Effects of biomass burning on climate, accounting for heat and moisture fluxes, black and brown carbon, and cloud absorption effects

2014 ◽  
Vol 119 (14) ◽  
pp. 8980-9002 ◽  
Author(s):  
Mark Z. Jacobson
Keyword(s):  
Biomass Burning ◽  
Brown Carbon ◽  
Moisture Fluxes ◽  
Heat And Moisture

scholarly journals Investigating the Local Atmospheric Response to a Realistic Shift in the Oyashio Sea Surface Temperature Front

2015 ◽  
Vol 28 (3) ◽  
pp. 1126-1147 ◽  
Author(s):  
Dimitry Smirnov ◽  
Matthew Newman ◽  
Michael A. Alexander ◽  
Young-Oh Kwon ◽  
Claude Frankignoul
Keyword(s):  
High Resolution ◽  
Surface Wind ◽  
Lower Troposphere ◽  
Vertical Motion ◽  
Atmospheric Response ◽  
Transient Eddy ◽  
Sst Front ◽  
Moisture Fluxes ◽  
Upper Level ◽  
Heat And Moisture

Abstract The local atmospheric response to a realistic shift of the Oyashio Extension SST front in the western North Pacific is analyzed using a high-resolution (HR; 0.25°) version of the global Community Atmosphere Model, version 5 (CAM5). A northward shift in the SST front causes an atmospheric response consisting of a weak surface wind anomaly but a strong vertical circulation extending throughout the troposphere. In the lower troposphere, most of the SST anomaly–induced diabatic heating is balanced by poleward transient eddy heat and moisture fluxes. Collectively, this response differs from the circulation suggested by linear dynamics, where extratropical SST forcing produces shallow anomalous heating balanced by strong equatorward cold air advection driven by an anomalous, stationary surface low to the east. This latter response, however, is obtained by repeating the same experiment except using a relatively low-resolution (LR; 1°) version of CAM5. Comparison to observations suggests that the HR response is closer to nature than the LR response. Strikingly, HR and LR experiments have almost identical vertical profiles of . However, diagnosis of the diabatic quasigeostrophic vertical pressure velocity (ω) budget reveals that HR has a substantially stronger response, which together with upper-level mean differential thermal advection balances stronger vertical motion. The results herein suggest that changes in transient eddy heat and moisture fluxes are critical to the overall local atmospheric response to Oyashio Front anomalies, which may consequently yield a stronger downstream response. These changes may require the high resolution to be fully reproduced, warranting further experiments of this type with other high-resolution atmosphere-only and fully coupled GCMs.

scholarly journals Effects of Vertical Eddy Diffusivity Parameterization on the Evolution of Landfalling Hurricanes

2017 ◽  
Vol 74 (6) ◽  
pp. 1879-1905 ◽  
Author(s):  
Feimin Zhang ◽  
Zhaoxia Pu
Keyword(s):  
Boundary Layer ◽  
Vertical Mixing ◽  
Eddy Diffusivity ◽  
Essential Components ◽  
Moisture Fluxes ◽  
Layer Velocity ◽  
Hurricane Boundary Layer ◽  
Heat And Moisture ◽  
Vertical Eddy Diffusivity ◽  
Vertical Eddy

Abstract As a result of rapid changes in surface conditions when a landfalling hurricane moves from ocean to land, interactions between the hurricane and surface heat and moisture fluxes become essential components of its evolution and dissipation. With a research version of the Hurricane Weather Research and Forecasting Model (HWRF), this study examines the effects of the vertical eddy diffusivity in the boundary layer on the evolution of three landfalling hurricanes (Dennis, Katrina, and Rita in 2005). Specifically, the parameterization scheme of eddy diffusivity for momentum Km is adjusted with the modification of the mixed-layer velocity scale in HWRF for both stable and unstable conditions. Results show that the change in the Km parameter leads to improved simulations of hurricane track, intensity, and quantitative precipitation against observations during and after landfall, compared to the simulations with the original Km. Further diagnosis shows that, compared to original Km, the modified Km produces stronger vertical mixing in the hurricane boundary layer over land, which tends to stabilize the hurricane boundary layer. Consequently, the simulated landfalling hurricanes attenuate effectively with the modified Km, while they mostly inherit their characteristics over the ocean and decay inefficiently with the original Km.

scholarly journals The Influence of the Barrier Layer on SST Response during Tropical Cyclone Wind Forcing Using Idealized Experiments

2018 ◽  
Vol 48 (7) ◽  
pp. 1471-1478 ◽  
Author(s):  
Johna E. Rudzin ◽  
Lynn K. Shay ◽  
William E. Johns
Keyword(s):  
Mixed Layer ◽  
Barrier Layer ◽  
Wind Forcing ◽  
Upper Ocean ◽  
Salinity Stratification ◽  
Sst Cooling ◽  
Temperature Regimes ◽  
Moisture Fluxes ◽  
Upper Ocean Response ◽  
Heat And Moisture

AbstractMultiple studies have shown that reduced sea surface temperature (SST) cooling occurs under tropical cyclones (TCs) where a fresh surface layer and subsurface halocline exist. Reduced SST cooling in these scenarios has been attributed to a barrier layer, an upper-ocean feature in the tropical global oceans in which a halocline resides within the isothermal mixed layer. Because upper-ocean stratification theoretically reduces ocean mixing induced by winds, the barrier layer is thought to reduce SST cooling during TC passage, sustaining heat and moisture fluxes into the storm. This research examines how both the inclusion of salinity and upper-ocean salinity stratification influences SST cooling for a variety of upper-ocean thermal regimes using one-dimensional (1D) ocean mixed layer (OML) models. The Kraus–Turner, Price–Weller–Pinkel, and Pollard–Rhines–Thompson 1D OML schemes are used to examine SST cooling and OML deepening during 30 m s−1 wind forcing (~category 1 TC) for both temperature-only and temperature–salinity stratification cases. Generally, the inclusion of salinity (a barrier layer) reduces SST cooling for all temperature regimes. However, results suggest that SST cooling sensitivities exist depending on thermal regime, salinity stratification, and the 1D OML model used. Upper-ocean thermal and haline characteristics are put into context of SST cooling with the creation of a barrier layer baroclinic wave speed to emphasize the influence of salinity stratification on upper-ocean response under TC wind forcing.

scholarly journals Chemical and optical properties of carbonaceous aerosols in Nanjing, eastern China: regionally transported biomass burning contribution

2019 ◽  
Vol 19 (17) ◽  
pp. 11213-11233 ◽  
Author(s):  
Xiaoyan Liu ◽  
Yan-Lin Zhang ◽  
Yiran Peng ◽  
Lulu Xu ◽  
Chunmao Zhu ◽  
...  
Keyword(s):  
Optical Properties ◽  
Organic Carbon ◽  
Solar Energy ◽  
Energy Absorption ◽  
Biomass Burning ◽  
Eastern China ◽  
Water Soluble ◽  
Carbonaceous Aerosols ◽  
Southeastern China ◽  
Brown Carbon

Abstract. Biomass burning can significantly impact the chemical and optical properties of carbonaceous aerosols. Here, the biomass burning impacts were studied during wintertime in a megacity of Nanjing, eastern China. The high abundance of biomass burning tracers such as levoglucosan (lev), mannosan (man), galactosan (gal) and non-sea-salt potassium (nss-K+) was found during the studied period with the concentration ranges of 22.4–1476 ng m−3, 2.1–56.2 ng m−3, 1.4–32.2 ng m−3 and 0.2–3.8 µg m−3, respectively. The significant contribution of biomass burning to water-soluble organic carbon (WSOC; 22.3±9.9 %) and organic carbon (OC; 20.9±9.3 %) was observed in this study. Backward air mass origin analysis, potential emission sensitivity of elemental carbon (EC) and MODIS fire spot information indicated that the elevations of the carbonaceous aerosols were due to the transported biomass-burning aerosols from southeastern China. The characteristic mass ratio maps of lev∕man and lev∕nss-K+ suggested that the biomass fuels were mainly crop residuals. Furthermore, the strong correlation (p < 0.01) between biomass burning tracers (such as lev) and light absorption coefficient (babs) for water-soluble brown carbon (BrC) revealed that biomass burning emissions played a significant role in the light-absorption properties of carbonaceous aerosols. The solar energy absorption due to water-soluble brown carbon and EC was estimated by a calculation based on measured light-absorbing parameters and a simulation based on a radiative transfer model (RRTMG_SW). The solar energy absorption of water-soluble BrC in short wavelengths (300–400 nm) was 0.8±0.4 (0.2–2.3) W m−2 (figures in parentheses represent the variation range of each parameter) from the calculation and 1.2±0.5 (0.3–1.9) W m−2 from the RRTMG_SW model. The absorption capacity of water-soluble BrC accounted for about 20 %–30 % of the total absorption of EC aerosols. The solar energy absorption of water-soluble BrC due to biomass burning was estimated as 0.2±0.1 (0.0–0.9) W m−2, considering the biomass burning contribution to carbonaceous aerosols. Potential source contribution function model simulations showed that the solar energy absorption induced by water-soluble BrC and EC aerosols was mostly due to the regionally transported carbonaceous aerosols from source regions such as southeastern China. Our results illustrate the importance of the absorbing water-soluble brown carbon aerosols in trapping additional solar energy in the low-level atmosphere, heating the surface and inhibiting the energy from escaping the atmosphere.

scholarly journals The characteristics of atmospheric brown carbon in Xi'an, inland China: sources, size distributions and optical properties

2020 ◽  
Vol 20 (4) ◽  
pp. 2017-2030 ◽  
Author(s):  
Can Wu ◽  
Gehui Wang ◽  
Jin Li ◽  
Jianjun Li ◽  
Cong Cao ◽  
...  
Keyword(s):  
Optical Properties ◽  
Biomass Burning ◽  
Isotope Composition ◽  
Stable Carbon Isotope ◽  
Urban Atmosphere ◽  
Semiarid Region ◽  
Chemical Compositions ◽  
Brown Carbon ◽  
Polycyclic Aromatic ◽  
Fine Mode

Abstract. To investigate the characteristics of atmospheric brown carbon (BrC) in the semiarid region of East Asia, PM2.5 and size-resolved particles in the urban atmosphere of Xi'an, inland China, during the winter and summer of 2017 were collected and analyzed for optical properties and chemical compositions. Methanol extracts (MeOH extracts) were more light-absorbing than water extracts (H2O extracts) in the optical wavelength of 300–600 nm and well correlated with nitrophenols, polycyclic aromatic hydrocarbons (PAHs) and oxygenated PAHs (r > 0.78). The light absorptions (absλ=365 nm) of H2O extracts and MeOH extracts in winter were 28±16 and 49±32 M m−1, respectively, which are about 10 times higher than those in summer, mainly due to the enhanced emissions from biomass burning for house heating. Water-extracted BrC predominately occurred in the fine mode (< 2.1 µm) during winter and summer, accounting for 81 % and 65 % of the total absorption of BrC, respectively. The light absorption and stable carbon isotope composition measurements showed an increasing ratio of absλ=365 nm-MeOH to absλ=550 nm-EC along with an enrichment of 13C in PM2.5 during the haze development, indicating an accumulation of secondarily formed BrC (e.g., nitrophenols) in the aerosol aging process. Positive matrix factorization (PMF) analysis showed that biomass burning, fossil fuel combustion, secondary formation, and fugitive dust are the major sources of BrC in the city, accounting for 55 %, 19 %, 16 %, and 10 % of the total BrC of PM2.5, respectively.

scholarly journals Dry Intrusions: Lagrangian Climatology and Dynamical Impact on the Planetary Boundary Layer

2017 ◽  
Vol 30 (17) ◽  
pp. 6661-6682 ◽  
Author(s):  
Shira Raveh-Rubin
Keyword(s):  
Boundary Layer ◽  
Planetary Boundary Layer ◽  
Potential Temperature ◽  
Storm Track ◽  
Lower Troposphere ◽  
Western Coast ◽  
Moisture Fluxes ◽  
Quantitative Understanding ◽  
America South ◽  
Heat And Moisture

Dry-air intrusions (DIs) are dry, deeply descending airstreams from the upper troposphere toward the planetary boundary layer (PBL). The significance of DIs spans a variety of aspects, including the interaction with convection, extratropical cyclones and fronts, the PBL, and extreme surface weather. Here, a Lagrangian definition for DI trajectories is used and applied to ECMWF interim reanalysis (ERA-Interim) data. Based on the criterion of a minimum descent of 400 hPa during 48 h, a first global Lagrangian climatology of DI trajectories is compiled for the years 1979–2014, allowing quantitative understanding of the occurrence and variability of DIs, as well as the dynamical and thermodynamical interactions that determine their impact. DIs occur mainly in winter. While traveling equatorward from 40°–50° latitude, DIs typically reach the lower troposphere (with maximum frequencies of ~10% in winter) in the storm-track regions, as well as over the Mediterranean Sea, Arabian Sea, and eastern North Pacific, off the western coast of South America, South Africa, and Australia, and across the Antarctic coast. The DI descent is nearly adiabatic, with a mean potential temperature decrease of 3 K in two days. Relative humidity drops strongly during the first descent day and increases in the second day, because of mixing into the moist PBL. Significant destabilization of the lower levels occurs beneath DIs, accompanied by increased 10-m wind gusts, intense surface heat and moisture fluxes, and elevated PBL heights. Interestingly, only 1.2% of all DIs are found to originate from the stratosphere.

scholarly journals Parameterization of single-scattering albedo (SSA) and absorption Ångström exponent (AAE) with EC / OC for aerosol emissions from biomass burning

2016 ◽  
Vol 16 (15) ◽  
pp. 9549-9561 ◽  
Author(s):  
Rudra P. Pokhrel ◽  
Nick L. Wagner ◽  
Justin M. Langridge ◽  
Daniel A. Lack ◽  
Thilina Jayarathne ◽  
...  
Keyword(s):  
Black Carbon ◽  
Biomass Burning ◽  
Single Scattering ◽  
Emission Factors ◽  
Single Scattering Albedo ◽  
Biomass Fuels ◽  
Brown Carbon ◽  
Pearson's R ◽  
Biomass Burning Aerosol ◽  
Pearson’S R

Abstract. Single-scattering albedo (SSA) and absorption Ångström exponent (AAE) are two critical parameters in determining the impact of absorbing aerosol on the Earth's radiative balance. Aerosol emitted by biomass burning represent a significant fraction of absorbing aerosol globally, but it remains difficult to accurately predict SSA and AAE for biomass burning aerosol. Black carbon (BC), brown carbon (BrC), and non-absorbing coatings all make substantial contributions to the absorption coefficient of biomass burning aerosol. SSA and AAE cannot be directly predicted based on fuel type because they depend strongly on burn conditions. It has been suggested that SSA can be effectively parameterized via the modified combustion efficiency (MCE) of a biomass burning event and that this would be useful because emission factors for CO and CO2, from which MCE can be calculated, are available for a large number of fuels. Here we demonstrate, with data from the FLAME-4 experiment, that for a wide variety of globally relevant biomass fuels, over a range of combustion conditions, parameterizations of SSA and AAE based on the elemental carbon (EC) to organic carbon (OC) mass ratio are quantitatively superior to parameterizations based on MCE. We show that the EC ∕ OC ratio and the ratio of EC ∕ (EC + OC) both have significantly better correlations with SSA than MCE. Furthermore, the relationship of EC ∕ (EC + OC) with SSA is linear. These improved parameterizations are significant because, similar to MCE, emission factors for EC (or black carbon) and OC are available for a wide range of biomass fuels. Fitting SSA with MCE yields correlation coefficients (Pearson's r) of  ∼  0.65 at the visible wavelengths of 405, 532, and 660 nm while fitting SSA with EC / OC or EC / (EC + OC) yields a Pearson's r of 0.94–0.97 at these same wavelengths. The strong correlation coefficient at 405 nm (r =  0.97) suggests that parameterizations based on EC / OC or EC / (EC + OC) have good predictive capabilities even for fuels in which brown carbon absorption is significant. Notably, these parameterizations are effective for emissions from Indonesian peat, which have very little black carbon but significant brown carbon (SSA  =  0.990 ± 0.001 at 532 and 660 nm, SSA  =  0.937 ± 0.011 at 405 nm). Finally, we demonstrate that our parameterization based on EC / (EC + OC) accurately predicts SSA during the first few hours of plume aging with data from Yokelson et al. (2009) gathered during a biomass burning event in the Yucatán Peninsula of Mexico.

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