scholarly journals A case of extreme particulate matter concentrations over Central Europe caused by dust emitted over the southern Ukraine

2008 ◽  
Vol 8 (4) ◽  
pp. 997-1016 ◽  
Author(s):  
W. Birmili ◽  
K. Schepanski ◽  
A. Ansmann ◽  
G. Spindler ◽  
I. Tegen ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Particulate Matter ◽  
Central Europe ◽  
Large Scale ◽  
Dust Emission ◽  
Wavelength Dependence ◽  
Light Extinction ◽  
Crustal Material ◽  
Southern Ukraine

Abstract. On 24 March 2007, an extraordinary dust plume was observed in the Central European troposphere. Satellite observations revealed its origins in a dust storm in Southern Ukraine, where large amounts of soil were resuspended from dried-out farmlands at wind gusts up to 30 m s−1. Along the pathway of the plume, maximum particulate matter (PM10) mass concentrations between 200 and 1400 μg m−3 occurred in Slovakia, the Czech Republic, Poland, and Germany. Over Germany, the dust plume was characterised by a volume extinction coefficient up to 400 Mm−1 and a particle optical depth of 0.71 at wavelength 0.532 μm. In-situ size distribution measurements as well as the wavelength dependence of light extinction from lidar and Sun photometer measurements confirmed the presence of a coarse particle mode with diameters around 2–3 μm. Chemical particle analyses suggested a fraction of 75% crustal material in daily average PM10 and up to 85% in the coarser fraction PM10–2.5. Based on the particle characteristics as well as a lack of increased CO and CO2 levels, a significant impact of biomass burning was ruled out. The reasons for the high particle concentrations in the dust plume were twofold: First, dust was transported very rapidly into Central Europe in a boundary layer jet under dry conditions. Second, the dust plume was confined to a relatively stable boundary layer of 1.4–1.8 km height, and could therefore neither expand nor dilute efficiently. Our findings illustrate the capacity of combined in situ and remote sensing measurements to characterise large-scale dust plumes with a variety of aerosol parameters. Although such plumes from Southern Eurasia seem to occur rather infrequently in Central Europe, its unexpected features highlights the need to improve the description of dust emission, transport and transformation processes needs, particularly when facing the possible effects of further anthropogenic desertification and climate change.

scholarly journals An episode of extremely high PM concentrations over Central Europe caused by dust emitted over the southern Ukraine

2007 ◽  
Vol 7 (4) ◽  
pp. 12231-12288 ◽  
Author(s):  
W. Birmili ◽  
K. Schepanski ◽  
A. Ansmann ◽  
G. Spindler ◽  
I. Tegen ◽  
...  
Keyword(s):  
Central Europe ◽  
Dust Cloud ◽  
Dust Emission ◽  
Light Extinction ◽  
High Mass ◽  
Particle Analysis ◽  
Back Trajectory ◽  
Southern Ukraine ◽  
Mass Concentrations

Abstract. On 24 March 2007, the atmosphere over Central Europe was affected by an episode of exceptionally high mass concentrations of aerosol particles, most likely caused by a dust storm in the Southern Ukraine on the preceding day. At ground-based measurement stations in Slovakia, the Czech Republic, Poland and Germany PM10 mass concentrations rose to values between 200 and 1400 μg m−3. An evaluation of PM10 measurements from 360 monitoring stations showed that the dust cloud advanced along a narrow corridor at speeds of up to 70 km h−1. According to lidar observations over Leipzig, Germany, the high aerosol concentrations were confined to a homogeneous boundary layer of 1800 m height. The wavelength dependence of light extinction using both lidar and sun photometer measurements suggested the dominance of coarse particles during the main event. At a wavelength of 532 nm, relatively high volume extinction coefficients (300–400 Mm−1) and a particle optical depth of 0.65 was observed. In-situ measurements with an aerodynamic particle sizer at Melpitz, Germany, confirmed the presence of a coarse particle mode with a mode diameter >2 μm, whose maximum concentration coincided with that of PM10. A chemical particle analysis confirmed the dominance of non-volatile and insoluble matter in the coarse mode as well as high enrichments of Ti and Fe, which are characteristic of soil dust. A combination of back trajectory calculations and satellite images allowed to identify the dust source with confidence: On 23 March 2007, large amounts of dust were emitted from dried-out farmlands in the southern Ukraine, facilitated by wind gusts up to 100 km h−1. The unusual vertical stability and confined height of this dust layer as well as the rapid transport under dry conditions led to the conservation of high aerosol mass concentrations along the transect and thus to the extraordinary high aerosol concentrations over Central Europe. Our observations demonstrate the capacity of a combined apparatus of in situ and remote sensing measurements to characterise such a dust with a variety of aerosol parameters. As a conclusion, the description of dust emission, transport and transformation processes needs to be improved, especially when facing the possible effects of further anthropogenic desertification and climate change.

scholarly journals Observed Evolution of Northward-Propagating Intraseasonal Variation over the Western Pacific: A Case Study in Boreal Early Summer

2013 ◽  
Vol 141 (2) ◽  
pp. 690-706 ◽  
Author(s):  
Masaki Katsumata ◽  
Hiroyuki Yamada ◽  
Hisayuki Kubota ◽  
Qoosaku Moteki ◽  
Ryuichi Shirooka
Keyword(s):  
Boundary Layer ◽  
Large Scale ◽  
Lower Troposphere ◽  
Western Pacific ◽  
Boreal Summer ◽  
Intraseasonal Variation ◽  
Middle Troposphere ◽  
Inactive Period ◽  
The Western Pacific

Abstract This report describes the in situ observed evolution of the atmospheric profile during an event of the boreal summer intraseasonal variation (BSISV) in the tropical western Pacific Ocean. The convectively active region of the BSISV proceeded northward over the sounding and radar network. Over the array, the situation changed from a convectively inactive period to an active period. Inspection of the sounding data revealed the gradual moistening of the lower troposphere during the convectively inactive period. The sounding-derived heat and moisture budget analyses indicated that both the convective- and large-scale processes caused moistening of the lower and middle troposphere where the radar echo tops were observed most frequently. This study is the first to identify such a “preconditioning” process for the BSISV in the western Pacific using detailed in situ observational data. During the preconditioning, an increase in CAPE was observed, as in previous studies of the MJO. An increase of moisture in the boundary layer was responsible for the increase of CAPE. The large-scale horizontal convergence in the boundary layer may be a key factor to moisten the boundary layer through the convective-scale processes, as well as through the large-scale processes to moisten the lower and middle troposphere.

Modeling of particulate matter transport in atmospheric boundary layer following dust emission from source areas

2016 ◽  
Vol 20 ◽  
pp. 147-156 ◽  
Author(s):  
Itzhak Katra ◽  
Tov Elperin ◽  
Andrew Fominykh ◽  
Boris Krasovitov ◽  
Hezi Yizhaq
Keyword(s):  
Boundary Layer ◽  
Particulate Matter ◽  
Atmospheric Boundary Layer ◽  
Dust Emission ◽  
Source Areas ◽  
Matter Transport

scholarly journals Measurements of Boundary Layer Profiles with In Situ Sensors and Doppler Lidar

2008 ◽  
Vol 25 (8) ◽  
pp. 1328-1340 ◽  
Author(s):  
Rod Frehlich ◽  
Yannick Meillier ◽  
Michael L. Jensen
Keyword(s):  
Boundary Layer ◽  
Large Scale ◽  
Energy Dissipation Rate ◽  
High Rate ◽  
Doppler Lidar ◽  
Stratified Turbulence ◽  
In Situ Sensors ◽  
The Impact ◽  
Turbulence Parameters

Abstract A new in situ measurement system and lidar processing algorithms were developed for improved measurements of boundary layer profiles. The first comparisons of simultaneous Doppler lidar–derived profiles of the key turbulence statistics of the two orthogonal horizontal velocity components (longitudinal and transverse) are presented. The instrument requirements for accurate observations of stably stratified turbulence were determined. A region of stably stratified low turbulence with constant gradients of temperature and velocity was observed above the nocturnal boundary layer using high-rate sensors. The important turbulence parameters were estimated, and turbulence spectra were consistent with new theoretical descriptions of stratified turbulence. The impact of removing the larger-scale velocity features in Doppler lidar estimates of turbulent velocity variance and length scales was investigated. The Doppler lidar–derived estimates of energy dissipation rate ε were found to be insensitive to spatial filtering of the large-scale atmospheric processes. The in situ and lidar-derived profiles were compared for the stable boundary layer in a suburban environment.

scholarly journals Two case studies on the interaction of large-scale transport, mesoscale photochemistry, and boundary-layer processes on the lower tropospheric ozone dynamics in early spring

2001 ◽  
Vol 19 (4) ◽  
pp. 469-486 ◽  
Author(s):  
S. Brönnimann ◽  
F. C. Siegrist ◽  
W. Eugster ◽  
R. Cattin ◽  
C. Sidle ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Large Scale ◽  
Lower Troposphere ◽  
Early Spring ◽  
Atmospheric Composition ◽  
Late Winter ◽  
Chemical Production ◽  
Ozone Concentrations ◽  
Boundary Layer Ozone

Abstract. The vertical distribution of ozone in the lower troposphere over the Swiss Plateau is investigated in detail for two episodes in early spring (February 1998 and March 1999). Profile measurements of boundary-layer ozone performed during two field campaigns with a tethered balloon sounding system and a kite are investigated using regular aerological and ozone soundings from a nearby site, measurements from monitoring stations at various altitudes, backward trajectories, and synoptic analyses of meteorological fields. Additionally, the effect of in situ photochemistry was estimated for one of the episodes employing the Metphomod Eulerian photochemical model. Although the meteorological situations were completely different, both cases had elevated layers with high ozone concentrations, which is not untypical for late winter and early spring. In the February episode, the highest ozone concentrations of 55 to 60 ppb, which were found at around 1100 m asl, were partly advected from Southern France, but a considerable contribution of in situ photochemistry is also predicted by the model. Below that elevation, the local chemical sinks and surface deposition probably overcompensated chemical production, and the vertical ozone distribution was governed by boundary-layer dynamics. In the March episode, the results suggest that ozone-rich air parcels, probably of stratospheric or upper tropospheric origin, were advected aloft the boundary layer on the Swiss Plateau.Key words. Atmospheric composition and structure (pollution – urban and regional; troposphere – composition and  chemistry) – Meteorology and atmospheric dynamics (mesoscale meteorology)

scholarly journals Observationally constrained analysis of sea salt aerosol in the marine atmosphere

2019 ◽  
Vol 19 (16) ◽  
pp. 10773-10785 ◽  
Author(s):  
Huisheng Bian ◽  
Karl Froyd ◽  
Daniel M. Murphy ◽  
Jack Dibb ◽  
Anton Darmenov ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Marine Boundary Layer ◽  
In Situ Measurements ◽  
Sea Salt ◽  
Light Extinction ◽  
Boreal Summer ◽  
Integrated Analysis ◽  
Marine Atmosphere ◽  
Model Simulations

Abstract. Atmospheric sea salt plays important roles in marine cloud formation and atmospheric chemistry. We performed an integrated analysis of NASA GEOS model simulations run with the GOCART aerosol module, in situ measurements from the PALMS and SAGA instruments obtained during the NASA ATom campaign, and aerosol optical depth (AOD) measurements from the AERONET Marine Aerosol Network (MAN) and from MODIS satellite observations to better constrain sea salt in the marine atmosphere. ATom measurements and GEOS model simulations both show that sea salt concentrations over the Pacific and Atlantic oceans have a strong vertical gradient, varying up to 4 orders of magnitude from the marine boundary layer to free troposphere. The modeled residence times suggest that the lifetime of sea salt particles with a dry diameter of less than 3 µm is largely controlled by wet removal, followed by turbulent process. During both boreal summer and winter, the GEOS-simulated sea salt mass mixing ratios agree with SAGA measurements in the marine boundary layer (MBL) and with PALMS measurements above the MBL. However, comparison of AOD from GEOS with AERONET/MAN and MODIS aerosol retrievals indicated that the model underestimated AOD over the oceans where sea salt dominates. The apparent discrepancy of slightly overpredicted concentration and large underpredicted AOD could not be explained by biases in the model RH affecting the particle hygroscopic growth, as modeled RH was found to be comparable to or larger than the in situ measurements. This conundrum could at least partially be explained by the difference in sea salt size distribution; the GEOS simulation has much less sea salt percentage-wise in the smaller particle size range and thus less efficient light extinction than what was observed by PALMS.

scholarly journals H<sub>2</sub> vertical profiles in the continental boundary layer: measurements at the Cabauw tall tower in The Netherlands

2011 ◽  
Vol 11 (13) ◽  
pp. 6425-6443 ◽  
Author(s):  
M. E. Popa ◽  
A. T. Vermeulen ◽  
W. C. M. van den Bulk ◽  
P. A. C. Jongejan ◽  
A. M. Batenburg ◽  
...  
Keyword(s):  
Boundary Layer ◽  
The Netherlands ◽  
Large Scale ◽  
Ground Level ◽  
Vertical Profiles ◽  
Short Term ◽  
Soil Uptake ◽  
Sampling Height ◽  
Tall Tower

Abstract. In-situ, quasi-continuous measurements of atmospheric hydrogen (H2) have been performed since October 2007 at the Cabauw tall tower station in the Netherlands. Mole fractions of H2, CO and several greenhouse gases are determined simultaneously in air sampled successively at four heights, between 20 and 200 m above ground level. 222Rn measurements are performed in air sampled at 20 and 200 m. This H2 dataset represents the first in-situ, quasi-continuous long-term measurement series of vertical profiles of H2 in the lower continental boundary layer. Seasonal cycles are present at all heights in both H2 and CO, and their amplitude varies with the sampling height. The seasonality is evident in both the "baseline" values and in the short term (diurnal to synoptic time scales) variability, the latter being significantly larger during winter. The observed H2 short term signals and vertical gradients are in many cases well correlated to other species, especially to CO. On the other hand, H2 has at times a unique behaviour, due to its particular distribution of sources and sinks. Our estimation for the regional H2 soil uptake flux, using the radon tracer method, is (−1.89 ± 0.26) × 10−5 g/(m2 h), significantly smaller than other recent results from Europe. H2/CO ratios of the traffic emissions computed from our data, with an average of 0.54 ± 0.07 mol:mol, are larger and more variable than estimated in some of the previous studies in Europe. This difference can be explained by a different driving regime, due to the frequent traffic jams in the influence area of Cabauw. The H2/CO ratios of the large scale pollution events have an average of 0.36 ± 0.05 mol:mol; these ratios were observed to slightly increase with sampling height, possibly due to a stronger influence of soil uptake at the lower sampling heights.

scholarly journals IMPROVING SYSTEM READINESS, STAFF PREPAREDNESS AND PATIENT SAFETY IN A NEW SINGLE FAMILY ROOM NICU THROUGH IN SITU SIMULATION

2018 ◽  
Vol 23 (suppl_1) ◽  
pp. e16-e16
Author(s):  
Ahmed Moussa ◽  
Audrey Larone-Juneau ◽  
Laura Fazilleau ◽  
Marie-Eve Rochon ◽  
Justine Giroux ◽  
...  
Keyword(s):  
Patient Safety ◽  
Repeated Measures ◽  
Large Scale ◽  
Multidisciplinary Teams ◽  
Single Family ◽  
In Situ Simulation ◽  
Ensure Patient Safety ◽  
System Readiness ◽  
Dependent Samples

Abstract BACKGROUND Transitions to new healthcare environments can negatively impact patient care and threaten patient safety. Immersive in situ simulation conducted in newly constructed single family room (SFR) Neonatal Intensive Care Units (NICUs) prior to occupancy, has been shown to be effective in testing new environments and identifying latent safety threats (LSTs). These simulations overlay human factors to identify LSTs as new and existing process and systems are implemented in the new environment OBJECTIVES We aimed to demonstrate that large-scale, immersive, in situ simulation prior to the transition to a new SFR NICU improves: 1) systems readiness, 2) staff preparedness, 3) patient safety, 4) staff comfort with simulation, and 5) staff attitude towards culture change. DESIGN/METHODS Multidisciplinary teams of neonatal healthcare providers (HCP) and parents of former NICU patients participated in large-scale, immersive in-situ simulations conducted in the new NICU prior to occupancy. One eighth of the NICU was outfitted with equipment and mannequins and staff performed in their native roles. Multidisciplinary debriefings, which included parents, were conducted immediately after simulations to identify LSTs. Through an iterative process issues were resolved and additional simulations conducted. Debriefings were documented and debriefing transcripts transcribed and LSTs classified using qualitative methods. To assess systems readiness and staff preparedness for transition into the new NICU, HCPs completed surveys prior to transition, post-simulation and post-transition. Systems readiness and staff preparedness were rated on a 5-point Likert scale. Average survey responses were analyzed using dependent samples t-tests and repeated measures ANOVAs. RESULTS One hundred eight HCPs and 24 parents participated in six half-day simulation sessions. A total of 75 LSTs were identified and were categorized into eight themes: 1) work organization, 2) orientation and parent wayfinding, 3) communication devices/systems, 4) nursing and resuscitation equipment, 5) ergonomics, 6) parent comfort; 7) work processes, and 8) interdepartmental interactions. Prior to the transition to the new NICU, 76% of the LSTs were resolved. Survey response rate was 31%, 16%, 7% for baseline, post-simulation and post-move surveys, respectively. System readiness at baseline was 1.3/5,. Post-simulation systems readiness was 3.5/5 (p = 0.0001) and post-transition was 3.9/5 (p = 0.02). Staff preparedness at baseline was 1.4/5. Staff preparedness post-simulation was 3.3/5 (p = 0.006) and post-transition was 3.9/5 (p = 0.03). CONCLUSION Large-scale, immersive in situ simulation is a feasible and effective methodology for identifying LSTs, improving systems readiness and staff preparedness in a new SFR NICU prior to occupancy. However, to optimize patient safety, identified LSTs must be mitigated prior to occupancy. Coordinating large-scale simulations is worth the time and cost investment necessary to optimize systems and ensure patient safety prior to transition to a new SFR NICU.

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