scholarly journals Early atmospheric contamination on the top of the Himalayas since the onset of the European Industrial Revolution

2020 ◽  
Vol 117 (8) ◽  
pp. 3967-3973 ◽  
Author(s):  
Paolo Gabrielli ◽  
Anna Wegner ◽  
M. Roxana Sierra-Hernández ◽  
Emilie Beaudon ◽  
Mary Davis ◽  
...  
Keyword(s):  
Trace Metals ◽  
Western Europe ◽  
Industrial Revolution ◽  
Ice Core ◽  
Toxic Metal ◽  
Enrichment Factors ◽  
High Elevation ◽  
Snow Accumulation ◽  
Metal Levels ◽  
Toxic Trace Metals

Because few ice core records from the Himalayas exist, understanding of the onset and timing of the human impact on the atmosphere of the “roof of the world” remains poorly constrained. We report a continuous 500-y trace metal ice core record from the Dasuopu glacier (7,200 m, central Himalayas), the highest drilling site on Earth. We show that an early contamination from toxic trace metals, particularly Cd, Cr, Mo, Ni, Sb, and Zn, emerged at high elevation in the Himalayas at the onset of the European Industrial Revolution (∼1780 AD). This was amplified by the intensification of the snow accumulation (+50% at Dasuopu) likely linked to the meridional displacement of the winter westerlies from 1810 until 1880 AD. During this period, the flux and crustal enrichment factors of the toxic trace metals were augmented by factors of 2 to 4 and 2 to 6, respectively. We suggest this contamination was the consequence of the long-range transport and wet deposition of fly ash from the combustion of coal (likely from Western Europe where it was almost entirely produced and used during the 19th century) with a possible contribution from the synchronous increase in biomass burning emissions from deforestation in the Northern Hemisphere. The snow accumulation decreased and dry winters were reestablished in Dasuopu after 1880 AD when lower than expected toxic metal levels were recorded. This indicates that contamination on the top of the Himalayas depended primarily on multidecadal changes in atmospheric circulation and secondarily on variations in emission sources during the last 200 y.

scholarly journals Use of Paleoflood Deposits to Determine the Contribution of Anthropogenic Trace Metals to Alluvial Sediments in the Hyperarid Rio Loa Basin, Chile

Geosciences ◽  
2019 ◽  
Vol 9 (6) ◽  
pp. 244 ◽  
Author(s):  
Jerry R. Miller ◽  
Danvey Walsh ◽  
Lionel F. Villarroel
Keyword(s):  
Trace Metals ◽  
Organic Matter Content ◽  
Enrichment Factors ◽  
Matter Content ◽  
Anthropogenic Sources ◽  
Biogeochemical Processes ◽  
Riverine Ecosystems ◽  
Local Background ◽  
Toxic Trace Metals ◽  
Source Materials

Toxic trace metals are a common and significant contaminant in riverine ecosystems, and are derived from both natural and anthropogenic sources. Determining the contributions of metals from these sources has proven difficult, in part, because physical and biogeochemical processes alter the nature (e.g., grain size, mineral composition, organic matter content) of the source materials as they are transported through the drainage network. This study examined the use of paleoflood deposits located along the hyperarid Rio Salado, a tributary to the Rio Loa of northern Chile, to construct local background functions and enrichment factors (LEFs) to differentiate between natural and anthropogenic metal sources. Significant variations in metal content occurred between river reaches and flood deposits of a given reach; these variations were primarily related to changes in sediment source that may reflect differences in El Niño and La Niña precipitation patterns. Three conservative elements (Al, Fe, Co) were examined to construct background functions for seven trace metals. Cobalt yielded the most effective background functions for As, Cd, Ni, Pb, and Zn; Fe was selected for Cr, and Al for Cu. The resulting LEFs approximated 1, illustrating that paleoflood deposits produced effective background functions, and could be applied to downstream sites contaminated by mining activity.

Identifying Sources of Sulfate Aerosols Reaching Whiteface Mountain, NY

1985 ◽  
Vol 43 ◽  
pp. 98-101
Author(s):  
James S. Webber
Keyword(s):  
Trace Metals ◽  
Acid Deposition ◽  
Surface Waters ◽  
Dry Deposition ◽  
Coal Combustion ◽  
Public Awareness ◽  
Sulfate Aerosols ◽  
Wet And Dry Deposition ◽  
Whiteface Mountain ◽  
Toxic Trace Metals

INTRODUCTION“Acid rain” and “acid deposition” are terms no longer confined to the lexicon of atmospheric scientists and 1imnologists. Public awareness of and concern over this phenomenon, particularly as it affects acid-sensitive regions of North America, have increased dramatically in the last five years. Temperate ecosystems are suffering from decreased pH caused by acid deposition. Human health may be directly affected by respirable sulfates and by the increased solubility of toxic trace metals in acidified waters. Even man's monuments are deteriorating as airborne acids etch metal and stone features.Sulfates account for about two thirds of airborne acids with wet and dry deposition contributing equally to acids reaching surface waters or ground. The industrial Midwest is widely assumed to be the source of most sulfates reaching the acid-sensitive Northeast since S02 emitted as a byproduct of coal combustion in the Midwest dwarfs S02 emitted from all sources in the Northeast.

Do Greenland Ice Cores Reflect NW European Interglacial Climate Variations?

1995 ◽  
Vol 43 (2) ◽  
pp. 125-132 ◽  
Author(s):  
Eiliv Larsen ◽  
Hans Petter Sejrup ◽  
Sigfus J. Johnsen ◽  
Karen Luise Knudsen
Keyword(s):  
Western Europe ◽  
Ice Core ◽  
Greenland Ice Sheet ◽  
Ice Cores ◽  
High Amplitude ◽  
Atlantic Water ◽  
Polar Front ◽  
Norwegian Sea ◽  
The Holocene ◽  
Climatic Evolution

AbstractThe climatic evolution during the Eemian and the Holocene in western Europe is compared with the sea-surface conditions in the Norwegian Sea and with the oxygen-isotope-derived paleotemperature signal in the GRIP and Renland ice cores from Greenland. The records show a warm phase (ca. 3000 yr long) early in the Eemian (substage 5e). This suggests that the Greenland ice sheet, in general, recorded the climate in the region during this time. Rapid fluctuations during late stage 6 and late substage 5e in the GRIP ice core apparently are not recorded in the climatic proxies from western Europe and the Norwegian Sea. This may be due to low resolution in the terrestrial and marine records and/or long response time of the biotic changes. The early Holocene climatic optimum recorded in the terrestrial and marine records in the Norwegian Sea-NW European region is not found in the Summit (GRIP and GISP2) ice cores. However, this warm phase is recorded in the Renland ice core. Due to the proximity of Renland to the Norwegian Sea, this area is probably more influenced by changes in polar front positions which may partly explain this discrepancy. A reduction in the elevation at Summit during the Holocene may, however, be just as important. The high-amplitude shifts during substage 5e in the GRIP core could be due to Atlantic water oscillating closer to, and also reaching, the coast of East Greenland. During the Holocene, Atlantic water was generally located farther east in the Norwegian Sea than during the Eemian.

scholarly journals Spatial and temporal variability in isotope composition of recent snow in the vicinity of Vostok station, Antarctica: implications for ice-core record interpretation

2002 ◽  
Vol 35 ◽  
pp. 181-186 ◽  
Author(s):  
Alexey A. Ekaykin ◽  
Vladimir Ya. Lipenkov ◽  
Narcisse I. Barkov ◽  
Jean Robert Petit ◽  
Valerie Masson-Delmotte
Keyword(s):  
Isotope Composition ◽  
Ice Core ◽  
Snow Accumulation ◽  
Spatial And Temporal Variability ◽  
Weak Correlation ◽  
Ice Core Record ◽  
Vostok Station ◽  
The Mean ◽  
Mean Annual Air Temperature ◽  
Snow Samples

AbstractContinuous, detailed isotope (δD and δ18O) profiles were obtained from eight snow pits dug in the vicinity of Vostok station, Antarctica, during the period 1984– 2000. In addition, snow samples taken along the 1km long accumulation-stake profile were measured to determine spatial variability in isotope composition of recent snow. the stacked δD time series spanning the last 55 years shows only weak correlation with the mean annual air temperature recorded at Vostok station. Significant oscillations of both snow accumulation and snow isotope composition with the periods 2.5, 5, 20 and, possibly, ~102 years observed at single points are interpreted in terms of drift of snow-accumulation waves of various scales on the surface of the ice sheet.

Reconstructing Antarctic snow accumulation using nitrogen isotopes of nitrate

2021 ◽  
Author(s):  
Pete D. Akers ◽  
Joël Savarino ◽  
Nicolas Caillon ◽  
Mark Curran ◽  
Tas Van Ommen
Keyword(s):  
Nitrogen Isotopes ◽  
Full Range ◽  
Ice Core ◽  
Ice Cores ◽  
Snow Accumulation ◽  
East Antarctica ◽  
Accumulation Rates ◽  
Sea Levels ◽  
Antarctic Snow ◽  
Parallel Reconstruction

<p>Precise Antarctic snow accumulation estimates are needed to understand past and future changes in global sea levels, but standard reconstructions using water isotopes suffer from competing isotopic effects external to accumulation. We present here an alternative accumulation proxy based on the post-depositional photolytic fractionation of nitrogen isotopes (d<sup>15</sup>N) in nitrate. On the high plateau of East Antarctica, sunlight penetrating the uppermost snow layers converts snow-borne nitrate into nitrogen oxide gas that can be lost to the atmosphere. This nitrate loss favors <sup>14</sup>NO<sub>3</sub><sup>-</sup> over <sup>15</sup>NO<sub>3</sub><sup>-</sup>, and thus the d<sup>15</sup>N of nitrate remaining in the snow will steadily increase until the nitrate is eventually buried beneath the reach of light. Because the duration of time until burial is dependent upon the rate of net snow accumulation, sites with lower accumulation rates have a longer burial wait and thus higher d<sup>15</sup>N values. A linear relationship (r<sup>2</sup> = 0.86) between d<sup>15</sup>N and net accumulation<sup>-1</sup> is calculated from over 120 samples representing 105 sites spanning East Antarctica. These sites largely encompass the full range of snow accumulation rates observed in East Antarctica, from 25 kg m-<sup>2</sup> yr<sup>-1</sup> at deep interior sites to >400 kg m-<sup>2</sup> yr<sup>-1</sup> at near coastal sites. We apply this relationship as a transfer function to an Aurora Basin ice core to produce a 700-year record of accumulation changes. Our nitrate-based estimate compares very well with a parallel reconstruction for Aurora Basin that uses volcanic horizons and ice-penetrating radar. Continued improvements to our database may enable precise independent estimates of millennial-scale accumulation changes using deep ice cores such as EPICA Dome C and Beyond EPICA-Oldest Ice.</p>

scholarly journals A 2700-year annual timescale and accumulation history for an ice core from Roosevelt Island, West Antarctica

2017 ◽  
Author(s):  
Mai Winstrup ◽  
Paul Vallelonga ◽  
Helle A. Kjær ◽  
Tyler J. Fudge ◽  
James E. Lee ◽  
...  
Keyword(s):  
Accumulation Rate ◽  
Ice Core ◽  
Early Period ◽  
Volcanic Eruptions ◽  
Snow Accumulation ◽  
Atmospheric Methane ◽  
Accumulation Rates ◽  
West Antarctica ◽  
Ross Ice Shelf ◽  
Accumulation History

Abstract. We present a 2700-year annually resolved timescale for the Roosevelt Island Climate Evolution (RICE) ice core, and reconstruct a past snow accumulation history for the coastal sector of the Ross Ice Shelf in West Antarctica. The timescale was constructed by identifying annual layers in multiple ice-core impurity records, employing both manual and automated counting approaches, and constitutes the top part of the Roosevelt Island Ice Core Chronology 2017 (RICE17). The maritime setting of Roosevelt Island results in high sulfate influx from sea salts and marine biogenic emissions, which prohibits a routine detection of volcanic eruptions in the ice-core records. This led to the use of non-traditional chronological techniques for validating the timescale: RICE was synchronized to the WAIS Divide ice core, on the WD2014 timescale, using volcanic attribution based on direct measurements of ice-core acidity, as well as records of globally-synchronous, centennial-scale variability in atmospheric methane concentrations. The RICE accumulation history suggests stable values of 0.25 m water equivalent (w.e.) per year until around 1260 CE. Uncertainties in the correction for ice flow thinning of annual layers with depth do not allow a firm conclusion about long-term trends in accumulation rates during this early period but from 1260 CE to the present, accumulation rate trends have been consistently negative. The decrease in accumulation rates has been increasingly rapid over the last centuries, with the decrease since 1950 CE being more than 7 times greater than the average over the last 300 years. The current accumulation rate of 0.22 ± 0.06 m w.e. yr−1 (average since 1950 CE, ±1σ) is 1.49 standard deviations (86th percentile) below the mean of 50-year average accumulation rates observed over the last 2700 years.

Ecological Selves and Organizational Leadership Values that Matter

2014 ◽  
Vol 3 (1) ◽  
pp. 1-6 ◽  
Author(s):  
Katrina S. Rogers
Keyword(s):  
Seventeenth Century ◽  
Soil Erosion ◽  
Knowledge Base ◽  
Human Activity ◽  
Natural Environment ◽  
Western Europe ◽  
Industrial Revolution ◽  
Striking Feature ◽  
Natural Systems ◽  
Body Of Knowledge

One striking feature in the sweep of history is the extent to which humans have manipulated the natural environment to serve our needs and our desires. In the early written record, there are tales of deforestation and soil erosion (Plato, 360 BCE). As early as the seventeenth century, natural historians compared the grasslands around villages to inhabited areas and speculated on the consequences of human activity on natural systems ( Goudie, 2006 , p. 3). The onset of the industrial revolution in Western Europe combined with a growing understanding and knowledge base of science has rendered a circumstance of uncontrolled manipulation of the ecosystems and ever finer ways to measure these consequences. This article is an invitation to challenge us as scholars and practitioners to seek understanding as companies and other organizations take up their roles in a world that we are transforming irrevocably. Why does it matter, after all, that we seek to build a body of knowledge around corporate functioning? It is my intention that this article helps us ponder and reflect on that question.

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