Rational design of a mesoporous silica-based cathode for efficient trapping of polysulfides in Li–S batteries

2020 ◽  
Vol 56 (5) ◽  
pp. 786-789 ◽  
Author(s):  
Chao Chen ◽  
Huifang Xu ◽  
Bingkai Zhang ◽  
Qingbin Jiang ◽  
Yaping Zhang ◽  
...  

We develop a mesoporous silica-based cathode for efficient trapping of lithium polysulfides. This cathode consists of a mesoporous silica (HMS), highly dispersed NiO nanoparticles embedded in the silica structure and a conductive polymer prepared by in situ polymerization.

RSC Advances ◽  
2016 ◽  
Vol 6 (113) ◽  
pp. 112193-112200 ◽  
Author(s):  
Shengyang Tao ◽  
Huan Wang ◽  
Huilong Wang

We present an in situ reduction strategy to prepare mesoporous silica supported by highly-dispersed noble metals.


ACS Omega ◽  
2020 ◽  
Vol 5 (46) ◽  
pp. 30237-30242
Author(s):  
Chunling Xin ◽  
Xia Wang ◽  
LiLi Liu ◽  
Jinmei Yang ◽  
Suqing Wang ◽  
...  

2021 ◽  
Vol 14 (1) ◽  
Author(s):  
Maria Gridina ◽  
Evgeniy Mozheiko ◽  
Emil Valeev ◽  
Ludmila P. Nazarenko ◽  
Maria E. Lopatkina ◽  
...  

Abstract Background The Hi-C technique is widely employed to study the 3-dimensional chromatin architecture and to assemble genomes. The conventional in situ Hi-C protocol employs restriction enzymes to digest chromatin, which results in nonuniform genomic coverage. Using sequence-agnostic restriction enzymes, such as DNAse I, could help to overcome this limitation. Results In this study, we compare different DNAse Hi-C protocols and identify the critical steps that significantly affect the efficiency of the protocol. In particular, we show that the SDS quenching strategy strongly affects subsequent chromatin digestion. The presence of biotinylated oligonucleotide adapters may lead to ligase reaction by-products, which can be avoided by rational design of the adapter sequences. Moreover, the use of nucleotide-exchange enzymes for biotin fill-in enables simultaneous labelling and repair of DNA ends, similar to the conventional Hi-C protocol. These improvements simplify the protocol, making it less expensive and time-consuming. Conclusions We propose a new robust protocol for the preparation of DNAse Hi-C libraries from cultured human cells and blood samples supplemented with experimental controls and computational tools for the evaluation of library quality.


2021 ◽  
Vol 5 (7) ◽  
pp. 191
Author(s):  
Yanshuai Wang ◽  
Siyao Guo ◽  
Biqin Dong ◽  
Feng Xing

The functionalization of graphene has been reported widely, showing special physical and chemical properties. However, due to the lack of surface functional groups, the poor dispersibility of graphene in solvents strongly limits its engineering applications. This paper develops a novel green “in-situ titania intercalation” method to prepare a highly dispersed graphene, which is enabled by the generation of the titania precursor between the layer of graphene at room temperature to yield titania-graphene nanocomposites (TiO2-RGO). The precursor of titania will produce amounts of nano titania between the graphene interlayers, which can effectively resist the interfacial van der Waals force of the interlamination in graphene for improved dispersion state. Such highly dispersed TiO2-RGO nanocomposites were used to modify epoxy resin. Surprisingly, significant enhancement of the mechanical performance of epoxy resin was observed when incorporating the titania-graphene nanocomposites, especially the improvements in tensile strength and elongation at break, with 75.54% and 176.61% increases at optimal usage compared to the pure epoxy, respectively. The approach presented herein is easy and economical for industry production, which can be potentially applied to the research of high mechanical property graphene/epoxy composite system.


CrystEngComm ◽  
2021 ◽  
Author(s):  
Mikkel Herzberg ◽  
Anders Støttrup Larsen ◽  
Tue Hassenkam ◽  
Anders Østergaard Madsen ◽  
Jukka Rantanen

Solvents can dramatically affect molecular crystals. Obtaining favorable properties for these crystals requires rational design based on molecular level understanding of the solid-solution interface. Here we show how atomic force...


2021 ◽  
pp. 129630
Author(s):  
Bong Kyun Kang ◽  
Yoo Jung Choi ◽  
Hyung Wook Choi ◽  
Seok Bin Kwon ◽  
Suji Kim ◽  
...  

2021 ◽  
Vol 514 ◽  
pp. 111859
Author(s):  
Samaneh Sohrabi ◽  
Reza Khaleghi Abasabadi ◽  
Abbas Ali Khodadadi ◽  
Yadollah Mortazavi ◽  
Ali Hoseinzadeh

2014 ◽  
Vol 2 (45) ◽  
pp. 9625-9630 ◽  
Author(s):  
Huangxin Zhou ◽  
Xun Lv ◽  
Ling Zhang ◽  
An Gong ◽  
Aiguo Wu ◽  
...  
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