scholarly journals A Novel High-Throughput Chaotic Advection Microreactor for the Preparation of Uniform BaSO4 Nanoparticles

2021 ◽  
Author(s):  
Hua Yang ◽  
Shi-Xiao Wei ◽  
Han Chen ◽  
Lang Chen ◽  
Chak-tong Au ◽  
...  
Keyword(s):  
High Throughput ◽  
Three Dimensional ◽  
Volumetric Flow Rate ◽  
Secondary Flows ◽  
Chaotic Advection ◽  
Narrow Particle Size Distribution ◽  
Chaotic Mixing ◽  
Mixing Efficiency ◽  
Size Uniformity ◽  
Average Size

Owing to high mixing efficiency, microreactors are used to synthesize uniform BaSO4 nanoparticles, but application in industrial scale is limited due to poor throughput. In this work, a high-throughput passive four-stage asymmetric oscillating feedback microreactor using chaotic mixing mechanism was developed to prepare BaSO4 nanoparticles of high size uniformity. Three-dimensional unsteady simulations showed that chaotic mixing could be induced by three unique secondary flows (i.e., vortex, recirculation, and oscillation), and the fluid oscillation mechanism was examined in detail. Simulations and Villermaux-Dushman experiments indicate that almost complete mixing in molecular level could be achieved when total volumetric flow rate Qtotal was larger than 10 mL/min, and the prepared BaSO4 nanoparticles were with narrow particle size distribution (PSD). Through the adjustment of Qtotal and reactant concentrations, it is easy to control the average size. An average size of 26 nm with narrow PSD could be achieved at Qtotal = 160 mL/min.

Three Dimensional Triangle Chaotic Micromixer

2014 ◽  
Vol 875-877 ◽  
pp. 1189-1193 ◽  
Author(s):  
Lin Li ◽  
Qing De Chen ◽  
C.T. Tsai
Keyword(s):  
Numerical Investigation ◽  
Three Dimensional ◽  
Microfluidic System ◽  
Chaotic Advection ◽  
Mixing Efficiency ◽  
Mixing Index ◽  
Ansys Fluent ◽  
Essential Component ◽  
Highly Efficient

Micromixer is essential component of microfluidic system which has wide application in the field of chemistry and biochemistry. A highly efficient and easily fabricated three dimensional micromixer based on chaotic advection is proposed and investigated. The depth of 25μm for each layer of micromixer and two kinds of fluids, which have viscosities of 0.00097kgm-1s-1and 0.186kgm-1s-1with Re number from 0.001 to 150, are adopted for numerical investigation of mixing efficiency by using ANSYS-Fluent. High mixing index of more than 90% can be obtained by using less than 300μm of length under Re number of 0.01 for mixing Fluid 1. However, it requires 850μm to achieve mixing index of more than 90% for hard-to-mix Fluid 2.

Particle Transport via Three-Dimensional Chaotic Advection to Produce Electrically Conducting Plastics With Powder Additives

1999 ◽  
Author(s):  
R. I. Danescu ◽  
D. A. Zumbrunnen
Keyword(s):  
Carbon Black ◽  
Three Dimensional ◽  
Chaotic Advection ◽  
Chaotic Mixing ◽  
Complex Structures ◽  
Two Dimensional ◽  
Electrical Measurements ◽  
Electrically Conducting ◽  
Scale Structures ◽  
Large Clusters

Abstract Extended micron-scale structures were produced in thermoplastic melts from initially large clusters of conducting carbon black particles transported by three-dimensional chaotic mixing. The structures formed networks that were captured by solidification and rendered the composite materials electrically conducting. A systematic study was carried out to assess the influence of key parameters and relate the electrical properties to the microstructures. Micrographs showed complex structures exhibiting patterns characteristic of chaos. Electrical measurements indicated that conductivity was achieved at carbon black concentrations significantly lower than achievable by common mixing methods, and lower than reported recently for two-dimensional chaotic mixing.

The Influence of Blade Wakes on the Performance of Interturbine Diffusers

1996 ◽  
Vol 118 (2) ◽  
pp. 347-352 ◽  
Author(s):  
R. G. Dominy ◽  
D. A. Kirkham
Keyword(s):  
Performance Modeling ◽  
Three Dimensional ◽  
Secondary Flows ◽  
Two Dimensional ◽  
Correct Performance ◽  
Analysis Methods ◽  
Flow Factor ◽  
The Mean ◽  
Lp Turbine

Interturbine diffusers provide continuity between HP and LP turbines while diffusing the flow upstream of the LP turbine. Increasing the mean turbine diameter offers the potential advantage of reducing the flow factor in the following stages, leading to increased efficiency. The flows associated with these interturbine diffusers differ from those in simple annular diffusers both as a consequence of their high-curvature S-shaped geometry and of the presence of wakes created by the upstream turbine. It is shown that even the simplest two-dimensional wakes result in significantly modified flows through such ducts. These introduce strong secondary flows demonstrating that fully three-dimensional, viscous analysis methods are essential for correct performance modeling.

scholarly journals A Numerical Study of Sub-Millisecond Integrated Mix-and-Inject Microfluidic Devices for Sample Delivery at Synchrotron and XFELs

2021 ◽  
Vol 11 (8) ◽  
pp. 3404
Author(s):  
Majid Hejazian ◽  
Eugeniu Balaur ◽  
Brian Abbey
Keyword(s):  
Molecular Dynamics ◽  
Flow Rate ◽  
Numerical Study ◽  
Three Dimensional ◽  
Microfluidic Devices ◽  
Liquid Jets ◽  
Mixing Efficiency ◽  
X Ray Diffraction ◽  
Cross Sectional ◽  
Time Required

Microfluidic devices which integrate both rapid mixing and liquid jetting for sample delivery are an emerging solution for studying molecular dynamics via X-ray diffraction. Here we use finite element modelling to investigate the efficiency and time-resolution achievable using microfluidic mixers within the parameter range required for producing stable liquid jets. Three-dimensional simulations, validated by experimental data, are used to determine the velocity and concentration distribution within these devices. The results show that by adopting a serpentine geometry, it is possible to induce chaotic mixing, which effectively reduces the time required to achieve a homogeneous mixture for sample delivery. Further, we investigate the effect of flow rate and the mixer microchannel size on the mixing efficiency and minimum time required for complete mixing of the two solutions whilst maintaining a stable jet. In general, we find that the smaller the cross-sectional area of the mixer microchannel, the shorter the time needed to achieve homogeneous mixing for a given flow rate. The results of these simulations will form the basis for optimised designs enabling the study of molecular dynamics occurring on millisecond timescales using integrated mix-and-inject microfluidic devices.

scholarly journals Steady flow separation patterns in a 45 degree junction

2000 ◽  
Vol 411 ◽  
pp. 1-38 ◽  
Author(s):  
C. ROSS ETHIER ◽  
SUJATA PRAKASH ◽  
DAVID A. STEINMAN ◽  
RICHARD L. LEASK ◽  
GREGORY G. COUCH ◽  
...  
Keyword(s):  
Flow Separation ◽  
Stokes Equations ◽  
Bypass Graft ◽  
Three Dimensional ◽  
Symmetry Plane ◽  
Axial Flow ◽  
Reynolds Numbers ◽  
Secondary Flows ◽  
Measured Velocity ◽  
Curved Tube

Numerical and experimental techniques were used to study the physics of flow separation for steady internal flow in a 45° junction geometry, such as that observed between two pipes or between the downstream end of a bypass graft and an artery. The three-dimensional Navier–Stokes equations were solved using a validated finite element code, and complementary experiments were performed using the photochromic dye tracer technique. Inlet Reynolds numbers in the range 250 to 1650 were considered. An adaptive mesh refinement approach was adopted to ensure grid-independent solutions. Good agreement was observed between the numerical results and the experimentally measured velocity fields; however, the wall shear stress agreement was less satisfactory. Just distal to the ‘toe’ of the junction, axial flow separation was observed for all Reynolds numbers greater than 250. Further downstream (approximately 1.3 diameters from the toe), the axial flow again separated for Re [ges ] 450. The location and structure of axial flow separation in this geometry is controlled by secondary flows, which at sufficiently high Re create free stagnation points on the model symmetry plane. In fact, separation in this flow is best explained by a secondary flow boundary layer collision model, analogous to that proposed for flow in the entry region of a curved tube. Novel features of this flow include axial flow separation at modest Re (as compared to flow in a curved tube, where separation occurs only at much higher Re), and the existence and interaction of two distinct three-dimensional separation zones.

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