scholarly journals Development of prognostic aerosol–cloud interactions combining a chemistry transport model and a regional climate model

2015 ◽  
Vol 8 (2) ◽  
pp. 897-933
Author(s):  
M. A. Thomas ◽  
M. Kahnert ◽  
C. Andersson ◽  
H. Kokkola ◽  
U. Hansson ◽  
...  

Abstract. To reduce uncertainties and hence, to obtain a better estimate of aerosol (direct and indirect) radiative forcing, next generation climate models aim for a tighter coupling between chemistry transport models and regional climate models and a better representation of aerosol–cloud interactions. In this study, this coupling is done by first forcing the Rossby Center regional climate model, RCA4 by ERA-Interim lateral boundaries (LBCs) and SST using the standard CDNC (cloud droplet number concentration) formulation (hereafter, referred to as the "stand-alone RCA4 version" or "CTRL" simulation). In this simulation, the CDNCs are assigned fixed numbers based on if the underlying surface is land or oceanic. The meteorology from this simulation is then used to drive the chemistry transport model, MATCH which is coupled online with the aerosol dynamics model, SALSA. CDNC fields obtained from MATCH-SALSA are then fed back into a new RCA4 simulation. In this new simulation (referred to as "MOD" simulation), all parameters remain the same as in the first run except for the CDNCs provided by MATCH-SALSA. Simulations are carried out with this model set up for the period 2005–2012 over Europe and the differences in cloud microphysical properties and radiative fluxes as a result of local CDNC changes and possible model responses are analyzed. Our study shows substantial improvements in the cloud microphysical properties with the input of the MATCH-SALSA derived 3-D CDNCs compared to the stand-alone RCA4 version. This model set up improves the spatial, seasonal and vertical distribution of CDNCs with higher concentration observed over central Europe during summer half of the year and over Eastern Europe and Russia during the winter half of the year. Realistic cloud droplet radii (CD radii) values have been simulated with the maxima reaching 13 μm whereas in the stand-alone version, the values reached only 5 μm. A substantial improvement in the distribution of cloud liquid water path was observed when compared to the satellite retrievals from MODIS for the boreal summer months. The median and SD values from the "MOD" simulation are closer to observations than those obtained using the stand-alone RCA4 version. These changes resulted in a significant decrease in the total annual mean net fluxes at the top of the atmosphere (TOA) by −5 W m−2 over the domain selected in the study. The TOA net fluxes from the "MOD" simulation show a better agreement with the retrievals from CERES instrument. The aerosol indirect effects are evaluated based on 1900 emissions. Our simulations estimated the domain averaged annual mean total radiative forcing of −0.64 W m−2 with larger contribution from the first indirect aerosol effect than from the second indirect aerosol effect.

2015 ◽  
Vol 8 (6) ◽  
pp. 1885-1898 ◽  
Author(s):  
M. A. Thomas ◽  
M. Kahnert ◽  
C. Andersson ◽  
H. Kokkola ◽  
U. Hansson ◽  
...  

Abstract. To reduce uncertainties and hence to obtain a better estimate of aerosol (direct and indirect) radiative forcing, next generation climate models aim for a tighter coupling between chemistry transport models and regional climate models and a better representation of aerosol–cloud interactions. In this study, this coupling is done by first forcing the Rossby Center regional climate model (RCA4) with ERA-Interim lateral boundaries and sea surface temperature (SST) using the standard cloud droplet number concentration (CDNC) formulation (hereafter, referred to as the "stand-alone RCA4 version" or "CTRL" simulation). In the stand-alone RCA4 version, CDNCs are constants distinguishing only between land and ocean surface. The meteorology from this simulation is then used to drive the chemistry transport model, Multiple-scale Atmospheric Transport and Chemistry (MATCH), which is coupled online with the aerosol dynamics model, Sectional Aerosol module for Large Scale Applications (SALSA). CDNC fields obtained from MATCH–SALSA are then fed back into a new RCA4 simulation. In this new simulation (referred to as "MOD" simulation), all parameters remain the same as in the first run except for the CDNCs provided by MATCH–SALSA. Simulations are carried out with this model setup for the period 2005–2012 over Europe, and the differences in cloud microphysical properties and radiative fluxes as a result of local CDNC changes and possible model responses are analysed. Our study shows substantial improvements in cloud microphysical properties with the input of the MATCH–SALSA derived 3-D CDNCs compared to the stand-alone RCA4 version. This model setup improves the spatial, seasonal and vertical distribution of CDNCs with a higher concentration observed over central Europe during boreal summer (JJA) and over eastern Europe and Russia during winter (DJF). Realistic cloud droplet radii (CD radii) values have been simulated with the maxima reaching 13 μm, whereas in the stand-alone version the values reached only 5 μm. A substantial improvement in the distribution of the cloud liquid-water paths (CLWP) was observed when compared to the satellite retrievals from the Moderate Resolution Imaging Spectroradiometer (MODIS) for the boreal summer months. The median and standard deviation values from the "MOD" simulation are closer to observations than those obtained using the stand-alone RCA4 version. These changes resulted in a significant decrease in the total annual mean net fluxes at the top of the atmosphere (TOA) by −5 W m−2 over the domain selected in the study. The TOA net fluxes from the "MOD" simulation show a better agreement with the retrievals from the Clouds and the Earth's Radiant Energy System (CERES) instrument. The aerosol indirect effects are estimated in the "MOD" simulation in comparison to the pre-industrial aerosol emissions (1900). Our simulations estimated the domain averaged annual mean total radiative forcing of −0.64 W m−2 with a larger contribution from the first indirect aerosol effect (−0.57 W m−2) than from the second indirect aerosol effect (−0.14 W m−2).


2017 ◽  
Vol 13 (8) ◽  
pp. 1037-1048 ◽  
Author(s):  
Henrik Carlson ◽  
Rodrigo Caballero

Abstract. Recent work in modelling the warm climates of the early Eocene shows that it is possible to obtain a reasonable global match between model surface temperature and proxy reconstructions, but only by using extremely high atmospheric CO2 concentrations or more modest CO2 levels complemented by a reduction in global cloud albedo. Understanding the mix of radiative forcing that gave rise to Eocene warmth has important implications for constraining Earth's climate sensitivity, but progress in this direction is hampered by the lack of direct proxy constraints on cloud properties. Here, we explore the potential for distinguishing among different radiative forcing scenarios via their impact on regional climate changes. We do this by comparing climate model simulations of two end-member scenarios: one in which the climate is warmed entirely by CO2 (which we refer to as the greenhouse gas (GHG) scenario) and another in which it is warmed entirely by reduced cloud albedo (which we refer to as the low CO2–thin clouds or LCTC scenario) . The two simulations have an almost identical global-mean surface temperature and equator-to-pole temperature difference, but the LCTC scenario has  ∼  11 % greater global-mean precipitation than the GHG scenario. The LCTC scenario also has cooler midlatitude continents and warmer oceans than the GHG scenario and a tropical climate which is significantly more El Niño-like. Extremely high warm-season temperatures in the subtropics are mitigated in the LCTC scenario, while cool-season temperatures are lower at all latitudes. These changes appear large enough to motivate further, more detailed study using other climate models and a more realistic set of modelling assumptions.


2017 ◽  
Author(s):  
Daniel T. McCoy ◽  
Paul R. Field ◽  
Anja Schmidt ◽  
Daniel P. Grosvenor ◽  
Frida A.-M. Bender ◽  
...  

Abstract. Aerosol-cloud interactions are a major source of uncertainty in predicting 21st century climate change. Using high-resolution, convection-permitting global simulations we predict that increased cloud condensation nuclei (CCN) interacting with midlatitude cyclones will increase their cloud droplet number concentration (CDNC), liquid water (CLWP), and albedo. For the first time this effect is shown with 13 years of satellite observations. Causality between enhanced CCN and enhanced cyclone liquid content is supported by the 2014 eruption of Holuhraun. The change in midlatitude cyclone albedo due to enhanced CCN in a surrogate climate model is around 70 % of the change in a high-resolution convection-permitting model, indicating that climate models may underestimate this indirect effect.


2009 ◽  
Vol 9 (6) ◽  
pp. 25633-25661 ◽  
Author(s):  
U. Lohmann ◽  
L. Rotstayn ◽  
T. Storelvmo ◽  
A. Jones ◽  
S. Menon ◽  
...  

Abstract. Uncertainties in aerosol radiative forcings, especially those associated with clouds, contribute to a large extent to uncertainties in the total anthropogenic forcing. The interaction of aerosols with clouds and radiation introduces feedbacks which can affect the rate of rain formation. In former assessments of aerosol radiative forcings, these effects have not been quantified. Also, with global aerosol-climate models simulating interactively aerosols and cloud microphysical properties, a quantification of the aerosol forcings in the traditional way is difficult to properly define. Here we argue that fast feedbacks should be included because they act quickly compared with the time scale of global warming. We show that for different forcing agents (aerosols and greenhouse gases) the radiative forcings as traditionally defined agree rather well with estimates from a method, here referred to as radiative flux perturbations (RFP), that takes these fast feedbacks and interactions into account. Based on our results, we recommend RFP as a valid option to compare different forcing agents, and to compare the effects of particular forcing agents in different models.


2020 ◽  
Vol 117 (32) ◽  
pp. 18998-19006 ◽  
Author(s):  
Isabel L. McCoy ◽  
Daniel T. McCoy ◽  
Robert Wood ◽  
Leighton Regayre ◽  
Duncan Watson-Parris ◽  
...  

The change in planetary albedo due to aerosol−cloud interactions during the industrial era is the leading source of uncertainty in inferring Earth’s climate sensitivity to increased greenhouse gases from the historical record. The variable that controls aerosol−cloud interactions in warm clouds is droplet number concentration. Global climate models demonstrate that the present-day hemispheric contrast in cloud droplet number concentration between the pristine Southern Hemisphere and the polluted Northern Hemisphere oceans can be used as a proxy for anthropogenically driven change in cloud droplet number concentration. Remotely sensed estimates constrain this change in droplet number concentration to be between 8 cm−3and 24 cm−3. By extension, the radiative forcing since 1850 from aerosol−cloud interactions is constrained to be −1.2 W⋅m−2to −0.6 W⋅m−2. The robustness of this constraint depends upon the assumption that pristine Southern Ocean droplet number concentration is a suitable proxy for preindustrial concentrations. Droplet number concentrations calculated from satellite data over the Southern Ocean are high in austral summer. Near Antarctica, they reach values typical of Northern Hemisphere polluted outflows. These concentrations are found to agree with several in situ datasets. In contrast, climate models show systematic underpredictions of cloud droplet number concentration across the Southern Ocean. Near Antarctica, where precipitation sinks of aerosol are small, the underestimation by climate models is particularly large. This motivates the need for detailed process studies of aerosol production and aerosol−cloud interactions in pristine environments. The hemispheric difference in satellite estimated cloud droplet number concentration implies preindustrial aerosol concentrations were higher than estimated by most models.


2010 ◽  
Vol 10 (7) ◽  
pp. 3235-3246 ◽  
Author(s):  
U. Lohmann ◽  
L. Rotstayn ◽  
T. Storelvmo ◽  
A. Jones ◽  
S. Menon ◽  
...  

Abstract. Uncertainties in aerosol radiative forcings, especially those associated with clouds, contribute to a large extent to uncertainties in the total anthropogenic forcing. The interaction of aerosols with clouds and radiation introduces feedbacks which can affect the rate of precipitation formation. In former assessments of aerosol radiative forcings, these effects have not been quantified. Also, with global aerosol-climate models simulating interactively aerosols and cloud microphysical properties, a quantification of the aerosol forcings in the traditional way is difficult to define properly. Here we argue that fast feedbacks should be included because they act quickly compared with the time scale of global warming. We show that for different forcing agents (aerosols and greenhouse gases) the radiative forcings as traditionally defined agree rather well with estimates from a method, here referred to as radiative flux perturbations (RFP), that takes these fast feedbacks and interactions into account. Based on our results, we recommend RFP as a valid option to compare different forcing agents, and to compare the effects of particular forcing agents in different models.


2005 ◽  
Vol 5 (5) ◽  
pp. 9039-9063 ◽  
Author(s):  
R.-M. Hu ◽  
J.-P. Blanchet ◽  
E. Girard

Abstract. Cloud radiative forcing is a very important concept to understand what kind of role the clouds play in climate change with thermal effect or albedo effect. In spite of that much progress has been achieved, the clouds are still poorly described in the climate models. Due to the complex aerosol-cloud-radiation interactions, high surface albedo of snow and ice cover, and without solar radiation in long period of the year, the Arctic strong warming caused by increasing greenhouse gases (as most GCMs suggested) has not been verified by the observations. In this study, we were dedicated to quantify the aerosol effect on the Arctic cloud radiative forcing by Northern Aerosol Regional Climate Model (NARCM). Major aerosol species such as Arctic haze sulphate, black carbon, sea salt, organics and dust have been included during our simulations. By inter-comparisons with the Atmospheric Radiation Measurement (ARM) data, we find surface cloud radiative forcing (SCRF) is −22 W/m2 for shortwave and 36 W/m2 for longwave. Total cloud forcing is 14 W/m2 with minimum of −35 W/m2 in early July. If aerosols are taken into account, the SCRF has been increased during winter while negative SCRF has been enhanced during summer. Our estimate of aerosol forcing is about −6 W/m2 in the Arctic.


2017 ◽  
Vol 17 (5) ◽  
pp. 17-26 ◽  
Author(s):  
Hristo Chervenkov ◽  
Vladimir Ivanov ◽  
Georgi Gadzhev ◽  
Kostadin Ganev

Abstract The oncoming climate changes will exert influence on the ecosystems, on all branches of the international economy, and on the quality of life. Global Circulation Models (GCMs) are the most widespread and successful tools employed for both numerical weather forecast and climate research since the 1980s. However, growing demands on accurate and reliable information on regional and sub-regional scale are not directly met by relatively coarse resolution global models, mainly due to the excessive costs affiliated with the use of the model in very high resolution. Regional Climate Models (RCMs) are important instruments used for downscaling climate simulations from GCMs. Main aim of the numerical experiment Tuning an Validation of Regional Climate Model (RegCM-TVRegCM) is to quantify the impact of some tunable factors in the RegCM set-up on the model outputs. Thus, on the first stage of the study, the skill of 20 different model configurations in representing the basic spatial and temporal patterns of the Southeast European (SE) climate for the period 1999-2009, is evaluated. Based on these outcomes, the present work is dedicated on more detailed inspection of the model set-ups with recognizable better performance. The Pearson’s correlation coefficient between the time series of the temperature and precipitation of the 6 most promising model set-ups and the E-OBS on monthly basis are calculated. The main conclusion is that this test does not reveal single one model set-up that definitely over performs the other considered ones.


2017 ◽  
Vol 114 (19) ◽  
pp. 4899-4904 ◽  
Author(s):  
Edward Gryspeerdt ◽  
Johannes Quaas ◽  
Sylvaine Ferrachat ◽  
Andrew Gettelman ◽  
Steven Ghan ◽  
...  

Much of the uncertainty in estimates of the anthropogenic forcing of climate change comes from uncertainties in the instantaneous effect of aerosols on cloud albedo, known as the Twomey effect or the radiative forcing from aerosol–cloud interactions (RFaci), a component of the total or effective radiative forcing. Because aerosols serving as cloud condensation nuclei can have a strong influence on the cloud droplet number concentration (Nd), previous studies have used the sensitivity of theNdto aerosol properties as a constraint on the strength of the RFaci. However, recent studies have suggested that relationships between aerosol and cloud properties in the present-day climate may not be suitable for determining the sensitivity of theNdto anthropogenic aerosol perturbations. Using an ensemble of global aerosol–climate models, this study demonstrates how joint histograms betweenNdand aerosol properties can account for many of the issues raised by previous studies. It shows that if the anthropogenic contribution to the aerosol is known, the RFaci can be diagnosed to within 20% of its actual value. The accuracy of different aerosol proxies for diagnosing the RFaci is investigated, confirming that using the aerosol optical depth significantly underestimates the strength of the aerosol–cloud interactions in satellite data.


2012 ◽  
Vol 5 (6) ◽  
pp. 1565-1587 ◽  
Author(s):  
G. Lacressonnière ◽  
V.-H. Peuch ◽  
J. Arteta ◽  
B. Josse ◽  
M. Joly ◽  
...  

Abstract. Predicting how European air quality could evolve over the next decades in the context of changing climate requires the use of climate models to produce results that can be averaged in a climatologically and statistically sound manner. This is a very different approach from the one that is generally used for air quality hindcasts for the present period; analysed meteorological fields are used to represent specifically each date and hour. Differences arise both from the fact that a climate model run results in a pure model output, with no influence from observations (which are useful to correct for a range of errors), and that in a "climate" set-up, simulations on a given day, month or even season cannot be related to any specific period of time (but can just be interpreted in a climatological sense). Hence, although an air quality model can be thoroughly validated in a "realistic" set-up using analysed meteorological fields, the question remains of how far its outputs can be interpreted in a "climate" set-up. For this purpose, we focus on Europe and on the current decade using three 5-yr simulations performed with the multiscale chemistry-transport model MOCAGE and use meteorological forcings either from operational meteorological analyses or from climate simulations. We investigate how statistical skill indicators compare in the different simulations, discriminating also the effects of meteorology on atmospheric fields (winds, temperature, humidity, pressure, etc.) and on the dependent emissions and deposition processes (volatile organic compound emissions, deposition velocities, etc.). Our results show in particular how differing boundary layer heights and deposition velocities affect horizontal and vertical distributions of species. When the model is driven by operational analyses, the simulation accurately reproduces the observed values of O3, NOx, SO2 and, with some bias that can be explained by the set-up, PM10. We study how the simulations driven by climate forcings differ, both due to the realism of the forcings (lack of data assimilated and lower resolution) and due to the lack of representation of the actual chronology of events. We conclude that the indicators such as mean bias, mean normalized bias, RMSE and deviation standards can be used to interpret the results with some confidence as well as the health-related indicators such as the number of days of exceedance of regulatory thresholds. These metrics are thus considered to be suitable for the interpretation of simulations of the future evolution of European air quality.


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