scholarly journals The AOTF-based NO<sub>2</sub> camera

2016 ◽  
Author(s):  
Emmanuel Dekemper ◽  
Jurgen Vanhamel ◽  
Bert Van Opstal ◽  
Didier Fussen

Abstract. The abundance of NO2 in the boundary layer relates to air quality and pollution sources monitoring. Observing the spatio-temporal distribution of NO2 above well-delimited (flue gas stacks, volcanoes, ships) or more extended sources (cities) allows for several applications: monitoring emission fluxes or studying the plume dynamic chemistry and its transport. So far, most attempts to map the NO2 field from the ground have been made with visible-light scanning spectrometers. Benefiting from a high retrieval accuracy, they only achieve a relatively low temporal resolution that hampers the detection of dynamic features. We present a new type of passive remote sensing instrument aiming at the measurement of the 2-D distributions of NO2 slant column densities (SCD) with a high spatio-temporal resolution. The measurement principle has strong similarities with the popular filter-based SO2 camera as it relies on spectral images taken at wavelengths where the molecule absorption cross-section is different. Contrary to the SO2 camera, the spectral selection is performed by an acousto-optical tunable filter (AOTF) capable of resolving the target molecule's spectral features. The NO2 camera capabilities are demonstrated by imaging the NO2 abundance in the plume of a coal-fired power plant. During this experiment, the 2-D distribution of the NO2 SCD was retrieved with a temporal resolution of 3 minutes and a spatial sampling of 50 cm (over a 250 x 250 m2 area). The detection limit was close to 5 x 1016 molecules cm−2, with a maximum detected SCD of 4 x 1017 molecules cm−2. Illustrating the added-value of the NO2 camera measurements, the data reveal the dynamics of the NO to NO2 conversion in the early plume with an unprecedent resolution: from its release in the air, and for 100 m upwards, the observed NO2 plume concentration increased at a rate of 0.75–1.25 g s−1. In joint campaigns with SO2 cameras, the NO2 camera could also help in removing the bias introduced by the NO2 interference in the SO2 measurements.

2016 ◽  
Vol 9 (12) ◽  
pp. 6025-6034 ◽  
Author(s):  
Emmanuel Dekemper ◽  
Jurgen Vanhamel ◽  
Bert Van Opstal ◽  
Didier Fussen

Abstract. The abundance of NO2 in the boundary layer relates to air quality and pollution source monitoring. Observing the spatiotemporal distribution of NO2 above well-delimited (flue gas stacks, volcanoes, ships) or more extended sources (cities) allows for applications such as monitoring emission fluxes or studying the plume dynamic chemistry and its transport. So far, most attempts to map the NO2 field from the ground have been made with visible-light scanning grating spectrometers. Benefiting from a high retrieval accuracy, they only achieve a relatively low spatiotemporal resolution that hampers the detection of dynamic features. We present a new type of passive remote sensing instrument aiming at the measurement of the 2-D distributions of NO2 slant column densities (SCDs) with a high spatiotemporal resolution. The measurement principle has strong similarities with the popular filter-based SO2 camera as it relies on spectral images taken at wavelengths where the molecule absorption cross section is different. Contrary to the SO2 camera, the spectral selection is performed by an acousto-optical tunable filter (AOTF) capable of resolving the target molecule's spectral features. The NO2 camera capabilities are demonstrated by imaging the NO2 abundance in the plume of a coal-fired power plant. During this experiment, the 2-D distribution of the NO2 SCD was retrieved with a temporal resolution of 3 min and a spatial sampling of 50 cm (over a 250 × 250 m2 area). The detection limit was close to 5 × 1016 molecules cm−2, with a maximum detected SCD of 4 × 1017 molecules cm−2. Illustrating the added value of the NO2 camera measurements, the data reveal the dynamics of the NO to NO2 conversion in the early plume with an unprecedent resolution: from its release in the air, and for 100 m upwards, the observed NO2 plume concentration increased at a rate of 0.75–1.25 g s−1. In joint campaigns with SO2 cameras, the NO2 camera could also help in removing the bias introduced by the NO2 interference with the SO2 spectrum.


2011 ◽  
Vol 15 (2) ◽  
pp. 437-451 ◽  
Author(s):  
E. L. A. Wolters ◽  
B. J. J. M. van den Hurk ◽  
R. A. Roebeling

Abstract. This paper describes the evaluation of the KNMI Cloud Physical Properties – Precipitation Properties (CPP-PP) algorithm over West Africa. The algorithm combines condensed water path (CWP), cloud phase (CPH), cloud particle effective radius (re), and cloud-top temperature (CTT) retrievals from visible, near-infrared and thermal infrared observations of the Spinning Enhanced Visible and Infrared Imager (SEVIRI) onboard the Meteosat Second Generation (MSG) satellites to estimate rain occurrence frequency and rain rate. For the 2005 and 2006 monsoon seasons, it is investigated whether the CPP-PP algorithm is capable of retrieving rain occurrence frequency and rain rate over West Africa with sufficient accuracy, using Tropical Monsoon Measurement Mission Precipitation Radar (TRMM-PR) as reference. As a second goal, it is assessed whether SEVIRI is capable of monitoring the seasonal and daytime evolution of rainfall during the West African monsoon (WAM), using Climate Prediction Center Morphing Technique (CMORPH) rainfall observations. The SEVIRI-detected rainfall area agrees well with TRMM-PR, with the areal extent of rainfall by SEVIRI being ~10% larger than from TRMM-PR. The mean retrieved rain rate from CPP-PP is about 8% higher than from TRMM-PR. Examination of the TRMM-PR and CPP-PP cumulative frequency distributions revealed that differences between CPP-PP and TRMM-PR are generally within +/−10%. Relative to the AMMA rain gauge observations, CPP-PP shows very good agreement up to 5 mm h−1. However, at higher rain rates (5–16 mm h−1) CPP-PP overestimates compared to the rain gauges. With respect to the second goal of this paper, it was shown that both the accumulated precipitation and the seasonal progression of rainfall throughout the WAM is in good agreement with CMORPH, although CPP-PP retrieves higher amounts in the coastal region of West Africa. Using latitudinal Hovmüller diagrams, a fair correspondence between CPP-PP and CMORPH was found, which is reflected by high correlation coefficients (~0.7) for both rain rate and rain occurrence frequency. The daytime cycle of rainfall from CPP-PP shows distinctly different patterns for three different regions in West Africa throughout the WAM, with a decrease in dynamical range of rainfall near the Inter Tropical Convergence Zone (ITCZ). The dynamical range as retrieved from CPP-PP is larger than that from CMORPH. It is suggested that this results from both the better spatio-temporal resolution of SEVIRI, as well as from thermal infrared radiances being partly used by CMORPH, which likely smoothes the daytime precipitation signal, especially in case of cold anvils from convective systems. The promising results show that the CPP-PP algorithm, taking advantage of the high spatio-temporal resolution of SEVIRI, is of added value for monitoring daytime precipitation patterns in tropical areas.


2018 ◽  
Vol 10 (12) ◽  
pp. 1950 ◽  
Author(s):  
Luca Cenci ◽  
Luca Pulvirenti ◽  
Giorgio Boni ◽  
Nazzareno Pierdicca

The next generation of synthetic aperture radar (SAR) systems could foresee satellite missions based on a geosynchronous orbit (GEO SAR). These systems are able to provide radar images with an unprecedented combination of spatial (≤1 km) and temporal (≤12 h) resolutions. This paper investigates the GEO SAR potentialities for soil moisture (SM) mapping finalized to hydrological applications, and defines the best compromise, in terms of image spatio-temporal resolution, for SM monitoring. A synthetic soil moisture–data assimilation (SM-DA) experiment was thus set up to evaluate the impact of the hydrological assimilation of different GEO SAR-like SM products, characterized by diverse spatio-temporal resolutions. The experiment was also designed to understand if GEO SAR-like SM maps could provide an added value with respect to SM products retrieved from SAR images acquired from satellites flying on a quasi-polar orbit, like Sentinel-1 (POLAR SAR). Findings showed that GEO SAR systems provide a valuable contribution for hydrological applications, especially if the possibility to generate many sub-daily observations is sacrificed in favor of higher spatial resolution. In the experiment, it was found that the assimilation of two GEO SAR-like observations a day, with a spatial resolution of 100 m, maximized the performances of the hydrological predictions, for both streamflow and SM state forecasts. Such improvements of the model performances were found to be 45% higher than the ones obtained by assimilating POLAR SAR-like SM maps.


2019 ◽  
Vol 23 (1) ◽  
pp. 255-275 ◽  
Author(s):  
Samiro Khodayar ◽  
Amparo Coll ◽  
Ernesto Lopez-Baeza

Abstract. This study uses the synergy of multi-resolution soil moisture (SM) satellite estimates from the Soil Moisture Ocean Salinity (SMOS) mission, a dense network of ground-based SM measurements, and a soil–vegetation–atmosphere transfer (SVAT) model, SURFEX (externalized surface), module ISBA (interactions between soil, biosphere and atmosphere), to examine the benefits of the SMOS level 4 (SMOS-L4) version 3.0, or “all weather” high-resolution soil moisture disaggregated product (SMOS-L43.0; ∼1 km). The added value compared to SMOS level 3 (SMOS-L3; ∼25 km) and SMOS level 2 (SMOS-L2; ∼15 km) is investigated. In situ SM observations over the Valencia anchor station (VAS; SMOS calibration and validation – Cal/Val – site in Europe) are used for comparison. The SURFEX (ISBA) model is used to simulate point-scale surface SM (SSM) and, in combination with high-quality atmospheric information data, namely from the European Centre for Medium-Range Weather Forecasts (ECMWF) and the Système d'analyse fournissant des renseignements atmosphériques à la neige (SAFRAN) meteorological analysis system, to obtain a representative SSM mapping over the VAS. The sensitivity to realistic initialization with SMOS-L43.0 is assessed to simulate the spatial and temporal distribution of SSM. Results demonstrate the following: (a) All SMOS products correctly capture the temporal patterns, but the spatial patterns are not accurately reproduced by the coarser resolutions, probably in relation to the contrast with point-scale in situ measurements. (b) The potential of the SMOS-L43.0 product is pointed out to adequately characterize SM spatio-temporal variability, reflecting patterns consistent with intensive point-scale SSM samples on a daily timescale. The restricted temporal availability of this product dictated by the revisit period of the SMOS satellite compromises the averaged SSM representation for longer periods than a day. (c) A seasonal analysis points out improved consistency during December–January–February and September–October–November, in contrast to significantly worse correlations in March–April–May (in relation to the growing vegetation) and June–July–August (in relation to low SSM values < 0.1 m3 m−3 and low spatial variability). (d) The combined use of the SURFEX (ISBA) SVAT model with the SAFRAN system, initialized with SMOS-L43.0 1 km disaggregated data, is proven to be a suitable tool for producing regional SM maps with high accuracy, which could be used as initial conditions for model simulations, flood forecasting, crop monitoring and crop development strategies, among others.


2018 ◽  
Author(s):  
Samiro Khodayar ◽  
Amparo Coll ◽  
Ernesto Lopez-Baeza

Abstract. This study uses the synergy of multiresolution soil moisture (SM) satellite estimates from the Soil Moisture Ocean Salinity (SMOS) mission, a dense network of ground-based SM measurements, and a Soil Vegetation Atmosphere Transfer (SVAT) model, SURFEX (Externalized Surface) – module ISBA (Interactions between Soil-Biosphere-Atmosphere), to examine, i) the comparison and suitability of different operational SMOS SM products to provide realistic information on the water content of the soil as well as the added value of the newly released SMOS Level 4 3.0 all weather disaggregated ~ 1 km SM (SMOS_L43.0), and ii) its potential impact for improving uncertainty associated to SM initialization in land surface modelling. Three different data products from SMOS-L3 (~ 25 km), L2 (~ 15 km), and disaggregated L4 3.0 (~ 1 km) are investigated. In situ SM observations over the Valencia Anchor Station (VAS; SMOS Calibration/Validation (Cal/Val) site in Europe) are used for comparison. The SURFEX-ISBA model is used to simulate point-scale surface SM (SSM) and, in combination with high-quality atmospheric information data, namely ECMWF and the SAFRAN meteorological analysis system, to obtain a representative SSM mapping over the VAS. The sensitivity to SSM initialization, particularly to realistic initialization with SMOS_L43.0 to simulate the spatial and temporal distribution of SSM is assessed. Results demonstrate: (a) all SMOS products correctly capture the temporal patterns, but, the spatial patterns are not accurately reproduced by the coarser resolutions probably in relation to the contrast with point-scale in situ measurements. (b) The potential of SMOS-L43.0 product is pointed out to adequately characterize SM spatio-temporal variability reflecting patterns consistent with intensive point scale SSM samples on a daily time scale. The restricted temporal availability of this product dictated by the revisit period of the SMOS satellite compromises the averaged SSM representation for longer periods than a day. (c) A seasonal analysis points out improved consistency during December-January-February and September-October-November in contrast to significantly worse correlations in March-April-May (in relation to the growing vegetation) and June-July-August (in relation to low SSM values


2021 ◽  
Author(s):  
Namendra Kumar Shahi ◽  
Jan Polcher‬ ◽  
Sophie Bastin ◽  
Romain Pennel ◽  
Lluís Fita

Abstract In this study, we have assessed the added value on the spatio-temporal distribution of the precipitation of convection-permitting simulation (3km) compared to the parent coarser-scale parameterized convection simulation (20km) with the high-resolution observational datasets i.e. SPREAD (5km) and IBERIA01 (10km) over the Iberian Peninsula in all four seasons during 2000-2009. Both simulations are evaluation runs based on ERA-Interim reanalysis and performed with the RegIPSL regional earth system model in the frame of the European Climate Prediction system (EUCP) H2020 project and COordinated Regional climate Downscaling Experiment (CORDEX). We have not found significant improvement in the convection-permitting simulation compared to the parent coarser-scale simulation for the seasonal mean precipitation of the Iberian Peninsula except the spatial variation over mountainous peaks. The kilometer-scale simulation significantly underestimates the observed seasonal mean precipitation over the western parts of the Iberian Peninsula compared to the coarser-scale simulation, which may be attributed to a change of local dynamics in the kilometer-scale simulation with a weakening and southward shifts of the westerly winds and also an enhancement of warm and dry southerly winds over the Iberian Peninsula. However, the added value of kilometer-scale simulation over the driving coarser-scale simulation is obtained for various indices; in the representation of the spatio-temporal distribution of the wet-day precipitation frequency and intensity, and the extreme/heavy precipitation events for each season at both resolutions i.e. downscaled and upscaled. It has also been noted that the spatio-temporal distribution of precipitation for all metrics used varies between the two observational datasets for all seasons.


2019 ◽  
Vol 19 (15) ◽  
pp. 10217-10237 ◽  
Author(s):  
Henrik Grythe ◽  
Susana Lopez-Aparicio ◽  
Matthias Vogt ◽  
Dam Vo Thanh ◽  
Claudia Hak ◽  
...  

Abstract. We present here emissions estimated from a newly developed emission model for residential wood combustion (RWC) at high spatial and temporal resolution, which we name the MetVed model. The model estimates hourly emissions resolved on a 250 m grid resolution for several compounds, including particulate matter (PM), black carbon (BC) and polycyclic aromatic hydrocarbons (PAHs) in Norway for a 12-year period. The model uses novel input data and calculation methods that combine databases built with an unprecedented high level of detail and near-national coverage. The model establishes wood burning potential at the grid based on the dependencies between variables that influence emissions: i.e. outdoor temperature, number of and type and size of dwellings, type of available heating technologies, distribution of wood-based heating installations and their associated emission factors. RWC activity with a 1 h temporal profile was produced by combining heating degree day and hourly and weekday activity profiles reported by wood consumers in official statistics. This approach results in an improved characterisation of the spatio-temporal distribution of wood use, and subsequently of emissions, required for urban air quality assessments. Whereas most variables are calculated based on bottom-up approaches on a 250 m spatial grid, the MetVed model is set up to use official wood consumption at the county level and then distributes consumption to individual grids proportional to the physical traits of the residences within it. MetVed combines consumption with official emission factors that makes the emissions also upward scalable from the 250 m grid to the national level. The MetVed spatial distribution obtained was compared at the urban scale to other existing emissions at the same scale. The annual urban emissions, developed according to different spatial proxies, were found to have differences up to an order of magnitude. The MetVed total annual PM2.5 emissions in the urban domains compare well to emissions adjusted based on concentration measurements. In addition, hourly PM2.5 concentrations estimated by an Eulerian dispersion model using MetVed emissions were compared to measurements at air quality stations. Both hourly daily profiles and the seasonality of PM2.5 show a slight overestimation of PM2.5 levels. However, a comparison with black carbon from biomass burning and benzo(a)pyrene measurements indicates higher emissions during winter than that obtained by MetVed. The accuracy of urban emissions from RWC relies on the accuracy of the wood consumption (activity data), emission factors and the spatio-temporal distribution. While there are still knowledge gaps regarding emissions, MetVed represents a vast improvement in the spatial and temporal distribution of RWC.


2019 ◽  
Author(s):  
Henrik Grythe ◽  
Susana Lopez-Aparicio ◽  
Matthias Vogt ◽  
Dam Vo Thanh ◽  
Claudia Hak ◽  
...  

Abstract. We present here emissions estimated from a newly developed emission model for residential wood combustion (RWC) at high spatial and temporal resolution, which we title the MetVed model. The model estimates hourly emissions resolved on a 250 m grid resolution for several compounds, including particulate matter (PM), black carbon (BC) and polycyclic aromatic hydrocarbons (PAH) in Norway for a 12 year period. The model uses novel input data and calculation methods that combine databases built with an unprecedented high level of detail and near national coverage. The model establishes wood burning potential at the grid based on the dependencies between variables that influence emissions; i.e., outdoor temperature, number of and type and size of dwellings, type of available heating technologies, distribution of wood-based heating installations and their associated emission factors. RWC activity with a 1 hr temporal profile was produced by combining heating degree day, and hourly and weekday activity profiles reported by wood consumer in official statistics. This approach results in an improved characterisation of the spatio-temporal distribution of wood use and subsequently of emissions, required for urban air quality assessments. Whereas most variables are calculated based on bottom up approaches on a 250 m spatial grid, the MetVed model is set up to use official wood consumption at county level, and then distributes consumption to individual grids proportional to the physical traits of the residences within it. MetVed combines consumption with official emission factors that makes the emissions also upward scalable from the 250 m grid to national level. The MetVed spatial distribution obtained was compared at urban scale to other existing emissions at the same scale. The annual urban emissions, developed according to different spatial proxies, were found to have differences up to order of magnitude. The MetVed total annual PM2.5 emissions in the urban domains compare well to emissions adjusted based on concentration measurements. In addition, hourly PM2.5 concentrations estimated by an Eulerian dispersion model using MetVed emissions was compared to measurements at air quality stations. Both hourly daily profiles and the seasonality of PM2.5 show a slight overestimation of PM2.5 levels. However, a comparison with black carbon from biomass burning and benzo(a)pyrene measurements indicates higher emissions during winter than that obtained by MetVed. The accuracy of urban emissions from RWC relies on the accuracy of the wood consumption (activity data), emission factors and the spatio-temporal distribution. While there are still knowledge gaps regarding emissions, MetVed represents a vast improvement in the spatial and temporal distribution of RWC.


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