scholarly journals The effects of cloud–aerosol interaction complexity on simulations of presummer rainfall over southern China

2020 ◽  
Vol 20 (8) ◽  
pp. 5093-5110
Author(s):  
Kalli Furtado ◽  
Paul Field ◽  
Yali Luo ◽  
Tianjun Zhou ◽  
Adrian Hill
Keyword(s):  
Southern China ◽  
Deep Convection ◽  
Short Wave ◽  
Wave Radiation ◽  
Cloud Droplets ◽  
Cloud Processing ◽  
Surface Rainfall ◽  
Clean Environment ◽  
Aerosol Number Concentration ◽  
Condensed Water

Abstract. Convection-permitting simulations are used to understand the effects of cloud–aerosol interactions in a case of heavy rainfall over southern China. The simulations are evaluated using radar observations from the Southern China Monsoon Rainfall Experiment (SCMREX) and remotely sensed estimates of precipitation, clouds and radiation. We focus on the effects of complexity in cloud–aerosol interactions, especially the depletion and transport of aerosol material by clouds. In particular, simulations with aerosol concentrations held constant are compared with a fully cloud–aerosol-interacting system to investigate the effects of two-way coupling between aerosols and clouds on a line of organised deep convection. It is shown that the cloud processing of aerosols can change the vertical structure of the storm by using up aerosols within the core of line, thereby maintaining a relatively clean environment which propagates with the heaviest rainfall. This induces changes in the statistics of surface rainfall, with a cleaner environment being associated with less-intense but more-frequent rainfall. These effects are shown to be related to a shortening of the timescale for converting cloud droplets to rain as the aerosol number concentration is decreased. The simulations are compared to satellite-derived estimates of surface rainfall, a condensed-water path and the outgoing flux of short-wave radiation. Simulations for fewer aerosol particles outperform the more polluted simulations for surface rainfall but give poorer representations of top-of-atmosphere (TOA) radiation.

scholarly journals The effects of cloud-aerosol-interaction complexity on simulations of presummer rainfall over southern China

2019 ◽  
Author(s):  
Kalli Furtado ◽  
Paul Field ◽  
Yali Luo ◽  
Tianjun Zhou ◽  
Adrian Hill
Keyword(s):  
South China ◽  
Vertical Structure ◽  
Monsoon Rainfall ◽  
Southern China ◽  
Deep Convection ◽  
Cloud Droplets ◽  
Cloud Processing ◽  
Squall Lines ◽  
Surface Rainfall ◽  
Fully Coupled

Abstract. Convection-permitting simulations are used to understand the effects of cloud-aerosol interactions on a case of heavy rainfall over south China. The simulations are evaluated using radar observations from the South China Monsoon Rainfall Experiment and remotely sensed estimates of precipitation, clouds and radiation. We focus on the effects of complexity in cloud-aerosol interactions, especially processing and transport of dissolved material inside clouds. In particular, simulations with aerosol concentrations held constant are compared with a fully coupled cloud-aerosol-interacting system to isolate the effects of processing on a line of organised-deep convection. It is shown that in-cloud processing of aerosols can change the vertical structure of squall lines thereby inducing changes in the statistics of surface rainfall. These effects are shown to be consistent with a modulation by aerosol of the timescale of the converting cloud-droplets to rain.

scholarly journals In-cloud formation of secondary species in iron-containing particles

2019 ◽  
Vol 19 (2) ◽  
pp. 1195-1206 ◽  
Author(s):  
Qinhao Lin ◽  
Xinhui Bi ◽  
Guohua Zhang ◽  
Yuxiang Yang ◽  
Long Peng ◽  
...  
Keyword(s):  
Southern China ◽  
Formation Rate ◽  
Cloud Formation ◽  
Dust Particles ◽  
Cloud Droplets ◽  
Aerosol Mass Spectrometer ◽  
Secondary Species ◽  
Cloud Processing ◽  
Aerosol Mass ◽  
Combustion Sources

Abstract. The increase in secondary species through cloud processing potentially increases aerosol iron (Fe) bioavailability. In this study, a ground-based counterflow virtual impactor coupled with a real-time single-particle aerosol mass spectrometer was used to characterize the formation of secondary species in Fe-containing cloud residues (dried cloud droplets) at a mountain site in southern China for nearly 1 month during the autumn of 2016. Fe-rich, Fe-dust, Fe-elemental carbon (Fe-EC), and Fe-vanadium (Fe-V) cloud residual types were obtained in this study. The Fe-rich particles, related to combustion sources, contributed 84 % (by number) to the Fe-containing cloud residues, and the Fe-dust particles represented 12 %. The remaining 4 % consisted of the Fe-EC and Fe-V particles. It was found that above 90 % (by number) of Fe-containing particles had already contained sulfate before cloud events, leading to no distinct change in number fraction (NF) of sulfate during cloud events. Cloud processing contributed to the enhanced NFs of nitrate, chloride, and oxalate in the Fe-containing cloud residues. However, the in-cloud formation of nitrate and chloride in the Fe-rich type was less obvious relative to the Fe-dust type. The increased NF of oxalate in the Fe-rich cloud residues was produced via aqueous oxidation of oxalate precursors (e.g., glyoxylate). Moreover, Fe-driven Fenton reactions likely increase the formation rate of aqueous-phase OH, improving the conversion of the precursors to oxalate in the Fe-rich cloud residues. During daytime, the decreased NF of oxalate in the Fe-rich cloud residues was supposed to be due to the photolysis of Fe-oxalate complexes. This work emphasizes the role of combustion Fe sources in participating in cloud processing and has important implications for evaluating Fe bioavailability from combustion sources during cloud processing.

scholarly journals In-cloud formation of secondary species in iron-containing particles

2018 ◽  
Author(s):  
Qinhao Lin ◽  
Xinhui Bi ◽  
Guohua Zhang ◽  
Yuxiang Yang ◽  
Long Peng ◽  
...  
Keyword(s):  
Southern China ◽  
Cloud Formation ◽  
Dust Particles ◽  
Cloud Droplets ◽  
Aerosol Mass Spectrometer ◽  
Secondary Species ◽  
Cloud Processing ◽  
Aerosol Mass ◽  
Combustion Sources

Abstract. The increase of secondary species through cloud processing potentially increases aerosol iron (Fe) bioavailability. In this study, a ground-based counterflow virtual impactor coupled with a real-time single-particle aerosol mass spectrometer was used to characterize the formation of secondary species in Fe-containing cloud residues (dried cloud droplets) at a mountain site in southern China for nearly one month during the autumn of 2016. Fe-rich, Fe-dust, Fe-elemental carbon (Fe-EC), and Fe-vanadium (Fe-V) cloud residual types were obtained in this study. The Fe-rich particles, related to combustion sources, contributed 84 % to the Fe-containing cloud residues, and the Fe-dust particles represented 12 %. The remaining 4 % consisted of the Fe-EC and Fe-V particles. It was found that extremely high amounts of sulfate had already accumulated on the Fe-containing particles before cloud events, leading to no distinct changes in sulfate during cloud events. Cloud processing contributed to the enhancement of nitrate, chloride, and oxalate in the Fe-containing cloud residues. However, the in-cloud formation of nitrate and chloride in the Fe-rich type was less obvious relative to the Fe-dust type. The enhancement of oxalate in the Fe-rich cloud residues was produced via aqueous oxidation of oxalate precursors (e.g., glyoxylate). Moreover, Fe chemistry involved in the Fenton reaction further promoted the conversion of the oxalate precursors to oxalate during cloud events, although the photolysis of Fe-oxalate complexes also existed in the Fe-rich cloud residues. This work emphasizes the role of combustion Fe sources in participating in cloud processing and has important implications for evaluating Fe bioavailability from combustion sources during cloud processing.

scholarly journals Evaluating the Effects of Façade Greening on Human Bioclimate in a Complex Urban Environment

2015 ◽  
Vol 2015 ◽  
pp. 1-15 ◽  
Author(s):  
Britta Jänicke ◽  
Fred Meier ◽  
Marie-Therese Hoelscher ◽  
Dieter Scherer
Keyword(s):  
Heat Stress ◽  
Short Wave ◽  
Wave Radiation ◽  
Short Wave Radiation ◽  
Long Wave ◽  
Building Facades ◽  
Urban Heat ◽  
The Mean ◽  
Human Bioclimate ◽  
Radiant Temperature

The evaluation of the effectiveness of countermeasures for a reduction of urban heat stress, such as façade greening, is challenging due to lacking transferability of results from one location to another. Furthermore, complex variables such as the mean radiant temperature(Tmrt)are necessary to assess outdoor human bioclimate. We observedTmrtin front of a building façade in Berlin, Germany, which is half-greened while the other part is bare.Tmrtwas reduced (mean 2 K) in front of the greened compared to the bare façade. To overcome observational shortcomings, we applied the microscale models ENVI-met, RayMan, and SOLWEIG. We evaluated these models based on observations. Our results show thatTmrt(MD = −1.93 K) and downward short-wave radiation (MD = 14.39 W/m2) were sufficiently simulated in contrast to upward short-wave and long-wave radiation. Finally, we compare the simulated reduction ofTmrtwith the observed one in front of the façade greening, showing that the models were not able to simulate the effects of façade greening with the applied settings. Our results reveal that façade greening contributes only slightly to a reduction of heat stress in front of building façades.

scholarly journals Albedo of Melting Sea Ice in the Southern Beaufort Sea

1971 ◽  
Vol 10 (58) ◽  
pp. 101-104 ◽  
Author(s):  
M.P. Langleben
Keyword(s):  
Sea Ice ◽  
Northwest Territories ◽  
Beaufort Sea ◽  
Ice Cover ◽  
Short Wave ◽  
Wave Radiation ◽  
Short Wave Radiation ◽  
Melting Period ◽  
Fast Ice ◽  
Made In

AbstractTwo Kipp hemispherical radiometers mounted back to back and suspended by an 18 m cable from a helicopter flying at an altitude of about 90 m were used to make measurements of incident and reflected short-wave radiation. The helicopter was brought to a hovering position at the instant of measurement to ensure that the radiometers were in the proper attitude and a photograph of the ice cover was taken at the same time. The observations were made in 1969 during 16 flights out of Tuktoyaktuk, Northwest Territories (lat. 69° 26’N., long. 133° 02’W.) over the fast ice extending 80 km north of Tuktoyaktuk. Values of albedo of the ice cover were found to decrease during the melting period according to the equation A = 0.59 —0.32P where P is the degree of puddling of the surface.

Short-wave radiation from a tube with a gas screen

1974 ◽  
Vol 20 (4) ◽  
pp. 434-438
Author(s):  
E. M. Golubev ◽  
N. N. Ogurtsova ◽  
I. V. Podmoshenskii ◽  
P. N. Rogovtsev
Keyword(s):  
Short Wave ◽  
Wave Radiation ◽  
Short Wave Radiation ◽  
Gas Screen

scholarly journals Measurements of Ablation and Heat Balance On Alpine Glaciers: With some remarks on the cause of glacier recession in the Alps

1955 ◽  
Vol 2 (17) ◽  
pp. 497-501 ◽  
Author(s):  
H. Hoinkes
Keyword(s):  
Latent Heat ◽  
Heat Balance ◽  
Eastern Alps ◽  
Short Wave ◽  
Wave Radiation ◽  
Perfect Agreement ◽  
Glacier Recession ◽  
A Value ◽  
Alpine Glaciers ◽  
Summer Temperatures

AbstractMeasurements of heat balance and ablation on glaciers of the Eastern Alps carried out during a total of 45 days since the summer of 1950 indicate that in flat glaciated areas at approximately 3000 m. above sea level 81 to 84 per cent of the energy causing ablation is supplied by short wave radiation from the sun and sky. Only 16 to 19 per cent come from the air in the form of actual and latent heat. On glacier tongues at altitudes of approximately 2300 m. the percentage of ablation caused by radiation is only 58 to 65 per cent. This is primarily the result of the shortened duration of sunshine in the deeper valleys. The supply of perceptible and latent heat from the air can, at most, reach a value of 15 to 30 per cent on glacier tongues. Evaporation from the ice and heat supply by liquid precipitation are negligible during the normal ablation period (June till September).It is to be expected therefore that the alpine glaciers will primarily react to variations of radiation and albedo during the months of June to September. The effects of changing summer temperatures are considered insufficient to cause the vast changes of the ice-cover. The variations of the duration of summer sunshine and the number of days with snowfall as a rough indication of albedo, respectively, are in perfect agreement with the behaviour of alpine glaciers during the last sixty years.

scholarly journals Size distributions of elemental carbon in the atmosphere of a coastal urban area in South China: characteristics, evolution processes, and implications for the mixing state

2008 ◽  
Vol 8 (19) ◽  
pp. 5843-5853 ◽  
Author(s):  
X.-F. Huang ◽  
J. Z. Yu
Keyword(s):  
Urban Area ◽  
Elemental Carbon ◽  
Southern China ◽  
Global Climate ◽  
Particle Growth ◽  
Size Distributions ◽  
Hygroscopic Growth ◽  
Mixing State ◽  
Cloud Processing ◽  
Fine Mode

Abstract. Elemental carbon (EC), as one of the primary light-absorbing components in the atmosphere, has a significant impact on both regional and global climate. The environmental impacts of EC are strongly dependent on its particle size. Little is known about the size distribution characteristics of EC particles in China's ambient environments. We report size distributions of EC particles in the urban area of Shenzhen in Southern China. In our samples, EC was consistently found in two modes, a fine mode and a coarse mode. The majority of EC mass (~80%) in this coastal metropolitan city resided in particles smaller than 3.2 μm in diameter. The fine mode peaked at around either 0.42 μm or 0.75 μm. While the mode at 0.42 μm could be ascribed to fresh vehicular emissions in the region, the mode at 0.75 μm was likely a result of particle growth from smaller EC particles. We theoretically investigated the particle growth processes that caused the EC particles to grow from 0.42 μm to 0.75 µm in the atmosphere. Our calculations indicate that the EC peak at 0.75 μm was not produced through either coagulation or H2SO4 condensation; both processes are too slow to lead to significant EC growth. Hygroscopic growth was also determined to be insignificant. Instead, addition of sulfate through in-cloud processing was found to cause significant growth of the EC particles and to explain the EC peak at 0.75 μm. We also estimated the mixing state of EC from the EC size distributions. In the droplet size, at least 45–60% of the EC mass in the summer samples and 68% of the EC mass in the winter samples was internally mixed with sulfate as a result of in-cloud processing. This information on EC should be considered in models of the optical properties of aerosols in this region. Our results also suggest that the in-cloud processing of primary EC particles could increase the light absorbing capacities through mixing EC with sulfate.

scholarly journals The Influence of Cloudiness on The Net Radiation Balance of A Snow Surface with High Albedo

1974 ◽  
Vol 13 (67) ◽  
pp. 73-84 ◽  
Author(s):  
W. Ambach
Keyword(s):  
Greenland Ice Sheet ◽  
Short Wave ◽  
Mean Value ◽  
Wave Radiation ◽  
Radiation Balance ◽  
Net Radiation ◽  
Long Wave ◽  
Energy Excess ◽  
Overcast Sky ◽  
Long Wave Radiation

The short-wave and long-wave radiant fluxes measured in the accumulation area of the Greenland ice sheet during a mid-summer period are discussed with respect to their dependence on cloudiness. At a cloudiness of 10/10, a mean value of 270 J/cm2 d is obtained for the daily totals of net radiation balance, whereas a mean value of only 75 J/cm2 d is observed at 0/10. The energy excess of the net radiation balance with overcast sky is due to the significant influence of the incoming long-wave radiation and the high albedo of the surface (average of 84%). High values of net radiation balance are therefore correlated with high values of long-wave radiation balance and low values of short-wave radiation balance.

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