Climate and composition impacts of a net-zero anthropogenic methane future using an emissions-driven chemistry-climate model

Author(s):  
Zosia Staniaszek ◽  
Paul T. Griffiths ◽  
Gerd A. Folberth ◽  
Fiona M. O'Connor ◽  
Alexander T. Archibald

<div> <p>Methane (CH<sub>4</sub>), the second most important greenhouse gas in terms of radiative forcing, is on the rise; but there are extensive opportunities for mitigation with existing technologies. Anthropogenic emissions account for around 60% of the global methane source, and the recent atmospheric methane growth rate puts us on a trajectory comparable to the most extreme future methane scenarios in the sixth Coupled Model Intercomparison Project (CMIP6). </p> </div><div> <p>We use a new methane emissions-driven configuration of the UK Earth System Model (UKESM1) to explore the role of anthropogenic methane in the earth system. The full methane cycle is represented, including surface deposition, chemistry and interactive wetland emissions. As a baseline scenario we used Shared Socioeconomic Pathway 3-7.0 (SSP3-7.0) – the highest methane emissions scenario in CMIP6. In an idealised experiment, all anthropogenic methane emissions were instantaneously stopped from 2015 onwards in a coupled atmosphere-ocean simulation running from 2015-2050, to make a net-zero anthropogenic methane emissions scenario.  </p> </div><div> <p>Within a decade, significant changes can be seen in atmospheric composition and climate, compared to SSP3-7.0. The atmospheric methane burden declines to below pre-industrial levels within 12 years, and by the late 2030s reaches a constant level around 44% below that of the present day (2015). The tropospheric ozone burden and surface mean ozone concentrations decreased by 12% and 15% respectively by 2050 – key in terms of limiting global warming as well as improving air quality and human health. </p> </div><div> <p>By 2050 the net-zero anthropogenic methane scenario results in a global mean surface temperature (GMST) 1˚C lower than the baseline, a significant value in the context of climate goals such as the Paris Agreement. Through decomposition of the radiation budget, the change in climate can be directly attributed to the reduction in methane and indirectly to the resulting changes in ozone, clouds and ozone precursors such as CO. In addition, the changes in climate result in impacts on the interactive wetland emissions via changes in temperature and wetland extent, highlighting the coupled nature of methane in the earth system. </p> </div><div> <p>Cessation of anthropogenic methane emissions has profound impacts on near-term warming and on tropospheric ozone, but ultimately cannot single-handedly achieve the necessary reductions for meeting Paris goals. </p> </div>

2011 ◽  
Vol 11 (3) ◽  
pp. 8777-8799
Author(s):  
B. Barja ◽  
J. C. Antuña

Abstract. Cirrus clouds play a key role in the radiation budget of the Earth system. They are an important aspect in the climate system, as they interact with the atmospheric radiation field. They control both the solar radiation that reaches the Earth surface and the longwave radiation that leaves the Earth system. The feedback produced by cirrus clouds in climate is not well understood. Therefore it is necessary to improve the understanding and characterization of the radiative forcing of cirrus clouds. We analyze the effect of optically thin cirrus clouds characterized with the lidar technique in Camagüey, Cuba, on solar radiation, by numerical simulation. Nature and amplitude of the effect of cirrus clouds on solar radiation is evaluated. Cirrus clouds have a cooling effect in the solar spectrum at the Top of the Atmosphere (TOA) and at the surface (SFC). The daily mean value of solar cirrus cloud radiative forcing (SCRF) has an average value of −9.1 W m−2 at TOA and −5.6 W m−2 at SFC. The cirrus clouds also have a local heating effect on the atmospheric layer where they are located. Cirrus clouds have mean daily values of heating rates of 0.63 K day−1 with a range between 0.35 K day−1 and 1.24 K day−1. The principal effect is in the near infrared spectral band of the solar spectrum. There is a linear relation between SCRF and cirrus clouds optical depth (COD), with −30 W m−2 COD−1 and −26 W m−2 COD−1, values for the slopes of the fits at the TOA and SFC, respectively in the broadband solar spectrum. Also there is a relation between the solar zenith angle and cirrus clouds radiative forcing displayed in the diurnal cycle.


2009 ◽  
Vol 9 (2) ◽  
pp. 5505-5547 ◽  
Author(s):  
J. Joiner ◽  
M. R. Schoeberl ◽  
A. P. Vasilkov ◽  
L. Oreopoulos ◽  
S. Platnick ◽  
...  

Abstract. Estimates of the radiative forcing due to anthropogenically-produced tropospheric O3 are derived primarily from models. Here, we use tropospheric ozone and cloud data from several instruments in the A-train constellation of satellites as well as information from the GEOS-5 Data Assimilation System to accurately estimate the radiative effect of tropospheric O3 for January and July 2005. Since we cannot distinguish between natural and anthropogenic sources with the satellite data, our derived radiative effect reflects the unadjusted (instantaneous) effect of the total tropospheric O3 rather than the anthropogenic component. We improve upon previous estimates of tropospheric ozone mixing ratios from a residual approach using the NASA Earth Observing System (EOS) Aura Ozone Monitoring Instrument (OMI) and Microwave Limb Sounder (MLS) by incorporating cloud pressure information from OMI. We focus specifically on the magnitude and spatial structure of the cloud effect on both the short- and long-wave radiative budget. The estimates presented here can be used to evaluate the various aspects of model-generated radiative forcing. For example, our derived cloud impact is to reduce the radiative effect of tropospheric ozone by ~16%. This is centered within the published range of model-produced cloud effect on instantaneous radiative forcing.


Author(s):  
Marion Gehlen ◽  
Nicolas Gruber

By the year 2008, the ocean had taken up approximately 140 Gt carbon corresponding to about a third of the total anthropogenic CO2 emitted to the atmosphere since the onset of industrialization (Khatiwala et al. 2009 ). As the weak acid CO2 invades the ocean, it triggers changes in ocean carbonate chemistry and ocean pH (see Chapter 1). The pH of modern ocean surface waters is already 0.1 units lower than in pre-industrial times and a decrease by 0.4 units is projected by the year 2100 in response to a business-as- usual emission pathway (Caldeira and Wickett 2003). These changes in ocean carbonate chemistry are likely to affect major ocean biogeochemical cycles, either through direct pH effects or indirect impacts on the structure and functioning of marine ecosystems. This chapter addresses the potential biogeochemical consequences of ocean acidification and associated feedbacks to the earth system, with focus on the alteration of element fluxes at the scale of the global ocean. The view taken here is on how the different effects interact and ultimately alter the atmospheric concentration of radiatively active substances, i.e. primarily greenhouse gases such as CO2 and nitrous oxide (N2O). Changes in carbonate chemistry have the potential for interacting with ocean biogeochemical cycles and creating feedbacks to climate in a myriad of ways (Box 12.1). In order to provide some structure to the discussion, direct and indirect feedbacks of ocean acidification on the earth system are distinguished. Direct feedbacks are those which directly affect radiative forcing in the atmosphere by altering the air–sea flux of radiatively active substances. Indirect feedbacks are those that first alter a biogeochemical process in the ocean, and through this change then affect the air–sea flux and ultimately the radiative forcing in the atmosphere. For example, when ocean acidification alters the production and export of organic matter by the biological pump, then this is an indirect feedback. This is because a change in the biological pump alters radiative forcing in the atmosphere indirectly by first changing the nearsurface concentrations of dissolved inorganic carbon and total alkalinity.


2021 ◽  
Author(s):  
Ilona Riipinen ◽  
Annica Ekman ◽  
Matthew Salter ◽  
Karoliina Pulkkinen ◽  

<p>Together with imminent climate action, building a sustainable future for the humanity requires striving for healthier environments. Atmospheric aerosol particles (also referred to as particulate matter, PM) play a key role in defining the air that the future generations will breathe but also the climates they live in, PM being an important short-lived climate forcer but also a key component of air quality and global environmental health hazard. The contribution of aerosol particles has been a key uncertainty in estimates of the Earth’s radiative forcing since the establishment of the Intergovernmental Panel for Climate Change (IPCC) and still remains as the single largest quoted source of uncertainty in the anthropogenic climate forcing during the industrial period. In the latest assessment by the IPCC, the radiative forcing by aerosol particles has been estimated to be -0.45 W m-2 (between -0.95 and 0.05 W m-2) for aerosol-radiation interactions (RFari) and -0.45 W m-2 (between -1.25 and 0 W m-2) for aerosol-cloud interactions (RFaci). Recent reviews indicate no significant reduction in the uncertainty. The large range of possible aerosol forcing values has serious consequences for climate projections and therefore developing strategies for reaching Paris agreement targets. It is currently not possible to say if a reduction in aerosol emissions due to air pollution mitigation and a phase-out of aerosol emissions will result in a noticeable increase in global mean temperature  or in a negligible climate effect. We will discuss the components and reasons of this uncertainty, focusing on those that are important for aerosol-cloud interactions. We will identify critical bottlenecks in 1) scientific understanding of fundamental aerosol and cloud microphysical processes; 2) method development for improving the understanding of aerosol, cloud, and aerosol-cloud processes as well as their representation in Earth System Models (ESMs); and 3) knowledge transfer within and between the relevant research communities. We will argue for key actions to overcome these bottlenecks, giving examples of good practices for breaking new ground in this long-standing problem that continues to intrigue the atmospheric and climate science communities. Besides enhancing the scientific understanding of the Earth system within the realm of natural science based on multiple lines of evidence, and developing novel (e.g. machine learning –based) methodologies for analyzing existing observational data and model output, we call for additional perspectives from social science and humanities on the communication and knowledge transfer practices within atmospheric and climate research. Making the relevant knowledge transfer pathways and processes transparent is urgently needed to enable systematic determination of the actions required to maximally utilize the existing knowledge, and to ensure effective implementation of new results that may help to narrow down the uncertainty associated with aerosols in climate projections. Improved understanding of the role of aerosols in the climate system will result in enhanced credibility of ESMs and hence also tighter constraints for policies aiming for simultaneous climate neutrality and zero pollution targets.</p>


2013 ◽  
Vol 17 (7) ◽  
pp. 2873-2892 ◽  
Author(s):  
A. Kleidon ◽  
M. Renner

Abstract. The hydrologic cycle results from the combination of energy conversions and atmospheric transport, and the laws of thermodynamics set limits to both. Here, we apply thermodynamics to derive the limits of the strength of hydrologic cycling within the Earth system and about the properties and processes that shape these limits. We set up simple models to derive analytical expressions of the limits of evaporation and precipitation in relation to vertical and horizontal differences in solar radiative forcing. These limits result from a fundamental trade-off by which a greater evaporation rate reduces the temperature gradient and thus the driver for atmospheric motion that exchanges moistened air from the surface with the drier air aloft. The limits on hydrologic cycling thus reflect the strong interaction between the hydrologic flux, motion, and the driving gradient. Despite the simplicity of the models, they yield estimates for the limits of hydrologic cycling that are within the observed magnitude, suggesting that the global hydrologic cycle operates near its maximum strength. We close with a discussion of how thermodynamic limits can provide a better characterization of the interaction of vegetation and human activity with hydrologic cycling.


2020 ◽  
Author(s):  
Benjamin Sanderson

Abstract. Cumulative emissions budgets and net-zero emission target dates are often used to frame climate negotiations (Frameet al., 2014; Millar et al., 2016; Van Vuuren et al., 2016; Rogelj et al., 2015b; Matthews et al., 2012). However, their utilityfor near-term policy decisions is confounded by an uncertainties in future negative emissions capacity (Fuss et al., 2014; Smith et al., 2016; Larkin et al., 2018; Anderson and Peters, 2016) and in long term Earth System response to climate forcers(Rugenstein et al., 2019; Knutti et al., 2017; Armour, 2017) which may impact the utility of an indefinite carbon budget if peak temperatures occur significantly after net zero emissions are achieved, the likelihood of which in a simple model is conditionalon prior assumptions about the long term dynamics of the Earth System. Here we illustrate that the risks associated with nearterm positive emissions can be framed using a definite cumulative emissions budget with a 2040 time horizon, allowing thenecessity and scope for negative emissions deployment later in the century to be better informed by observed warming overcoming decades.


Science ◽  
1989 ◽  
Vol 243 (4887) ◽  
pp. 57-63 ◽  
Author(s):  
V. RAMANATHAN ◽  
R. D. CESS ◽  
E. F. HARRISON ◽  
P. MINNIS ◽  
B. R. BARKSTROM ◽  
...  

2020 ◽  
Vol 3 (1) ◽  
Author(s):  
Dantong Liu ◽  
Cenlin He ◽  
Joshua P. Schwarz ◽  
Xuan Wang

Abstract Light-absorbing carbonaceous aerosols (LACs), including black carbon and light-absorbing organic carbon (brown carbon, BrC), have an important role in the Earth system via heating the atmosphere, dimming the surface, modifying the dynamics, reducing snow/ice albedo, and exerting positive radiative forcing. The lifecycle of LACs, from emission to atmospheric evolution further to deposition, is key to their overall climate impacts and uncertainties in determining their hygroscopic and optical properties, atmospheric burden, interactions with clouds, and deposition on the snowpack. At present, direct observations constraining some key processes during the lifecycle of LACs (e.g., interactions between LACs and hydrometeors) are rather limited. Large inconsistencies between directly measured LAC properties and those used for model evaluations also exist. Modern models are starting to incorporate detailed aerosol microphysics to evaluate transformation rates of water solubility, chemical composition, optical properties, and phases of LACs, which have shown improved model performance. However, process-level understanding and modeling are still poor particularly for BrC, and yet to be sufficiently assessed due to lack of global-scale direct measurements. Appropriate treatments of size- and composition-resolved processes that influence both LAC microphysics and aerosol–cloud interactions are expected to advance the quantification of aerosol light absorption and climate impacts in the Earth system. This review summarizes recent advances and up-to-date knowledge on key processes during the lifecycle of LACs, highlighting the essential issues where measurements and modeling need improvement.


2017 ◽  
Vol 114 (13) ◽  
pp. E2571-E2579 ◽  
Author(s):  
Gareth Izon ◽  
Aubrey L. Zerkle ◽  
Kenneth H. Williford ◽  
James Farquhar ◽  
Simon W. Poulton ◽  
...  

Emerging evidence suggests that atmospheric oxygen may have varied before rising irreversibly ∼2.4 billion years ago, during the Great Oxidation Event (GOE). Significantly, however, pre-GOE atmospheric aberrations toward more reducing conditions—featuring a methane-derived organic-haze—have recently been suggested, yet their occurrence, causes, and significance remain underexplored. To examine the role of haze formation in Earth’s history, we targeted an episode of inferred haze development. Our redox-controlled (Fe-speciation) carbon- and sulfur-isotope record reveals sustained systematic stratigraphic covariance, precluding nonatmospheric explanations. Photochemical models corroborate this inference, showing Δ36S/Δ33S ratios are sensitive to the presence of haze. Exploiting existing age constraints, we estimate that organic haze developed rapidly, stabilizing within ∼0.3 ± 0.1 million years (Myr), and persisted for upward of ∼1.4 ± 0.4 Myr. Given these temporal constraints, and the elevated atmospheric CO2 concentrations in the Archean, the sustained methane fluxes necessary for haze formation can only be reconciled with a biological source. Correlative δ13COrg and total organic carbon measurements support the interpretation that atmospheric haze was a transient response of the biosphere to increased nutrient availability, with methane fluxes controlled by the relative availability of organic carbon and sulfate. Elevated atmospheric methane concentrations during haze episodes would have expedited planetary hydrogen loss, with a single episode of haze development providing up to 2.6–18 × 1018 moles of O2 equivalents to the Earth system. Our findings suggest the Neoarchean likely represented a unique state of the Earth system where haze development played a pivotal role in planetary oxidation, hastening the contingent biological innovations that followed.


2004 ◽  
Vol 4 (6) ◽  
pp. 8471-8538 ◽  
Author(s):  
F. Dentener ◽  
D. Stevenson ◽  
J. Cofala ◽  
R. Mechler ◽  
M. Amann ◽  
...  

Abstract. To explore the relationship between tropospheric ozone and radiative forcing with changing emissions, we compiled two sets of global scenarios for the emissions of the ozone precursors methane (CH4), carbon monoxide (CO), non-methane volatile organic compounds (NMVOC) and nitrogen oxides (NOx) up to the year 2030 and implemented them in two global Chemistry Transport Models. The "Current Legislation" (CLE) scenario reflects the current perspectives of individual countries on future economic development and takes the anticipated effects of presently decided emission control legislation in the individual countries into account. In addition, we developed a "Maximum technically Feasible Reduction" (MFR) scenario that outlines the scope for emission reductions offered by full implementation of the presently available emission control technologies, while maintaining the projected levels of anthropogenic activities. Whereas the resulting projections of methane emissions lie within the range suggested by other greenhouse gas projections, the recent pollution control legislation of many Asian countries, requiring introduction of catalytic converters for vehicles, leads to significantly lower growth in emissions of the air pollutants NOx, NMVOC and CO than was suggested by the widely used IPCC (Intergovernmental Panel on Climate Change) SRES (Special Report on Emission Scenarios) scenarios (Nakicenovic et al., 2000). With the TM3 and STOCHEM models we performed several long-term integrations (1990–2030) to assess global, hemispheric and regional changes in CH4, CO, hydroxyl radicals, ozone and the radiative climate forcings resulting from these two emission scenarios. Both models reproduce realistically the observed trends in background ozone, CO, and CH4 concentrations from 1990 to 2002. For the "current legislation" case, both models indicate an increase of the annual average ozone levels in the Northern hemisphere by 5 ppbv, and up to 15 ppbv over the Indian sub-continent, comparing the 2020s with the 1990s. The corresponding higher ozone and methane burdens in the atmosphere increase radiative forcing by approximately 0.2 Wm−2. Full application of today's emissions control technologies, however, would bring down ozone below the levels experienced in the 1990s and would reduce the current radiative forcing of ozone and methane by approximately 0.1Wm−2. While methane reductions lead to lower ozone burdens and to less radiative forcing, further reductions of the air pollutants NO4 and NMVOC result in lower ozone, but at the same time increase the lifetime of methane. Control of methane emissions appears an efficient option to reduce tropospheric ozone as well as radiative forcing.


Sign in / Sign up

Export Citation Format

Share Document