scholarly journals Simulation of tropospheric chemistry and aerosols with the climate model EC-Earth

2014 ◽  
Vol 7 (2) ◽  
pp. 1933-2006 ◽  
Author(s):  
T. P. C. van Noije ◽  
P. Le Sager ◽  
A. J. Segers ◽  
P. F. J. van Velthoven ◽  
M. C. Krol ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Atmospheric Chemistry ◽  
General Circulation ◽  
Data Exchange ◽  
Climate Model ◽  
Global Climate Model ◽  
Surface Ozone ◽  
Circulation Model ◽  
Tropospheric Chemistry

Abstract. We have integrated the atmospheric chemistry and transport model TM5 into the global climate model EC-Earth version 2.4. We present an overview of the TM5 model and the two-way data exchange between TM5 and the integrated forecasting system (IFS) model from the European Centre for Medium-Range Weather Forecasts (ECMWF), the atmospheric general circulation model of EC-Earth. In this paper we evaluate the simulation of tropospheric chemistry and aerosols in a one-way coupled configuration. We have carried out a decadal simulation for present-day conditions and calculated chemical budgets and climatologies of tracer concentrations and aerosol optical depth. For comparison we have also performed offline simulations driven by meteorological fields from ECMWF's ERA-Interim reanalysis and output from the EC-Earth model itself. Compared to the offline simulations, the online-coupled system produces more efficient vertical mixing in the troposphere, which likely reflects an improvement of the treatment of cumulus convection. The chemistry in the EC-Earth simulations is affected by the fact that the current version of EC-Earth produces a cold bias with too dry air in large parts of the troposphere. Compared to the ERA-Interim driven simulation, the oxidizing capacity in EC-Earth is lower in the tropics and higher in the extratropics. The methane lifetime is 7% higher in EC-Earth, but remains well within the range reported in the literature. We evaluate the model by comparing the simulated climatologies of surface carbon monoxide, tropospheric and surface ozone, and aerosol optical depth against observational data. The work presented in this study is the first step in the development of EC-Earth into an Earth system model with fully interactive atmospheric chemistry and aerosols.

scholarly journals Simulation of tropospheric chemistry and aerosols with the climate model EC-Earth

2014 ◽  
Vol 7 (5) ◽  
pp. 2435-2475 ◽  
Author(s):  
T. P. C. van Noije ◽  
P. Le Sager ◽  
A. J. Segers ◽  
P. F. J. van Velthoven ◽  
M. C. Krol ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Atmospheric Chemistry ◽  
General Circulation ◽  
Data Exchange ◽  
Climate Model ◽  
Global Climate Model ◽  
Surface Ozone ◽  
Circulation Model ◽  
Tropospheric Chemistry

Abstract. We have integrated the atmospheric chemistry and transport model TM5 into the global climate model EC-Earth version 2.4. We present an overview of the TM5 model and the two-way data exchange between TM5 and the IFS model from the European Centre for Medium-Range Weather Forecasts (ECMWF), the atmospheric general circulation model of EC-Earth. In this paper we evaluate the simulation of tropospheric chemistry and aerosols in a one-way coupled configuration. We have carried out a decadal simulation for present-day conditions and calculated chemical budgets and climatologies of tracer concentrations and aerosol optical depth. For comparison we have also performed offline simulations driven by meteorological fields from ECMWF's ERA-Interim reanalysis and output from the EC-Earth model itself. Compared to the offline simulations, the online-coupled system produces more efficient vertical mixing in the troposphere, which reflects an improvement of the treatment of cumulus convection. The chemistry in the EC-Earth simulations is affected by the fact that the current version of EC-Earth produces a cold bias with too dry air in large parts of the troposphere. Compared to the ERA-Interim driven simulation, the oxidizing capacity in EC-Earth is lower in the tropics and higher in the extratropics. The atmospheric lifetime of methane in EC-Earth is 9.4 years, which is 7% longer than the lifetime obtained with ERA-Interim but remains well within the range reported in the literature. We further evaluate the model by comparing the simulated climatologies of surface radon-222 and carbon monoxide, tropospheric and surface ozone, and aerosol optical depth against observational data. The work presented in this study is the first step in the development of EC-Earth into an Earth system model with fully interactive atmospheric chemistry and aerosols.

scholarly journals Interpreting the cloud cover – aerosol optical depth relationship found in satellite data using a general circulation model

2010 ◽  
Vol 10 (13) ◽  
pp. 6129-6135 ◽  
Author(s):  
J. Quaas ◽  
B. Stevens ◽  
P. Stier ◽  
U. Lohmann
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Satellite Data ◽  
General Circulation ◽  
Cloud Cover ◽  
Climate Model ◽  
Circulation Model ◽  
Total Cloud Cover ◽  
Positive Correlation ◽  
Depth Relationship

Abstract. Statistical analysis of satellite data shows a positive correlation between aerosol optical depth (AOD) and total cloud cover (TCC). Reasons for this relationship have been disputed in recent literature. The aim of this study is to explore how different processes contribute to one model's analog of the positive correlation between aerosol optical depth and total cloud cover seen in the satellite retrievals. We compare the slope of the linear regression between the logarithm of TCC and the logarithm of AOD, or the strength of the relationship, as derived from three satellite data sets to the ones simulated by a global aerosol-climate model. We analyse model results from two different simulations with and without a parameterisation of aerosol indirect effects, and using dry compared to humidified AOD. Perhaps not surprisingly we find that no single one of the hypotheses discussed in the literature is able to uniquely explain the positive relationship. However the dominant contribution to the model's AOD-TCC relationship can be attributed to aerosol swelling in regions where humidity is high and clouds are coincidentally found. This finding leads us to hypothesise that much of the AOD-TCC relationship seen in the satellite data is also carried by such a process, rather than the direct effects of the aerosols on the cloud fields themselves.

scholarly journals Interpreting the cloud cover – aerosol optical depth relationship found in satellite data using a general circulation model

2009 ◽  
Vol 9 (6) ◽  
pp. 26013-26027 ◽  
Author(s):  
J. Quaas ◽  
B. Stevens ◽  
P. Stier ◽  
U. Lohmann
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Satellite Data ◽  
General Circulation ◽  
Cloud Cover ◽  
Positive Relationship ◽  
Climate Model ◽  
Circulation Model ◽  
Data Sets ◽  
Depth Relationship

Abstract. Statistical analysis of satellite data shows a positive correlation between aerosol optical depth (AOD) and total cloud cover (TCC). Here we compare the slope of the linear regression between the logarithm of TCC and the logarithm of AOD, or the strength of the relationship, as derived from three satellite data sets to the ones simulated by a global aerosol-climate model. We analyze model results from two different simulations with and without a parameterization of aerosol indirect effects, and using dry compared to humidified AOD. We find that none of the hypotheses discussed in the literature is able to uniquely explain the positive relationship. The most important contribution in the model is from the swelling of aerosol in the vicinity of clouds, where relative humidity is high. The model also shows contribution of the aerosol cloud lifetime effect to the positive relationship, which, however, is of lesser importance.

Aerosol Radiative Forcing and Forcing Efficiency in the UVB for Regions Affected by Saharan and Asian Mineral Dust

2009 ◽  
Vol 66 (4) ◽  
pp. 1033-1040 ◽  
Author(s):  
O. E. García ◽  
A. M. Díaz ◽  
F. J. Expósito ◽  
J. P. Díaz ◽  
A. Redondas ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Radiative Forcing ◽  
Climate Model ◽  
Mineral Dust ◽  
Global Climate ◽  
Global Climate Model ◽  
Aerosol Radiative Forcing ◽  
Benchmark Database ◽  
Aerosol Radiative

Abstract The influence of mineral dust on ultraviolet energy transfer is studied for two different mineralogical origins. The aerosol radiative forcing ΔF and the forcing efficiency at the surface ΔFeff in the range 290–325 nm were estimated in ground-based stations affected by the Saharan and Asian deserts during the dusty seasons. UVB solar measurements were taken from the World Ozone and Ultraviolet Data Center (WOUDC) for four Asian stations (2000–04) and from the Santa Cruz Observatory, Canary Islands (2002–03), under Gobi and Sahara Desert influences, respectively. The Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol optical depth at 550 nm was used to characterize the aerosol load τ, whereas the aerosol index provided by the Total Ozone Mapping Spectrometer (TOMS) sensor was employed to identify the mineral dust events. The ΔF is strongly affected by the aerosol load, the values found being comparable in both regions during the dusty seasons. Under those conditions, ΔF values as large as −1.29 ± 0.53 W m−2 (τ550 = 0.48 ± 0.24) and −1.43 ± 0.38 W m−2 (τ550 = 0.54 ± 0.26) were reached under Saharan and Asian dust conditions, respectively. Nevertheless, significant differences have been observed in the aerosol radiative forcing per unit of aerosol optical depth in the slant path, τS. The maximum ΔFeff values associated with dust influences were −1.55 ± 0.20 W m−2 τS550−1 for the Saharan region and −0.95 ± 0.11 W m−2 τS550−1 in the Asian area. These results may be used as a benchmark database for establishing aerosol corrections in UV satellite products or in global climate model estimations.

scholarly journals Preindustrial-to-present-day radiative forcing by tropospheric ozone from improved simulations with the GISS chemistry-climate GCM

2003 ◽  
Vol 3 (5) ◽  
pp. 1675-1702 ◽  
Author(s):  
D. T. Shindell ◽  
G. Faluvegi ◽  
N. Bell
Keyword(s):  
Tropospheric Ozone ◽  
Radiative Forcing ◽  
General Circulation ◽  
Climate Model ◽  
Circulation Model ◽  
Tropospheric Chemistry ◽  
True Value ◽  
Tropopause Region ◽  
Dynamics Simulations ◽  
Goddard Institute

Abstract. Improved estimates of the radiative forcing from tropospheric ozone increases since the preindustrial have been calculated with the tropospheric chemistry model used at the Goddard Institute for Space Studies (GISS) within the GISS general circulation model (GCM). The chemistry in this model has been expanded to include simplified representations of peroxyacetylnitrates and non-methane hydrocarbons in addition to background NOx-HOx-Ox-CO-CH4 chemistry. The GCM has improved resolution and physics in the boundary layer, improved resolution near the tropopause, and now contains a full representation of stratospheric dynamics. Simulations of present-day conditions show that this coupled chemistry-climate model is better able to reproduce observed tropospheric ozone, especially in the tropopause region, which is critical to climate forcing. Comparison with preindustrial simulations gives a global annual average radiative forcing due to tropospheric ozone increases of 0.30 W/m2 with standard assumptions for preindustrial emissions. Locally, the forcing reaches more than 0.8 W/m2 in parts of the northern subtropics during spring and summer, and is more than 0.6 W/m2 through nearly all the Northern subtropics and mid-latitudes during summer. An alternative preindustrial simulation with soil NOx emissions reduced by two-thirds and emissions of isoprene, paraffins and alkenes from vegetation increased by 50% gives a forcing of 0.33 W/m2. Given the large uncertainties in preindustrial ozone amounts, the true value may lie well outside this range.

scholarly journals Composite Analysis of Winter Cyclones in a GCM: Influence on Climatological Humidity

2006 ◽  
Vol 19 (9) ◽  
pp. 1652-1672 ◽  
Author(s):  
Mike Bauer ◽  
Anthony D. Del Genio
Keyword(s):  
Water Vapor ◽  
General Circulation ◽  
Climate Model ◽  
Global Climate ◽  
Global Climate Model ◽  
Circulation Model ◽  
Cloud Properties ◽  
Frontal Zones ◽  
Goddard Institute ◽  
Ageostrophic Circulation

Abstract The role of midlatitude baroclinic cyclones in maintaining the extratropical winter distribution of water vapor in an operational global climate model is investigated. A cyclone identification and tracking algorithm is used to compare the frequency of occurrence, propagation characteristics, and composite structure of 10 winters of storms in the Goddard Institute for Space Studies general circulation model (GCM) and in two reanalysis products. Cyclones are the major dynamical source of water vapor over the extratropical oceans in the reanalyses. The GCM produces fewer, generally weaker, and slower-moving cyclones than the reanalyses and is especially deficient in storms associated with secondary cyclogenesis. Composite fields show that GCM cyclones are shallower and drier aloft than those in the reanalyses and that their vertical structure is less tilted in the frontal region because of the GCM’s weaker ageostrophic circulation. This is consistent with the GCM’s underprediction of midlatitude cirrus. The GCM deficiencies do not appear to be primarily due to parameterization errors; the model is too dry despite producing less storm precipitation than is present in the reanalyses and in an experimental satellite precipitation dataset, and the weakness and shallow structure of GCM cyclones is already present at storm onset. These shortcomings may be common to most climate GCMs that do not resolve the mesoscale structure of frontal zones, and this may account for some universal problems in climate GCM midlatitude cloud properties.

scholarly journals Development cycle 2 of the Modular Earth Submodel System (MESSy2)

2010 ◽  
Vol 3 (2) ◽  
pp. 717-752 ◽  
Author(s):  
P. Jöckel ◽  
A. Kerkweg ◽  
A. Pozzer ◽  
R. Sander ◽  
H. Tost ◽  
...  
Keyword(s):  
Atmospheric Chemistry ◽  
General Circulation ◽  
Atmospheric General Circulation Model ◽  
Climate Model ◽  
Circulation Model ◽  
Second Development ◽  
Development Cycle ◽  
Climate Simulations ◽  
Diagnostic Capabilities ◽  
Earth System Models

Abstract. The Modular Earth Submodel System (MESSy) is an open, multi-institutional project providing a strategy for developing comprehensive Earth System Models (ESMs) with highly flexible complexity. The first version of the MESSy infrastructure and process submodels, mainly focusing on atmospheric chemistry, has been successfully coupled to an atmospheric General Circulation Model (GCM) expanding it into an Atmospheric Chemistry GCM (AC-GCM) for nudged simulations and into a Chemistry Climate Model (CCM) for climate simulations. Here, we present the second development cycle of MESSy, which comprises (1) an improved and extended infrastructure for the basemodel independent coupling of process-submodels, (2) new, highly valuable diagnostic capabilities for the evaluation with observational data and (3) an improved atmospheric chemistry setup. With the infrastructural changes, we place the headstone for further model extensions from a CCM towards a comprehensive ESM. The new diagnostic submodels will be used for regular re-evaluations of the continuously further developing model system. The updates of the chemistry setup are briefly evaluated.

scholarly journals Evaluation of CLaMS, KASIMA and ECHAM5/MESSy1 simulations in the lower stratosphere using observations of Odin/SMR and ILAS/ILAS-II

2009 ◽  
Vol 9 (1) ◽  
pp. 1977-2020
Author(s):  
F. Khosrawi ◽  
R. Müller ◽  
M. H. Proffitt ◽  
R. Ruhnke ◽  
O. Kirner ◽  
...  
Keyword(s):  
Atmospheric Chemistry ◽  
General Circulation ◽  
Lower Stratosphere ◽  
Climate Model ◽  
Middle Atmosphere ◽  
Circulation Model ◽  
Lagrangian Model ◽  
Data Sets ◽  
Data Set ◽  
The Impact

Abstract. 1-year data sets of monthly averaged nitrous oxide (N2O) and ozone (O3) derived from satellite measurements were used as a tool for the evaluation of atmospheric photochemical models. Two 1-year data sets, one derived from the Improved Limb Atmospheric Spectrometer (ILAS and ILAS-II) and one from the Odin Sub-Millimetre Radiometer (Odin/SMR) were employed. Here, these data sets are used for the evaluation of two Chemical Transport Models (CTMs), the Karlsruhe Simulation Model of the Middle Atmosphere (KASIMA) and the Chemical Lagrangian Model of the Stratosphere (CLaMS) as well as for one Chemistry-Climate Model (CCM), the atmospheric chemistry general circulation model ECHAM5/MESSy1 (E5M1) in the lower stratosphere with focus on the Northern Hemisphere. Since the Odin/SMR measurements cover the entire hemisphere, the evaluation is performed for the entire hemisphere as well as for the low latitudes, midlatitudes and high latitudes using the Odin/SMR 1-year data set as reference. To assess the impact of using different data sets for such an evaluation study we repeat the evaluation for the polar lower stratosphere using the ILAS/ILAS-II data set. Only small differences were found using ILAS/ILAS-II instead of Odin/SMR as a reference, thus, showing that the results are not influenced by the particular satellite data set used for the evaluation. The evaluation of CLaMS, KASIMA and E5M1 shows that all models are in good agreement with Odin/SMR and ILAS/ILAS-II. Differences are generally in the range of ±20%. Larger differences (up to −40%) are found in all models at 500±25 K for N2O mixing ratios greater than 200 ppb. Generally, the largest differences were found for the tropics and the lowest for the polar regions. However, an underestimation of polar winter ozone loss was found both in KASIMA and E5M1 both in the Northern and Southern Hemisphere.

scholarly journals The influence of the vertical distribution of emissions on tropospheric chemistry

2009 ◽  
Vol 9 (4) ◽  
pp. 16051-16083
Author(s):  
A. Pozzer ◽  
P. Jöckel ◽  
J. Van Aardenne
Keyword(s):  
Vertical Distribution ◽  
Atmospheric Chemistry ◽  
General Circulation ◽  
Circulation Model ◽  
Tropospheric Chemistry ◽  
Aircraft Observations ◽  
Field Campaigns ◽  
The Vertical Distribution ◽  
Lower Correlation ◽  
Model Layer

Abstract. The atmospheric chemistry general circulation model EMAC (ECHAM5/MESSy atmospheric chemistry) is used to investigate the effect of height dependent emissions on tropospheric chemistry. In a sensitivity simulation, anthropogenic and biomass burning emissions are released in the lowest model layer. The resulting tracer distributions are compared to those of a former simulation applying height dependent emissions. Although the differences between the two simulations in the free troposphere are small (less than 5%), large differences are present in polluted regions at the surface, in particular for NOx (more than 100%) and non-methane hydrocarbons (up to 30%), whereas for OH the differences at the same locations are somewhat lower (15%). Global ozone formation is virtually unaffected by the choice of the vertical distribution of emissions. Nevertheless, local ozone changes can be up to 30%. Model results of both simulations are further compared to observations from field campaigns and to data from measurement stations. The two simulations show no significant differences when compared to aircraft observations. In contrast, for measurements from surface stations, the simulation with emissions in the lowest model layer gives a 20% lower correlation to the observations compared to the simulation with height dependent emissions.

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