scholarly journals Global response of parameterised convective cloud fields to anthropogenic aerosol forcing

2019 ◽  
Author(s):  
Zak Kipling ◽  
Laurent Labbouz ◽  
Philip Stier
Keyword(s):  
Large Scale ◽  
Climate Model ◽  
Global Climate ◽  
Convective Cloud ◽  
Climate Impact ◽  
Limited Area ◽  
Climate Modelling ◽  
Anthropogenic Aerosol ◽  
Convective Clouds ◽  
Aerosol Effects

Abstract. The interactions between aerosols and convective clouds represent some of the greatest uncertainties in the climate impact of aerosols in the atmosphere. A wide variety of mechanisms have been proposed by which aerosols may invigorate, suppress, or change the properties of individual convective clouds, some of which can be reproduced in high-resolution limited-area models. However, there may also be mesoscale, regional or global adjustments which modulate or dampen such impacts which cannot be captured in the limited domain of such models. The Convective Cloud Field Model (CCFM) provides a mechanism to explicitly simulate a population of convective clouds within each grid column at resolutions used for global climate modelling, so that a representation of the microphysical aerosol response within each parameterised cloud type is possible. Using CCFM within the global aerosol–climate model ECHAM–HAM, we demonstrate how the parameterised cloud field responds to the present-day anthropogenic aerosol perturbation in different regions. In particular, we show that in regions with strongly-forced deep convection and/or significant aerosol effects via large-scale processes, the changes in the convective cloud field due to microphysical effects is rather small; however in a more weakly-forced regime such as the Caribbean, where large-scale aerosol effects are small, a signature of convective invigoration does become apparent.

scholarly journals Global response of parameterised convective cloud fields to anthropogenic aerosol forcing

2020 ◽  
Vol 20 (7) ◽  
pp. 4445-4460
Author(s):  
Zak Kipling ◽  
Laurent Labbouz ◽  
Philip Stier
Keyword(s):  
Large Scale ◽  
Climate Model ◽  
Global Climate ◽  
Convective Cloud ◽  
Climate Impact ◽  
Limited Area ◽  
Climate Modelling ◽  
Anthropogenic Aerosol ◽  
Convective Clouds ◽  
Aerosol Effects

Abstract. The interactions between aerosols and convective clouds represent some of the greatest uncertainties in the climate impact of aerosols in the atmosphere. A wide variety of mechanisms have been proposed by which aerosols may invigorate, suppress or change the properties of individual convective clouds, some of which can be reproduced in high-resolution limited-area models. However, there may also be mesoscale, regional or global adjustments which modulate or dampen such impacts which cannot be captured in the limited domain of such models. The Convective Cloud Field Model (CCFM) provides a mechanism to simulate a population of convective clouds, complete with microphysics and interactions between clouds, within each grid column at resolutions used for global climate modelling, so that a representation of the microphysical aerosol response within each parameterised cloud type is possible. Using CCFM within the global aerosol–climate model ECHAM–HAM, we demonstrate how the parameterised cloud field responds to the present-day anthropogenic aerosol perturbation in different regions. In particular, we show that in regions with strongly forced deep convection and/or significant aerosol effects via large-scale processes, the changes in the convective cloud field due to microphysical effects are rather small; however in a more weakly forced regime such as the Caribbean, where large-scale aerosol effects are small, a signature of convective invigoration does become apparent.

scholarly journals Organic aerosol and global climate modelling: a review

2005 ◽  
Vol 5 (4) ◽  
pp. 1053-1123 ◽  
Author(s):  
M. Kanakidou ◽  
J. H. Seinfeld ◽  
S. N. Pandis ◽  
I. Barnes ◽  
F. J. Dentener ◽  
...  
Keyword(s):  
Climate Model ◽  
Global Climate ◽  
Global Climate Model ◽  
Organic Aerosol ◽  
Climate Impact ◽  
Climate Modelling ◽  
Carbonaceous Particles ◽  
Global Climate Modelling ◽  
Removal Processes ◽  
Wet Removal

Abstract. The present paper reviews existing knowledge with regard to Organic Aerosol (OA) of importance for global climate modelling and defines critical gaps needed to reduce the involved uncertainties. All pieces required for the representation of OA in a global climate model are sketched out with special attention to Secondary Organic Aerosol (SOA): The emission estimates of primary carbonaceous particles and SOA precursor gases are summarized. The up-to-date understanding of the chemical formation and transformation of condensable organic material is outlined. Knowledge on the hygroscopicity of OA and measurements of optical properties of the organic aerosol constituents are summarized. The mechanisms of interactions of OA with clouds and dry and wet removal processes parameterisations in global models are outlined. This information is synthesized to provide a continuous analysis of the flow from the emitted material to the atmosphere up to the point of the climate impact of the produced organic aerosol. The sources of uncertainties at each step of this process are highlighted as areas that require further studies.

scholarly journals How Well Can We Represent the Spectrum of Convective Clouds in a Climate Model? Comparisons between Internal Parameterization Variables and Radar Observations

2018 ◽  
Vol 75 (5) ◽  
pp. 1509-1524 ◽  
Author(s):  
Laurent Labbouz ◽  
Zak Kipling ◽  
Philip Stier ◽  
Alain Protat
Keyword(s):  
Large Scale ◽  
Climate Models ◽  
Climate Model ◽  
Aerodynamic Drag ◽  
Model Development ◽  
Convective Cloud ◽  
Height Distribution ◽  
Radar Observations ◽  
Convective Parameterization ◽  
Convective Clouds

Current climate models cannot resolve individual convective clouds, and hence parameterizations are needed. The primary goal of convective parameterization is to represent the bulk impact of convection on the gridbox-scale variables. Spectral convective parameterizations also aim to represent the key features of the subgrid-scale convective cloud field such as cloud-top-height distribution and in-cloud vertical velocities in addition to precipitation rates. Ground-based radar retrievals of these quantities have been made available at Darwin, Australia, permitting direct comparisons of internal parameterization variables and providing new observational references for further model development. A spectral convective parameterization [the convective cloud field model (CCFM)] is discussed, and its internal equation of motion is improved. Results from the ECHAM–HAM model in single-column mode using the CCFM and the bulk mass flux Tiedtke–Nordeng scheme are compared with the radar retrievals at Darwin. The CCFM is found to outperform the Tiedtke–Nordeng scheme for cloud-top-height and precipitation-rate distributions. Radar observations are further used to propose a modified CCFM configuration with an aerodynamic drag and reduced entrainment parameter, further improving both the convective cloud-top-height distribution (important for large-scale impact of convection) and the in-cloud vertical velocities (important for aerosol activation). This study provides a new development in the CCFM, improving the representation of convective cloud spectrum characteristics observed in Darwin. This is a step toward an improved representation of convection and ultimately of aerosol effects on convection. It also shows how long-term radar observations of convective cloud properties can help constrain parameters of convective parameterization schemes.

scholarly journals Process-oriented analysis of aircraft soot-cirrus interactions constrains the climate impact of aviation

2021 ◽  
Vol 2 (1) ◽  
Author(s):  
Bernd Kärcher ◽  
Fabian Mahrt ◽  
Claudia Marcolli
Keyword(s):  
Radiative Forcing ◽  
Large Scale ◽  
Climate Models ◽  
Climate Model ◽  
Global Climate ◽  
Climate Impact ◽  
Global Climate Models ◽  
Soot Particles ◽  
Cloud Ice ◽  
The Impact

AbstractFully accounting for the climate impact of aviation requires a process-level understanding of the impact of aircraft soot particle emissions on the formation of ice clouds. Assessing this impact with the help of global climate models remains elusive and direct observations are lacking. Here we use a high-resolution cirrus column model to investigate how aircraft-emitted soot particles, released after ice crystals sublimate at the end of the lifetime of contrails and contrail cirrus, perturb the formation of cirrus. By allying cloud simulations with a measurement-based description of soot-induced ice formation, we find that only a small fraction (<1%) of the soot particles succeeds in forming cloud ice alongside homogeneous freezing of liquid aerosol droplets. Thus, soot-perturbed and homogeneously-formed cirrus fundamentally do not differ in optical depth. Our results imply that climate model estimates of global radiative forcing from interactions between aircraft soot and large-scale cirrus may be overestimates. The improved scientific understanding reported here provides a process-based underpinning for improved climate model parametrizations and targeted field observations.

scholarly journals Global anthropogenic aerosol effects on convective clouds in ECHAM5-HAM

2008 ◽  
Vol 8 (7) ◽  
pp. 2115-2131 ◽  
Author(s):  
U. Lohmann
Keyword(s):  
General Circulation ◽  
Large Scale ◽  
Hydrological Cycle ◽  
Circulation Model ◽  
Cloud Microphysics ◽  
Convective Precipitation ◽  
Anthropogenic Aerosol ◽  
Convective Clouds ◽  
Double Moment ◽  
Aerosol Effects

Abstract. Aerosols affect the climate system by changing cloud characteristics in many ways. They act as cloud condensation and ice nuclei and may have an influence on the hydrological cycle. Here we investigate aerosol effects on convective clouds by extending the double-moment cloud microphysics scheme developed for stratiform clouds, which is coupled to the HAM double-moment aerosol scheme, to convective clouds in the ECHAM5 general circulation model. This enables us to investigate whether more, and smaller cloud droplets suppress the warm rain formation in the lower parts of convective clouds and thus release more latent heat upon freezing, which would then result in more vigorous convection and more precipitation. In ECHAM5, including aerosol effects in large-scale and convective clouds (simulation ECHAM5-conv) reduces the sensitivity of the liquid water path increase with increasing aerosol optical depth in better agreement with observations and large-eddy simulation studies. In simulation ECHAM5-conv with increases in greenhouse gas and aerosol emissions since pre-industrial times, the geographical distribution of the changes in precipitation better matches the observed increase in precipitation than neglecting microphysics in convective clouds. In this simulation the convective precipitation increases the most suggesting that the convection has indeed become more vigorous.

scholarly journals Organic aerosol and global climate modelling: a review

2004 ◽  
Vol 4 (5) ◽  
pp. 5855-6024 ◽  
Author(s):  
M. Kanakidou ◽  
J. H. Seinfeld ◽  
S. N. Pandis ◽  
I. Barnes ◽  
F. J. Dentener ◽  
...  
Keyword(s):  
Climate Model ◽  
Global Climate ◽  
Global Climate Model ◽  
Organic Aerosol ◽  
Climate Impact ◽  
Climate Modelling ◽  
Carbonaceous Particles ◽  
Global Climate Modelling ◽  
Removal Processes ◽  
Wet Removal

Abstract. The present paper reviews existing knowledge with regard to Organic Aerosol (OA) of importance for global climate modelling and defines critical gaps needed to reduce the involved uncertainties. All pieces required for the representation of OA in a global climate model are sketched out with special attention to Secondary Organic Aerosol (SOA): The emission estimates of primary carbonaceous particles and SOA precursor gases are summarized. The up-to-date understanding of the chemical formation and transformation of condensable organic material is outlined. Knowledge on the hygroscopicity of OA and measurements of optical properties of the organic aerosol constituents are summarized. The mechanisms of interactions of OA with clouds and dry and wet removal processes parameterisations in global models are outlined. This information is synthesized to provide a continuous analysis of the flow from the emitted material to the atmosphere up to the point of the climate impact of the produced organic aerosol. The sources of uncertainties at each step of this process are highlighted as areas that require further studies.

scholarly journals Aerosol indirect effects in a multi-scale aerosol-climate model PNNL-MMF

2011 ◽  
Vol 11 (1) ◽  
pp. 3399-3459 ◽  
Author(s):  
M. Wang ◽  
S. Ghan ◽  
M. Ovchinnikov ◽  
X. Liu ◽  
R. Easter ◽  
...  
Keyword(s):  
Indirect Effects ◽  
Large Scale ◽  
Climate Models ◽  
Climate Model ◽  
Global Climate ◽  
Global Climate Models ◽  
Anthropogenic Aerosols ◽  
Anthropogenic Aerosol ◽  
Aerosol Indirect Effects ◽  
Multi Scale

Abstract. Much of the large uncertainty in estimates of anthropogenic aerosol effects on climate arises from the multi-scale nature of the interactions between aerosols, clouds and large-scale dynamics, which are difficult to represent in conventional global climate models (GCMs). In this study, we use a multi-scale aerosol-climate model that treats aerosols and clouds across multiple scales to study aerosol indirect effects. This multi-scale aerosol-climate model is an extension of a multi-scale modeling framework (MMF) model that embeds a cloud-resolving model (CRM) within each grid cell of a GCM. The extension allows the explicit simulation of aerosol/cloud interactions in both stratiform and convective clouds on the global scale in a computationally feasible way. Simulated model fields, including liquid water path (LWP), ice water path, cloud fraction, shortwave and longwave cloud forcing, precipitation, water vapor, and cloud droplet number concentration are in agreement with observations. The new model performs quantitatively similar to the previous version of the MMF model in terms of simulated cloud fraction and precipitation. The simulated change in shortwave cloud forcing from anthropogenic aerosols is −0.77 W m−2, which is less than half of that in the host GCM (NCAR CAM5) (−1.79 W m−2) and is also at the low end of the estimates of most other conventional global aerosol-climate models. The smaller forcing in the MMF model is attributed to its smaller increase in LWP from preindustrial conditions (PI) to present day (PD): 3.9% in the MMF, compared with 15.6% increase in LWP in large-scale clouds in CAM5. The much smaller increase in LWP in the MMF is caused by a much smaller response in LWP to a given perturbation in cloud condensation nuclei (CCN) concentrations from PI to PD in the MMF (about one-third of that in CAM5), and, to a lesser extent, by a smaller relative increase in CCN concentrations from PI to PD in the MMF (about 26% smaller than that in CAM5). The smaller relative increase in CCN concentrations in the MMF is caused in part by a smaller increase in aerosol lifetime from PI to PD in the MMF, a positive feedback in aerosol indirect effects induced by cloud lifetime effects. The smaller response in LWP to anthropogenic aerosols in the MMF model is consistent with observations and with high resolution model studies, which may indicate that aerosol indirect effects simulated in conventional global climate models are overestimated and point to the need to use global high resolution models, such as MMF models or global CRMs, to study aerosol indirect effects. The simulated total anthropogenic aerosol effect in the MMF is −1.05 W m−2, which is close to the Murphy et al. (2009) inverse estimate of −1.1 ± 0.4 W m−2 (1σ) based on the examination of the Earth's energy balance. Further improvements in the representation of ice nucleation and low clouds are needed.

scholarly journals Aerosol effects on clouds and precipitation during the 1997 smoke episode in Indonesia

2009 ◽  
Vol 9 (2) ◽  
pp. 743-756 ◽  
Author(s):  
H.-F. Graf ◽  
J. Yang ◽  
T. M. Wagner
Keyword(s):  
Large Scale ◽  
Convective Cloud ◽  
Reanalysis Data ◽  
Cumulus Parameterization ◽  
Convective Precipitation ◽  
Limited Area ◽  
Convective Rainfall ◽  
High Background ◽  
Convective Clouds ◽  
The Mean

Abstract. In 1997/1998 a severe smoke episode due to extensive biomass burning, especially of peat, was observed over Indonesia. September 1997 was the month with the highest aerosol burden. This month was simulated using the limited area model REMOTE driven at its lateral boundaries by ERA40 reanalysis data. REMOTE was extended by a new convective cloud parameterization mimicking individual clouds competing for instability energy. This allows for the interaction of aerosols, convective clouds and precipitation. Results show that in the monthly mean convective precipitation is diminished at nearly all places with high aerosol loading, but at some areas with high background humidity precipitation from large-scale clouds may over-compensate the loss in convective rainfall. The simulations revealed that both large-scale and convective clouds' microphysics are influenced by aerosols. Since aerosols are washed and rained out by rainfall, high aerosol concentrations can only persist at low rainfall rates. Hence, aerosol concentrations are not independent of the rainfall amount and in the mean the maximum absolute effects on rainfall from large scale clouds are found at intermediate aerosol concentrations. The reason for this behavior is that at high aerosol concentrations rainfall rates are small and consequently also the anomalies are small. For large-scale as well as for convective rain negative and positive anomalies are found for all aerosol concentrations. Negative anomalies dominate and are highly statistically significant especially for convective rainfall since part of the precipitation loss from large-scale clouds is compensated by moisture detrained from the convective clouds. The mean precipitation from large-scale clouds is less reduced (however still statistically significant) than rain from convective clouds. This effect is due to detrainment of cloud water from the less strongly raining convective clouds and because of the generally lower absolute amounts of rainfall from large-scale clouds. With increasing aerosol load both, convective and large scale clouds produce less rain. At very few individual time steps cases were found when polluted convective clouds produced intensified rainfall via mixed phase microphysics. However, these cases are not unequivocal and opposite results were also simulated, indicating that other than aerosol-microphysics effects have important impact on the results. Overall, the introduction of the new cumulus parameterization and aerosol-cloud interaction reduced some of the original REMOTE biases of precipitation patterns and total amount.

scholarly journals Aerosol effects on clouds and precipitation during the 1997 smoke episode in Indonesia

2007 ◽  
Vol 7 (6) ◽  
pp. 17099-17116 ◽  
Author(s):  
H.-F. Graf ◽  
J. Yang ◽  
T. M. Wagner
Keyword(s):  
Large Scale ◽  
Convective Cloud ◽  
Reanalysis Data ◽  
Cumulus Parameterization ◽  
Convective Precipitation ◽  
Limited Area ◽  
High Background ◽  
Convective Clouds ◽  
Era40 Reanalysis ◽  
Instability Energy

Abstract. In 1997/98 a severe smoke episode due to extensive biomass burning, especially of peat, was observed over Indonesia. September 1997 was the month with the highest aerosol burden. This month was simulated using the limited area model REMOTE driven at its lateral boundaries by ERA40 reanalysis data. REMOTE was extended by a new convective cloud parameterization mimicking individual clouds competing for instability energy. This allows for the interaction of aerosols and convective clouds and precipitation. Results show that convective precipitation is diminished at all places with high aerosol loading, but at some areas with high background humidity precipitation from large-scale clouds may over-compensate the loss in convective rainfall. At individual time steps, very few cases were found when polluted convective clouds produced intensified rainfall via mixed phase microphysics. However, these cases are not unequivocal and opposite results were also simulated, indicating that other than aerosol-microphysics effects have important impact on the results. Overall, the introduction of the new cumulus parameterization and of aerosol-cloud interaction improved the simulation of precipitation patterns and total amount.

scholarly journals The nature of ice-nucleating particles affects the radiative properties of tropical convective cloud systems

2020 ◽  
Author(s):  
Rachel E. Hawker ◽  
Annette K. Miltenberger ◽  
Jonathan M. Wilkinson ◽  
Adrian A. Hill ◽  
Ben J. Shipway ◽  
...  
Keyword(s):  
Temperature Dependence ◽  
Climate Model ◽  
Global Climate ◽  
Critical Role ◽  
Convective Cloud ◽  
Radiative Properties ◽  
Ice Formation ◽  
Climate Modelling ◽  
Microphysics Scheme ◽  
Cloud Systems

Abstract. Convective cloud systems in the maritime tropics play a critical role in global climate, but accurately representing aerosol interactions within these clouds persists as a major challenge for weather and climate modelling. We quantify the effect of ice-nucleating particles (INP) on the radiative properties of a complex Tropical Atlantic deep convective cloud field using a regional model with an advanced double-moment microphysics scheme. Our results show that the domain-mean daylight outgoing radiation varies by up to 18 W m−2 depending on the bio- and physico-chemical properties of INP. The key distinction between different INPs is the temperature dependence of ice formation, which alters the vertical distribution of cloud microphysical processes. The controlling effect of the INP temperature dependence is substantial even in the presence of secondary ice production, and the effects of secondary ice formation depend strongly on the nature of the INP. Our results have implications for climate model simulations of tropical clouds and radiation, which currently do not consider a link between INP particle type and ice water content. The results also provide a challenge to the INP measurement community, since we demonstrate that INP concentration measurements are required over the full mixed-phase temperature regime, which covers around 10 orders of magnitude in INP concentration.

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