scholarly journals Carbon monoxide distributions from the IASI/METOP mission: evaluation with other space-borne remote sensors

2009 ◽  
Vol 9 (21) ◽  
pp. 8317-8330 ◽  
Author(s):  
M. George ◽  
C. Clerbaux ◽  
D. Hurtmans ◽  
S. Turquety ◽  
P.-F. Coheur ◽  
...  
Keyword(s):  
Carbon Monoxide ◽  
A Priori ◽  
Global Scale ◽  
Equatorial Region ◽  
Vertical Profiles ◽  
Atmospheric Infrared Sounder ◽  
Upper Troposphere ◽  
Remote Sensors ◽  
Atmospheric Sounding ◽  
Total Column

Abstract. The Infrared Atmospheric Sounding Interferometer (IASI) onboard the MetOp satellite measures carbon monoxide (CO) on a global scale, twice a day. CO total columns and vertical profiles are retrieved in near real time from the nadir radiance spectra measured by the instrument in the thermal infrared (TIR) spectral range. This paper describes the measurement vertical sensitivity and provides a first assessment of the capabilities of IASI to measure CO distributions. On the global scale, 0.8 to 2.4 independent pieces of information are available for the retrieval. At mid latitudes, the information ranges between 1.5 and 2, which enables the lower and upper troposphere to be distinguished, especially when thermal contrast is significant. Global distributions of column CO are evaluated with correlative observations available from other nadir looking TIR missions currently in operation: the Measurements of Pollution in the Troposphere (MOPITT) onboard TERRA, the Atmospheric Infrared Sounder (AIRS) onboard AQUA and the Tropospheric Emission Spectrometer (TES) onboard AURA. The IASI CO columns are compared with MOPITT, AIRS and TES CO columns, adjusted with the a priori, for three different months: August 2008, November 2008 and February 2009. On average, total column discrepancies of about 7% are found between IASI and the three other sounders in the Northern Hemisphere and in the equatorial region. However when strong CO concentrations are present, such as during fire events, these discrepancies can climb as high as 17%. Instrument specifications of IASI versus other missions are also discussed.

scholarly journals Carbon monoxide distributions from the IASI/METOP mission: evaluation with other space-borne remote sensors

2009 ◽  
Vol 9 (2) ◽  
pp. 9793-9822 ◽  
Author(s):  
M. George ◽  
C. Clerbaux ◽  
D. Hurtmans ◽  
S. Turquety ◽  
P.-F. Coheur ◽  
...  
Keyword(s):  
Carbon Monoxide ◽  
A Priori ◽  
Global Scale ◽  
Vertical Profiles ◽  
Atmospheric Infrared Sounder ◽  
Upper Troposphere ◽  
Remote Sensors ◽  
Atmospheric Sounding ◽  
Total Column ◽  
Co Concentrations

Abstract. The Infrared Atmospheric Sounding Interferometer (IASI) onboard the MetOp satellite measures carbon monoxide (CO) on a global scale, twice a day. CO total columns and vertical profiles are retrieved in near real time from the nadir radiance spectra measured by the instrument in the thermal infrared (TIR) spectral range. This paper describes the measurement vertical sensitivity of IASI. On the global scale, 0.8 to 2.4 independent pieces of information are available for the retrieval. At mid latitudes, the information ranges between 1.5 and 2, which enables the lower and upper troposphere to be distinguished, especially when thermal contrast is important. Global distributions of column CO are evaluated with correlative observations available from other nadir looking TIR missions currently in operation: the Measurements of Pollution in the Troposphere (MOPITT) onboard TERRA, the Atmospheric Infrared Sounder (AIRS) onboard AQUA and the Tropospheric Emission Spectrometer (TES) onboard AURA. On the global scale and on average, total column discrepancies ranging from 10 to 15% are found for latitudes above 45° N and lower than 15° S, but can reach 30% in cases of strong CO concentrations, e.g. when fires events occur. The choice of the a priori assumptions influences the retrievals and can explain some of the observed differences. Instrument specifications of IASI versus other missions are also discussed.

scholarly journals An examination of the long-term CO records from MOPITT and IASI: comparison of retrieval methodology

2015 ◽  
Vol 8 (4) ◽  
pp. 4095-4135 ◽  
Author(s):  
M. George ◽  
C. Clerbaux ◽  
I. Bouarar ◽  
P.-F. Coheur ◽  
M. N. Deeter ◽  
...  
Keyword(s):  
A Priori ◽  
Correlation Coefficients ◽  
Global Scale ◽  
Vertical Profiles ◽  
Unexpected Events ◽  
Advantages And Disadvantages ◽  
Atmospheric State ◽  
Total Column ◽  
Aircraft Data

Abstract. Carbon monoxide (CO) is a key atmospheric compound that can be remotely sensed by satellite on the global scale. Fifteen years of continuous observations are now available from the MOPITT/Terra mission (2000 to present). Another fifteen and more years of observations will be provided by the IASI/MetOp instrument series (2007–2023>). In order to study long term variability and trends, a homogeneous record is required, which is not straightforward as the retrieved products are instrument and processing dependent. The present study aims at evaluating the consistency between the CO products derived from the MOPITT and IASI missions, both for total columns and vertical profiles, during a six year overlap period (2008–2013). The analysis is performed by first comparing the available 2013 versions of the retrieval algorithms, and second using a dedicated reprocessing of MOPITT CO profiles and columns based on the IASI a priori constraints. MOPITT v5T total columns are generally slightly higher over land (bias ranging from 0 to 13%) than IASI v20100815 data. When IASI and MOPITT data are retrieved with the same a priori constraints, correlation coefficients are slightly improved. Large discrepancies (total column bias over 15%) observed in the Northern Hemisphere during the winter months are reduced by a factor of 2 to 2.5. The detailed analysis of retrieved vertical profiles compared with collocated aircraft data from the MOZAIC-IAGOS network, illustrates the advantages and disadvantages of a constant vs. a variable a priori. On one hand, MOPITT agrees better with the aircraft profiles for observations with persisting high levels of CO throughout the year due to pollution or seasonal fire activity (because the climatology-based a priori is supposed to be closer to the real atmospheric state). On the other hand, IASI performs better when unexpected events leading to high levels of CO occur, due to the less constrained variance-covariance matrix.

scholarly journals An examination of the long-term CO records from MOPITT and IASI: comparison of retrieval methodology

2015 ◽  
Vol 8 (10) ◽  
pp. 4313-4328 ◽  
Author(s):  
M. George ◽  
C. Clerbaux ◽  
I. Bouarar ◽  
P.-F. Coheur ◽  
M. N. Deeter ◽  
...  
Keyword(s):  
A Priori ◽  
Correlation Coefficients ◽  
Global Scale ◽  
Vertical Profiles ◽  
Advantages And Disadvantages ◽  
Atmospheric State ◽  
Priori Information ◽  
Total Column ◽  
Aircraft Data

Abstract. Carbon monoxide (CO) is a key atmospheric compound that can be remotely sensed by satellite on the global scale. Fifteen years of continuous observations are now available from the MOPITT/Terra mission (2000 to present). Another 15 and more years of observations will be provided by the IASI/MetOp instrument series (2007–2023 >). In order to study long-term variability and trends, a homogeneous record is required, which is not straightforward as the retrieved quantities are instrument and processing dependent. The present study aims at evaluating the consistency between the CO products derived from the MOPITT and IASI missions, both for total columns and vertical profiles, during a 6-year overlap period (2008–2013). The analysis is performed by first comparing the available 2013 versions of the retrieval algorithms (v5T for MOPITT and v20100815 for IASI), and second using a dedicated reprocessing of MOPITT CO profiles and columns using the same a priori information as the IASI product. MOPITT total columns are generally slightly higher over land (bias ranging from 0 to 13 %) than IASI data. When IASI and MOPITT data are retrieved with the same a priori constraints, correlation coefficients are slightly improved. Large discrepancies (total column bias over 15 %) observed in the Northern Hemisphere during the winter months are reduced by a factor of 2 to 2.5. The detailed analysis of retrieved vertical profiles compared with collocated aircraft data from the MOZAIC-IAGOS network, illustrates the advantages and disadvantages of a constant vs. a variable a priori. On one hand, MOPITT agrees better with the aircraft profiles for observations with persisting high levels of CO throughout the year due to pollution or seasonal fire activity (because the climatology-based a priori is supposed to be closer to the real atmospheric state). On the other hand, IASI performs better when unexpected events leading to high levels of CO occur, due to a larger variability associated with the a priori.

scholarly journals Retrieval of desert dust aerosol vertical profiles from IASI measurements in the TIR atmospheric window

2013 ◽  
Vol 6 (10) ◽  
pp. 2577-2591 ◽  
Author(s):  
S. Vandenbussche ◽  
S. Kochenova ◽  
A. C. Vandaele ◽  
N. Kumps ◽  
M. De Mazière
Keyword(s):  
Optical Depth ◽  
Radiative Forcing ◽  
Degrees Of Freedom ◽  
A Priori ◽  
Global Scale ◽  
Dust Aerosol ◽  
Vertical Profiles ◽  
Desert Dust ◽  
Dust Aerosols ◽  
Infrared Measurements

Abstract. Desert dust aerosols are the most prominent tropospheric aerosols, playing an important role in the earth's climate. However, their radiative forcing is currently not known with sufficient precision to even determine its sign. The sources of uncertainty are multiple, one of them being a poor characterisation of the dust aerosol's vertical profile on a global scale. In this work, we tackle this scientific issue by designing a method for retrieving dust aerosol vertical profiles from Thermal Infrared measurements by Infrared Atmospheric Sounding Interferometer (IASI) instruments onboard the Metop satellite series. IASI offers almost global coverage twice a day, and long (past and future) time series of radiances, therefore being extremely well suited for climate studies. Our retrieval follows Rodger's formalism and is based on a two-step approach, treating separately the issues of low altitude sensitivity and difficult a priori definition. We compare our results for a selected test case above the Atlantic Ocean and North Africa in June 2009, with optical depth data from MODIS, aerosol absorbing index from GOME-2 and OMI, and vertical profiles of extinction coefficients from CALIOP. We also use literature information on desert dust sources to interpret our results above land. Our retrievals provide perfectly reasonable results in terms of optical depth. The retrieved vertical profiles (with on average 1.5 degrees of freedom) show most of the time sensitivity down to the lowest layer, and agree well with CALIOP extinction profiles for medium to high dust optical depth. We conclude that this new method is extremely promising for improving the scientific knowledge about the 3-D distribution of desert dust aerosols in the atmosphere.

scholarly journals Global carbon monoxide products from combined AIRS, TES and MLS measurements on A-train satellites

2013 ◽  
Vol 13 (6) ◽  
pp. 15409-15441
Author(s):  
J. X. Warner ◽  
R. Yang ◽  
Z. Wei ◽  
F. Carminati ◽  
A. Tangborn ◽  
...  
Keyword(s):  
Carbon Monoxide ◽  
Data Fusion ◽  
Lower Troposphere ◽  
Atmospheric Infrared Sounder ◽  
Upper Troposphere ◽  
In Situ Data ◽  
Diode Laser Spectrometer ◽  
Spatial Coverage ◽  
Transport Experiment

Abstract. This study tests a novel methodology to add value to satellite datasets. This methodology, data fusion, is similar to data assimilation, except that the background model-based field is replaced by a satellite dataset, in this case AIRS (Atmospheric Infrared Sounder) carbon monoxide (CO) measurements. The observational information comes from CO measurements with lower spatial coverage than AIRS, namely, from TES (Tropospheric Emission Spectrometer) and MLS (Microwave Limb Sounder). We show that combining these datasets with data fusion uses the higher spectral resolution of TES to extend AIRS CO observational sensitivity to the lower troposphere, a region especially important for air quality studies. We also show that combined CO measurements from AIRS and MLS provide enhanced information in the UTLS (upper troposphere/lower stratosphere) region compared to each product individually. The combined AIRS/TES and AIRS/MLS CO products are validated against DACOM (differential absorption mid-IR diode laser spectrometer) in situ CO measurements from the INTEX-B (Intercontinental Chemical Transport Experiment: MILAGRO and Pacific phases) field campaign and in situ data from HIPPO (HIAPER Pole-to-Pole Observations) flights. The data fusion results show improved sensitivities in the lower and upper troposphere (20–30% and above 20%, respectively) as compared with AIRS-only retrievals, and improved coverage compared with TES and MLS CO data.

scholarly journals Retrieval of desert dust aerosol vertical profiles from IASI measurements in the TIR atmospheric window

2013 ◽  
Vol 6 (3) ◽  
pp. 4511-4550
Author(s):  
S. Vandenbussche ◽  
S. Kochenova ◽  
A. C. Vandaele ◽  
N. Kumps ◽  
M. De Mazière
Keyword(s):  
Optical Depth ◽  
Radiative Forcing ◽  
Degrees Of Freedom ◽  
A Priori ◽  
Global Scale ◽  
Test Case ◽  
Vertical Profiles ◽  
Desert Dust ◽  
Dust Aerosols ◽  
Infrared Measurements

Abstract. Desert dust aerosols are the most prominent tropospheric aerosols, playing an important role in the Earth's climate. However, their radiative forcing is currently not known with sufficient precision to even determine its sign. The sources of uncertainty are multiple, one of them being a poor characterisation of dust aerosols vertical profile on a global scale. In this work, we tackle this scientific issue by designing a method for retrieving dust aerosols vertical profiles from Thermal Infrared measurements by IASI instruments onboard the Metop satellite series. IASI offers almost global coverage twice a day, and long (past and future) time series of radiances, being therefore extremely well-suited for climate studies. Our retrieval follows Rodger's formalism and is based on a two-steps approach, treating separately the issues of low altitude sensitivity and of difficult a priori definition. We compare our results for a selected test-case, above the Atlantic Ocean and North Africa in June 2009, with optical depth data from MODIS, aerosol absorbing index from GOME-2 and OMI, and vertical profiles of extinction coefficients from CALIOP. We also use literature information on desert dust sources to interpret our results above land. Our retrievals provide perfectly reasonable results in terms of optical depth. The retrieved vertical profiles (with on average 1.5 degrees of freedom) show most of the time sensitivity down to the lowest layer, and agree well with CALIOP extinction profiles for medium to high dust optical depth. We conclude that this new method is extremely promising for improving the scientific knowledge about the 3-D distribution of desert dust aerosols in the atmosphere.

scholarly journals Global distribution of CO<sub>2</sub> in the Upper-Troposphere and Stratosphere

2016 ◽  
Author(s):  
M. Diallo ◽  
B. Legras ◽  
E. Ray ◽  
A. Engel ◽  
J. A. Añel
Keyword(s):  
Global Scale ◽  
Lagrangian Model ◽  
Vertical Profiles ◽  
Mixing Ratio ◽  
Tropical Regions ◽  
High Co2 ◽  
Upper Troposphere ◽  
Satellite Validation ◽  
Carbon Dioxide Co2 ◽  
The Tropics

Abstract. In this study, we aim to reconstruct a relevant and new database of monthly zonal mean distribution of carbon dioxide (CO2) at global scale extending from the upper-troposphere (UT) to stratosphere (S). This product can be used for model and satellite validation in the UT/S, as a prior for inversion modelling and mainly to analyse a plausible feature of the stratospheric-tropospheric exchange as well as the stratospheric circulation and its variability. To do so, we investigate the ability of a Lagrangian trajectory model guided by ERA-Interim reanalysis to construct the CO2 abundance in the UT/S. From 10 year backward trajectories and tropospheric observations of CO2, we reconstruct upper-tropospheric and stratospheric CO2 over the period 2000–2010. The inter-comparisons of the reconstructed CO2 with mid-latitude vertical profiles measured by balloon samples as well as quasi-horizontal air samples from ER-2 aircraft during SOLVE and CONTRAIL campaigns exhibit a remarkable agreement. That demonstrates the potential of Lagrangian model to reconstruct CO2 in the UT/S. The zonal mean distribution exhibits relatively large CO2 in the tropical stratosphere due to the seasonal variation of the tropical upwelling of Brewer-Dobson circulation. During winter and spring, the tropical pipe is relatively isolated but is less narrow during summer and autumn so that high CO2 values are more readily transported out of the tropics to the mid- and high latitude stratosphere. The shape of the vertical profiles suggests that relatively high CO2 above 20 km altitude mainly enter the stratosphere through tropical upwelling. CO2 mixing ratio is relatively low in the polar and tropical regions above 25 km. On average the CO2 mixing ratio decreases with altitude by 6–8 ppmv from the UT to stratosphere (e.g. up to 35 km) and is nearly constant with altitude.

scholarly journals Retrieval of MetOp-A/IASI CO profiles and validation with MOZAIC data

2012 ◽  
Vol 5 (11) ◽  
pp. 2843-2857 ◽  
Author(s):  
E. De Wachter ◽  
B. Barret ◽  
E. Le Flochmoën ◽  
E. Pavelin ◽  
M. Matricardi ◽  
...  
Keyword(s):  
Lower Troposphere ◽  
Correlation Coefficients ◽  
Lower Surface ◽  
Global Scale ◽  
Upper Troposphere ◽  
Retrieval Algorithms ◽  
Atmospheric Sounding ◽  
The Impact ◽  
Limited Sensitivity

Abstract. The IASI (Infrared Atmospheric Sounding Interferometer) nadir-looking thermal infrared sounder onboard MetOp-A enables the monitoring of atmospheric constituents on a global scale. This paper presents a quality assessment of IASI CO profiles retrieved by the two different retrieval algorithms SOFRID and FORLI, by an intercomparison with airborne in-situ CO profiles from the MOZAIC program for the 2008–2009 period. Lower (surface–480 hPa) and upper tropospheric partial column (480–225 hPa) comparisons as well as profile comparisons are made. The retrieval errors of the IASI products are less than 21% in the lower troposphere and less than 10% in the upper troposphere. A statistical analysis shows similar correlation coefficients for the two retrieval algorithms and smoothed MOZAIC of r ~ 0.8 and r ~ 0.7 in the lower and upper troposphere respectively. Comparison with smoothed MOZAIC data of the temporal variation of the CO profiles at the airports of Frankfurt and Windhoek demonstrates that the IASI products are able to capture the seasonal variability at these sites. At Frankfurt SOFRID (respectively FORLI) is positively biased by 10.5% (13.0%) compared to smoothed MOZAIC in the upper (lower) troposphere, and the limited sensitivity of the IASI instrument to the boundary layer when thermal contrast is low is identified. At Windhoek, the impact of the vegetation fires in Southern Africa from July to November is captured by both SOFRID and FORLI, with an overestimation of the CO background values (fire maxima) by SOFRID (FORLI) by 12.8% (10%). Profile comparisons at Frankfurt and Windhoek show that the largest discrepancies are found between the two IASI products and MOZAIC for the nighttime retrievals.

scholarly journals Retrieval of sulphur dioxide from the infrared atmospheric sounding interferometer (IASI)

2012 ◽  
Vol 5 (3) ◽  
pp. 581-594 ◽  
Author(s):  
L. Clarisse ◽  
D. Hurtmans ◽  
C. Clerbaux ◽  
J. Hadji-Lazaro ◽  
Y. Ngadi ◽  
...  
Keyword(s):  
High Resolution ◽  
Error Analysis ◽  
Sulphur Dioxide ◽  
Absorption Bands ◽  
Atmospheric Infrared Sounder ◽  
Volcanic Plumes ◽  
Atmospheric Sounding ◽  
Valuable Complement ◽  
Total Column ◽  
Novel Algorithm

Abstract. Thermal infrared sounding of sulphur dioxide (SO2) from space has gained appreciation as a valuable complement to ultraviolet sounding. There are several strong absorption bands of SO2 in the infrared, and atmospheric sounders, such as AIRS (Atmospheric Infrared Sounder), TES (Tropospheric Emission Spectrometer) and IASI (Infrared Atmospheric Sounding Interferometer) have the ability to globally monitor SO2 abundances. Most of the observed SO2 is found in volcanic plumes. In this paper we outline a novel algorithm for the sounding of SO2 above ~5 km altitude using high resolution infrared sounders and apply it to measurements of IASI. The main features of the algorithm are a wide applicable total column range (over 4 orders of magnitude, from 0.5 to 5000 dobson units), a low theoretical uncertainty (3–5%) and near real time applicability. We make an error analysis and demonstrate the algorithm on the recent eruptions of Sarychev, Kasatochi, Grimsvötn, Puyehue-Cordón Caulle and Nabro.

scholarly journals First detection of ammonia (NH<sub>3</sub>) in the Asian monsoon upper troposphere

2016 ◽  
Author(s):  
Michael Höpfner ◽  
Rainer Volkamer ◽  
Udo Grabowski ◽  
Michel Grutter ◽  
Johannes Orphal ◽  
...  
Keyword(s):  
Asian Monsoon ◽  
Aerosol Particles ◽  
Emission Spectra ◽  
Global Scale ◽  
Model Simulations ◽  
Upper Troposphere ◽  
Mixing Ratios ◽  
Monsoon Area ◽  
Atmospheric Sounding ◽  
Different Seasons

Abstract. Ammonia (NH3) has been detected in the upper troposphere by analysis of averaged MIPAS (Michelson Interferomter for Passive Atmospheric Sounding) infrared limb-emission spectra. We have found enhanced amounts of NH3 within the region of the Asian monsoon at 12–15 km altitude. Three-monthly, 10° longitude x 10° latitude average profiles reaching maximum mixing ratios of around 30 pptv in this altitude range have been retrieved with a vertical resolution of 3–8 km and estimated errors of about 5 pptv. These observations show that loss processes during transport from the boundary layer to the upper troposphere within the Asian monsoon do not deplete the air entirely of NH3. Thus, ammonia might contribute to the so-called Asian tropopause aersol layer by formation of ammonium aerosol particles. On a global scale, outside the monsoon area and during different seasons, we could not detect enhanced values of NH3 above the actual detection limit of about 3–5 pptv. This upper bound helps to constrain global model simulations.

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