Generation of stable and tunable optical frequency linked to a radio frequency by use of a high finesse cavity and its application in absorption spectroscopy

The laser frequency could be linked to an radio frequency through an external cavity by the combination of Pound-Drever-Hall and Devoe-Brewer locking techniques. A stable and tunable optical frequency at wavelength of 1.5 μm obtained by a cavity with high finesse of 96,000 and a fiber laser, calibrated by a commercial optical frequency comb, has been demonstrated. The locking performances have been analyzed by in-loop and out-loop noises, indicating that the absolute frequency instability could be down to 50 kHz over 1 s and keep to less than 110 kHz over 2.5 h. Then, the application of this stabilized laser to the direct absorption spectroscopy has been performed. With the help of balanced detection, the detection sensitivity, in terms of optical density, can reach to 9.4×10-6.

Polariton Condensate and Landau-Zener-Stückelberg Interferometry Transition in Multilayer Transition Metal Dichalcogenides

This paper gives a detailed description of a high-performance polariton condensate for a quantum mechanical two-level system (TLS). We propose a transition metal dichalcogenides (TMDs) setup and theoretically carry out the spectroscopy of these polariton condensates. Through theoretical and numerical analysis, we obtain many features in two dimensional (2D) multilayer TMDs. We compute the energy of the system and the Landau-Zener-Stückelberg (LZS) quantum tunneling probability under the effect of a sequence of laser light. At certain critical 2D TMDs parameters, the system exhibits a multi-crossing scenario in a privileged position of 2D multilayer TMDs. We predict the consecutive modulations and highlight the conservation of the LZS interference patterns mapped from the 2D TMDs system. At weak coupling regime, a successful conversion of interferometry signals is identified for some values of laser frequency. We explain such a result as a valley sensitive cavity rate model due to coherent exchange and incoherent scattering, meaning that polariton condensate is formed in the valley around the Brillouin zone. The latter is used quantitatively and qualitatively to achieve high-precision measurements beyond that of its elementary constituents. The obtained results confirm that MoSe2 has the highest sensitivity to radiation field as compared to other 2D multilayer TMDs materials. Therefore, MoSe2 stands as an appropriate candidate among other 2D TMDs to form polariton condensates.

Magic Wavelengths for 1S–nS and 2S–nS Transitions in Hydrogenlike Systems

We study the magic wavelength for two-photon 1S–nS transitions in a hydrogen and deuterium atom, as well as 2S–nS transitions, where the lower level is the metastable 2S state. At the magic wavelength, the dynamic Stark shifts of the ground and the excited state of the transition coincide, so that the transition frequency is independent of the intensity of the trapping laser field. Experimentally feasible magic wavelengths of transitions with small slopes in the atomic polarizabilities are determined; these are the most stable magic wavelengths against variations of the laser frequency. We provide data for the magic wavelengths for the 1S–nS and 2S–nS transitions in hydrogen and deuterium, with n=2,⋯,8. We also analyze the stability of the elimination of the ac Stark shift at the magic wavelength against tiny variations of the trapping laser frequency from the magic value.

Kinetic Simulations of in-situ Diffracted Intensities During Pulsed Laser Deposition of LuFeO3: Effect of Pulse Laser Frequency

Atomistic processes during pulsed-laser deposition (PLD) growth influence the physical properties of the resulting films. We investigated the PLD of epitaxial layers of hexagonal LuFeO3 by measuring the x-ray diffraction intensity in the quasiforbidden reflection 0003 in situ during deposition. From measured x-ray diffraction intensities we determined coverages of each layer and studied their time evolution which is described by scaling exponent β directly connected to the surface roughness. Subsequently we modelled the growth using kinetic Monte Carlo simulations. While the experimentally obtained scaling exponent β decreases with the laser frequency, the simulations provided the opposite behaviour. We demonstrate that the increase of the surface temperature caused by impinging ablated particles satisfactorily explains the recorded decrease in the scaling exponent with the laser frequency. This phenomena is often overlooked during the PLD growth.