scholarly journals A novel method for estimating shortwave direct radiative effect of above-cloud aerosols using CALIOP and MODIS data

2014 ◽  
Vol 7 (6) ◽  
pp. 1777-1789 ◽  
Author(s):  
Z. Zhang ◽  
K. Meyer ◽  
S. Platnick ◽  
L. Oreopoulos ◽  
D. Lee ◽  
...  

Abstract. This paper describes an efficient and unique method for computing the shortwave direct radiative effect (DRE) of aerosol residing above low-level liquid-phase clouds using CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) and MODIS (Moderate Resolution Imaging Spectroradiometer) data. It addresses the overlap of aerosol and cloud rigorously by utilizing the joint histogram of cloud optical depth and cloud top pressure while also accounting for subgrid-scale variations of aerosols. The method is computationally efficient because of its use of grid-level cloud and aerosol statistics, instead of pixel-level products, and a precomputed look-up table based on radiative transfer calculations. We verify that for smoke and polluted dust over the southeastern Atlantic Ocean the method yields a seasonal mean instantaneous (approximately 13:30 local time) shortwave DRE of above-cloud aerosol (ACA) that generally agrees with a more rigorous pixel-level computation within 4%. We also estimate the impact of potential CALIOP aerosol optical depth (AOD) retrieval bias of ACA on DRE. We find that the regional and seasonal mean instantaneous DRE of ACA over southeastern Atlantic Ocean would increase, from the original value of 6.4 W m−2 based on operational CALIOP AOD to 9.6 W m−2 if CALIOP AOD retrievals are biased low by a factor of 1.5 (Meyer et al., 2013) and further to 30.9 W m−2 if CALIOP AOD retrievals are biased low by a factor of 5 as suggested in Jethva et al. (2014). In contrast, the instantaneous ACA radiative forcing efficiency (RFE) remains relatively invariant in all cases at about 53 W m−2 AOD−1, suggesting a near-linear relation between the instantaneous RFE and AOD. We also compute the annual mean instantaneous shortwave DRE of light-absorbing aerosols (i.e., smoke and polluted dust) over global oceans based on 4 years of CALIOP and MODIS data. We find that given an above-cloud aerosol type the optical depth of the underlying clouds plays a larger role than above-cloud AOD in the variability of the annual mean shortwave DRE of above-cloud light-absorbing aerosol. While we demonstrate our method using CALIOP and MODIS data, it can also be extended to other satellite data sets.

2013 ◽  
Vol 6 (6) ◽  
pp. 9993-10020 ◽  
Author(s):  
Z. Zhang ◽  
K. Meyer ◽  
S. Platnick ◽  
L. Oreopoulos ◽  
D. Lee ◽  
...  

Abstract. This paper describes an efficient and unique method for computing the shortwave direct radiative effect (DRE) of aerosol residing above low-level liquid-phase clouds using CALIOP and MODIS data. It accounts for the overlapping of aerosol and cloud rigorously by utilizing the joint histogram of cloud optical depth and cloud top pressure. Effects of sub-grid scale cloud and aerosol variations on DRE are accounted for. It is computationally efficient through using grid-level cloud and aerosol statistics, instead of pixel-level products, and a pre-computed look-up table in radiative transfer calculations. We verified that for smoke over the southeast Atlantic Ocean the method yields a seasonal mean instantaneous shortwave DRE that generally agrees with more rigorous pixel-level computation within 4%. We have also computed the annual mean instantaneous shortwave DRE of light-absorbing aerosols (i.e., smoke and polluted dust) over global ocean based on 4 yr of CALIOP and MODIS data. We found that the variability of the annual mean shortwave DRE of above-cloud light-absorbing aerosol is mainly driven by the optical depth of the underlying clouds.


2013 ◽  
Vol 13 (15) ◽  
pp. 7895-7901 ◽  
Author(s):  
A. Arola ◽  
T. F. Eck ◽  
J. Huttunen ◽  
K. E. J. Lehtinen ◽  
A. V. Lindfors ◽  
...  

Abstract. The diurnal variability of aerosol optical depth (AOD) can be significant, depending on location and dominant aerosol type. However, these diurnal cycles have rarely been taken into account in measurement-based estimates of aerosol direct radiative forcing (ADRF) or aerosol direct radiative effect (ADRE). The objective of our study was to estimate the influence of diurnal aerosol variability at the top of the atmosphere ADRE estimates. By including all the possible AERONET sites, we wanted to assess the influence on global ADRE estimates. While focusing also in more detail on some selected sites of strongest impact, our goal was to also see the possible impact regionally. We calculated ADRE with different assumptions about the daily AOD variability: taking the observed daily AOD cycle into account and assuming diurnally constant AOD. Moreover, we estimated the corresponding differences in ADREs, if the single AOD value for the daily mean was taken from the the Moderate Resolution Imaging Spectroradiometer (MODIS) Terra or Aqua overpass times, instead of accounting for the true observed daily variability. The mean impact of diurnal AOD variability on 24 h ADRE estimates, averaged over all AERONET sites, was rather small and it was relatively small even for the cases when AOD was chosen to correspond to the Terra or Aqua overpass time. This was true on average over all AERONET sites, while clearly there can be much stronger impact in individual sites. Examples of some selected sites demonstrated that the strongest observed AOD variability (the strongest morning afternoon contrast) does not typically result in a significant impact on 24 h ADRE. In those cases, the morning and afternoon AOD patterns are opposite and thus the impact on 24 h ADRE, when integrated over all solar zenith angles, is reduced. The most significant effect on daily ADRE was induced by AOD cycles with either maximum or minimum AOD close to local noon. In these cases, the impact on 24 h ADRE was typically around 0.1–0.2 W m−2 (both positive and negative) in absolute values, 5–10% in relative ones.


2013 ◽  
Vol 13 (4) ◽  
pp. 10327-10344 ◽  
Author(s):  
A. Arola ◽  
T. F. Eck ◽  
J. Huttunen ◽  
K. E. J. Lehtinen ◽  
A. V. Lindfors ◽  
...  

Abstract. The diurnal variability of aerosol optical depth (AOD) can be significant, depending on location and dominant aerosol type. However, these diurnal cycles have rarely been taken into account in measurement-based estimates of aerosol direct radiative forcing (ADRF) or aerosol direct radiative effect (ADRE). The objective of our study was to estimate the influence of diurnal aerosol variability on the top of the atmosphere ADRE estimates. By including all the possible AERONET sites, we wanted to assess the influence on global ADRE estimates, while by focusing also in more detail on some selected sites of strongest impact, our goal was to also see the possible impact regionally. We calculated ADRE with different assumptions about the daily AOD variability: taking the observed daily AOD cycle into account and assuming diurnally constant AOD. Moreover, we estimated the corresponding differences in ADREs, if the single AOD value for the daily mean was taken from the the Moderate Resolution Imaging Spectroradiometer (MODIS) Terra or Aqua overpass times, instead of accounting for the true observed daily variability. The mean impact of diurnal AOD variability on 24 h ADRE estimates, averaged over all AERONET sites, was rather small and it was relatively small even for the cases when AOD was chosen to correspond to the Terra or Aqua overpass time. This was true on average over all AERONET sites, while clearly there can be much stronger impact in individual sites. Examples of some selected sites demonstrated that the strongest observed AOD variability (the strongest morning afternoon contrast) does not typically result in a significant impact on 24 h ADRE. In those cases, the morning and afternoon AOD patterns are opposite and thus the impact on 24 h ADRE, when integrated over all solar zenith angles, is reduced. The most significant effect on daily ADRE was induced by AOD cycles with either maximum or minimum AOD close to local noon. In these cases, the impact on 24 h ADRE was typically around 0.1–0.2 W m−2 (both positive and negative).


2018 ◽  
Vol 115 (12) ◽  
pp. 2924-2929 ◽  
Author(s):  
Zheng Lu ◽  
Xiaohong Liu ◽  
Zhibo Zhang ◽  
Chun Zhao ◽  
Kerry Meyer ◽  
...  

Marine stratocumulus clouds cover nearly one-quarter of the ocean surface and thus play an extremely important role in determining the global radiative balance. The semipermanent marine stratocumulus deck over the southeastern Atlantic Ocean is of particular interest, because of its interactions with seasonal biomass burning aerosols that are emitted in southern Africa. Understanding the impacts of biomass burning aerosols on stratocumulus clouds and the implications for regional and global radiative balance is still very limited. Previous studies have focused on assessing the magnitude of the warming caused by solar scattering and absorption by biomass burning aerosols over stratocumulus (the direct radiative effect) or cloud adjustments to the direct radiative effect (the semidirect effect). Here, using a nested modeling approach in conjunction with observations from multiple satellites, we demonstrate that cloud condensation nuclei activated from biomass burning aerosols entrained into the stratocumulus (the microphysical effect) can play a dominant role in determining the total radiative forcing at the top of the atmosphere, compared with their direct and semidirect radiative effects. Biomass burning aerosols over the region and period with heavy loadings can cause a substantial cooling (daily mean −8.05 W m−2), primarily as a result of clouds brightening by reducing the cloud droplet size (the Twomey effect) and secondarily through modulating the diurnal cycle of cloud liquid water path and coverage (the cloud lifetime effect). Our results highlight the importance of realistically representing the interactions of stratocumulus with biomass burning aerosols in global climate models in this region.


2020 ◽  
Vol 16 (1) ◽  
pp. 1-14
Author(s):  
Monim Jiboori ◽  
Nadia Abed ◽  
Mohamed Abdel Wahab

2018 ◽  
Vol 11 (10) ◽  
pp. 5837-5864 ◽  
Author(s):  
Hiren Jethva ◽  
Omar Torres ◽  
Changwoo Ahn

Abstract. Aerosol–cloud interaction continues to be one of the leading uncertain components of climate models, primarily due to the lack of adequate knowledge of the complex microphysical and radiative processes of the aerosol–cloud system. Situations when light-absorbing aerosols such as carbonaceous particles and windblown dust overlay low-level cloud decks are commonly found in several regions of the world. Contrary to the known cooling effects of these aerosols in cloud-free scenario over darker surfaces, an overlapping situation of the absorbing aerosols over the cloud can lead to a significant level of atmospheric absorption exerting a positive radiative forcing (warming) at the top of the atmosphere. We contribute to this topic by introducing a new global product of above-cloud aerosol optical depth (ACAOD) of absorbing aerosols retrieved from the near-UV observations made by the Ozone Monitoring Instrument (OMI) onboard NASA's Aura platform. Physically based on an unambiguous “color ratio” effect in the near-UV caused by the aerosol absorption above the cloud, the OMACA (OMI above-cloud aerosols) algorithm simultaneously retrieves the optical depths of aerosols and clouds under a prescribed state of the atmosphere. The OMACA algorithm shares many similarities with the two-channel cloud-free OMAERUV algorithm, including the use of AIRS carbon monoxide for aerosol type identification, CALIOP-based aerosol layer height dataset, and an OMI-based surface albedo database. We present the algorithm architecture, inversion procedure, retrieval quality flags, initial validation results, and results from a 12-year long OMI record (2005–2016) including global climatology of the frequency of occurrence, ACAOD, and aerosol-corrected cloud optical depth. A comparative analysis of the OMACA-retrieved ACAOD, collocated with equivalent accurate measurements from the HSRL-2 lidar for the ORACLES Phase I operation (August–September 2016), revealed a good agreement (R = 0.77, RMSE = 0.10). The long-term OMACA record reveals several important regions of the world, where the carbonaceous aerosols from the seasonal biomass burning and mineral dust originated over the continents are found to overlie low-level cloud decks with moderate (0.3 < ACAOD < 0.5, away from the sources) to higher levels of ACAOD (> 0.8 in the proximity to the sources), including the southeastern Atlantic Ocean, southern Indian Ocean, Southeast Asia, the tropical Atlantic Ocean off the coast of western Africa, and northern Arabian sea. No significant long-term trend in the frequency of occurrence of aerosols above the clouds and ACAOD is noticed when OMI observations that are free from the “row anomaly” throughout the operation are considered. If not accounted for, the effects of aerosol absorption above the clouds introduce low bias in the retrieval of cloud optical depth with a profound impact on increasing ACAOD and cloud brightness. The OMACA aerosol product from OMI presented in this paper offers a crucial missing piece of information from the aerosol loading above cloud that will help us to quantify the radiative effects of clouds when overlaid with aerosols and their resultant impact on cloud properties and climate.


2019 ◽  
Vol 12 (9) ◽  
pp. 5087-5099 ◽  
Author(s):  
Jonathan K. P. Shonk ◽  
Jui-Yuan Christine Chiu ◽  
Alexander Marshak ◽  
David M. Giles ◽  
Chiung-Huei Huang ◽  
...  

Abstract. Clouds present many challenges to climate modelling. To develop and verify the parameterisations needed to allow climate models to represent cloud structure and processes, there is a need for high-quality observations of cloud optical depth from locations around the world. Retrievals of cloud optical depth are obtainable from radiances measured by Aerosol Robotic Network (AERONET) radiometers in “cloud mode” using a two-wavelength retrieval method. However, the method is unable to detect cloud phase, and hence assumes that all of the cloud in a profile is liquid. This assumption has the potential to introduce errors into long-term statistics of retrieved optical depth for clouds that also contain ice. Using a set of idealised cloud profiles we find that, for optical depths above 20, the fractional error in retrieved optical depth is a linear function of the fraction of the optical depth that is due to the presence of ice cloud (“ice fraction”). Clouds that are entirely ice have positive errors with magnitudes of the order of 55 % to 70 %. We derive a simple linear equation that can be used as a correction at AERONET sites where ice fraction can be independently estimated. Using this linear equation, we estimate the magnitude of the error for a set of cloud profiles from five sites of the Atmospheric Radiation Measurement programme. The dataset contains separate retrievals of ice and liquid retrievals; hence ice fraction can be estimated. The magnitude of the error at each location was related to the relative frequencies of occurrence in thick frontal cloud at the mid-latitude sites and of deep convection at the tropical sites – that is, of deep cloud containing both ice and liquid particles. The long-term mean optical depth error at the five locations spans the range 2–4, which we show to be small enough to allow calculation of top-of-atmosphere flux to within 10 % and surface flux to about 15 %.


2015 ◽  
Vol 15 (13) ◽  
pp. 7173-7193 ◽  
Author(s):  
A. Veira ◽  
S. Kloster ◽  
N. A. J. Schutgens ◽  
J. W. Kaiser

Abstract. Wildfires represent a major source for aerosols impacting atmospheric radiation, atmospheric chemistry and cloud micro-physical properties. Previous case studies indicated that the height of the aerosol–radiation interaction may crucially affect atmospheric radiation, but the sensitivity to emission heights has been examined with only a few models and is still uncertain. In this study we use the general circulation model ECHAM6 extended by the aerosol module HAM2 to investigate the impact of wildfire emission heights on atmospheric long-range transport, black carbon (BC) concentrations and atmospheric radiation. We simulate the wildfire aerosol release using either various versions of a semi-empirical plume height parametrization or prescribed standard emission heights in ECHAM6-HAM2. Extreme scenarios of near-surface or free-tropospheric-only injections provide lower and upper constraints on the emission height climate impact. We find relative changes in mean global atmospheric BC burden of up to 7.9±4.4 % caused by average changes in emission heights of 1.5–3.5 km. Regionally, changes in BC burden exceed 30–40 % in the major biomass burning regions. The model evaluation of aerosol optical thickness (AOT) against Moderate Resolution Imaging Spectroradiometer (MODIS), AErosol RObotic NETwork (AERONET) and Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) observations indicates that the implementation of a plume height parametrization slightly reduces the ECHAM6-HAM2 biases regionally, but on the global scale these improvements in model performance are small. For prescribed emission release at the surface, wildfire emissions entail a total sky top-of-atmosphere (TOA) radiative forcing (RF) of −0.16±0.06 W m−2. The application of a plume height parametrization which agrees reasonably well with observations introduces a slightly stronger negative TOA RF of −0.20±0.07 W m−2. The standard ECHAM6-HAM2 model in which 25 % of the wildfire emissions are injected into the free troposphere (FT) and 75 % into the planetary boundary layer (PBL), leads to a TOA RF of −0.24±0.06 W m−2. Overall, we conclude that simple plume height parametrizations provide sufficient representations of emission heights for global climate modeling. Significant improvements in aerosol wildfire modeling likely depend on better emission inventories and aerosol process modeling rather than on improved emission height parametrizations.


2012 ◽  
Vol 51 (7) ◽  
pp. 1407-1425 ◽  
Author(s):  
Anne Garnier ◽  
Jacques Pelon ◽  
Philippe Dubuisson ◽  
Michaël Faivre ◽  
Olivier Chomette ◽  
...  

AbstractThe paper describes the operational analysis of the Imaging Infrared Radiometer (IIR) data, which have been collected in the framework of the Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) mission for the purpose of retrieving high-altitude (above 7 km) cloud effective emissivity and optical depth that can be used in synergy with the vertically resolved Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) collocated observations. After an IIR scene classification is built under the CALIOP track, the analysis is applied to features detected by CALIOP when found alone in the atmospheric column or when CALIOP identifies an opaque layer underneath. The fast-calculation radiative transfer (FASRAD) model fed by ancillary meteorological and surface data is used to compute the different components involved in the effective emissivity retrievals under the CALIOP track. The track analysis is extended to the IIR swath using homogeneity criteria that are based on radiative equivalence. The effective optical depth at 12.05 μm is shown to be a good proxy for about one-half of the cloud optical depth, allowing direct comparisons with other databases in the visible spectrum. A step-by-step quantitative sensitivity and performance analysis is provided. The method is validated through comparisons of collocated IIR and CALIOP optical depths for elevated single-layered semitransparent cirrus clouds, showing excellent agreement (within 20%) for values ranging from 1 down to 0.05. Uncertainties have been determined from the identified error sources. The optical depth distribution of semitransparent clouds is found to have a nearly exponential shape with a mean value of about 0.5–0.6.


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