Sodium Silicate Based Thermal Interface Material for High Thermal Contact Conductance

1999 ◽  
Vol 122 (2) ◽  
pp. 128-131 ◽  
Author(s):  
Yunsheng Xu ◽  
Xiangcheng Luo ◽  
D. D. L. Chung

Sodium silicate based thermal interface pastes give higher thermal contact conductance across conductor surfaces than polymer based pastes and oils, due to their higher fluidity and the consequent greater conformability. Addition of hexagonal boron nitride particles up to 16.0 vol. percent further increases the conductance of sodium silicate, due to the higher thermal conductivity of BN. However, addition beyond 16.0 vol. percent BN causes the conductance to decrease, due to the decrease in fluidity. At 16.0 vol. percent BN, the conductance is up to 63 percent higher than those given by silicone based pastes and is almost as high as that given by solder. Water is almost as effective as sodium silicate without filler, but the thermal contact conductance decreases with time due to the evaporation of water. Mineral oil and silicone without filler are much less effective than water or sodium silicate without filler. [S1043-7398(00)00402-3]

2006 ◽  
Vol 128 (4) ◽  
pp. 319-323 ◽  
Author(s):  
Zongrong Liu ◽  
D. D. L. Chung

Wax (predominantly tricosane paraffin wax, with a melting temperature of 48°C) filled with hexagonal boron nitride (BN) particles (5-11μm) was found to be an effective phase-change thermal interface material. The thermal contact conductance, as measured with the interface material between copper surfaces, decreased with increasing temperature from 22to48°C, but increased with increasing temperature from 48to55°C. The melting of the wax enhanced the conductance, due to increased conformability to the mating surfaces. For a given BN volume fraction and a given temperature, the thermal contact conductance increased with increasing contact pressure. However, a pressure above 0.30MPa resulted in no significant increase in the conductance. The conductance increased with BN content up to 6.2vol.%, but decreased upon further increase to 8.6vol.%. The highest conductance above the melting temperature was 18×104W∕m2.°C, as attained for a BN content of 4.0vol.% at 55°C and 0.30MPa. Below the melting temperature, the highest conductance was 19×104W∕m2.°C, as attained for a BN content of 6.2vol.% at 22°C and 0.30MPa.


2002 ◽  
Vol 124 (3) ◽  
pp. 188-191 ◽  
Author(s):  
Yunsheng Xu ◽  
Xiangcheng Luo ◽  
D. D. L. Chung

Polyethylene-glycol-based thermal interface paste containing trifluoroacetic acid lithium salt (1.5 wt. percent optimum) and boron nitride particles (∼18.0 vol. percent optimum), as well as water and N, N-dimethylformamide for helping the dissociation of the salt to release Li+ ions, gives thermal contact conductance that is almost as high as that given by Sn-Pb solder, similar to that given by boron nitride particle filled sodium silicate, and much higher than that given by boron nitride particle filled silicone.


2000 ◽  
Vol 123 (3) ◽  
pp. 309-311 ◽  
Author(s):  
Xiangcheng Luo, ◽  
Yunsheng Xu, and ◽  
D. D. L. Chung

Thermal interface pastes based on silicone, lithium doped polyethylene glycol (PEG), and sodium silicate were evaluated in their performance before and after heating up to 120°C. The thermal contact conductance of any of the pastes between copper disks decreased after heating, such that the fractional decrease was less for the silicone-based paste than the PEG-based and sodium-silicate-based pastes. Nevertheless, the conductance was lower for the silicone-based paste than the other pastes both before and after heating up to 100 cycles.


Energies ◽  
2021 ◽  
Vol 14 (4) ◽  
pp. 999
Author(s):  
Yafang Zhang ◽  
Juhua Huang ◽  
Ming Cao ◽  
Guoping Du ◽  
Ziqiang Liu ◽  
...  

Hexagonal boron nitride and silicone rubber (h-BN/SR) composites were prepared by the mechanical stirring method, and their crystal morphology, chemical structure, thermal properties, and compression stress–strain performance were investigated. The experimental results suggest that silicone rubber combined with h-BN exhibits better thermal conductivity and mechanical properties. When the proportion of h-BN is 30 wt%, the thermal conductivity of the h-BN/SR composite material is 0.58 W/m∙K, which is 3.4 times that of pure silicone rubber. At the same time, the compressive strength of h-BN/SR is 4.27 MPa, which is 6.7 times that of pure silicone rubber. Furthermore, the finite element model was employed to numerically analyze the thermal behavior of a battery with a h-BN/SR composite as the thermal interface material. The analytical results show that the highest temperature of the battery decreased when using h-BN/SR as the thermal interface material in the battery thermal management system. The h-BN/SR composite can thus effectively improve the safety properties of batteries.


Author(s):  
U. B. Jayadeep ◽  
R. Krishna Sabareesh ◽  
R. Nirmal ◽  
K. V. Rijin ◽  
C. B. Sobhan

Thermal contact conductance is used to indicate the resistance offered by a contact interface to the flow of heat. When an interface material is applied as nano-layered coatings on super-finished contacting surfaces, the possibility of size effects necessitates the use of a discrete computation method for its analysis. Hence, a methodology is proposed which utilizes Molecular Dynamics (MD) simulations to obtain the size affected thermal conductivity of the interfacial layer, which in turn characterizes the thermal contact conductance behavior. Molecular Dynamics codes have been developed, making use of Sutton-Chen many-body potential, suitable for metallic materials. The model includes the asperities at the contact interface, assuming the asperities to be of a simplified geometry. The paper also presents the validation of the codes developed, and parametric studies on the effect of temperature, number of asperities and the material used for thermal interface coating on the size-affected interfacial conductivity.


2018 ◽  
Vol 7 (4.33) ◽  
pp. 530
Author(s):  
Mazlan Mohamed ◽  
Mohd Nazri Omar ◽  
Mohamad Shaiful Ashrul Ishak ◽  
Rozyanty Rahman ◽  
Zaiazmin Y.N ◽  
...  

Epoxy mixed with others filler for thermal interface material (TIM) had been well conducted and developed. There are problem occurs when previous material were used as matrix material likes epoxy that has non-uniform thickness of thermal interface material produce, time taken for solidification and others. Thermal pad or thermal interface material using graphene as main material to overcome the existing problem and at the same time to increase thermal conductivity and thermal contact resistance. Three types of composite graphene were used for thermal interface material in this research. The sample that contain 10 wt. %, 20 wt. % and 30 wt. % of graphene was used with different contain of graphene oxide (GO).  The thermal conductivity of thermal interface material is both measured and it was found that the increase of amount of graphene used will increase the thermal conductivity of thermal interface material. The highest thermal conductivity is 12.8 W/ (mK) with 30 w. % graphene. The comparison between the present thermal interface material and other thermal interface material show that this present graphene-epoxy is an excellent thermal interface material in increasing thermal conductivity.  


Author(s):  
Jin Cui ◽  
Liang Pan ◽  
Justin A. Weibel

Abstract Pluggable optoelectronic transceiver modules are widely used in the fiber-optic communication infrastructure. It is essential to mitigate thermal contact resistance between the high-power optical module and its riding heat sink in order to maintain the required operation temperature. The pluggable nature of the modules requires dry contact thermal interfaces that permit repeated insertion–disconnect cycles under low compression pressures (∼10–100 kPa). Conventional wet thermal interface materials (TIM), such as greases, or those that require high compression pressures, are not suitable for pluggable operation. Here we demonstrate the use of compliant micro-structured TIM to enhance the thermal contact conductance between an optical module and its riding heat sink under a low compression pressure (20 kPa). The metallized and polymer-coated structures are able to accommodate the surface nonflatness and microscale roughness of the mating surface while maintaining a high effective thermal conductance across the thickness. This dry contact TIM is demonstrated to maintain reliable thermal performance after 100 plug-in and plug-out cycles while under compression.


2018 ◽  
Vol 6 (36) ◽  
pp. 17540-17547 ◽  
Author(s):  
Zhilin Tian ◽  
Jiajia Sun ◽  
Shaogang Wang ◽  
Xiaoliang Zeng ◽  
Shuang Zhou ◽  
...  

A high thermal conductivity boron nitride based thermal interface material was developed by a foam-templated method.


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