scholarly journals The importance of interactive chemistry for stratosphere–troposphere–coupling

2018 ◽  
Author(s):  
Sabine Haase ◽  
Katja Matthes

Abstract. Recent observational and modeling studies suggest that not only southern hemispheric surface climate is influenced by stratospheric ozone depletion but also northern hemisphere (NH) spring, implying a strong interaction between dynamics and chemistry. Here, we systematically analyze the importance of interactive chemistry for the representation of stratosphere–troposphere–coupling and in particular the effects on NH surface climate during the recent past. We use the interactive and specified chemistry version of NCAR's Whole Atmosphere Community Climate Model coupled to an ocean model to investigate differences in the mean state of the NH stratosphere as well as in stratospheric extreme events, namely sudden stratospheric warmings (SSWs), and their surface impacts. We also test the effects of zonally symmetric versus asymmetric prescribed ozone, testing the importance of ozone waves for the representation of stratospheric mean state and variability. The interactive chemistry simulation is characterized by a statistically significant stronger and colder polar night jet (PNJ) during spring when ozone depletion becomes important. We identify a negative feedback between lower stratospheric ozone and atmospheric dynamics during the break down of the stratospheric polar vortex in the NH, which contributes to the different characteristics of the PNJ between the simulations. Not only the mean state, but also stratospheric variability is better represented in the interactive chemistry simulation, which shows a more realistic distribution of SSWs as well as a more persisting surface impact afterwards compared to the simulation where the feedback between chemistry and dynamics is switched off. We hypothesize that this is also related to the feedback between ozone and dynamics through the intrusion of ozone rich air into polar latitudes during SSWs. The results from the zonally asymmetric ozone simulation are closer to the interactive chemistry simulations, implying that a three-dimensional representation of prescribed ozone is necessary and desirable in case interactive chemistry is not available or possible for (multi-) centennial simulations. Our findings underline the importance of the representation of interactive chemistry and its feedback on the stratospheric mean state and variability not only on the SH but also on the NH during the recent past.

2019 ◽  
Vol 19 (5) ◽  
pp. 3417-3432 ◽  
Author(s):  
Sabine Haase ◽  
Katja Matthes

Abstract. Recent observational and modeling studies suggest that stratospheric ozone depletion not only influences the surface climate in the Southern Hemisphere (SH), but also impacts Northern Hemisphere (NH) spring, which implies a strong interaction between dynamics and chemistry. Here, we systematically analyze the importance of interactive chemistry with respect to the representation of stratosphere–troposphere coupling and in particular the effects on NH surface climate during the recent past. We use the interactive and specified chemistry version of NCAR's Whole Atmosphere Community Climate Model coupled to an ocean model to investigate differences in the mean state of the NH stratosphere as well as in stratospheric extreme events, namely sudden stratospheric warmings (SSWs), and their surface impacts. To be able to focus on differences that arise from two-way interactions between chemistry and dynamics in the model, the specified chemistry model version uses a time-evolving, model-consistent ozone field generated by the interactive chemistry model version. We also test the effects of zonally symmetric versus asymmetric prescribed ozone, evaluating the importance of ozone waves in the representation of stratospheric mean state and variability. The interactive chemistry simulation is characterized by a significantly stronger and colder polar night jet (PNJ) during spring when ozone depletion becomes important. We identify a negative feedback between lower stratospheric ozone and atmospheric dynamics during the breakdown of the stratospheric polar vortex in the NH, which contributes to the different characteristics of the PNJ between the simulations. Not only the mean state, but also stratospheric variability is better represented in the interactive chemistry simulation, which shows a more realistic distribution of SSWs as well as a more persistent surface impact afterwards compared with the simulation where the feedback between chemistry and dynamics is switched off. We hypothesize that this is also related to the feedback between ozone and dynamics via the intrusion of ozone-rich air into polar latitudes during SSWs. The results from the zonally asymmetric ozone simulation are closer to the interactive chemistry simulations, implying that under a model-consistent ozone forcing, a three-dimensional (3-D) representation of the prescribed ozone field is desirable. This suggests that a 3-D ozone forcing, as recommended for the upcoming CMIP6 simulations, has the potential to improve the representation of stratospheric dynamics and chemistry. Our findings underline the importance of the representation of interactive chemistry and its feedback on the stratospheric mean state and variability not only in the SH but also in the NH during the recent past.


2021 ◽  
Author(s):  
Marina Friedel ◽  
Gabriel Chiodo ◽  
Andrea Stenke ◽  
Daniela Domeisen ◽  
Stephan Fueglistaler ◽  
...  

Abstract Massive spring ozone loss due to anthropogenic emissions of ozone depleting substances is not limited to the austral hemisphere, but can also occur in the Arctic. Previous studies have suggested a link between springtime Arctic ozone depletion and Northern Hemispheric surface climate, which might add surface predictability. However, so far it has not been possible to isolate the role of stratospheric ozone from dynamical downward impacts. For the first time, we quantify the impact of springtime Arctic ozone depletion on surface climate using observations and targeted chemistry-climate model experiments to isolate the effects of ozone feedbacks. We find that springtime stratospheric ozone depletion is followed by surface anomalies in precipitation and temperature resembling a positive Arctic Oscillation. Most notably, we show that these anomalies, affecting large portions of the Northern Hemisphere, cannot be explained by dynamical variability alone, but are to a significant degree driven by stratospheric ozone. The surface signal is linked to reduced shortwave absorption by stratospheric ozone, forcing persistent negative temperature anomalies in the lower stratosphere and a delayed breakup of the polar vortex - analogous to ozone-surface coupling in the Southern Hemisphere.These results suggest that Arctic stratospheric ozone actively forces springtime Northern Hemispheric surface climate and thus provides a source of predictability on seasonal scales.


2020 ◽  
Author(s):  
Brian Zambri ◽  
Susan Solomon ◽  
David Thompson ◽  
Qiang Fu

<p>Ozone depletion in the Southern Hemisphere (SH) stratosphere in the late 20<sup>th</sup> century cooled the air there, strengthening the SH stratospheric westerly winds near 60ºS and altering SH surface climate. Since ~1999, trends in Antarctic ozone have begun to recover, exhibiting a flattening followed by a sign reversal in response to decreases in stratospheric chlorine concentration due to the Montreal Protocol, an international treaty banning the production and consumption of ozone-depleting substances. Here we show that the post–1999 increase in ozone has resulted in thermal and circulation changes of opposite sign to those that resulted from stratospheric ozone losses, including a warming of the SH polar lower stratosphere and a weakening of the SH stratospheric polar vortex.  Further, these altered trends extend to the upper troposphere, albeit of smaller magnitudes.  Observed post–1999 trends of temperature and circulation in the stratosphere are about 20–25% the magnitude of those of the ozone depletion era, and are broadly consistent with expectations based on modeled depletion-era trends and variability of both ozone and reactive chlorine, thereby indicating the emergence of healing of dynamical impacts of the Antarctic ozone hole.</p>


2013 ◽  
Vol 70 (12) ◽  
pp. 3977-3994 ◽  
Author(s):  
John R. Albers ◽  
Terrence R. Nathan

Abstract A mechanistic chemistry–dynamical model is used to evaluate the relative importance of radiative, photochemical, and dynamical feedbacks in communicating changes in lower-stratospheric ozone to the circulation of the stratosphere and lower mesosphere. Consistent with observations and past modeling studies of Northern Hemisphere late winter and early spring, high-latitude radiative cooling due to lower-stratospheric ozone depletion causes an increase in the modeled meridional temperature gradient, an increase in the strength of the polar vortex, and a decrease in vertical wave propagation in the lower stratosphere. Moreover, it is shown that, as planetary waves pass through the ozone loss region, dynamical feedbacks precondition the wave, causing a large increase in wave amplitude. The wave amplification causes an increase in planetary wave drag, an increase in residual circulation downwelling, and a weaker polar vortex in the upper stratosphere and lower mesosphere. The dynamical feedbacks responsible for the wave amplification are diagnosed using an ozone-modified refractive index; the results explain recent chemistry–coupled climate model simulations that suggest a link between ozone depletion and increased polar downwelling. The effects of future ozone recovery are also examined and the results provide guidance for researchers attempting to diagnose and predict how stratospheric climate will respond specifically to ozone loss and recovery versus other climate forcings including increasing greenhouse gas abundances and changing sea surface temperatures.


2020 ◽  
Author(s):  
Jessica Oehrlein ◽  
Gabriel Chiodo ◽  
Lorenzo M. Polvani

Abstract. Modeling and observational studies have reported effects of stratospheric ozone extremes on Northern Hemisphere spring climate. Recent work has further suggested that the coupling of ozone chemistry and dynamics amplifies the surface response to midwinter sudden stratospheric warmings (SSWs). Here, we study the importance of interactive ozone chemistry in representing the stratospheric polar vortex and Northern Hemisphere winter surface climate variability. We contrast two simulations from the interactive and specified chemistry (and thus ozone) versions of the Whole Atmosphere Community Climate Model, designed to isolate the impact of interactive ozone on polar vortex variability. In particular, we analyze the response with and without interactive chemistry to midwinter SSWs, March SSWs, and strong polar vortex events (SPVs). With interactive chemistry, the stratospheric polar vortex is stronger, and more SPVs occur, but we find little effect on the frequency of midwinter SSWs. At the surface, interactive chemistry results in a pattern resembling a more negative North Atlantic Oscillation following midwinter SSWs, but with little impact on the surface signatures of late winter SSWs and SPVs. These results suggest that including interactive ozone chemistry is important for representing North Atlantic and European winter climate variability.


2020 ◽  
Vol 20 (17) ◽  
pp. 10531-10544
Author(s):  
Jessica Oehrlein ◽  
Gabriel Chiodo ◽  
Lorenzo M. Polvani

Abstract. Modeling and observational studies have reported effects of stratospheric ozone extremes on Northern Hemisphere spring climate. Recent work has further suggested that the coupling of ozone chemistry and dynamics amplifies the surface response to midwinter sudden stratospheric warmings (SSWs). Here we study the importance of interactive ozone chemistry in representing the stratospheric polar vortex and Northern Hemisphere winter surface climate variability. We contrast two simulations from the interactive and specified chemistry (and thus ozone) versions of the Whole Atmosphere Community Climate Model, which is designed to isolate the impact of interactive ozone on polar vortex variability. In particular, we analyze the response with and without interactive chemistry to midwinter SSWs, March SSWs, and strong polar vortex events (SPVs). With interactive chemistry, the stratospheric polar vortex is stronger and more SPVs occur, but we find little effect on the frequency of midwinter SSWs. At the surface, interactive chemistry results in a pattern resembling a more negative North Atlantic Oscillation following midwinter SSWs but with little impact on the surface signatures of late winter SSWs and SPVs. These results suggest that including interactive ozone chemistry is important for representing North Atlantic and European winter climate variability.


2020 ◽  
Vol 33 (11) ◽  
pp. 4641-4658
Author(s):  
Jiankai Zhang ◽  
Wenshou Tian ◽  
Fei Xie ◽  
John A. Pyle ◽  
James Keeble ◽  
...  

AbstractRecent studies have found a shift of the Arctic stratospheric polar vortex toward Siberia during late winter since 1980, intensifying the zonally asymmetric ozone (ZAO) depletion in the northern middle and high latitudes with a stronger total column ozone decline over Siberia compared with that above other regions at the same latitudes. Using observations and a climate model, this study shows that zonally asymmetric stratospheric ozone depletion gives a significant feedback on the position of the polar vortex and further favors the stratospheric polar vortex shift toward Siberia in February for the period 1980–99. The polar vortex shift is not significant in the experiment forced by zonal mean ozone fields. The February ZAO trend with a stronger ozone decline over Siberia causes a lower temperature over this region than over the other regions at the same latitudes, due to shortwave radiative cooling and dynamical cooling. The combined cooling effects induce an anomalous cyclonic flow over Siberia, corresponding to the polar vortex shift toward Siberia. In addition, the ZAO depletion also increases the meridional gradient of potential vorticity over Siberia, which is favorable for the upward propagation of planetary wave fluxes from the troposphere over this region. Increased horizontal divergence of planetary waves fluxes over the region 60°–75°N, 60°–90°E associated with ZAO changes accelerates the high-latitude zonal westerlies in the middle stratosphere, further enhancing the shift of the stratospheric polar vortex toward Siberia. After 2000, the ZAO trend in February is weaker and induces a smaller polar vortex shift than that in the period 1980–99.


2014 ◽  
Vol 71 (7) ◽  
pp. 2335-2353 ◽  
Author(s):  
Lantao Sun ◽  
Gang Chen ◽  
Walter A. Robinson

Abstract This paper investigates the connection between the delay in the final breakdown of the stratospheric polar vortex, the stratospheric final warming (SFW), and Southern Hemisphere climate trends. The authors first analyze Interim European Centre for Medium-Range Weather Forecasts (ECMWF) Re-Analysis (ERA-Interim) and three climate model outputs with different climate forcings. Climate trends appear when there is a delay in the timing of SFWs. When regressed onto the SFW dates (which reflect the anomaly when the SFW is delayed for one standard deviation of its onset dates), the anomaly pattern bears a resemblance to the observed climate trends, for all the model outputs, even without any trends. This suggests that the stratospheric and tropospheric circulations are organized by the timing of SFWs in both the interannual time scale and climate trends because of external forcings. The authors further explore the role of the SFW using a simplified dynamical model in which the ozone depletion is mimicked by a springtime polar stratospheric cooling. The responses of zonal-mean atmospheric circulation, including zonal wind, temperature, and poleward edge of the Hadley cell and the Ferrel cell, are similar to the observed climate trends. The authors divide the years into those in which the SFW is delayed and those in which it is not. The responses for the years in which the SFW is delayed are very similar to the overall response, while the stratosphere is only characterized by the localized cooling for those years in which the SFW is not delayed, with no subsequent downward influence into the troposphere. This suggests that, in order to affect the troposphere, ozone depletion must first delay the SFW so as to induce a deep response in planetary wave drag and the associated eddy-driven circulation.


2012 ◽  
Vol 69 (8) ◽  
pp. 2608-2618 ◽  
Author(s):  
Daniel M. Mitchell ◽  
Scott M. Osprey ◽  
Lesley J. Gray ◽  
Neal Butchart ◽  
Steven C. Hardiman ◽  
...  

Abstract With extreme variability of the Arctic polar vortex being a key link for stratosphere–troposphere influences, its evolution into the twenty-first century is important for projections of changing surface climate in response to greenhouse gases. Variability of the stratospheric vortex is examined using a state-of-the-art climate model and a suite of specifically developed vortex diagnostics. The model has a fully coupled ocean and a fully resolved stratosphere. Analysis of the standard stratospheric zonal mean wind diagnostic shows no significant increase over the twenty-first century in the number of major sudden stratospheric warmings (SSWs) from its historical value of 0.7 events per decade, although the monthly distribution of SSWs does vary, with events becoming more evenly dispersed throughout the winter. However, further analyses using geometric-based vortex diagnostics show that the vortex mean state becomes weaker, and the vortex centroid is climatologically more equatorward by up to 2.5°, especially during early winter. The results using these diagnostics not only characterize the vortex structure and evolution but also emphasize the need for vortex-centric diagnostics over zonally averaged measures. Finally, vortex variability is subdivided into wave-1 (displaced) and -2 (split) components, and it is implied that vortex displacement events increase in frequency under climate change, whereas little change is observed in splitting events.


2011 ◽  
Vol 24 (16) ◽  
pp. 4210-4229 ◽  
Author(s):  
Tiffany A. Shaw ◽  
Judith Perlwitz ◽  
Nili Harnik ◽  
Paul A. Newman ◽  
Steven Pawson

Abstract The impact of stratospheric ozone changes on downward wave coupling between the stratosphere and troposphere in the Southern Hemisphere is investigated using a suite of Goddard Earth Observing System chemistry–climate model (GEOS CCM) simulations. Downward wave coupling occurs when planetary waves reflected in the stratosphere impact the troposphere. In reanalysis data, the climatological coupling occurs from September to December when the stratospheric basic state has a well-defined high-latitude meridional waveguide in the lower stratosphere that is bounded above by a reflecting surface, called a bounded wave geometry. Reanalysis data suggests that downward wave coupling during November–December has increased during the last three decades. The GEOS CCM simulation of the recent past captures the main features of downward wave coupling in the Southern Hemisphere. Consistent with the Modern Era Retrospective-Analysis for Research and Application (MERRA) dataset, wave coupling in the model maximizes during October–November when there is a bounded wave geometry configuration. However, the wave coupling in the model is stronger than in the MERRA dataset, and starts earlier and ends later in the seasonal cycle. The late season bias is caused by a bias in the timing of the stratospheric polar vortex breakup. Temporal changes in stratospheric ozone associated with past depletion and future recovery significantly impact downward wave coupling in the model. During the period of ozone depletion, the spring bounded wave geometry, which is favorable for downward wave coupling, extends into early summer, due to a delay in the vortex breakup date, and leads to increased downward wave coupling during November–December. During the period of ozone recovery, the stratospheric basic state during November–December shifts from a spring configuration back to a summer configuration, where waves are trapped in the troposphere, and leads to a decrease in downward wave coupling. Model simulations with chlorine fixed at 1960 values and increasing greenhouse gases show no significant changes in downward wave coupling and confirm that the changes in downward wave coupling in the model are caused by ozone changes. The results reveal a new mechanism wherein stratospheric ozone changes can affect the tropospheric circulation.


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