Effect of Chemical Composition of Syngas on Combustion Dynamics Inside Bluff-Body Type Turbulent Syngas Combustor

Author(s):  
Nikhil Ashokbhai Baraiya ◽  
Satynarayanan R. Chakravarthy

In the present work, the chemical composition of syngas is changed by varying the H2/CO ratio, to map the change in the acoustic behavior of a bluff-body combustor. It was observed that with increase in hydrogen concentration in the syngas mixture, the frequency shifts to higher modes and the flame structures changes. The flame oscillations are mapped by means of simultaneous high-speed OH* and CO2* chemiluminescence imaging along with dynamic pressure measurement. The plots of spatial distribution of OH* and CO2* intensity are used to understand change in flame structure with change in chemical composition and also to help in understanding the kinetics affecting acoustic behavior of the flame. The change in flow structures with change in chemical composition of fuel is studied by simultaneous high-speed PIV, OH* chemiluminescence and dynamic pressure measurements.

Author(s):  
Nikhil Ashokbhai Baraiya ◽  
Baladandayuthapani Nagarajan ◽  
Satynarayanan R. Chakravarthy

In the present work, the proportion of carbon monoxide to hydrogen is widely varied to simulate different compositions of synthesis gas and the potential of the fuel mixture to excite combustion oscillations in a laboratory-scale turbulent bluff body combustor is investigated. The effect of parameters such as the bluff body location and equivalence ratio on the self-excited acoustic oscillations of the combustor is studied. The flame oscillations are mapped by means of simultaneous high-speed CH* and OH* chemiluminescence imaging along with dynamic pressure measurement. Mode shifts are observed as the bluff body location or the air flow Reynolds number/overall equivalence ratio are varied for different fuel compositions. It is observed that the fuel mixtures that are hydrogen-rich excite high amplitude pressure oscillations as compared to other fuel composition cases. Higher H2 content in the mixture is also capable of exciting significantly higher natural acoustic modes of the combustor so long as CO is present, but not without the latter. The interchangeability factor Wobbe Index is not entirely sufficient to understand the unsteady flame response to the chemical composition.


Author(s):  
Raymond L. Speth ◽  
H. Murat Altay ◽  
Duane E. Hudgins ◽  
Ahmed F. Ghoniem

The combustion dynamics, stability bands and flame structure of syngas flames under different operating conditions are investigated in an atmospheric pressure swirl-stabilized combustor. Pressure measurements and high-speed video data are used to distinguish several operating modes. Increasing the equivalence ratio makes the flame more compact, and in general increases the overall sound pressure level. Very close to the lean blowout limit, a long stable flame anchored to the inner recirculation zone is observed. At higher equivalence ratios, a low frequency, low amplitude pulsing mode associated with the fluid dynamic instabilities of axial swirling flows is present. Further increasing the equivalence ratio produces unstable flames oscillating at frequencies coupled with the acoustic eigenmodes. Additionally, a second unstable mode, coupled with a lower eigen-mode of the system, is observed for flames with CO concentration higher than 50%. As the amount of hydrogen in the fuel is increased, the lean flammability limit is extended and transitions between operating regimes move to lower equivalence ratios.


Author(s):  
Nikhil Ashokbhai Baraiya ◽  
Vikram Ramanan ◽  
Baladandayuthapani Nagarajan ◽  
Chetankumar S Vegad ◽  
S. R. Chakravarthy

Abstract A bluff-body turbulent combustor is mapped for its thermo-acoustic stability across variation in airflow rate, non-dimensionalized as the Reynolds number (Re) and fuel composition. The combustor stability is evaluated for three fuels, namely, pure hydrogen (PH), synthesis natural gas (SNG), and syngas (SG). The combustion dynamics display markedly different behavior across the fuels, in the extent of the unstable region, as well as the observed dominant Eigenvalues. At low Re, SNG displays stable combustion, while SG exhibits high amplitude oscillations at the fundamental duct acoustic mode. As the Re is increased, SNG displays very high amplitude oscillations at the duct acoustic mode, while SG exhibit relatively low amplitude oscillations at the third harmonic. In the case of PH, high amplitude oscillations observed at higher Re at the first harmonic. These peculiarities are investigated in light of the role of mean flame stabilization. The combustion dynamics of fuels is influenced by the global equivalence ratio, as well as the jet momentum ratio. These effects significantly demarcates the dynamics of SNG and SG combustion. This is seen manifested in mean flame structure of flame at high amplitude oscillations, whereby result in SNG flame to be present in the wake, while the SG flame resides in the shear layer. The driving by the flame because of their mean stabilization quantified by a spatial Rayleigh index. It confirms the presence of large driving regions for SNG compared to that of SG, results in the observed differences in amplitude of the oscillations.


Author(s):  
Ryan Blanchard ◽  
A. J. Wickersham ◽  
Lin Ma ◽  
Wing Ng ◽  
Uri Vandsburger

Contemporary tools for experimentation and computational modeling of unsteady and reacting flow open new opportunities for engineering insight into dynamic phenomena. In this article, we describe a novel use of proper orthogonal decomposition (POD) for validation of the unsteady heat release of a turbulent premixed flame stabilized by a vee-gutter bluff-body. Large-eddy simulations were conducted for the same geometry and flow conditions as examined in an experimental rig with chemiluminescence measurements obtained with a high-speed camera. In addition to comparing the experiment to the simulation using traditional time-averaging and pointwise statistical techniques, the dynamic modes of each are isolated using proper orthogonal decomposition (POD) and then compared mode-by-mode against each other. The results show good overall agreement between the shapes and magnitudes of the first modes of the measured and simulated data. A numerical study of into the effects of various simulation parameters on these heat release modes showed significant effects on the flame's effective angle but also on the size, shape, and symmetry patterns of the flame's dynamic modes.


Author(s):  
Farzan Parsinejad ◽  
Christian Arcari ◽  
Edwin Shirk ◽  
Hameed Metghalchi

Burning speed measurement and structure of JP-8 air mixtures at a wide range of temperature and pressure have been studied using two matched constant volume chambers. The experimental facilities include a spherical chamber and cylindrical vessel with glasses at the end caps to enable us visualizing flame structure. Cylindrical vessel is located in a Schlieren set up including spherical mirrors and a high speed CCD camera. Facilities also include and oven which can raise the initial temperature of the mixtures in spherical vessel to 500 K and similar heating elements that perform the same task in cylindrical chamber. A thermodynamic model has been developed to calculate burning speeds using dynamic pressure rise in the chamber. The model considers a central burned gas core of variable temperature surrounded by an unburned gas shell with uniform temperature with a thermal boundary layer at the wall. Burning speed and flame structure of different gaseous fuel-air mixtures have been investigated. Autoignition characteristics of JP-8 air mixtures have also been determined by the sudden pressure rise in spherical vessel.


Energies ◽  
2021 ◽  
Vol 14 (6) ◽  
pp. 1609
Author(s):  
Donghyun Hwang ◽  
Kyubok Ahn

An experimental study was performed to investigate the combustion instability characteristics of swirl-stabilized combustors. A premixed gas composed of ethylene and air was burned under various flow and geometric conditions. Experiments were conducted by changing the inlet mean velocity, equivalence ratio, swirler vane angle, and combustor length. Two dynamic pressure sensors, a hot-wire anemometer, and a photomultiplier tube were installed to detect the pressure oscillations, velocity perturbations, and heat release fluctuations in the inlet and combustion chambers, respectively. An ICCD camera was used to capture the time-averaged flame structure. The objective was to understand the relationship between combustion instability and the Rayleigh criterion/the flame structure. When combustion instability occurred, the pressure oscillations were in-phase with the heat release oscillations. Even if the Rayleigh criterion between the pressure and heat release oscillations was satisfied, stable combustion with low pressure fluctuations was possible. This was explained by analyzing the dynamic flow and combustion data. The root-mean-square value of the heat release fluctuations was observed to predict the combustion instability region better than that of the inlet velocity fluctuations. The bifurcation of the flame structure was a necessary condition for combustion instability in this combustor. The results shed new insight into combustion instability in swirl-stabilized combustors.


Pharmaceutics ◽  
2021 ◽  
Vol 13 (1) ◽  
pp. 119
Author(s):  
Simone A.G. Langeveld ◽  
Inés Beekers ◽  
Gonzalo Collado-Lara ◽  
Antonius F. W. van der Steen ◽  
Nico de Jong ◽  
...  

Phospholipid-coated microbubbles are ultrasound contrast agents that can be employed for ultrasound molecular imaging and drug delivery. For safe and effective implementation, microbubbles must respond uniformly and predictably to ultrasound. Therefore, we investigated how lipid handling and phase distribution affected the variability in the acoustic behavior of microbubbles. Cholesterol was used to modify the lateral molecular packing of 1,2-distearoyl-sn-glycero-3-phosphocholine (DSPC)-based microbubbles. To assess the effect of lipid handling, microbubbles were produced by a direct method, i.e., lipids directly dispersed in an aqueous medium or indirect method, i.e., lipids first dissolved in an organic solvent. The lipid phase and ligand distribution in the microbubble coating were investigated using confocal microscopy, and the acoustic response was recorded with the Brandaris 128 ultra-high-speed camera. In microbubbles with 12 mol% cholesterol, the lipids were miscible and all in the same phase, which resulted in more buckle formation, lower shell elasticity and higher shell viscosity. Indirect DSPC microbubbles had a more uniform response to ultrasound than direct DSPC and indirect DSPC-cholesterol microbubbles. The difference in lipid handling between direct and indirect DSPC microbubbles significantly affected the acoustic behavior. Indirect DSPC microbubbles are the most promising candidate for ultrasound molecular imaging and drug delivery applications.


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