Влияние электрического поля на водородоподобные состояния в кристаллах моноклинного дифосфида цинка

The effect of the electric field on hydrogen-like states in β-ZnP2 is investigated. It was found that the exciton states Cn=1 in the electric field of the Schottky barrier undergo an anomalous Stark shift, and the states that form a reverse hydrogen-like series of absorption lines (IOS) are practically insensitive to the electric field. The laws governing the behavior of the exciton Xn=2 state "flammable" in an electric field in β-ZnP2 have been determined.

Magic Wavelengths for 1S–nS and 2S–nS Transitions in Hydrogenlike Systems

We study the magic wavelength for two-photon 1S–nS transitions in a hydrogen and deuterium atom, as well as 2S–nS transitions, where the lower level is the metastable 2S state. At the magic wavelength, the dynamic Stark shifts of the ground and the excited state of the transition coincide, so that the transition frequency is independent of the intensity of the trapping laser field. Experimentally feasible magic wavelengths of transitions with small slopes in the atomic polarizabilities are determined; these are the most stable magic wavelengths against variations of the laser frequency. We provide data for the magic wavelengths for the 1S–nS and 2S–nS transitions in hydrogen and deuterium, with n=2,⋯,8. We also analyze the stability of the elimination of the ac Stark shift at the magic wavelength against tiny variations of the trapping laser frequency from the magic value.

On the optical measurement of microparticle charge using quantum dots

We investigated the possibility of using a layer of quantum dots (QDs) deposited on the microparticle surface for the measurement of the charge the microparticle acquires when immersed into a plasma. To that end, we performed the calculations of the Stark shift of the photoluminescence spectrum of QDs caused by the fluctuating local electric field. In our calculations, we assumed the plasma-delivered surplus electrons to be distributed on the surface of a microparticle. According to our calculations, the Stark shift will acquire measurable values when the lifetime of the quasi-stationary configuration of the surplus electrons will be determined by their diffusion along the surface. Experiments with flat QD-covered floating plasma-facing surfaces suggest that measurable Stark shift of the photoluminescence spectrum can be achieved. Based on our model, modern microscopic plasma-surface interaction theories and analysis of the experiments, we suggest the possible design of the charge microsensor, which will allow to measure the charge accumulated on its surface by means of visible-light optics.

Ultrafast Quenching of Excitons in the ZnxCd1-xS/ ZnS Quantum Dots Doped with Mn2+ through Charge Transfer Intermediates Results in Manganese Luminescence

For the first time, a specific time-delayed peak was registered in the femtosecond transient absorption (TA) spectra of ZnxCd1-xS/ZnS (x~0.5) alloy quantum dots (QDs) doped with Mn2+, which was interpreted as the electrochromic Stark shift of the band-edge exciton. The time-delayed rise and decay kinetics of the Stark peak in the manganese-doped QDs significantly distinguish it from the kinetics of the Stark peak caused by exciton–exciton interaction in the undoped QDs. The Stark shift in the Mn2+-doped QDs developed at a 1 ps time delay in contrast to the instantaneous appearance of the Stark shift in the undoped QDs. Simultaneously with the development of the Stark peak in the Mn2+-doped QDs, stimulated emission corresponding to 4T1-6A1 Mn2+ transition was detected in the subpicosecond time domain. The time-delayed Stark peak in the Mn2+-doped QDs, associated with the development of an electric field in QDs, indicates the appearance of charge transfer intermediates in the process of exciton quenching by manganese ions, leading to the ultrafast Mn2+ excitation. The usually considered mechanism of the nonradiative energy transfer from an exciton to Mn2+ does not imply the development of an electric field in a QD. Femtosecond TA data were analyzed using a combination of empirical and computational methods. A kinetic scheme of charge transfer processes is proposed to explain the excitation of Mn2+. The kinetic scheme includes the reduction of Mn2+ by a 1Se electron and the subsequent oxidation of Mn1+ with a hole, leading to the formation of an excited state of manganese.

Underlying SUSY in a generalized Jaynes–Cummings model

We present a general qubit-boson interaction Hamiltonian that describes the Jaynes–Cummings model and its extensions as a single Hamiltonian class. Our model includes non-linear processes for both the free qubit and boson field as well as non-linear, multi-boson excitation exchange between them. It shows an underlying algebra with supersymmetric quantum mechanics features allowing an operator based diagonalization that simplifies the calculations of observables. As a practical example, we show the evolution of the population inversion and the boson quadratures for an initial state consisting of the qubit in the ground state interacting with a coherent field for a selection of cases covering the standard Jaynes–Cummings model and some of its extensions including Stark shift, Kerr-like, intensity dependent coupling, multi-boson exchange and algebraic deformations.