scholarly journals Where do fossil fuel carbon dioxide emissions from California go? An analysis based on radiocarbon observations and an atmospheric transport model

Author(s):  
W. J. Riley ◽  
D. Y. Hsueh ◽  
J. T. Randerson ◽  
M. L. Fischer ◽  
J. G. Hatch ◽  
...  
2017 ◽  
Author(s):  
Yu Liu ◽  
Nicolas Gruber ◽  
Dominik Brunner

Abstract. The emission of CO2 from the burning of fossil fuel is a prime determinant of variations in atmospheric CO2. Here, we simulate this fossil fuel signal together with the natural and background components with a regional high-resolution atmospheric transport model for central and southern Europe considering separately the emissions from different sectors and countries on the basis of emission inventories and hourly emission time functions. The simulated variations in atmospheric CO2 agree very well with observation-based estimates, although the observed variance is slightly underestimated, particularly for the fossil fuel component. Despite relatively rapid atmospheric mixing, the simulated fossil fuel signal reveals distinct annual mean structures deep into the troposphere reflecting the spatially dense aggregation of most emissions. The fossil fuel signal accounts for more than half of the total (fossil fuel + biospheric + background) temporal variations in atmospheric CO2 in most areas of northern and western central Europe, with the largest variations occurring on diurnal timescales owing to the combination of diurnal variations in emissions and atmospheric mixing/transport out of the surface layer. Their co-variance leads to a fossil-fuel diurnal rectifier effect with a magnitude as large as 9 ppm compared to a case with time-constant emissions. The spatial pattern of CO2 from the different sectors largely reflects the distribution and relative magnitude of the corresponding emissions, with power plant emissions leaving the most distinguished mark. An exception is southern and western Europe, where the emissions from the transportation sector dominate the fossil fuel signal. Most of the fossil fuel CO2 remains within the country responsible for the emission, although in smaller countries, up to 80 % of the fossil fuel signal can come from abroad. A fossil fuel emission reduction of 30 % is clearly detectable for a surface-based observing system for atmospheric CO2, while it is beyond the edge of detectability for the current generation of satellites with the exception of a few hotspot sites. Changes in variability in atmospheric CO2 might open an additional door for the monitoring and verification of changes in fossil fuel emissions, primarily for surface based systems.


2009 ◽  
Vol 114 (D22) ◽  
Author(s):  
Jocelyn Turnbull ◽  
Peter Rayner ◽  
John Miller ◽  
Tobias Naegler ◽  
Philippe Ciais ◽  
...  

2017 ◽  
Vol 17 (22) ◽  
pp. 14145-14169 ◽  
Author(s):  
Yu Liu ◽  
Nicolas Gruber ◽  
Dominik Brunner

Abstract. The emission of CO2 from the burning of fossil fuel is a prime determinant of variations in atmospheric CO2. Here, we simulate this fossil-fuel signal together with the natural and background components with a regional high-resolution atmospheric transport model for central and southern Europe considering separately the emissions from different sectors and countries on the basis of emission inventories and hourly emission time functions. The simulated variations in atmospheric CO2 agree very well with observation-based estimates, although the observed variance is slightly underestimated, particularly for the fossil-fuel component. Despite relatively rapid atmospheric mixing, the simulated fossil-fuel signal reveals distinct annual mean structures deep into the troposphere, reflecting the spatially dense aggregation of most emissions. The fossil-fuel signal accounts for more than half of the total (fossil fuel + biospheric + background) temporal variations in atmospheric CO2 in most areas of northern and western central Europe, with the largest variations occurring on diurnal timescales owing to the combination of diurnal variations in emissions and atmospheric mixing and transport out of the surface layer. The covariance of the fossil-fuel emissions and atmospheric transport on diurnal timescales leads to a diurnal fossil-fuel rectifier effect of up to 9 ppm compared to a case with time-constant emissions. The spatial pattern of CO2 from the different sectors largely reflects the distribution and relative magnitude of the corresponding emissions, with power plant emissions leaving the most distinguished mark. An exception is southern and western Europe, where the emissions from the transportation sector dominate the fossil-fuel signal. Most of the fossil-fuel CO2 remains within the country responsible for the emission, although in smaller countries up to 80 % of the fossil-fuel signal can come from abroad. A fossil-fuel emission reduction of 30 % is clearly detectable for a surface-based observing system for atmospheric CO2, while it is beyond the edge of detectability for the current generation of satellites with the exception of a few hotspot sites. Changes in variability in atmospheric CO2 might open an additional door for the monitoring and verification of changes in fossil-fuel emissions, primarily for surface-based systems.


Energies ◽  
2020 ◽  
Vol 13 (15) ◽  
pp. 3956 ◽  
Author(s):  
Elkhan Richard Sadik-Zada ◽  
Wilhelm Loewenstein

The present inquiry addresses the income-environment relationship in oil-producing countries and scrutinizes the further drivers of atmospheric pollution in the respective settings. The existing literature that tests the environmental Kuznets curve hypothesis within the framework of the black-box approaches provides only a bird’s-eye perspective on the long-run income-environment relationship. The aspiration behind this study is making the first step toward the disentanglement of the sources of carbon dioxide emissions, which could be employed in the pollution mitigation policies of this group of countries. Based on the combination of two strands of literature, the environmental Kuznets curve conjecture and the resource curse, the paper at hand proposes an augmented theoretical framework of this inquiry. To approach the research questions empirically, the study employs advanced panel cointegration techniques. To avoid econometric misspecification, the study also employs for the first time a nonparametric time-varying coefficient panel data estimator with fixed effects (NPFE) for the dataset of 37 oil-producing countries in the time interval spanning between 1989 and 2019. The empirical analysis identifies the level of per capita income, the magnitude of oil rents, the share of fossil fuel-based electricity generation in the energy mix, and the share of the manufacturing sector in GDP as essential drivers of carbon dioxide emissions in the oil-rich countries. Tertiarization, on the contrary, leads to a substantial reduction of emissions. Another striking result of this study is that level of political rights and civil liberties are negatively associated with per capita carbon emissions in this group of countries. Furthermore, the study decisively rejects an inverted U-shaped income-emission relationship and validates the monotonically or exponentially increasing impact of average income on carbon dioxide emissions.


2018 ◽  
Vol 18 (18) ◽  
pp. 13305-13320 ◽  
Author(s):  
Tim Arnold ◽  
Alistair J. Manning ◽  
Jooil Kim ◽  
Shanlan Li ◽  
Helen Webster ◽  
...  

Abstract. Decadal trends in the atmospheric abundances of carbon tetrafluoride (CF4) and nitrogen trifluoride (NF3) have been well characterised and have provided a time series of global total emissions. Information on locations of emissions contributing to the global total, however, is currently poor. We use a unique set of measurements between 2008 and 2015 from the Gosan station, Jeju Island, South Korea (part of the Advanced Global Atmospheric Gases Experiment network), together with an atmospheric transport model, to make spatially disaggregated emission estimates of these gases in East Asia. Due to the poor availability of good prior information for this study, our emission estimates are largely influenced by the atmospheric measurements. Notably, we are able to highlight emission hotspots of NF3 and CF4 in South Korea due to the measurement location. We calculate emissions of CF4 to be quite constant between the years 2008 and 2015 for both China and South Korea, with 2015 emissions calculated at 4.3±2.7 and 0.36±0.11 Gg yr−1, respectively. Emission estimates of NF3 from South Korea could be made with relatively small uncertainty at 0.6±0.07 Gg yr−1 in 2015, which equates to ∼1.6 % of the country's CO2 emissions. We also apply our method to calculate emissions of CHF3 (HFC-23) between 2008 and 2012, for which our results find good agreement with other studies and which helps support our choice in methodology for CF4 and NF3.


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