Excitonic couplings and interband energy transfer in a double-wall molecular aggregate imaged by coherent two-dimensional electronic spectroscopy

2009 ◽  
Vol 131 (5) ◽  
pp. 054510 ◽  
Author(s):  
F. Milota ◽  
J. Sperling ◽  
A. Nemeth ◽  
D. Abramavicius ◽  
S. Mukamel ◽  
...  
Chem ◽  
2019 ◽  
Vol 5 (8) ◽  
pp. 2111-2125 ◽  
Author(s):  
Brian K. Petkov ◽  
Tobias A. Gellen ◽  
Camille A. Farfan ◽  
William P. Carbery ◽  
Belinda E. Hetzler ◽  
...  

2019 ◽  
Vol 205 ◽  
pp. 09034
Author(s):  
Minjung Son ◽  
Alberta Pinnola ◽  
Roberto Bassi ◽  
Gabriela S. Schlau-Cohen

We utilise ultrabroadband two-dimensional electronic spectroscopy to map out pathways of energy flow in LHCII across the entire visible region. In addition to the well-established, low-lying chlorophyll Qy bands, our results reveal additional pathways of energy relaxation on the higher-lying excited states involving the S2 energy levels of carotenoids, including ultrafast carotenoid-to-chlorophyll energy transfer on 90-150 fs timescales.


2019 ◽  
Vol 205 ◽  
pp. 09038
Author(s):  
Thanh Nhut Do ◽  
Adriana Huerta-Viga ◽  
Cheng Zhang ◽  
Parveen Akhtar ◽  
Pawei J. Nowakowski ◽  
...  

Light-harvesting complex II (LHCII) – the light-harvesting antenna of Photosystem II – is a naturally abundant system that plays an important role in photosynthesis. In this study, we present a phenomenological analysis of the excitonic energy transfer in LHCII using ultrafast two-dimensional electronic spectroscopy, that we find compares well with previous theoretical and experimental results.


2013 ◽  
Vol 85 (7) ◽  
pp. 1307-1319 ◽  
Author(s):  
Jessica M. Anna ◽  
Yin Song ◽  
Rayomond Dinshaw ◽  
Gregory D. Scholes

We demonstrate the ability of two-dimensional electronic spectroscopy (2DES) to map ultrafast energy transfer and dynamics in two systems: the pigment–protein complex photosystem I (PSI) and aggregates of the conjugated polymer poly(3-hexylthiophene) (P3HT). A detailed description of our experimental set-up and data processing procedure is also given.


2018 ◽  
Vol 24 (46) ◽  
pp. 12084-12092
Author(s):  
Francesco Segatta ◽  
Itay Gdor ◽  
Julien Réhault ◽  
Simone Taioli ◽  
Noga Friedman ◽  
...  

2018 ◽  
Vol 9 (15) ◽  
pp. 3694-3703 ◽  
Author(s):  
John P. Otto ◽  
Lili Wang ◽  
Igor Pochorovski ◽  
Samuel M. Blau ◽  
Alán Aspuru-Guzik ◽  
...  

Two-dimensional electronic spectroscopy of energy transfer and competing dynamics highlights how conformational changes create issues with lifetime-based FRET measurements.


Author(s):  
Mattia Russo ◽  
Anna Paola Casazza ◽  
Giulio Cerullo ◽  
Stefano Santabarbara ◽  
Margherita Maiuri

2013 ◽  
Vol 4 (22) ◽  
pp. 3977-3977 ◽  
Author(s):  
Peter D. Dahlberg ◽  
Andrew F. Fidler ◽  
Justin R. Caram ◽  
Phillip D. Long ◽  
Gregory S. Engel

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