scholarly journals Enhancement Thermoelectric Properties of Cux-doped Nanostructure Bi-Sb-Te Thermoelectric Materials by Spark Plasma Sintering

2022 ◽  
Vol 2160 (1) ◽  
pp. 012029
Author(s):  
Zhe Chen ◽  
Wenhua Zhang ◽  
Rui Hu ◽  
Xuelong He ◽  
Guodong Xu ◽  
...  
Keyword(s):  
Spark Plasma Sintering ◽  
Thermoelectric Properties ◽  
Thermoelectric Materials ◽  
Carrier Mobility ◽  
Lattice Thermal Conductivity ◽  
Lattice Vibration ◽  
As Doping ◽  
Plasma Sintering ◽  
Thermoelectric Energy ◽  
Spark Plasma

Abstract Nanostructure Cux-doped Bi0.5Sb1.5-xTe3 thermoelectric materials was successfully prepared by Mechanical alloys and spark plasma sintering. In the reasearch, the crystallinity, particle size, and chemical composition were characterized by XRD, EDS, respectively. Thermoelectric properties with a maximum ZT value up to 1.17 has been obtained at 407 K in prepared Cu0.04-doped Bi0.5Sb1.496Te3 sample. The achieved higher ZT value is attributed that Cu as doping at the Sb sites introduced additional holes to enhance carrier mobility and Cu dopants interrupted the periodicity of lattice vibration to decrease lattice thermal conductivity. It is suggested that the as-prepared nanostructure Cux-doped Bi0.5Sb1.5-xTe3 thermoelectric materials has high potential for thermoelectric energy conversion application.

scholarly journals Thermoelectric properties of Cu3SbSe3 with intrinsically ultralow lattice thermal conductivity

2014 ◽  
Vol 2 (38) ◽  
pp. 15829-15835 ◽  
Author(s):  
Kriti Tyagi ◽  
Bhasker Gahtori ◽  
Sivaiah Bathula ◽  
A. K. Srivastava ◽  
A. K. Shukla ◽  
...  
Keyword(s):  
Thermal Conductivity ◽  
Solid State ◽  
Spark Plasma Sintering ◽  
Thermoelectric Properties ◽  
Solid State Reaction ◽  
Electrical Transport ◽  
Single Phase ◽  
Lattice Thermal Conductivity ◽  
Plasma Sintering ◽  
Spark Plasma

Intrinsically ultra-low thermal conductivity and electrical transport in single-phase Cu2SbSe3 synthesized employing a solid state reaction and spark plasma sintering.

scholarly journals Flash spark plasma sintering of magnesium silicide stannide with improved thermoelectric properties

2017 ◽  
Vol 5 (6) ◽  
pp. 1514-1521 ◽  
Author(s):  
Baoli Du ◽  
Francesco Gucci ◽  
Harshit Porwal ◽  
Salvatore Grasso ◽  
Amit Mahajan ◽  
...  
Keyword(s):  
Spark Plasma Sintering ◽  
Thermoelectric Properties ◽  
Thermoelectric Materials ◽  
Surface Oxidation ◽  
Magnesium Silicide ◽  
Flash Sintering ◽  
Plasma Sintering ◽  
Spark Plasma

Flash sintering is capable of rapid densification of thermoelectric materials with optimised microstructure, conductivity, and distribution of surface oxidation.

THERMOELECTRIC PROPERTIES OF p-TYPE SKUTTERUDITES (Pr0.25Nd0.75)xFe3CoSb12 BY LEVITATION MELTING AND SPARK PLASMA SINTERING

2013 ◽  
Vol 06 (05) ◽  
pp. 1340006 ◽  
Author(s):  
JINGSHU XU ◽  
CHENGUANG FU ◽  
JIAN XIE ◽  
XINBING ZHAO ◽  
TIEJUN ZHU
Keyword(s):  
Thermal Conductivity ◽  
Electrical Conductivity ◽  
Seebeck Coefficient ◽  
Spark Plasma Sintering ◽  
Thermoelectric Properties ◽  
Lattice Thermal Conductivity ◽  
Levitation Melting ◽  
Plasma Sintering ◽  
Spark Plasma ◽  
P Type

The p-type skutterudite compounds of ( Pr 0.25 Nd 0.75)x Fe 3 CoSb 12 (x = 0.67–0.78) have been successfully synthesized by levitation melting followed by annealing and spark plasma sintering. The thermoelectric properties have been characterized by the measurements of Seebeck coefficient, electrical conductivity and thermal conductivity in the temperature range from 300 K to 850 K. The improvement in the thermoelectric properties was realized due to the reduction in the lattice thermal conductivity when the voids were partially filled by Pr 0.25 Nd 0.75. The maximum ZT value of ~ 0.83 for ( Pr 0.25 Nd 0.75)0.76 Fe 3 CoSb 12 was obtained at 700 K.

scholarly journals Thermal Conductivity of A-Site Cation-Deficient La-Substituted SrTiO3 Produced by Spark Plasma Sintering

2015 ◽  
Vol 2 (1-2) ◽  
Author(s):  
Thomas E. Loland ◽  
Jaran Sele ◽  
Mari-Ann Einarsrud ◽  
Per Erik Vullum ◽  
Mats Johnsson ◽  
...  
Keyword(s):  
Thermal Conductivity ◽  
Spark Plasma Sintering ◽  
High Temperatures ◽  
Thermoelectric Properties ◽  
Thermoelectric Materials ◽  
High Stability ◽  
Plasma Sintering ◽  
Spark Plasma ◽  
A Site

AbstractDuring the last decade oxide-based thermoelectric materials have received increased attention due to their high stability and thermal robustness at high temperatures as well as the availability and nontoxic nature of a number of promising candidates. In the present study we are investigating the thermoelectric properties of an n-type La-substituted SrTiO

scholarly journals Effect of Powder Heat Treatment on Chemical Composition and Thermoelectric Properties of Bismuth Antimony Telluride Alloys Fabricated by Combining Water Atomization and Spark Plasma Sintering

Materials ◽  
2021 ◽  
Vol 14 (11) ◽  
pp. 2993
Author(s):  
Dong-won Shin ◽  
Peyala Dharmaiah ◽  
Jun-Woo Song ◽  
Soon-Jik Hong
Keyword(s):  
Spark Plasma Sintering ◽  
Thermoelectric Properties ◽  
Hole Concentration ◽  
Bismuth Antimony Telluride ◽  
Plasma Sintering ◽  
Heat Treated ◽  
Water Atomization ◽  
Powder Samples ◽  
Different Temperatures ◽  
Spark Plasma

In this work, Bi0.5Sb1.5Te3 materials were produced by an economically viable and time efficient water atomization process. The powder samples were heat treated at different temperatures (673 K, 723 K, 743 K, 773 K, 803 K, and 823 K) followed by spark plasma sintering (SPS). It was found that the Te evaporated slightly at 723 K and 743 K and became dominated at 773 K, 803 K, and 823 K, which severely influences the thermoelectric properties. The electrical conductivity was significantly improved for over 803 K heat treated samples due to the remarkable improvement in hole concentration. The power factor values for the 803 K and 823 K samples were significantly larger at T > 350 K compared to other samples. Consequently, the peak ZT of 0.92 at 350 K was obtained for the 803 K sample, which could be useful in commercial thermoelectric power generation.

Thermoelectric properties of Sb-doped Mg2(Si0.95Ge0.05) synthesized by spark plasma sintering

2015 ◽  
Vol 195 ◽  
pp. 45-49 ◽  
Author(s):  
Koya Arai ◽  
Asumi Sasaki ◽  
Yuto Kimori ◽  
Miharu Iida ◽  
Tomoyuki Nakamura ◽  
...  
Keyword(s):  
Spark Plasma Sintering ◽  
Thermoelectric Properties ◽  
Plasma Sintering ◽  
Spark Plasma

Fabrication of Bi-Te Based Thermoelectric Semiconductors by Using Hybrid Powders

2005 ◽  
Vol 297-300 ◽  
pp. 875-880
Author(s):  
Cheol Ho Lim ◽  
Ki Tae Kim ◽  
Yong Hwan Kim ◽  
Dong Choul Cho ◽  
Young Sup Lee ◽  
...  
Keyword(s):  
Mechanical Properties ◽  
Single Crystals ◽  
Thermoelectric Properties ◽  
Thermoelectric Materials ◽  
Figure Of Merit ◽  
Bending Strength ◽  
Mixing Ratio ◽  
Plasma Sintering ◽  
Spark Plasma ◽  
P Type

P-type Bi0.5Sb1.5Te3 compounds doped with 3wt% Te were fabricated by spark plasma sintering and their mechanical and thermoelectric properties were investigated. The sintered compounds with the bending strength of more than 50MPa and the figure-of-merit 2.9×10-3/K were obtained by controlling the mixing ratio of large powders (PL) and small powders (PS). Compared with the conventionally prepared single crystal thermoelectric materials, the bending strength was increased up to more than three times and the figure-of-merit Z was similar those of single crystals. It is expected that the mechanical properties could be improved by using hybrid powders without degradation of thermoelectric properties.

Optimization of the thermoelectric properties of Bi2O2Se ceramics by altering the temperature of spark plasma sintering

2016 ◽  
Vol 37 (1-4) ◽  
pp. 66-72 ◽  
Author(s):  
Xing Tan ◽  
Jin-Le Lan ◽  
Yao-Chun Liu ◽  
Guang-Kun Ren ◽  
Cheng-Cheng Zeng ◽  
...  
Keyword(s):  
Spark Plasma Sintering ◽  
Thermoelectric Properties ◽  
Plasma Sintering ◽  
Spark Plasma
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