scholarly journals Karymsky volcano eruptive plume properties based on MISR multi-angle imagery and the volcanological implications

2018 ◽  
Vol 18 (6) ◽  
pp. 3903-3918 ◽  
Author(s):  
Verity J. B. Flower ◽  
Ralph A. Kahn
Keyword(s):  
Atmospheric Aerosols ◽  
Thermal Anomaly ◽  
Effective Radius ◽  
Particle Properties ◽  
Remote Locations ◽  
Microphysical Properties ◽  
Event Timing ◽  
Stereo Imagery ◽  
Karymsky Volcano ◽  
Over Time

Abstract. Space-based operational instruments are in unique positions to monitor volcanic activity globally, especially in remote locations or where suborbital observing conditions are hazardous. The Multi-angle Imaging SpectroRadiometer (MISR) provides hyper-stereo imagery, from which the altitude and microphysical properties of suspended atmospheric aerosols can be derived. These capabilities are applied to plumes emitted at Karymsky volcano from 2000 to 2017. Observed plumes from Karymsky were emitted predominantly to an altitude of 2–4 km, with occasional events exceeding 6 km. MISR plume observations were most common when volcanic surface manifestations, such as lava flows, were identified by satellite-based thermal anomaly detection. The analyzed plumes predominantly contained large (1.28 µm effective radius), strongly absorbing particles indicative of ash-rich eruptions. Differences between the retrievals for Karymsky volcano's ash-rich plumes and the sulfur-rich plumes emitted during the 2014–2015 eruption of Holuhraun (Iceland) highlight the ability of MISR to distinguish particle types from such events. Observed plumes ranged from 30 to 220 km in length and were imaged at a spatial resolution of 1.1 km. Retrieved particle properties display evidence of downwind particle fallout, particle aggregation and chemical evolution. In addition, changes in plume properties retrieved from the remote-sensing observations over time are interpreted in terms of shifts in eruption dynamics within the volcano itself, corroborated to the extent possible with suborbital data. Plumes emitted at Karymsky prior to 2010 display mixed emissions of ash and sulfate particles. After 2010, all plumes contain consistent particle components, indicative of entering an ash-dominated regime. Post-2010 event timing, relative to eruption phase, was found to influence the optical properties of observed plume particles, with light absorption varying in a consistent sequence as each respective eruption phase progressed.

scholarly journals Tracking microphysical variations in emissions from Karymsky volcano using MISR multi-angle imagery, and implications for volcano geologic interpretation

2017 ◽  
Author(s):  
Verity J. B. Flower ◽  
Ralph A. Kahn
Keyword(s):  
Atmospheric Aerosols ◽  
Thermal Anomaly ◽  
Remote Locations ◽  
Microphysical Properties ◽  
Stereo Imagery ◽  
Geologic Interpretation ◽  
Particle Property ◽  
Karymsky Volcano ◽  
Activity Cycles ◽  
Over Time

Abstract. Space-based, operational instruments are in unique positions to monitor volcanic activity globally, especially in remote locations or where suborbital observing conditions are hazardous. The Multi-angle Imaging SpectroRadiometer (MISR) provides hyper-stereo imagery, from which the altitude and microphysical properties of suspended atmospheric aerosols can be derived. These capabilities are applied to plumes emitted at Karymsky volcano from 2000 to 2017. Plumes from Karymsky were predominantly emitted to an altitude of 2–4 km, with occasional events exceeding 6 km. MISR plume observations were most common when volcanic surface manifestations were high, such as lava flows identified by satellite-based thermal anomaly detection. The plumes contained large, strongly absorbing particles indicative of ash-rich eruptions. Differences between the retrievals for Karymsky volcano's ash-rich plumes and the sulfur-rich plumes from the 2014–2015 eruption of Bárðarbunga (Iceland) highlight the ability of MISR to distinguish particle types from such events. Plumes emitted at Karymsky prior to 2010 contain the sulfate proxy. After 2011, plumes contain similar particle components, but with varying fractions of absorption linked to timing within respective eruption phases. From the 1.1 km spatial-resolution retrievals within 30–220 km plumes, particle fallout, physical aggregation, and chemical evolution are indicated by the particle property variations observed downwind. In addition, changes in plume properties retrieved from the remote-sensing observations over time are interpreted in terms of activity cycles within the volcano itself, corroborated to the extent possible with suborbital data.

scholarly journals FAME-C: cloud property retrieval using synergistic AATSR and MERIS observations

2014 ◽  
Vol 7 (11) ◽  
pp. 3873-3890 ◽  
Author(s):  
C. K. Carbajal Henken ◽  
R. Lindstrot ◽  
R. Preusker ◽  
J. Fischer
Keyword(s):  
Optical Thickness ◽  
Single Layer ◽  
Cloud Water ◽  
Effective Radius ◽  
Cloud Property ◽  
Microphysical Properties ◽  
Microphysical Property ◽  
Resolution Imaging ◽  
Cloud Optical Thickness ◽  
Cloud Water Path

Abstract. A newly developed daytime cloud property retrieval algorithm, FAME-C (Freie Universität Berlin AATSR MERIS Cloud), is presented. Synergistic observations from the Advanced Along-Track Scanning Radiometer (AATSR) and the Medium Resolution Imaging Spectrometer (MERIS), both mounted on the polar-orbiting Environmental Satellite (Envisat), are used for cloud screening. For cloudy pixels two main steps are carried out in a sequential form. First, a cloud optical and microphysical property retrieval is performed using an AATSR near-infrared and visible channel. Cloud phase, cloud optical thickness, and effective radius are retrieved, and subsequently cloud water path is computed. Second, two cloud top height products are retrieved based on independent techniques. For cloud top temperature, measurements in the AATSR infrared channels are used, while for cloud top pressure, measurements in the MERIS oxygen-A absorption channel are used. Results from the cloud optical and microphysical property retrieval serve as input for the two cloud top height retrievals. Introduced here are the AATSR and MERIS forward models and auxiliary data needed in FAME-C. Also, the optimal estimation method, which provides uncertainty estimates of the retrieved property on a pixel basis, is presented. Within the frame of the European Space Agency (ESA) Climate Change Initiative (CCI) project, the first global cloud property retrievals have been conducted for the years 2007–2009. For this time period, verification efforts are presented, comparing, for four selected regions around the globe, FAME-C cloud optical and microphysical properties to cloud optical and microphysical properties derived from measurements of the Moderate Resolution Imaging Spectroradiometer (MODIS) on the Terra satellite. The results show a reasonable agreement between the cloud optical and microphysical property retrievals. Biases are generally smallest for marine stratocumulus clouds: −0.28, 0.41 μm and −0.18 g m−2 for cloud optical thickness, effective radius and cloud water path, respectively. This is also true for the root-mean-square deviation. Furthermore, both cloud top height products are compared to cloud top heights derived from ground-based cloud radars located at several Atmospheric Radiation Measurement (ARM) sites. FAME-C mostly shows an underestimation of cloud top heights when compared to radar observations. The lowest bias of −0.3 km is found for AATSR cloud top heights for single-layer clouds, while the highest bias of −3.0 km is found for AATSR cloud top heights for multilayer clouds. Variability is low for MERIS cloud top heights for low-level clouds, and high for MERIS cloud top heights for mid-level and high-level single-layer clouds, as well as for both AATSR and MERIS cloud top heights for multilayer clouds.

scholarly journals Retrieval of aerosol microphysical properties from atmospheric lidar sounding: an investigation using synthetic measurements and data from the ACEPOL campaign

2021 ◽  
Vol 14 (6) ◽  
pp. 4755-4771
Author(s):  
William G. K. McLean ◽  
Guangliang Fu ◽  
Sharon P. Burton ◽  
Otto P. Hasekamp
Keyword(s):  
Refractive Index ◽  
Effective Radius ◽  
High Spectral Resolution ◽  
Imaginary Component ◽  
The Real ◽  
Microphysical Properties ◽  
Lidar Measurements ◽  
Fine Mode ◽  
Truth Value ◽  
Real Refractive Index

Abstract. This study presents an investigation of aerosol microphysical retrievals from high spectral resolution lidar (HSRL) measurements. Firstly, retrievals are presented for synthetically generated lidar measurements, followed by an application of the retrieval algorithm to real lidar measurements. Here, we perform the investigation for an aerosol state vector that is typically used in multi-angle polarimeter (MAP) retrievals, so that the results can be interpreted in relation to a potential combination of lidar and MAP measurements. These state vectors correspond to a bimodal size distribution, where column number, effective radius, and effective variance of both modes are treated as fit parameters, alongside the complex refractive index and particle shape. The focus is primarily on a lidar configuration based on that of the High Spectral Resolution Lidar-2 (HSRL-2), which participated in the ACEPOL (Aerosol Characterization from Polarimeter and Lidar) campaign, a combined project between NASA and SRON (Netherlands Institute for Space Research). The measurement campaign took place between October and November 2017, over the western region of the USA. Six different instruments were mounted on the aeroplane: four MAPs and two lidar instruments, HSRL-2 and the Cloud Physics Lidar (CPL). Most of the flights were carried out over land, passing over scenes with a low aerosol load. One of the flights passed over a prescribed forest fire in Arizona on 9 November, with a relatively higher aerosol optical depth (AOD), and it is the data from this flight that are focussed on in this study. A retrieval of the aerosol microphysical properties of the smoke plume mixture was attempted with the data from HSRL-2 and compared with a retrieval from the MAPs carried out in previous work pertaining to the ACEPOL data. The synthetic HSRL-2 retrievals resulted for the fine mode in a mean absolute error (MAE) of 0.038 (0.025) µm for the effective radius (with a mean truth value of 0.195 µm), 0.052 (0.037) for the real refractive index, 0.010 (7.20×10-3) for the imaginary part of the refractive index, 0.109 (0.071) for the spherical fraction, and 0.054 (0.039) for the AOD at 532 nm, where the retrievals inside brackets indicate the MAE for noise-free retrievals. For the coarse mode, we find the MAE is 0.459 (0.254) µm for the effective radius (with a mean truth value of 1.970 µm), 0.085 (0.075) for the real refractive index, 2.06×10-4 (1.90×10-4) for the imaginary component, 0.120 (0.090) for the spherical fraction, and 0.051 (0.039) for the AOD. A study of the sensitivity of retrievals to the choice of prior and first guess showed that, on average, the retrieval errors increase when the prior deviates too much from the truth value. These experiments revealed that the measurements primarily contain information on the size and shape of the aerosol, along with the column number. Some information on the real component of the refractive index is also present, with the measurements providing little on absorption or on the effective variance of the aerosol distribution, as both of these were shown to depend heavily on the choice of prior. Retrievals using the HSRL-2 smoke-plume data yielded, for the fine mode, an effective radius of 0.107 µm, a real refractive index of 1.561, an imaginary component of refractive index of 0.010, a spherical fraction of 0.719, and an AOD at 532 nm of 0.505. Additionally, the single-scattering albedo (SSA) from the HSRL-2 retrievals was 0.940. Overall, these results are in good agreement with those from the Spectropolarimeter for Planetary Exploration (SPEX) and Research Scanning Polarimeter (RSP) retrievals.

Information Content of AVHRR Channels 4 and 5 with Respect to the Effective Radius of Cirrus Cloud Particles

1991 ◽  
Vol 30 (7) ◽  
pp. 973-984 ◽  
Author(s):  
F. Parol ◽  
J. C. Buriez ◽  
G. Brogniez ◽  
Y. Fouquart
Keyword(s):  
Absorption Coefficient ◽  
Mean Value ◽  
Effective Radius ◽  
Forward Peak ◽  
Effective Absorption Coefficient ◽  
Brightness Temperatures ◽  
Microphysical Properties ◽  
Effective Absorption ◽  
Cloud Particles ◽  
The Relationship

Abstract This paper investigates the important difference in the relationship between brightness temperatures between the 11-μm and the 12-μn AVHRR data and the microphysical properties of the semitransparent cirrus clouds. In the nonscattering approximation, the emittance for channels 4 and 5 are related through the absorption coefficient ratio that is the key parameter giving access to the size of cloud particles. The observed mean value of this parameter corresponds to effective radius of 18 μm for polydisperse spheres and 12 μm for polydisperse infinitely long ice cylinders. Taking the multiple scattering into account, the brightness temperature difference enhances much more for cylinders than for spheres owing to the fact that the forward peak of scattering is less large for cylinders. To obtain the size of cloud particles, the method developed in the nonscattering case is still applicable if one makes use of the effective emittance that implicitly includes the effects of mattering. Thus, an effective absorption coefficient ratio is defined and we derive a direct relationship between this ratio and the optical properties of the cloud particles. The mean value of the effective absorption coefficient ratio corresponds to ice spheres of effective radius of 26 μm or a bit less in the case of water spheres (supercooled droplets), but no agreement can be obtained for fully randomly oriented cylinders.

scholarly journals The variability of tropical ice cloud properties as a function of the large-scale context from ground-based radar-lidar observations over Darwin, Australia

2011 ◽  
Vol 11 (16) ◽  
pp. 8363-8384 ◽  
Author(s):  
A. Protat ◽  
J. Delanoë ◽  
P. T. May ◽  
J. Haynes ◽  
C. Jakob ◽  
...  
Keyword(s):  
Large Scale ◽  
Effective Radius ◽  
Ice Clouds ◽  
Ice Cloud ◽  
Microphysical Properties ◽  
Cloud Properties ◽  
Ice Water Content ◽  
Mean Differences ◽  
Ice Water ◽  
Lidar Observations

Abstract. The high complexity of cloud parameterizations now held in models puts more pressure on observational studies to provide useful means to evaluate them. One approach to the problem put forth in the modelling community is to evaluate under what atmospheric conditions the parameterizations fail to simulate the cloud properties and under what conditions they do a good job. It is the ambition of this paper to characterize the variability of the statistical properties of tropical ice clouds in different tropical "regimes" recently identified in the literature to aid the development of better process-oriented parameterizations in models. For this purpose, the statistical properties of non-precipitating tropical ice clouds over Darwin, Australia are characterized using ground-based radar-lidar observations from the Atmospheric Radiation Measurement (ARM) Program. The ice cloud properties analysed are the frequency of ice cloud occurrence, the morphological properties (cloud top height and thickness), and the microphysical and radiative properties (ice water content, visible extinction, effective radius, and total concentration). The variability of these tropical ice cloud properties is then studied as a function of the large-scale cloud regimes derived from the International Satellite Cloud Climatology Project (ISCCP), the amplitude and phase of the Madden-Julian Oscillation (MJO), and the large-scale atmospheric regime as derived from a long-term record of radiosonde observations over Darwin. The vertical variability of ice cloud occurrence and microphysical properties is largest in all regimes (1.5 order of magnitude for ice water content and extinction, a factor 3 in effective radius, and three orders of magnitude in concentration, typically). 98 % of ice clouds in our dataset are characterized by either a small cloud fraction (smaller than 0.3) or a very large cloud fraction (larger than 0.9). In the ice part of the troposphere three distinct layers characterized by different statistically-dominant microphysical processes are identified. The variability of the ice cloud properties as a function of the large-scale atmospheric regime, cloud regime, and MJO phase is large, producing mean differences of up to a factor 8 in the frequency of ice cloud occurrence between large-scale atmospheric regimes and mean differences of a factor 2 typically in all microphysical properties. Finally, the diurnal cycle of the frequency of occurrence of ice clouds is also very different between regimes and MJO phases, with diurnal amplitudes of the vertically-integrated frequency of ice cloud occurrence ranging from as low as 0.2 (weak diurnal amplitude) to values in excess of 2.0 (very large diurnal amplitude). Modellers should now use these results to check if their model cloud parameterizations are capable of translating a given atmospheric forcing into the correct statistical ice cloud properties.

scholarly journals Overview of Ice Nucleating Particles

2017 ◽  
Vol 58 ◽  
pp. 1.1-1.33 ◽  
Author(s):  
Zamin A. Kanji ◽  
Luis A. Ladino ◽  
Heike Wex ◽  
Yvonne Boose ◽  
Monika Burkert-Kohn ◽  
...  
Keyword(s):  
Chemical Properties ◽  
Ice Nucleation ◽  
Ice Crystal ◽  
New Developments ◽  
Particle Properties ◽  
Microphysical Properties ◽  
Range Transport ◽  
Homogeneous Freezing ◽  
Aerosol Aging ◽  
Physical And Chemical

Abstract Ice particle formation in tropospheric clouds significantly changes cloud radiative and microphysical properties. Ice nucleation in the troposphere via homogeneous freezing occurs at temperatures lower than −38°C and relative humidity with respect to ice above 140%. In the absence of these conditions, ice formation can proceed via heterogeneous nucleation aided by aerosol particles known as ice nucleating particles (INPs). In this chapter, new developments in identifying the heterogeneous freezing mechanisms, atmospheric relevance, uncertainties, and unknowns about INPs are described. The change in conventional wisdom regarding the requirements of INPs as new studies discover physical and chemical properties of these particles is explained. INP sources and known reasons for their ice nucleating properties are presented. The need for more studies to systematically identify particle properties that facilitate ice nucleation is highlighted. The atmospheric relevance of long-range transport, aerosol aging, and coating studies (in the laboratory) of INPs are also presented. Possible mechanisms for processes that change the ice nucleating potential of INPs and the corresponding challenges in understanding and applying these in models are discussed. How primary ice nucleation affects total ice crystal number concentrations in clouds and the discrepancy between INP concentrations and ice crystal number concentrations are presented. Finally, limitations of parameterizing INPs and of models in representing known and unknown processes related to heterogeneous ice nucleation processes are discussed.

scholarly journals Comparison of CALIPSO-Like, LaRC, and MODIS Retrievals of Ice-Cloud Properties over SIRTA in France and Florida during CRYSTAL-FACE

2007 ◽  
Vol 46 (3) ◽  
pp. 249-272 ◽  
Author(s):  
M. Chiriaco ◽  
H. Chepfer ◽  
P. Minnis ◽  
M. Haeffelin ◽  
S. Platnick ◽  
...  
Keyword(s):  
Remote Sensing ◽  
Radiant Energy ◽  
Energy System ◽  
Effective Radius ◽  
Cloud Detection ◽  
Regional Study ◽  
Crystal Face ◽  
Ice Clouds ◽  
Microphysical Properties ◽  
Cloud Properties

Abstract This study compares cirrus-cloud properties and, in particular, particle effective radius retrieved by a Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO)-like method with two similar methods using Moderate-Resolution Imaging Spectroradiometer (MODIS), MODIS Airborne Simulator (MAS), and Geostationary Operational Environmental Satellite imagery. The CALIPSO-like method uses lidar measurements coupled with the split-window technique that uses the infrared spectral information contained at the 8.65-, 11.15-, and 12.05-μm bands to infer the microphysical properties of cirrus clouds. The two other methods, using passive remote sensing at visible and infrared wavelengths, are the operational MODIS cloud products (using 20 spectral bands from visible to infrared, referred to by its archival product identifier MOD06 for MODIS Terra) and MODIS retrievals performed by the Clouds and the Earth’s Radiant Energy System (CERES) team at Langley Research Center (LaRC) in support of CERES algorithms (using 0.65-, 3.75-, 10.8-, and 12.05-μm bands); the two algorithms will be referred to as the MOD06 and LaRC methods, respectively. The three techniques are compared at two different latitudes. The midlatitude ice-clouds study uses 16 days of observations at the Palaiseau ground-based site in France [Site Instrumental de Recherche par Télédétection Atmosphérique (SIRTA)], including a ground-based 532-nm lidar and the MODIS overpasses on the Terra platform. The tropical ice-clouds study uses 14 different flight legs of observations collected in Florida during the intensive field experiment known as the Cirrus Regional Study of Tropical Anvils and Cirrus Layers–Florida Area Cirrus Experiment (CRYSTAL-FACE), including the airborne cloud-physics lidar and the MAS. The comparison of the three methods gives consistent results for the particle effective radius and the optical thickness but discrepancies in cloud detection and altitudes. The study confirms the value of an active remote sensing method (CALIPSO like) for the study of subvisible ice clouds, in both the midlatitudes and Tropics. Nevertheless, this method is not reliable in optically very thick tropical ice clouds, because of their particular microphysical properties.

scholarly journals Validation of MODIS cloud microphysical properties with in situ measurements over the Southeast Pacific

2012 ◽  
Vol 12 (1) ◽  
pp. 1419-1449 ◽  
Author(s):  
Q. Min ◽  
E. Joseph ◽  
Y. Lin ◽  
L. Min ◽  
B. Yin ◽  
...  
Keyword(s):  
Number Concentration ◽  
Effective Radius ◽  
In Situ Measurements ◽  
Liquid Water Path ◽  
Cloud Drop ◽  
Microphysical Properties ◽  
Satellite Retrievals ◽  
Drop Number ◽  
Cloud Liquid Water Path

Abstract. Utilizing the unique characteristics of the cloud over the Southeast Pacific (SEP) off the coast of Chile during the VOCALS field campaign, we validated satellite remote sensing of cloud microphysical properties against in situ data from multi-aircraft observations, and studied the extent to which these retrieved properties are sufficiently constrained and consistent to reliably quantify the influence of aerosol loading on cloud droplet sizes. After constraining the spatial-temporal coincidence between satellite retrievals and in situ measurements, we selected 17 non-drizzle comparison pairs. For these cases the mean aircraft profiling times were within one hour of Terra overpass at both projected and un-projected (actual) aircraft positions for two different averaging domains of 5 km and 25 km. Retrieved quantities that were averaged over a larger domain of 25 km compared better statistically with in situ observations than averages over a smaller domain of 5 km. Validation at projected aircraft positions was slightly better than un-projected aircraft positions for some parameters. Overall, both MODIS-retrieved effective radius and LWP were larger but highly correlated with the in situ measured effective radius and LWP. The observed effective radius difference between the two decreased with increasing cloud drop number concentration, and increased with increasing cloud geometrical thickness. Also, MODIS retrievals for adiabatic clouds agreed better with the in situ measurements than for sub-adiabatic clouds. Our validation and sensitivity analysis of simulated retrievals demonstrate that both cloud geometrical thickness and cloud adiabaticity are important factors in satellite retrievals of effective radius and cloud drop number concentration. The large variabilities in cloud geometric thickness and adiabaticity, the dependencies of cloud microphysical properties on both quantities (as demonstrated in our sensitivity study of simulated retrievals), and the inability to accurately account for either of them in retrievals lead to substantial uncertainties and biases in satellite retrieved cloud effective radius, cloud liquid water path, and cloud drop number concentration. However, strong correlations between satellite retrievals and in situ measurements suggest that satellite retrievals of cloud effective radius, cloud liquid water path, and cloud drop number concentration can be used to investigate aerosol indirect effects qualitatively.

scholarly journals The challenge of simulating the sensitivity of the Amazonian clouds microstructure to cloud condensation nuclei number concentrations

2019 ◽  
Author(s):  
Pascal Polonik ◽  
Christoph Knote ◽  
Tobias Zinner ◽  
Florian Ewald ◽  
Tobias Kölling ◽  
...  
Keyword(s):  
Cloud Condensation Nuclei ◽  
Regional Scale ◽  
Cloud Droplet ◽  
Number Concentration ◽  
Effective Radius ◽  
Cloud Base ◽  
Condensation Nuclei ◽  
Aerosol Cloud ◽  
Microphysical Properties

Abstract. The realistic representation of cloud-aerosol interactions is of primary importance for accurate climate model projections. The investigation of these interactions in strongly contrasting clean and polluted atmospheric conditions in the Amazon area has been one of the motivations for several field observations, including the airborne Aerosol, Cloud, Precipitation, and Radiation Interactions and DynamIcs of CONvective cloud systems – Cloud Processes of the Main Precipitation Systems in Brazil: A Contribution to Cloud Resolving Modeling and to the GPM (Global Precipitation Measurement) (ACRIDICON-CHUVA) campaign based in Manaus, Brazil in September 2014. In this work we combine in situ and remotely sensed aerosol, cloud, and atmospheric radiation data collected during ACRIDICON-CHUVA with regional, online-coupled chemistry-transport simulations to evaluate the model’s ability to represent the indirect effects of biomass burning aerosol on cloud microphysical properties (droplet number concentration and effective radius). We found agreement between modeled and observed median cloud droplet number concentrations (CDNC) for low values of CDNC, i.e., low levels of pollution. In general, a linear relationship between modeled and observed CDNC with a slope of two was found, which means a systematic underestimation of modeled CDNC as compared to measurements. Variability in cloud condensation nuclei (CCN) number concentrations and cloud droplet effective radii (reff) was also underestimated by the model. Modeled effective radius profiles began to saturate around 500 CCN per cm3 at cloud base, indicating an upper limit for the model sensitivity well below CCN concentrations reached during the burning season in the Amazon Basin. Regional background aerosol concentrations were sufficiently high such that the additional CCN emitted from local fires did not cause a notable change in modelled cloud microphysical properties. In addition, we evaluate a parameterization of CDNC at cloud base using more readily available cloud microphysical properties, aimed at in situ observations and satellite retrievals. Our study casts doubt on the validity of regional scale modeling studies of the cloud albedo effect in convective situations for polluted situations where the number concentration of CCN is greater than 500 cm−3.

scholarly journals Optical and microphysical properties of natural mineral dust and anthropogenic soil dust near dust source regions over northwestern China

2018 ◽  
Vol 18 (3) ◽  
pp. 2119-2138 ◽  
Author(s):  
Xin Wang ◽  
Hui Wen ◽  
Jinsen Shi ◽  
Jianrong Bi ◽  
Zhongwei Huang ◽  
...  
Keyword(s):  
Atmospheric Aerosols ◽  
Mineral Dust ◽  
Particle Diameter ◽  
Northwestern China ◽  
Soil Dust ◽  
Dust Source ◽  
Dust Aerosols ◽  
Microphysical Properties ◽  
Source Regions ◽  
Anthropogenic Soil

Abstract. Mineral dust aerosols (MDs) not only influence the climate by scattering and absorbing solar radiation but also modify cloud properties and change the ecosystem. From 3 April to 16 May 2014, a ground-based mobile laboratory was deployed to measure the optical and microphysical properties of MDs near dust source regions in Wuwei, Zhangye, and Dunhuang (in chronological order) along the Hexi Corridor over northwestern China. Throughout this dust campaign, the hourly averaged (±standard deviation) aerosol scattering coefficients (σsp, 550 nm) of the particulates with aerodynamic diameters less than 2.5 µm (PM2.5) at these three sites were sequentially 101.5 ± 36.8, 182.2 ± 433.1, and 54.0 ± 32.0 Mm−1. Correspondingly, the absorption coefficients (σap, 637 nm) were 9.7 ± 6.1, 6.0 ± 4.6, and 2.3 ± 0.9 Mm−1; single-scattering albedos (ω, 637 nm) were 0.902 ± 0.025, 0.931 ± 0.037, and 0.949 ± 0.020; and scattering Ångström exponents (Åsp, 450–700 nm) of PM2.5 were 1.28 ± 0.27, 0.77 ± 0.51, and 0.52 ± 0.31. During a severe dust storm in Zhangye (i.e., from 23 to 25 April), the highest values of σsp2.5 (∼ 5074 Mm−1), backscattering coefficient (σbsp2.5, ∼ 522 Mm−1), and ω637 (∼ 0.993) and the lowest values of backscattering fraction (b2.5, ∼ 0.101) at 550 nm and Åsp2.5 (∼ −0.046) at 450–700 nm, with peak values of aerosol number size distribution (appearing at the particle diameter range of 1–3 µm), exhibited that the atmospheric aerosols were dominated by coarse-mode dust aerosols. It is hypothesized that the relatively higher values of mass scattering efficiency during floating dust episodes in Wuwei and Zhangye are attributed to the anthropogenic soil dust produced by agricultural cultivations.

Sign in / Sign up

Export Citation Format

Share Document