampling at Nainital (NTL) in northern India and Comilla (CLA) in Bangladesh from 2006 and 2012, respectively. Air samples were analyzed for dry-air gas mole fractions of CO2, CH4, CO, H2, N2O, and SF6 and carbon and oxygen isotopic ratios of CO2 (δ13C-CO2 and δ18O-CO2). Regional characteristics of these components over the Indo-Gangetic Plain are discussed compared to data from other Indian sites and Mauna Loa, Hawaii (MLO), which is representative of marine background air. We found that the CO2 mole fraction at CLA had two seasonal minima in February–March and September, corresponding to crop cultivation activities that depend on regional climatic conditions. Although NTL had only one clear minimum in September, the carbon isotopic signature suggested that photosynthetic CO2 absorption by crops cultivated in each season contributes differently to lower CO2 mole fractions at both sites. The CH4 mole fraction of NTL and CLA in August–October showed high values (i.e., sometimes over 4000 ppb at CLA), mainly due to the influence of CH4 emissions from the paddy fields. High CH4 mole fractions sustained over months at CLA were a characteristic feature on the Indo-Gangetic Plain, which were affected by both the local emission and air mass transport. The CO mole fractions at NTL were also high and showed peaks in May and October, while CLA had much higher peaks in October–March due to the influence of human activities such as emissions from biomass burning and brick production. The N2O mole fractions at NTL and CLA increased in June–August and November–February, which coincided with the application of nitrogen fertilizer and the burning of biomass such as the harvest residues and dung for domestic cooking. Based on H2 seasonal variation at both sites, it appeared that the emissions in this region were related to biomass burning in addition to production from the reaction of OH and CH4. The SF6 mole fraction was similar to that at MLO, suggesting that there were few anthropogenic SF6 emission sources in the district. The variability of the CO2 growth rate at NTL was different from the variability in the CO2 growth rate at MLO, which is more closely linked to the El Niño–Southern Oscillation (ENSO). In addition, the growth rates of the CH4 and SF6 mole fractions at NTL showed an anticorrelation with those at MLO, indicating that the frequency of southerly air masses strongly influenced these mole fractions. These findings showed that rather large regional climatic conditions considerably controlled interannual variations in GHGs, δ13C-CO2, and δ18O-CO2 through changes in precipitation and air mass.


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