scholarly journals UV Sensitivity to Changes in Ozone, Aerosols, and Clouds in Seoul, South Korea

2014 ◽  
Vol 53 (2) ◽  
pp. 310-322 ◽  
Author(s):  
Woogyung Kim ◽  
Jhoon Kim ◽  
Sang Seo Park ◽  
Hi-Ku Cho

AbstractThe total ozone (O3) and aerosol optical depth (AOD) at 320 nm have been observed from the ultraviolet (UV) measurements made at Yonsei University in Seoul, South Korea, with Dobson and Brewer spectrophotometers, respectively, during 2004–10. The daily datasets are analyzed to show the sensitivities of UV radiation to changes in O3, AOD, and cloud cover (CC) together with global solar radiation (GS), including the long-term characteristics of surface UV irradiance in Seoul. The UV sensitivities show that 1% increases of O3 and AOD relative to their reference values under all- and clear-sky conditions similarly manifest as 1–1.2% and 0.2% decreases of both daily erythemal UV (EUV) and total UV (TUV) irradiance at the ground level except for TUV sensitivity to O3 (~0.3%). Those UV sensitivities to CC and GS changes are associated with a 0.12% decrease and 0.7% increase, respectively, in fractional UV changes. The trends show that the positive trends of O3 (+7.2% decade−1), AOD (+22.4% decade−1), and CC (+52.4% decade−1) induce negative trends in EUV (−8.4% decade−1) and TUV (−2.5% decade−1), in both UV (−4.7% decade−1), and in EUV (−6.3% decade−1) and TUV (−6.8% decade−1), respectively. On the basis of the multiple linear regression analyses, it is found that UV sensitivity to O3 is relatively high in the forcing factors, but the contributions of the UV forcing factors to the daily variability and the range of UV disturbances due to the variability of the forcing factors are affected more by AOD than by O3 and CC in both UV fractional changes.

2008 ◽  
Vol 8 (23) ◽  
pp. 7033-7043 ◽  
Author(s):  
S. Simic ◽  
P. Weihs ◽  
A. Vacek ◽  
H. Kromp-Kolb ◽  
M. Fitzka

Abstract. The influence of variability of atmospheric parameters on short- and long-term changes of spectral UV irradiance measured at the Sonnblick observatory (47.03° N, 12.57° E, 3106 m) during the period from 1994 to 2006 is studied. Measurements were performed with the Brewer #093 single-monochromator spectrophotometer and with a Bentham DM 150 spectroradiometer (double-monochromator). The influence of ozone, albedo, snowline and clouds on UV variability is evaluated for each parameter separately using 10-year climatology. It is found that the effect of total ozone on short-term variability of UV irradiance at 305 nm can be more than 200% and on average more than 50%. Clouds can cause variability of 150% or more and on average 35%. Variability caused by albedo reaches a maximum of 32% in April (6% on average). In summer and autumn, total ozone and clouds strongly influence the variability of UV radiation, whereas in winter and spring ozone has the more pronounced effect. A decrease in snowline height from 3000 m to 800 m a.s.l. enhances the UV irradiance by a factor of 1.24 for clear sky conditions and by a factor of 1.7 for 8/8 cloud cover. Long-term trends are investigated for the time period from 1994 to 2006 based on clear-sky measurements, using the non-parametric Mann-Kendall trend test. Significant downward trends (99% confidence level) are found for solar zenith angle 55° at wavelengths from 305 nm to 324 nm and erythemally weighted irradiance according to CIE, which are caused by an increase in sunshine duration during periods of high total column ozone. Significant trends (90% confidence level) were also found for other combinations of wavelength and SZA.


2016 ◽  
Vol 16 (4) ◽  
pp. 2493-2505 ◽  
Author(s):  
Ilias Fountoulakis ◽  
Alkiviadis F. Bais ◽  
Konstantinos Fragkos ◽  
Charickleia Meleti ◽  
Kleareti Tourpali ◽  
...  

Abstract. In this study, we discuss the short- and the long-term variability of spectral UV irradiance at Thessaloniki, Greece, using a long, quality-controlled data set from two Brewer spectrophotometers. Long-term changes in spectral UV irradiance at 307.5, 324 and 350 nm for the period 1994–2014 are presented for different solar zenith angles and discussed in association with changes in total ozone column (TOC), aerosol optical depth (AOD) and cloudiness observed in the same period. Positive changes in annual mean anomalies of UV irradiance, ranging from 2 to 6 % per decade, have been detected both for clear- and all-sky conditions. The changes are generally greater for larger solar zenith angles and for shorter wavelengths. For clear-skies, these changes are, in most cases, statistically significant at the 95 % confidence limit. Decreases in the aerosol load and weakening of the attenuation by clouds lead to increases in UV irradiance in the summer, of 7–9 % per decade for 64° solar zenith angle. The increasing TOC in winter counteracts the effect of decreasing AOD for this particular season, leading to small, statistically insignificant, negative long-term changes in irradiance at 307.5 nm. Annual mean UV irradiance levels are increasing from 1994 to 2006 and remain relatively stable thereafter, possibly due to the combined changes in the amount and optical properties of aerosols. However, no statistically significant corresponding turning point has been detected in the long-term changes of AOD. The absence of signatures of changes in AOD in the short-term variability of irradiance in the UV-A may have been caused by changes in the single scattering albedo of aerosols, which may counteract the effects of changes in AOD on irradiance. The anti-correlation between the year-to-year variability of the irradiance at 307.5 nm and TOC is clear and becomes clearer as the AOD decreases.


2015 ◽  
Vol 15 (24) ◽  
pp. 35753-35785
Author(s):  
I. Fountoulakis ◽  
A. F. Bais ◽  
K. Fragkos ◽  
C. Meleti ◽  
K. Tourpali ◽  
...  

Abstract. In this study, we discuss the short- and the long-term variability of spectral UV irradiance at Thessaloniki, Greece using a long, quality-controlled data set from two Brewer spectrophotometers. Long-term changes in spectral UV irradiance at 307.5, 324 and 350 nm for the period 1994–2014 are presented for different solar zenith angles and discussed in association to changes in total ozone column (TOC), aerosol optical depth (AOD) and cloudiness observed in the same period. Positive changes in annual mean anomalies of UV irradiance, ranging from 2 to 6 % per decade, have been detected both for clear- and all-sky conditions. The changes are generally greater for larger solar zenith angles and for shorter wavelengths. For clear skies, these changes are, in most cases, statistically significant at the 95 % confidence limit. Decreases in the aerosol load and weakening of the attenuation by clouds lead to increases in UV irradiance in the summer, of 7–9 % per decade for 64° solar zenith angle. The increasing TOC in winter counteracts the effect of decreasing AOD for this particular season, leading to small, statistically insignificant, negative long-term changes in irradiance at 307.5 nm. Annual mean UV irradiance levels are increasing from 1994 to 2006 and remain relatively stable thereafter, possibly due to the combined changes in the amount and optical properties of aerosols. However, no statistically significant corresponding turning point has been detected in the long-term changes of AOD. Trends in irradiance during the two sub-periods are not discussed, because the length of the two datasets is too short for deriving statistically significant estimates. The absence of signatures of changes in AOD in the short-term variability of irradiance in the UV-A may have been caused by changes in the single scattering albedo of aerosols, which may counteract the effects of changes in AOD on irradiance. The anti-correlation between the year-to-year variability of the irradiance at 307.5 nm and TOC is clear and becomes clearer as the AOD decreases.


2008 ◽  
Vol 8 (16) ◽  
pp. 4517-4528 ◽  
Author(s):  
V. Buchard ◽  
C. Brogniez ◽  
F. Auriol ◽  
B. Bonnel ◽  
J. Lenoble ◽  
...  

Abstract. Ozone Monitoring Instrument (OMI), launched in July 2004, is dedicated to the monitoring of the Earth's ozone, air quality and climate. OMI is the successor of the Total Ozone Mapping Spectrometer (TOMS) instruments and provides among other atmospheric and radiometric quantities the total column of ozone (TOC), the surface ultraviolet (UV) irradiance at several wavelengths, the erythemal dose rates and the erythemal daily doses. The main objective of this work is to compare OMI data with data from ground-based instruments in order to use OMI products (collection 2) for scientific studies. The Laboratoire d'Optique Atmosphérique (LOA) located in Villeneuve d'Ascq (VdA) in the north of France performs solar UV measurements using a spectroradiometer. The site of Briançon in the French Southern Alps is also equipped with a spectroradiometer operated by Interaction Rayonnement Solaire Atmosphère (IRSA). The OMI total ozone column data is obtained from the OMI-TOMS and OMI-DOAS algorithms. The comparison between the TOC retrieved with ground-based measurements and OMI-TOMS data shows good agreement at both sites for all sky conditions with a relative difference for most of points better than 5%. For OMI-DOAS data, the agreement is generally better than 7% and these data show a significant dependence on solar zenith angle. Comparisons of spectral UV on clear sky conditions are also satisfying with relative differences smaller than 10% except at solar zenith angles larger than 65°. On the contrary, results of comparisons of the erythemal dose rates and erythemal daily doses for clear sky show that OMI overestimates surface UV doses at VdA by about 15% and that on cloudy skies, the bias increases. At Briançon, such a bias is observed if data corresponding to snow-covered surface are excluded.


2016 ◽  
Author(s):  
Lubna Dada ◽  
Pauli Paasonen ◽  
Tuomo Nieminen ◽  
Stephany Buenrostro Mazon ◽  
Jenni Kontkanen ◽  
...  

Abstract. New particle formation (NPF) events have been observed all around the world and are known to be a major source of atmospheric aerosol particles. Here we combine 20 years of observations in a boreal forest at the SMEAR II station (Station for Measuring Ecosystem-Atmosphere Relations) in Hyytiälä, Finland, by utilizing previously accumulated knowledge, and by focusing on clear-sky (non-cloudy) conditions. We first investigated the effect of cloudiness on NPF and then compared the NPF event and non-event days during clear-sky conditions. In this comparison we considered, for example, the effects of calculated particle formation rates, condensation sink, trace gas concentrations and various meteorological quantities. The formation rate of 1.5 nm particles was calculated by using proxies for gaseous sulfuric acid and oxidized products of low volatile organic compounds. As expected, our results indicate an increase in the frequency of NPF events under clear-sky conditions. Also, focusing on clearsky conditions enabled us to find a clear separation of many variables related to NPF. For instance, oxidized organic vapors showed higher concentration during the clear-sky NPF event days, whereas the condensation sink (CS) and some trace gases had higher concentrations during the non-event days. The calculated formation rate of 3 nm particles showed a notable difference between the NPF event and non-event days during clear-sky conditions, especially in winter and spring. For spring time, we are able to find a threshold value for the combined values of ambient temperature and CS, above which practically no clear-sky NPF event could be observed. Finally, we present a probability distribution for the frequency of NPF events at a specific CS and temperature.


2019 ◽  
Vol 76 (11) ◽  
pp. 3485-3504 ◽  
Author(s):  
Carsten Abraham ◽  
Adam H. Monahan

Abstract In a companion paper hidden Markov model (HMM) analyses have been conducted to classify the nocturnal stably stratified boundary layer (SBL) into weakly stable (wSBL) and very stable (vSBL) conditions at different tower sites on the basis of long-term Reynolds-averaged mean data. The resulting HMM regime sequences allow analysis of long-term (climatological) SBL regime statistics. In particular, statistical features of very persistent wSBL and vSBL nights, in which a single regime lasts for the entire night, are contrasted with those of nights with SBL regime transitions. The occurrence of very persistent nights is seasonally dependent and more likely in homogeneous surroundings than in regions with complex terrain. When transitions occur, their timing is not seasonally dependent, but transitions are enhanced close to sunset (for land-based sites). The regime event durations depict remarkably similar distributions across all stations with peaks in transition likelihood approximately 1–2 h after a preceding transition. At Cabauw in the Netherlands, very persistent wSBL and vSBL nights are usually accompanied by overcast conditions with strong geostrophic winds Ugeo or clear-sky conditions with weak Ugeo, respectively. In contrast, SBL regime transitions can neither be linked to magnitudes in Ugeo and cloud coverage nor to specific tendencies in Ugeo. However, regime transitions can be initiated by changes in low-level cloud cover.


2018 ◽  
Vol 10 (10) ◽  
pp. 1651 ◽  
Author(s):  
Bikhtiyar Ameen ◽  
Heiko Balzter ◽  
Claire Jarvis ◽  
Etienne Wey ◽  
Claire Thomas ◽  
...  

Several sectors need global horizontal irradiance (GHI) data for various purposes. However, the availability of a long-term time series of high quality in situ GHI measurements is limited. Therefore, several studies have tried to estimate GHI by re-analysing climate data or satellite images. Validation is essential for the later use of GHI data in the regions with a scarcity of ground-recorded data. This study contributes to previous studies that have been carried out in the past to validate HelioClim-3 version 5 (HC3v5) and the Copernicus Atmosphere Monitoring Service, using radiation service version 3 (CRSv3) data of hourly GHI from satellite-derived datasets (SDD) with nine ground stations in northeast Iraq, which have not been used previously. The validation is carried out with station data at the pixel locations and two other data points in the vicinity of each station, which is something that is rarely seen in the literature. The temporal and spatial trends of the ground data are well captured by the two SDDs. Correlation ranges from 0.94 to 0.97 in all-sky and clear-sky conditions in most cases, while for cloudy-sky conditions, it is between 0.51–0.72 and 0.82–0.89 for the clearness index. The bias is negative for most of the cases, except for three positive cases. It ranges from −7% to 4%, and −8% to 3% for the all-sky and clear-sky conditions, respectively. For cloudy-sky conditions, the bias is positive, and differs from one station to another, from 16% to 85%. The root mean square error (RMSE) ranges between 12–20% and 8–12% for all-sky and clear-sky conditions, respectively. In contrast, the RMSE range is significantly higher in cloudy-sky conditions: above 56%. The bias and RMSE for the clearness index are nearly the same as those for the GHI for all-sky conditions. The spatial variability of hourly GHI SDD differs only by 2%, depending on the station location compared to the data points around each station. The variability of two SDDs is quite similar to the ground data, based on the mean and standard deviation of hourly GHI in a month. Having station data at different timescales and the small number of stations with GHI records in the region are the main limitations of this analysis.


2012 ◽  
Vol 12 (5) ◽  
pp. 2469-2477 ◽  
Author(s):  
C. S. Zerefos ◽  
K. Tourpali ◽  
K. Eleftheratos ◽  
S. Kazadzis ◽  
C. Meleti ◽  
...  

Abstract. This study examines the long-term variability of UV solar irradiances at 305 nm and 325 nm over selected sites in Canada, Europe and Japan. Site selection was restricted to the availability of the most complete UV spectroradiometric datasets during the period 1990–2011. The analysis includes the long-term variability of total ozone, aerosol optical depth and cloud fraction at the sites studied. The results, based on observations and modeling, suggest that over Canada, Europe and Japan the period under study can be divided into three sub-periods of scientific merit: the first period (1991–1994) is the period perturbed by the Pinatubo volcanic eruption, during which excess volcanic aerosol has enhanced the "conventional" amplification factor of UV-B at ground level by an additional factor that depends on solar elevation. The increase of the UV-B amplification factor is the result of enhanced scattering processes caused by the injection of huge amounts of volcanic aerosols during the perturbed period. The second period (1995–2006) is characterized by a 0.14% yr−1 increase in total ozone and an increasing trend in spectral irradiance by 0.94% yr−1 at 305 nm and 0.88% yr−1 at 325 nm. That paradox was caused by the significant decline of the aerosol optical depth by more than 1% yr−1 (the "brightening" effect) and the absence of any statistically significant trend in the cloud fraction. The third period (2007–2011) shows statistically significant evidence of a slowdown or even a turning point in the previously reported upward UV-B trends over Canada, Europe and Japan.


2013 ◽  
Vol 31 (5) ◽  
pp. 795-804 ◽  
Author(s):  
X. Xia

Abstract. This study aims to investigate the effect of total cloud cover (TCC) and sunshine duration (SSD) in the variation of diurnal temperature range (DTR) in China during 1954–2009. As expected, the inter-annual variation of DTR was mainly determined by TCC. Analysis of trends of 30-year moving windows of DTR and TCC time series showed that TCC changes could account for that of DTR in some cases. However, TCC decreased during 1954–2009, which did not support DTR reduction across China. DTRs under sky conditions such as clear, cloudy and overcast showed nearly the same decreasing rate that completely accounted for the overall DTR reduction. Nevertheless, correlation between SSD and DTR was weak and not significant under clear sky conditions in which aerosol direct radiative effect should be dominant. Furthermore, 30–60% of DTR reduction was associated with DTR decrease under overcast conditions in south China. This implies that aerosol direct radiative effect appears not to be one of the main factors determining long-term changes in DTR in China.


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