Low-temperature synthesis of oxygen-rich fish-scale-like porous boron nitride for effective water cleaning

Author(s):  
Jie Li ◽  
Mengting Xia ◽  
Lin Zhang ◽  
Junhui Tao ◽  
Chuanhui Wang ◽  
...  

Effective removal of the organic pollutants from aqueous solution is significative and challenging for environmental sustainability. The high-performance adsorbent materials need to be developed. In this study, oxygen-rich fish-scale-like porous boron nitride (O-PBN) was facilely synthesized only at 900[Formula: see text]C (about 400[Formula: see text]C lower than that of the conventional process) through the molten salt method. The adsorption capacity of the as-prepared O-PBN for Methylene Blue (MB) from water was 422.6 mg/g, resulting from oxidizing groups and B–O bonds induced by oxygen doping as well as fish-scale-like structure composed of the BN nanoflakes. Moreover, the initial removal capacity of O-PBN only lost 7.6% even after 10 adsorption–regeneration cycles due to their strong resistance to oxidation. The unique B–O polar covalent bond, fish-scale-like two-dimensional nanostructure exposing the active adsorption sites to the surface ((002) crystal plane) and high specific surface area of O-PBN are confirmed to be the key factors in significantly enhancing water purification and regeneration performance. Overall, the synthetic method should help to a low-temperature and facile fabrication of O-PBN for effective water cleaning.

2013 ◽  
Vol 4 (1) ◽  
Author(s):  
Weiwei Lei ◽  
David Portehault ◽  
Dan Liu ◽  
Si Qin ◽  
Ying Chen

2020 ◽  
Author(s):  
N. P. Boroznina ◽  
M. A. Vdovin ◽  
I. V. Zaporotskova ◽  
S. V. Boroznin ◽  
P. A. Zaporotskov

Proceedings ◽  
2020 ◽  
Vol 65 (1) ◽  
pp. 25
Author(s):  
Antonio Garrido Marijuan ◽  
Roberto Garay ◽  
Mikel Lumbreras ◽  
Víctor Sánchez ◽  
Olga Macias ◽  
...  

District heating networks deliver around 13% of the heating energy in the EU, being considered as a key element of the progressive decarbonization of Europe. The H2020 REnewable Low TEmperature District project (RELaTED) seeks to contribute to the energy decarbonization of these infrastructures through the development and demonstration of the following concepts: reduction in network temperature down to 50 °C, integration of renewable energies and waste heat sources with a novel substation concept, and improvement on building-integrated solar thermal systems. The coupling of renewable thermal sources with ultra-low temperature district heating (DH) allows for a bidirectional energy flow, using the DH as both thermal storage in periods of production surplus and a back-up heating source during consumption peaks. The ultra-low temperature enables the integration of a wide range of energy sources such as waste heat from industry. Furthermore, RELaTED also develops concepts concerning district heating-connected reversible heat pump systems that allow to reach adequate thermal levels for domestic hot water as well as the use of the network for district cooling with high performance. These developments will be demonstrated in four locations: Estonia, Serbia, Denmark, and Spain.


2021 ◽  
Vol 60 (16) ◽  
pp. 8813-8817
Author(s):  
Shuting Pang ◽  
Zhiqiang Wang ◽  
Xiyue Yuan ◽  
Langheng Pan ◽  
Wanyuan Deng ◽  
...  

2021 ◽  
Vol 332 ◽  
pp. 129512
Author(s):  
Yingman Bian ◽  
Li Li ◽  
Hongjie Song ◽  
Yingying Su ◽  
Yi Lv

Solar RRL ◽  
2021 ◽  
pp. 2100108
Author(s):  
Shih-Chi Yang ◽  
Jordi Sastre ◽  
Maximilian Krause ◽  
Xiaoxiao Sun ◽  
Ramis Hertwig ◽  
...  

2021 ◽  
Vol 13 (1) ◽  
Author(s):  
Muhammad Naqi ◽  
Kyung Hwan Choi ◽  
Hocheon Yoo ◽  
Sudong Chae ◽  
Bum Jun Kim ◽  
...  

AbstractLow-temperature-processed semiconductors are an emerging need for next-generation scalable electronics, and these semiconductors need to feature large-area fabrication, solution processability, high electrical performance, and wide spectral optical absorption properties. Although various strategies of low-temperature-processed n-type semiconductors have been achieved, the development of high-performance p-type semiconductors at low temperature is still limited. Here, we report a unique low-temperature-processed method to synthesize tellurium nanowire networks (Te-nanonets) over a scalable area for the fabrication of high-performance large-area p-type field-effect transistors (FETs) with uniform and stable electrical and optical properties. Maximum mobility of 4.7 cm2/Vs, an on/off current ratio of 1 × 104, and a maximum transconductance of 2.18 µS are achieved. To further demonstrate the applicability of the proposed semiconductor, the electrical performance of a Te-nanonet-based transistor array of 42 devices is also measured, revealing stable and uniform results. Finally, to broaden the applicability of p-type Te-nanonet-based FETs, optical measurements are demonstrated over a wide spectral range, revealing an exceptionally uniform optical performance.


2021 ◽  
Vol 412 ◽  
pp. 127034
Author(s):  
Yang Yu ◽  
Zhuoya Ren ◽  
Qianqian Shang ◽  
Jiangang Han ◽  
Lei Li ◽  
...  

Nanomaterials ◽  
2021 ◽  
Vol 11 (7) ◽  
pp. 1738
Author(s):  
Saeid Vafaei ◽  
Alexander Wolosz ◽  
Catlin Ethridge ◽  
Udo Schnupf ◽  
Nagisa Hattori ◽  
...  

SnO2 nanoparticles are regarded as attractive, functional materials because of their versatile applications. SnO2 nanoaggregates with single-nanometer-scale lumpy surfaces provide opportunities to enhance hetero-material interfacial areas, leading to the performance improvement of materials and devices. For the first time, we demonstrate that SnO2 nanoaggregates with oxygen vacancies can be produced by a simple, low-temperature sol-gel approach combined with freeze-drying. We characterize the initiation of the low-temperature crystal growth of the obtained SnO2 nanoaggregates using high-resolution transmission electron microscopy (HRTEM). The results indicate that Sn (II) hydroxide precursors are converted into submicrometer-scale nanoaggregates consisting of uniform SnO2 spherical nanocrystals (2~5 nm in size). As the sol-gel reaction time increases, further crystallization is observed through the neighboring particles in a confined part of the aggregates, while the specific surface areas of the SnO2 samples increase concomitantly. In addition, X-ray photoelectron spectroscopy (XPS) measurements suggest that Sn (II) ions exist in the SnO2 samples when the reactions are stopped after a short time or when a relatively high concentration of Sn (II) is involved in the corresponding sol-gel reactions. Understanding this low-temperature growth of 3D SnO2 will provide new avenues for developing and producing high-performance, photofunctional nanomaterials via a cost-effective and scalable method.


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