scholarly journals Vertical profiles of submicron aerosol single scattering albedo over the Indian region immediately before monsoon onset and during its development: research from the SWAAMI field campaign

2020 ◽  
Vol 20 (6) ◽  
pp. 4031-4046
Author(s):  
Mohanan R. Manoj ◽  
Sreedharan K. Satheesh ◽  
Krishnaswamy K. Moorthy ◽  
Hugh Coe
Keyword(s):  
Active Phase ◽  
Single Scattering ◽  
Monsoon Onset ◽  
Single Scattering Albedo ◽  
Transfer Model ◽  
Heating Rates ◽  
Atmospheric Measurements ◽  
Middle Troposphere ◽  
Submicron Aerosol ◽  
Aerosol Absorption

Abstract. Vertical structures of aerosol single scattering albedo (SSA), from near the surface through the free troposphere, have been estimated for the first time at distinct geographical locations over the Indian mainland and adjoining oceans, using in situ measurements of aerosol scattering and absorption coefficients aboard the Facility for Airborne Atmospheric Measurements (FAAM) BAe-146 aircraft during the South West Asian Aerosol Monsoon Interactions (SWAAMI) campaign from June to July 2016. These are used to examine the spatial variation of SSA profiles and also to characterize its transformation from just prior to the onset of Indian Summer Monsoon (June 2016) to its active phase (July 2016). Very strong aerosol absorption, with SSA values as low as 0.7, persisted in the lower altitudes (<3 km) over the Indo-Gangetic Plains (IGP), prior to the monsoon onset, with a west-to-east gradient; lower values occurred in the north-western arid regions, peaking in the central IGP and somewhat decreasing towards the eastern end. During the active phase of the monsoon, the SSA is found to increase remarkably, indicating far less absorption. Nevertheless, significant aerosol absorption persisted in the lower and middle troposphere over the IGP. Inputting these SSA and extinction profiles into a radiative transfer model, we examined the effects of using height-resolved information in estimating atmospheric heating rates due to aerosols, over similar estimates made using a single columnar value. It was noted that use of a single SSA value leads to an underestimation (overestimation) of the heating rates over regions with low (high) SSA, emphasizing the importance of height-resolved information. Further, the use of realistic profiles showed significant heating of the atmosphere by submicron aerosol absorption at the middle troposphere, which may have strong implications for clouds and climate.

scholarly journals Vertical profiles of sub-micron aerosol single scattering albedo over Indian region immediately before monsoon onset and during its development: Research from the SWAAMI field campaign

2019 ◽  
Author(s):  
Mohanan R. Manoj ◽  
Sreedharan K. Satheesh ◽  
Krishnaswamy K. Moorthy ◽  
Hugh Coe
Keyword(s):  
Active Phase ◽  
Single Scattering ◽  
Single Scattering Albedo ◽  
Development Research ◽  
Aerosol Absorption ◽  
South West ◽  
Aerosol Scattering ◽  
First Time ◽  
Geographical Locations

Abstract. Vertical structures of aerosol single scattering albedo (SSA), from near the surface through the free troposphere, have been estimated for the first time at distinct geographical locations over the Indian mainland and adjoining oceans, using in-situ measurements of aerosol scattering and absorption coefficients aboard the FAAM BAe-146 aircraft during the South West Asian Aerosol Monsoon Interactions (SWAAMI) campaign from June to July 2016. These are used to examine the spatial variation of SSA profiles and also to characterize its transformation from just prior to the onset of Indian Summer Monsoon (June 2016) to its active phase (July 2016). Very strong aerosol absorption, with SSA values as low as 0.7, persisted in the lower altitudes (

scholarly journals Aerosol absorption retrieval at ultraviolet wavelengths in a complex environment

2012 ◽  
Vol 5 (5) ◽  
pp. 6991-7023 ◽  
Author(s):  
S. Kazadzis ◽  
N. Kouremeti ◽  
V. Amiridis ◽  
A. Arola ◽  
E. Gerasopoulos
Keyword(s):  
Wavelength Dependence ◽  
Single Scattering ◽  
Single Scattering Albedo ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Aerosol Composition ◽  
Aerosol Absorption ◽  
Uv Irradiance ◽  
Band Radiometer ◽  
Uv Range

Abstract. We have combined sun and sky radiance measurements from a CIMEL sun-photometer and total and diffuse UV irradiance measurements with a multi-filter rotating shadow-band radiometer (UVMFR), in order to calculate aerosol absorption properties (single scattering albedo) in the UV range, for a 10 month period in Athens, Greece. The aerosol extinction optical thickness measured by the CIMEL instrument has been used for the inter-calibration of the UVMFR. The measurements from both instruments were used as input to a radiative transfer model and the single scattering albedo (SSA) for 368 nm and 332 nm has been calculated. The SSA values at these wavelengths, together with synchronous SSA, CIMEL-derived, retrievals at 440 nm, show a mean of 0.88, 0.86 and 0.80, with lowest values (higher absorption) towards lower wavelengths. In addition, noticeable diurnal variations of the SSA in all wavelengths are revealed, with amplitudes in the order of 0.05. Higher SSA wavelength dependence is found for cases of lower Ångström exponents and also an SSA decrease with decreasing extinction optical depth, suggesting an effect of the different aerosol composition.

scholarly journals Study of the effect of different type of aerosols on UV-B radiation from measurements during EARLINET

2003 ◽  
Vol 3 (5) ◽  
pp. 4671-4700
Author(s):  
D. S. Balis ◽  
V. Amiridis ◽  
C. Zerefos ◽  
A. Kazantzidis ◽  
S. Kazadzis ◽  
...  
Keyword(s):  
Total Ozone ◽  
Single Scattering ◽  
Single Scattering Albedo ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Combined Use ◽  
Lidar Measurements ◽  
The Vertical Distribution ◽  
Aerosol Type

Abstract. Routine lidar measurements of the vertical distribution of the aerosol extinction coefficient and the extinction-to-backscatter ratio have been performed at Thessaloniki, Greece using a Raman lidar system in the frame of the EARLINET project since 2000. Spectral and broadband UV-B irradiance measurements, as well as total ozone observations, were available whenever lidar measurements were obtained. From the available measurements several cases could be identified that allowed the study of the effect of different types of aerosol on the levels of the UV-B solar irradiance at the Earth's surface. The TUV radiative transfer model has been used to simulate the irradiance measurements, using total ozone and the lidar aerosol data as input. From the comparison of the model results with the measured spectra the effective single scattering albedo was determined using an iterative procedure, which has been verified against results from the 1998 Lindenberg Aerosol Characterization Experiment. It is shown that the same aerosol optical depth and same total ozone values can show differences up to 10% in the UV-B irradiance at the Earth's surface, which can be attributed to differences in the aerosol type. It is shown that the combined use of the estimated single scattering albedo and the measured extinction-to-backscatter ratio leads to a better characterization of the aerosol type probed.

scholarly journals Global maps of aerosol single scattering albedo using combined CERES-MODIS retrieval

2021 ◽  
Author(s):  
Archana Devi ◽  
Sreedharan Krishnakumari Satheesh
Keyword(s):  
Climate Models ◽  
Radiant Energy ◽  
Energy System ◽  
Single Scattering ◽  
Global Scale ◽  
Single Scattering Albedo ◽  
Accurate Information ◽  
Climatic Impact ◽  
Aerosol Absorption ◽  
Moderate Resolution Imaging Spectroradiometer

Abstract. Single Scattering Albedo (SSA) is a leading contributor to the uncertainty in aerosol radiative impact assessments. Therefore accurate information on aerosol absorption is required on a global scale. In this study, we have applied a multi-satellite algorithm to retrieve SSA using the concept of ‘critical optical depth.’ Global maps of SSA were generated following this approach using spatially and temporally collocated data from Clouds and the Earth’s Radiant Energy System (CERES) and Moderate Resolution Imaging Spectroradiometer (MODIS) sensors on board Terra and Aqua satellites. The method has been validated using the data from aircraft-based measurements of various field campaigns. The retrieval uncertainty is ±0.03 and depends on both the surface albedo and aerosol absorption. Global mean SSA estimated over land and ocean is 0.93 and 0.97, respectively. Seasonal and spatial distribution of SSA over various regions are also presented. The global maps of SSA, thus derived with improved accuracy, provide important input to climate models for assessing the climatic impact of aerosols on regional and global scales.

scholarly journals Continental pollution in the Western Mediterranean basin: large variability of the aerosol single scattering albedo and influence on the direct shortwave radiative effect

2016 ◽  
Author(s):  
C. Di Biagio ◽  
P. Formenti ◽  
L. Doppler ◽  
C. Gaimoz ◽  
N. Grand ◽  
...  
Keyword(s):  
Mediterranean Basin ◽  
Single Scattering ◽  
Western Mediterranean ◽  
Single Scattering Albedo ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Radiative Effect ◽  
Large Variability ◽  
Western Mediterranean Basin ◽  
Study Results

Abstract. Pollution aerosols strongly influence the composition of the Western Mediterranean basin, but at present little is known on their optical properties. We report in this study in situ observations of the single scattering albedo (ω) of pollution aerosol plumes measured over the Western Mediterranean basin during the TRAQA (TRansport and Air QuAlity) airborne campaign in summer 2012. Cases of pollution export from different source regions around the basin and at different altitudes between ~160 and 3500 m above sea level have been sampled during the flights. Data from this study show a large variability of ω, with values between 0.84–0.98 at 370 nm and 0.70–0.99 at 950 nm. The single scattering albedo generally decreases with the wavelength, with some exception associated to the mixing of pollution with sea spray over the sea surface. Lowest values of ω (0.84–0.70 between 370 and 950 nm) are measured in correspondence of a fresh plume possibly linked to ship emissions over the basin. The range of variability of ω observed in this study seems to be independent of the source region around the basin, as well as of the altitude and ageing time of the plumes. The observed variability of ω reflects in a large variability for the complex refractive index of pollution aerosols, which is estimated to span in the large range 1.41–1.75 and 0.002–0.068 for the real and the imaginary parts, respectively, between 370 and 950 nm. Radiative calculations in clear-sky conditions have been performed with the GAME radiative transfer model to test the sensitivity of the aerosol shortwave Direct Radiative Effect (DRE) to the variability of ω as observed in this study. Results from the calculations suggest up to a 50 % and 30 % change of the forcing efficiency (FE), i.e. the DRE per unit of optical depth, at the surface (−160÷−235 Wm−2 τ−1 at 60° solar zenith angle) and at the Top-Of-Atmosphere (−137÷−92 5 Wm−2 τ−1) for ω varying between its maximum and minimum value. This induces a change of up to an order of magnitude (+23÷+143 Wm−2 τ−1) for the radiative effect within the atmosphere.

scholarly journals Spectral absorption properties of atmospheric aerosols

2007 ◽  
Vol 7 (23) ◽  
pp. 5937-5943 ◽  
Author(s):  
R. W. Bergstrom ◽  
P. Pilewskie ◽  
P. B. Russell ◽  
J. Redemann ◽  
T. C. Bond ◽  
...  
Keyword(s):  
Optical Depth ◽  
Atmospheric Aerosols ◽  
Wavelength Dependence ◽  
Single Scattering ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Spectral Absorption ◽  
Solar Absorption ◽  
Airborne Measurements ◽  
Aerosol Absorption

Abstract. We have determined the solar spectral absorption optical depth of atmospheric aerosols for specific case studies during several field programs (three cases have been reported previously; two are new results). We combined airborne measurements of the solar net radiant flux density and the aerosol optical depth with a detailed radiative transfer model for all but one of the cases. The field programs (SAFARI 2000, ACE Asia, PRIDE, TARFOX, INTEX-A) contained aerosols representing the major absorbing aerosol types: pollution, biomass burning, desert dust and mixtures. In all cases the spectral absorption optical depth decreases with wavelength and can be approximated with a power-law wavelength dependence (Absorption Angstrom Exponent or AAE). We compare our results with other recent spectral absorption measurements and attempt to briefly summarize the state of knowledge of aerosol absorption spectra in the atmosphere. We discuss the limitations in using the AAE for calculating the solar absorption. We also discuss the resulting spectral single scattering albedo for these cases.

scholarly journals Aerosol absorption retrieval at ultraviolet wavelengths in a complex environment

2016 ◽  
Author(s):  
Stelios Kazadzis ◽  
Panagiotis Ι. Raptis ◽  
Natalia Kouremeti ◽  
Vassilis Amiridis ◽  
Antti Arola ◽  
...  
Keyword(s):  
Wavelength Dependence ◽  
Single Scattering ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Aerosol Composition ◽  
Data Set ◽  
Aerosol Absorption ◽  
Uv Irradiance ◽  
Band Radiometer ◽  
Uv Range

Abstract. We have used total and diffuse UV irradiance measurements with a multi-filter rotating shadow-band radiometer (UVMFR), in order to calculate aerosol absorption properties (Single Scattering Albedo – SSA) in the UV range, for a 5 years period in Athens, Greece. Τhis data set was used as input to a radiative transfer model and the SSA for 368 nm and 332 nm has been calculated. Retrievals from a collocated CIMEL sun-photometer were used to validate the products and study absorption spectral behavior SSA values at these wavelengths. UVMFR SSA together with synchronous,CIMEL-derived, retrievals at 440 nm, show a mean of 0.90, 0.87 and 0.83, with lowest values (higher absorption) towards lower wavelengths. In addition, noticeable diurnal variations of the SSA in all wavelengths are revealed, with amplitudes in up to 0.05. High SSA wavelength dependence is found for cases of low Ångström exponents and also an SSA decrease with decreasing extinction optical depth, suggesting an effect of the different aerosol composition. Dust and Brown Carbon UV absorbing properties were investigated to understand seasonal variability of the results.

scholarly journals Seasonal differences in the vertical profiles of aerosol optical properties over rural Oklahoma

2011 ◽  
Vol 11 (4) ◽  
pp. 11939-11957 ◽  
Author(s):  
E. Andrews ◽  
P. J. Sheridan ◽  
J. A. Ogren
Keyword(s):  
Seasonal Variability ◽  
Seasonal Cycle ◽  
Gulf Coast ◽  
Single Scattering ◽  
Single Scattering Albedo ◽  
Vertical Profiles ◽  
Seasonal Differences ◽  
Aerosol Loading ◽  
Aerosol Absorption ◽  
Aerosol Scattering

Abstract. A small airplane made more than 450 aerosol optical property (light absorption and light scattering) vertical profile measurements (up to 4 km) over a rural Oklahoma site between March 2000 and July 2005. These profiles suggest significant seasonal differences in aerosol properties. The highest amounts of scattering and absorbing aerosol are observed during the summer, while the relative contribution of aerosol absorption is highest in the winter (i.e., single scattering albedo is lowest in winter). Aerosol absorption generally decreased with altitude below ∼1.5 km and then was relatively constant above that. Aerosol scattering decreased sharply with altitude below ∼1.5 km but, unlike absorption, also decreased at higher altitudes, albeit less sharply. The seasonal variability observed for aerosol loading is consistent with other aerosol measurements in the region including AERONET aerosol optical depth (AOD), CALIPSO vertical profiles, and IMPROVE aerosol mass. The column averaged single scattering albedo derived from in situ airplane measurements shows a similar seasonal cycle as the AERONET single scattering albedo inversion product, but a comparison of aerosol asymmetry parameter from airplane and AERONET platforms suggests differences in seasonal variability. The observed seasonal cycle of aerosol loading corresponds with changes in air mass back trajectories: the aerosol scattering was higher when transport was from polluted areas (e.g., the Gulf Coast) and lower when the air came from cleaner regions and/or the upper atmosphere.

scholarly journals Comparison of UV-RSS spectral measurements and TUV model runs for clear skies for the May 2003 ARM aerosol intensive observation period

2007 ◽  
Vol 7 (6) ◽  
pp. 17401-17427
Author(s):  
J. J. Michalsky ◽  
P. W. Kiedron
Keyword(s):  
Radiative Transfer ◽  
Single Scattering ◽  
Single Scattering Albedo ◽  
Spectral Irradiance ◽  
Radiative Transfer Model ◽  
Visible Range ◽  
Transfer Model ◽  
Intensive Observation ◽  
Aerosol Properties ◽  
Observation Period

Abstract. The first successful deployment of the fully-operational ultraviolet rotating shadow-band spectroradiometer occurred during the May 2003 U.S. Department of Energy's Atmospheric Radiation Measurement program's Aerosol Intensive Observation Period. The aerosol properties in the visible range were characterized using redundant measurements with several instruments to determine the column aerosol optical depth, the single scattering albedo, and the asymmetry parameter needed as input for radiative transfer calculations of the downwelling direct normal and diffuse horizontal solar irradiance in clear-sky conditions. The Tropospheric Ultraviolet and Visible (TUV) radiative transfer model developed by Madronich and his colleagues at the U.S. National Center for Atmospheric Research was used for the calculations of the spectral irradiance between 300–360 nm. Since there are few ultraviolet measurements of aerosol properties, most of the input aerosol data for the radiative transfer model are based on the assumption that UV input parameters can be extrapolated from the visible portion of the spectrum. Disagreements between available extraterrestrial spectra, which are discussed briefly, suggested that instead of comparing irradiances that measured and modeled spectral transmittances between 300–360 nm should be compared for the seven cases studied. These cases included low to moderate aerosol loads and low to high solar-zenith angles. A procedure for retrieving single scattering albedo in the ultraviolet based on the comparisons of direct and diffuse transmittance is outlined.

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