scholarly journals Age Spectra and Other Transport Diagnostics in the North American Monsoon UTLS from SEAC<sup>4</sup>RS In Situ Trace Gas Measurements

2021 ◽  
Author(s):  
Eric A. Ray ◽  
Elliot L. Atlas ◽  
Sue Schauffler ◽  
Sofia Chelpon ◽  
Laura Pan ◽  
...  

Abstract. The upper troposphere and lower stratosphere (UTLS) during the summer monsoon season over North America (NAM) is influenced by the transport of air from a variety of source regions over a wide range of time scales (hours to years). Age spectra are useful for characterizing the transport into such a region and in this study we use and build on recently developed techniques to infer age spectra from trace gas measurements with photochemical lifetimes from days to centuries. We show that the measurements taken by the Whole Air Sampler instrument during the SEAC4RS campaign can be used to not only derive age spectra, but also path-integrated lifetimes of each of the trace gases and surface source regions. The method used here can also clearly identify and adjust for measurement outliers that were influenced by polluted surface source regions. The results are generally consistent with expected transport features of the NAM but also provide a range of transport diagnostics that have not previously been computed solely from in situ measurements. These methods may be applied to many other existing in situ datasets and the transport diagnostics can be compared with chemistry-climate model transport in the UTLS.

2013 ◽  
Vol 26 (17) ◽  
pp. 6257-6286 ◽  
Author(s):  
Leila M. V. Carvalho ◽  
Charles Jones

Abstract Global warming has been linked to systematic changes in North and South America's climates and may severely impact the North American monsoon system (NAMS) and South American monsoon system (SAMS). This study examines interannual-to-decadal variations and changes in the low-troposphere (850 hPa) temperature (T850) and specific humidity (Q850) and relationships with daily precipitation over the tropical Americas using the NCEP–NCAR reanalysis, the Climate Forecast System Reanalysis (CFSR), and phase 5 of the Coupled Model Intercomparison Project (CMIP5) simulations for two scenarios: “historic” and high-emission representative concentration pathway 8.5 (RCP8.5). Trends in the magnitude and area of the 85th percentiles were distinctly examined over North America (NA) and South America (SA) during the peak of the respective monsoon season. The historic simulations (1951–2005) and the two reanalyses agree well and indicate that significant warming has occurred over tropical SA with a remarkable increase in the area and magnitude of the 85th percentile in the last decade (1996–2005). The RCP8.5 CMIP5 ensemble mean projects an increase in the T850 85th percentile of about 2.5°C (2.8°C) by 2050 and 4.8°C (5.5°C) over SA (NA) by 2095 relative to 1955. The area of SA (NA) with T850 ≥ the 85th percentile is projected to increase from ~10% (15%) in 1955 to ~58% (~33%) by 2050 and ~80% (~50%) by 2095. The respective increase in the 85th percentile of Q850 is about 3 g kg−1 over SAMS and NAMS by 2095. CMIP5 models project variable changes in daily precipitation over the tropical Americas. The most consistent is increased rainfall in the intertropical convergence zone in December–February (DJF) and June–August (JJA) and decreased precipitation over NAMS in JJA.


2005 ◽  
Vol 5 (4) ◽  
pp. 1125-1156 ◽  
Author(s):  
P. Stier ◽  
J. Feichter ◽  
S. Kinne ◽  
S. Kloster ◽  
E. Vignati ◽  
...  

Abstract. The aerosol-climate modelling system ECHAM5-HAM is introduced. It is based on a flexible microphysical approach and, as the number of externally imposed parameters is minimised, allows the application in a wide range of climate regimes. ECHAM5-HAM predicts the evolution of an ensemble of microphysically interacting internally- and externally-mixed aerosol populations as well as their size-distribution and composition. The size-distribution is represented by a superposition of log-normal modes. In the current setup, the major global aerosol compounds sulfate (SU), black carbon (BC), particulate organic matter (POM), sea salt (SS), and mineral dust (DU) are included. The simulated global annual mean aerosol burdens (lifetimes) for the year 2000 are for SU: 0.80 Tg(S) (3.9 days), for BC: 0.11 Tg (5.4 days), for POM: 0.99 Tg (5.4 days), for SS: 10.5 Tg (0.8 days), and for DU: 8.28 Tg (4.6 days). An extensive evaluation with in-situ and remote sensing measurements underscores that the model results are generally in good agreement with observations of the global aerosol system. The simulated global annual mean aerosol optical depth (AOD) is with 0.14 in excellent agreement with an estimate derived from AERONET measurements (0.14) and a composite derived from MODIS-MISR satellite retrievals (0.16). Regionally, the deviations are not negligible. However, the main patterns of AOD attributable to anthropogenic activity are reproduced.


2015 ◽  
Vol 15 (17) ◽  
pp. 10087-10092 ◽  
Author(s):  
L. Kattner ◽  
B. Mathieu-Üffing ◽  
J. P. Burrows ◽  
A. Richter ◽  
S. Schmolke ◽  
...  

Abstract. In 1997 the International Maritime Organisation (IMO) adopted MARPOL Annex VI to prevent air pollution by shipping emissions. It regulates, among other issues, the sulfur content in shipping fuels, which is transformed into the air pollutant sulfur dioxide (SO2) during combustion. Within designated Sulfur Emission Control Areas (SECA), the sulfur content was limited to 1 %, and on 1 January 2015, this limit was further reduced to 0.1 %. Here we present the set-up and measurement results of a permanent ship emission monitoring site near Hamburg harbour in the North Sea SECA. Trace gas measurements are conducted with in situ instruments and a data set from September 2014 to January 2015 is presented. By combining measurements of carbon dioxide (CO2) and SO2 with ship position data, it is possible to deduce the sulfur fuel content of individual ships passing the measurement station, thus facilitating the monitoring of compliance of ships with the IMO regulations. While compliance is almost 100 % for the 2014 data, it decreases only very little in 2015 to 95.4 % despite the much stricter limit. We analysed more than 1400 ship plumes in total and for months with favourable conditions, up to 40 % of all ships entering and leaving Hamburg harbour could be checked for their sulfur fuel content.


2015 ◽  
Vol 15 (12) ◽  
pp. 6943-6958 ◽  
Author(s):  
E. Crosbie ◽  
J.-S. Youn ◽  
B. Balch ◽  
A. Wonaschütz ◽  
T. Shingler ◽  
...  

Abstract. A 2-year data set of measured CCN (cloud condensation nuclei) concentrations at 0.2 % supersaturation is combined with aerosol size distribution and aerosol composition data to probe the effects of aerosol number concentrations, size distribution and composition on CCN patterns. Data were collected over a period of 2 years (2012–2014) in central Tucson, Arizona: a significant urban area surrounded by a sparsely populated desert. Average CCN concentrations are typically lowest in spring (233 cm−3), highest in winter (430 cm−3) and have a secondary peak during the North American monsoon season (July to September; 372 cm−3). There is significant variability outside of seasonal patterns, with extreme concentrations (1 and 99 % levels) ranging from 56 to 1945 cm−3 as measured during the winter, the season with highest variability. Modeled CCN concentrations based on fixed chemical composition achieve better closure in winter, with size and number alone able to predict 82 % of the variance in CCN concentration. Changes in aerosol chemical composition are typically aligned with changes in size and aerosol number, such that hygroscopicity can be parameterized even though it is still variable. In summer, models based on fixed chemical composition explain at best only 41 % (pre-monsoon) and 36 % (monsoon) of the variance. This is attributed to the effects of secondary organic aerosol (SOA) production, the competition between new particle formation and condensational growth, the complex interaction of meteorology, regional and local emissions and multi-phase chemistry during the North American monsoon. Chemical composition is found to be an important factor for improving predictability in spring and on longer timescales in winter. Parameterized models typically exhibit improved predictive skill when there are strong relationships between CCN concentrations and the prevailing meteorology and dominant aerosol physicochemical processes, suggesting that similar findings could be possible in other locations with comparable climates and geography.


2006 ◽  
Vol 134 (12) ◽  
pp. 3774-3781 ◽  
Author(s):  
Anne W. Nolin ◽  
Eileen A. Hall-McKim

Abstract The interannual and intraseasonal variability of the North American monsoon is of great interest because a large proportion of the annual precipitation for Arizona and New Mexico arrives during the summer monsoon. Forty-one years of daily monsoon season precipitation data for Arizona and New Mexico were studied using wavelet analysis. This time-localized spectral analysis method reveals that periodicities of less than 8 days are positively correlated with mean daily precipitation during the 1 July–15 September monsoon period. Roughly 17% of the years indicate no significant periodicity during the monsoon period for either region and are associated with low monsoon precipitation. High- and low-frequency modes explain an equivalent percentage of the variance in monsoon precipitation in both Arizona and New Mexico, and in many years concurrent multiple periodicities occur. Wavelet analysis was effective in identifying the contribution of high-frequency modes that had not been discerned in previous studies. These results suggest that precipitation processes during the monsoon season are modulated by phenomena operating at synoptic (2–8 days) and longer (&gt;8 days) time scales and point to the need for further studies to better understand the associated atmospheric processes.


2015 ◽  
Vol 28 (17) ◽  
pp. 6707-6728 ◽  
Author(s):  
Melissa S. Bukovsky ◽  
Carlos M. Carrillo ◽  
David J. Gochis ◽  
Dorit M. Hammerling ◽  
Rachel R. McCrary ◽  
...  

Abstract This study presents climate change results from the North American Regional Climate Change Assessment Program (NARCCAP) suite of dynamically downscaled simulations for the North American monsoon system in the southwestern United States and northwestern Mexico. The focus is on changes in precipitation and the processes driving the projected changes from the regional climate simulations and their driving coupled atmosphere–ocean global climate models. The effect of known biases on the projections is also examined. Overall, there is strong ensemble agreement for a large decrease in precipitation during the monsoon season; however, this agreement and the magnitude of the ensemble-mean change is likely deceiving, as the greatest decreases are produced by the simulations that are the most biased in the baseline/current climate. Furthermore, some of the greatest decreases in precipitation are being driven by changes in processes/phenomena that are less credible (e.g., changes in El Niño–Southern Oscillation, when it is initially not simulated well). In other simulations, the processes driving the precipitation change may be plausible, but other biases (e.g., biases in low-level moisture or precipitation intensity) appear to be affecting the magnitude of the projected changes. The most and least credible simulations are clearly identified, while the other simulations are mixed in their abilities to produce projections of value.


1991 ◽  
Vol 57 (2) ◽  
pp. 103-157 ◽  
Author(s):  
Richard S. Thorpe ◽  
Olwen Williams-Thorpe ◽  
D. Graham Jenkins ◽  
J. S. Watson ◽  
R. A. Ixer ◽  
...  

Stonehenge on Salisbury Plain is one of the most impressive British prehistoric(c.3000–1500 BC) monuments. It is dominated by large upright sarsen stones, some of which are joined by lintels. While these stones are of relatively local derivation, some of the stone settings, termed bluestones, are composed of igneous and minor sedimentary rocks which are foreign to the solid geology of Salisbury Plain and must have been transported to their present location. Following the proposal of an origin in south-west Wales, debate has focused on hypotheses of natural transport by glacial processes, or transport by human agency. This paper reports the results of a programme of sampling and chemical analysis of Stonehenge bluestones and proposed source outcrops in Wales.Analysis by X-ray-fluorescence of fifteen monolith samples and twenty-two excavated fragments from Stonehenge indicate that the dolerites originated at three sources in a small area in the eastern Preseli Hills, and that the rhyolite monoliths derive from four sources including northern Preseli and other (unidentified) locations in Pembrokeshire, perhaps on the north Pembrokeshire coast. Rhyolite fragments derive from four outcrops (including only one of the monolith sources) over a distance of at least 10 km within Preseli. The Altar Stone and a sandstone fragment (excavated at Stonehenge) are from two sources within the Palaeozoic of south-west Wales. This variety of source suggests that the monoliths were taken from a glacially-mixed deposit, not carefully selected from anin situsource. We then consider whether prehistoric man collected the bluestones from such a deposit in south Wales or whether glacial action could have transported bluestone boulders onto Salisbury Plain. Glacial erratics deposited in south Dyfed (dolerites chemically identical to Stonehenge dolerite monoliths), near Cardiff, on Flatholm and near Bristol indicate glacial action at least as far as the Avon area. There is an apparent absence of erratics east of here, with the possible exception of the Boles Barrow boulder, which may predate the Stonehenge bluestones by as much as 1000 years, and which derived from the same Preseli source as two of the Stonehenge monoliths. However, 18th-century geological accounts describe intensive agricultural clearance of glacial boulders, including igneous rocks, on Salisbury Plain, and contemporary practice was of burial of such boulders in pits. Such erratics could have been transported as ‘free boulders’ from ‘nunataks’ on the top of an extensive, perhaps Anglian or earlier, glacier some 400,000 years ago or more, leaving no trace of fine glacial material in present river gravels. Erratics may be deposited at the margins of ice-sheets in small groups at irregular intervals and with gaps of several kilometres between individual boulders.‘Bluestone’ fragments are frequently reported on and near Salisbury Plain in archaeological literature, and include a wide range of rock types from monuments of widely differing types and dates, and pieces not directly associated with archaeological structures. Examination of prehistoric stone monuments in south Wales shows no preference for bluestones in this area. The monoliths at Stonehenge include some structurally poor rock types, now completely eroded above ground. We conclude that the builders of the bluestone structures at Stonehenge utilized a heterogeneous deposit of glacial boulders readily available on Salisbury Plain. Remaining erratics are now seen as small fragments sometimes incorporated in a variety of archaeological sites, while others were destroyed and removed in the 18th century. The bluestones were transported to Salisbury Plain from varied sources in south Wales by a glacier rather than human activity.


2004 ◽  
Vol 4 (5) ◽  
pp. 1427-1442 ◽  
Author(s):  
P. Hoor ◽  
C. Gurk ◽  
D. Brunner ◽  
M. I. Hegglin ◽  
H. Wernli ◽  
...  

Abstract. We present airborne in-situ trace gas measurements which were performed on eight campaigns between November 2001 and July 2003 during the SPURT-project (SPURenstofftransport in der Tropopausenregion, trace gas transport in the tropopause region). The measurements on a quasi regular basis allowed an overview of the seasonal variations of the trace gas distribution in the tropopause region over Europe from 35°-75°N to investigate the influence of transport and mixing across the extratropical tropopause on the lowermost stratosphere. From the correlation of CO and O3 irreversible mixing of tropospheric air into the lowermost stratosphere is identified. The CO distribution indicates that transport and subsequent mixing of tropospheric air across the extratropical tropopause predominantly affects a layer, which closely follows the shape of the local tropopause. In addition, the seasonal cycle of CO2 illustrates the strong coupling of that layer to the extratropical troposphere. Both, horizontal gradients of CO on isentropes as well as the CO-O3-distribution in the lowermost stratosphere reveal that the influence of quasi-horizontal transport and subsequent mixing weakens with distance from the local tropopause. The mixing layer extends to about 25 K in potential temperature above the local tropopause exhibiting only a weak seasonality. However, at large distances from the tropopause a significant influence of tropospheric air is still evident. The relation between N2O and CO2 indicates that a significant contribution of air originating from the tropical tropopause contributes to the background air in the extratropical lowermost stratosphere.


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