Polariton Condensate and Landau-Zener-Stückelberg Interferometry Transition in Multilayer Transition Metal Dichalcogenides

2021 ◽  
Author(s):  
Clautaire Ekengoue ◽  
Christian Sadem Kenfack ◽  
Jérémie Edmond Danga ◽  
Gerard Bawe ◽  
Abdelaziz El Moussaouy ◽  
...  

Abstract This paper gives a detailed description of a high-performance polariton condensate for a quantum mechanical two-level system (TLS). We propose a transition metal dichalcogenides (TMDs) setup and theoretically carry out the spectroscopy of these polariton condensates. Through theoretical and numerical analysis, we obtain many features in two dimensional (2D) multilayer TMDs. We compute the energy of the system and the Landau-Zener-Stückelberg (LZS) quantum tunneling probability under the effect of a sequence of laser light. At certain critical 2D TMDs parameters, the system exhibits a multi-crossing scenario in a privileged position of 2D multilayer TMDs. We predict the consecutive modulations and highlight the conservation of the LZS interference patterns mapped from the 2D TMDs system. At weak coupling regime, a successful conversion of interferometry signals is identified for some values of laser frequency. We explain such a result as a valley sensitive cavity rate model due to coherent exchange and incoherent scattering, meaning that polariton condensate is formed in the valley around the Brillouin zone. The latter is used quantitatively and qualitatively to achieve high-precision measurements beyond that of its elementary constituents. The obtained results confirm that MoSe2 has the highest sensitivity to radiation field as compared to other 2D multilayer TMDs materials. Therefore, MoSe2 stands as an appropriate candidate among other 2D TMDs to form polariton condensates.

Author(s):  
Yoobeen Lee ◽  
Jin Won Jung ◽  
Jin Seok Lee

The reduction of intrinsic defects, including vacancies and grain boundaries, remains one of the greatest challenges to produce high-performance transition metal dichalcogenides (TMDCs) electronic systems. A deeper comprehension of the...


Author(s):  
Alwin Daus ◽  
Sam Vaziri ◽  
Victoria Chen ◽  
Çağıl Köroğlu ◽  
Ryan W. Grady ◽  
...  

2019 ◽  
Vol 10 (1) ◽  
Author(s):  
Lei Yin ◽  
Peng He ◽  
Ruiqing Cheng ◽  
Feng Wang ◽  
Fengmei Wang ◽  
...  

Abstract Defects play a crucial role in determining electric transport properties of two-dimensional transition metal dichalcogenides. In particular, defect-induced deep traps have been demonstrated to possess the ability to capture carriers. However, due to their poor stability and controllability, most studies focus on eliminating this trap effect, and little consideration was devoted to the applications of their inherent capabilities on electronics. Here, we report the realization of robust trap effect, which can capture carriers and store them steadily, in two-dimensional MoS2xSe2(1-x) via synergistic effect of sulphur vacancies and isoelectronic selenium atoms. As a result, infrared detection with very high photoresponsivity (2.4 × 105 A W−1) and photoswitching ratio (~108), as well as nonvolatile infrared memory with high program/erase ratio (~108) and fast switching time, are achieved just based on an individual flake. This demonstration of defect engineering opens up an avenue for achieving high-performance infrared detector and memory.


2017 ◽  
Vol 5 (29) ◽  
pp. 14950-14968 ◽  
Author(s):  
Gi Woong Shim ◽  
Woonggi Hong ◽  
Sang Yoon Yang ◽  
Sung-Yool Choi

This review provides insights for the design of synthetic schemes and catalytic systems of CVD-grown functional TMDs for high performance HER applications.


2016 ◽  
Vol 52 (59) ◽  
pp. 9251-9254 ◽  
Author(s):  
Jianfeng Shen ◽  
Pei Dong ◽  
Robert Baines ◽  
Xiaowei Xu ◽  
Zhuqing Zhang ◽  
...  

Novel ternary electrode materials based on graphene, NiCo2S4, and transition metal dichalcogenides were designed and fabricated with the intention of exploiting synergistic effects conducive to supercapacitive energy storage.


2019 ◽  
Vol 3 (10) ◽  
pp. 2577-2582 ◽  
Author(s):  
Chuang Wang ◽  
Xiao-Dong Zhu ◽  
Ke-Xin Wang ◽  
Liang-Liang Gu ◽  
Sheng-You Qiu ◽  
...  

Composite films comprising MXene nanosheets sandwiched by transition metal dichalcogenides/oxides are constructed as flexible lithium-ion battery anodes through vacuum-assisted filtration.


2021 ◽  
Author(s):  
Haoran Mu ◽  
Jian Yuan ◽  
Shenghuang Lin

2D Transition-Metal Dichalcogenides (TMDs) have been widely considered as a promising material for future optoelectronics due to the strong light-matter interaction, fantastic electronic properties and environmental stability. However, the relatively large bandgap and low mobility of conventional TMDs (such as MoS2 and WS2) limit their applications in infra optoelectronics and high-speed photodetection. In this chapter, we introduce a new type of group-10 noble TMDs (NTMDs), which exhibit outstanding properties such as unique structural phase, widely tunable energy gap and high mobility. Till now, various NTMDs-based photodetectors have been realized with ultrabroad detection waveband (200 nm to 10.6 μm), fast response time, high responsivity and detectivity, and polarization sensitivity. NTMDs have been excellent potential candidates for next-generation photodetection devices with high-performance, wafer-scalability and flexibility.


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