scholarly journals Calculations of Light Scattering Matrix of Dust Aerosols for Problems of Lidar Remote Sensing

2020 ◽  
Vol 237 ◽  
pp. 08008
Author(s):  
Natalia Kustova ◽  
Alexander Konoshonkin ◽  
Anatoli Borovoi ◽  
Zhenzhu Wang ◽  
Dong Liu ◽  
...  

The light scattering matrix is calculated for large dust particles with irregular shape and refractive index of 1.3116+i0.0. The scattering matrix in the backward direction needed for lidar studies is separately discussed. In this case, the obtained results for the lidar and depolarization ratios are in good agreement with experimental data. It is shown that for randomly oriented particles the number of particle orientations needed for numerical calculations by exact methods like DDA becomes a crucial parameter. In particular, for particles with size parameters larger than 40 the number of orientations should be more than 1000.

2020 ◽  
Vol 13 (8) ◽  
pp. 4097-4109
Author(s):  
Jia Liu ◽  
Qixing Zhang ◽  
Yinuo Huo ◽  
Jinjun Wang ◽  
Yongming Zhang

Abstract. Mineral dust suspended in the atmosphere has significant effects on radiative balance and climate change. The Chinese Loess Plateau (CLP) is generally considered one of the main sources of Asian dust aerosol. After being lifted by wind, dust particles with various size distributions can be transported over different distances. In this study, an original loess sample was collected from Luochuan, which is centrally located on the CLP, and two samples with different size distributions were obtained afterwards. “Pristine loess” was used to represent dust that only affects source regions, part of pristine loess was milled to finer “milled loess” that can be transported over long distances. Light scattering matrices for these two samples were measured at 532 nm wavelength from 5 to 175∘ angles. Particle size distribution, refractive index, chemical component, and microscopic appearance were also characterized for auxiliary analyses. Experimental results showed that there are obvious discrepancies in angular behaviors of matrix elements for pristine loess and milled loess, and these discrepancies are different from those for other kinds of dust with distinct size distributions. Given that the effective radii of these two loess samples differ by more than 20 times, it is reasonable to conclude that the difference in size distributions plays a major role in leading to different matrices, while differences in refractive index and microstructure have relatively small contributions. Qualitative analyses of numerical simulation results of irregular particles also validate this conclusion. Gaussian spheres may be promising morphological models for simulating the scattering matrix of loess but need further quantitative verification. Finally, synthetic scattering matrices for both pristine loess and milled loess were constructed over 0–180∘, and the previous average scattering matrix for loess dust was updated. This study presents measurement results of Chinese loess dust and an updated average scattering matrix for loess, which are useful for validating existing models, developing more advanced models for optical simulations of loess dust, and helping to improve retrieval accuracy of dust aerosol properties over both source and downwind areas.


1996 ◽  
Vol 150 ◽  
pp. 409-413
Author(s):  
Patrick P. Combet ◽  
Philippe L. Lamy

AbstractWe have set up an experimental device to optically study the scattering properties of dust particles. Measurements over the 8 — 174° interval of scattering angles are performed on a continuously flowing dust loaded jet illuminated by a polarized red HeNe laser beam. The scattering is averaged over the population of the dust particles in the jet, which can be determined independently, and give the “volume scattering function” for the two directions of polarization directly. While results for spherical particles are in good agreement with Mie theory, those for arbitrary particles show conspicuous deviations.


1973 ◽  
Vol 52 ◽  
pp. 131-137
Author(s):  
Th. Schmidt

Calculations have been carried out of single light scattering by Rayleigh type spheroidal dust particles. It can be shown that elliptical polarized radiation with e = v/p ≈ 0.15 can be produced from unpolarized incident radiation, in the case of dirty quartz particles with a refractive index m = 1.54 ± 0.4i and a geometrical axial ratio c: a ≈ 1:2.


2020 ◽  
Vol 237 ◽  
pp. 08012
Author(s):  
Victor Shishko ◽  
Alexander Konoshonkin ◽  
Natalia Kustova ◽  
Anatoli Borovoi ◽  
Dmitry Timofeev

The work presents the solution for the light scattering problem by arbitrarily-shaped particles in the vicinity of the backward scattering direction. The solution was obtained within the framework of the geometrical optics approximation. The refractive index was equal to 1.3116. It was shown that the general contribution of scattering light for arbitrarily-shaped particles in the vicinity of the backscattering direction consists of the specular reflection of the particles and two types of non-specular optical beams. It is shown that the optical characteristics of the ice particles with arbitrary shapes correspond to experimental data.


2021 ◽  
Author(s):  
Alain Miffre ◽  
Danaël Cholleton ◽  
Patrick Rairoux

<p>This abstract is dedicated to dual-wavelength polarization lidars (2β+2δ) and related particles backscattering Ångström exponents BAE<sub>p</sub>, as nowadays remotely evaluated by atmospheric multi-wavelength lidar instruments (Veselovskii et al., ACP, 2016). We here present two new lidar remote sensing developments applicable to every multi-wavelengths polarization lidars, as published in Miffre et al. (Rem. Sens. 2019, Opt. Lett. 2020).</p><p>As a first development, we investigate the size, shape and complex refractive index dependence of measured backscattering Ångström exponents (Miffre et al., Opt. Lett., 2020). If BAE<sub>p</sub> is generally considered as a particles size indicator, it actually depends on the particles size, shape (Mehri et al., Atm. Res., 2018) and complex refractive index as β<sub>p</sub> does. From a precise analysis of the polarization state of the backscattered radiation and of its wavelength dependence, in two components particle mixtures (p) = {s, ns} involving spherical (s) and nonspherical (ns)-particles, we could establish the relationship between BAE<sub>p</sub>, BAE<sub>s</sub> and BAE<sub>ns</sub>. Then, by numerically simulating the two latter, we could discuss on the range of involved particle sizes and complex refractive indices.</p><p>The second development is related to the remote sensing observation of a new particle formation event with a dual-wavelength polarization lidar (Miffre et al. Rem. Sens. 2019). Where previous thoughts were that it is not feasible due to the small size of involved particles, we identified the requirements ensuring a (UV, VIS) polarization lidar to be sensitive to the subsequent particles growth following nucleation events promoted by nonspherical mineral dust particles. The presentation will explicit these optical requirements in terms of polarization and spectroscopy, as recently published in (Miffre et al., Rem. Sens., 2019).</p><p>The oral presentation will first present our dual-wavelength polarization lidar remote sensing instrument (2β+2δ), based on an unique laboratory Pi-polarimeter (Miffre et al., JQSRT, 2016). Special focus will be made on the (UV, VIS) calibration of the polarization lidar, as a decisive point for precise observations and interpretations. As an application case study, the oral presentation will then consider the lidar remote sensing observation of a nucleation event promoted by mineral dust. There, the involved particles sizes of freshly nucleated sulfuric acid particles and mineral dust will be retrieved by considering the above backscattering Ångström exponents analysis. As expected, the retrieved involved particles sizes reveal the underlying physical-chemistry of the nucleation process promoted by mineral dust (Dupart et al., PNAS, 2012). We believe this work may then interest a wide community of scientists.</p><p>Veselovskii, I., P. Goloub, D. N. Whiteman, A. Diallo, T. Ndiaye, A. Kolgotin, and O. Dubovik, ACP, <strong>16</strong>(11), (2016).<br>Dupart, Y., A. Wiedensohler, H. Hermann, A. Miffre, P. Rairoux, B. D’Anna and C. George, PNAS, 109, 51, (2012).<br>Miffre, A., T. Mehri, M. Francis and P. Rairoux, JQSRT, 169, 79-90, (2016).<br>Mehri, T., P. Rairoux, T. Nousiainen, A. Miffre, Atm. Res. <strong>203</strong>, 44-61 (2018).<br>Miffre A, D Cholleton, T. Mehri and P Rairoux, Rem. Sens., 11(15), 1761, (2019).<br>Miffre, A., D. Cholleton, P. Rairoux, Opt. Lett.<strong> 45</strong>, 5, 1084-1087, (2020).</p>


2019 ◽  
Vol 15 (S350) ◽  
pp. 372-374
Author(s):  
Amritaksha Kar ◽  
Asoke K Sen

AbstractThe surfaces of most of the atmosphereless solar system bodies are referred to as regolith or layers of usually loosely connected fragmentary debris, produced by meteorite impacts. Measurement of light scattered from such surfaces provide information about the composition and structure of the surface. In the present work, the effect of porosity and particle size, on reflectance is studied for regolith like samples. For modelling the experimental data Hapke 2008 is used and found to be in good agreement with laboratory data. From the present study, it can be concluded that the physical properties of a regolith, such as porosity, particle size etc are effectively represented by albedo.


1984 ◽  
Vol 49 (8) ◽  
pp. 1731-1735 ◽  
Author(s):  
Viliam Klimo ◽  
Jozef Tiňo

Geometry and energy parameters of individual dissociation intermediate steps of the NH3 molecule, geometry of the saddle point, and the inversion barrier of NH3 have been calculated by the UMP2 method in the minimum basis set augmented with the bond functions. A good agreement has been reached with experimental data and with results of more exact methods except for the dissociation energies of the NH3 and NH2 molecules. New values of heats of formation are suggested on the basis of these results: ΔHfo0 = 197 and 362 kJ/mol for the NH2 and NH molecules, respectively.


1947 ◽  
Vol 25b (3) ◽  
pp. 255-265 ◽  
Author(s):  
J. Bardwell ◽  
C. Sivertz

A critical study has been made of the various observations necessary for the determination of the size of small dielectric particles by the Debye–Einstein equation, which can take the form:[Formula: see text]The turbidity measurements were made with a Beckman spectrophotometer and those of refractive index with a Zeiss dipping refractometer. This article deals especially with the determination of the turbidity and refractive index gradients. The method was applied to the determination of latex particle size and gave results in good agreement with independent methods.


2020 ◽  
Vol 21 (1) ◽  
pp. 57-60 ◽  
Author(s):  
H. Il'chuk ◽  
A. Kashuba ◽  
R. Petrus ◽  
I. Semkiv ◽  
N. Ukrainets

The spectral dependence of the transmittance as a function of the film thickness, the refractive index of the substrate, bandgap and the Cauchy parameters (α and β) of the semiconductor material was determined from condition of interference extremes. The absorption coefficient was simulated for the structure – thin film/substrate. Cadmium chalcogenides (CdTe, CdSe, and CdS) deposited on quartz substrates was selected as model samples. Experimental behavior of substrate transmittance was used to determine its refractive index. The theoretical results are compared with the experimental data and shows good agreement.


2019 ◽  
Author(s):  
Jia Liu ◽  
Qixing Zhang ◽  
Jinjun Wang ◽  
Yongming Zhang

Abstract. Mineral dust suspended in the atmosphere has significant effects on radiative balance and climate change. Chinese Loess Plateau (CLP) is generally considered as a main sources of Asian dust aerosol. After being lifted by wind, dust particles with various size distributions can be transported for different distances. In this study, original loess sample was collected from Luochuan, which is centrally located at CLP, and two samples with different size distributions were obtained after then. Pristine loess was used to represent dust that only affect source regions, part of pristine loess was milled to finer milled loess that can be transported for long distance. Light scattering matrices for these two samples were measured at 532 nm wavelength from 5° to 160° angles. Particle size distribution, refractive index, chemical component, and microscopic appearance were also measured for auxiliary analyses. Results showed that discrepancies in angular behaviours of matrix elements for pristine loess and milled loess cannot be ignored. Given that the effective radii of these two loess samples differ by more than 20 times, it is reasonable to conclude that the difference in size distributions plays a major role in leading to different matrices, while refractive index and micro structure have relatively small impacts. Analyses of numerical simulation results about irregular particles also variety this conclusion. At last, synthetic scattering matrices for both pristine loess and milled loess were calculated over 0°–180°, and the previous average scattering matrix for loess dust was updated.


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