scholarly journals Calculation of NH3 Emissions, Evaluation of Backward Lagrangian Stochastic Dispersion Model and Aerodynamic Gradient Method

Atmosphere ◽  
2021 ◽  
Vol 12 (1) ◽  
pp. 102
Author(s):  
Jesper Nørlem Kamp ◽  
Christoph Häni ◽  
Tavs Nyord ◽  
Anders Feilberg ◽  
Lise Lotte Sørensen

Two campaigns measuring ammonia (NH3) emissions with different measurement techniques were performed on a large grass field (26 ha) after the application of liquid animal manure. The aim was to compare emissions from a confined area estimated from either (i) concentration measurements, both point and line-integrated measurements, combined with backward Lagrangian stochastic (bLS) dispersion modeling or by (ii) estimation of the vertical flux by the aerodynamic gradient method (AGM) with and without footprint correction approximated by the bLS model estimates of the flux footprint. The objective of the comparison is to establish the best practice to derive NH3 emissions from a large field. NH3 emissions derived from bLS agreed well when comparing point and line-integrated measurements. Simple point measurements combined with bLS yield good emission estimations for the confined area. Without footprint correction, the AGM underestimates the emissions by up to 9% compared to the footprint-corrected AGM results. The sensitivity of the measurement methods makes it possible to quantify NH3 emissions with diurnal patterns even five days after a field application of liquid animal manure under wet conditions. The bLS model proves to be a strong tool to determine the NH3 emissions from point concentration measurements inside a large field after a slurry application.

2021 ◽  
pp. 128106
Author(s):  
Arezoo Dadrasnia ◽  
Isabella de Bona Muñoz ◽  
Eduardo Hernandez Yáñez ◽  
Imane Uald Lamkaddam ◽  
Mabel Mora ◽  
...  

2011 ◽  
Vol 11 (9) ◽  
pp. 4333-4351 ◽  
Author(s):  
A. Stohl ◽  
A. J. Prata ◽  
S. Eckhardt ◽  
L. Clarisse ◽  
A. Durant ◽  
...  

Abstract. The April–May, 2010 volcanic eruptions of Eyjafjallajökull, Iceland caused significant economic and social disruption in Europe whilst state of the art measurements and ash dispersion forecasts were heavily criticized by the aviation industry. Here we demonstrate for the first time that large improvements can be made in quantitative predictions of the fate of volcanic ash emissions, by using an inversion scheme that couples a priori source information and the output of a Lagrangian dispersion model with satellite data to estimate the volcanic ash source strength as a function of altitude and time. From the inversion, we obtain a total fine ash emission of the eruption of 8.3 ± 4.2 Tg for particles in the size range of 2.8–28 μm diameter. We evaluate the results of our model results with a posteriori ash emissions using independent ground-based, airborne and space-borne measurements both in case studies and statistically. Subsequently, we estimate the area over Europe affected by volcanic ash above certain concentration thresholds relevant for the aviation industry. We find that during three episodes in April and May, volcanic ash concentrations at some altitude in the atmosphere exceeded the limits for the "Normal" flying zone in up to 14 % (6–16 %), 2 % (1–3 %) and 7 % (4–11 %), respectively, of the European area. For a limit of 2 mg m−3 only two episodes with fractions of 1.5 % (0.2–2.8 %) and 0.9 % (0.1–1.6 %) occurred, while the current "No-Fly" zone criterion of 4 mg m−3 was rarely exceeded. Our results have important ramifications for determining air space closures and for real-time quantitative estimations of ash concentrations. Furthermore, the general nature of our method yields better constraints on the distribution and fate of volcanic ash in the Earth system.


2021 ◽  
Author(s):  
Alistair Manning ◽  
Alison Redington ◽  
Simon O'Doherty ◽  
Dickon Young ◽  
Dan Say ◽  
...  

<p align="justify">Verification of the nationally reported greenhouse gas (GHG) inventories using inverse modelling and atmospheric observations is considered to be best practice by the United Nations Framework Convention on Climate Change (UNFCCC). It allows for an independent assessment of the nationally reported GHG emissions using a comprehensively different approach to the inventory methods. Significant differences in the emissions estimated using the two approaches are a means of identifying areas worthy of further investigation.</p><p align="justify"> </p><p align="justify"><span>An inversion methodology called Inversion Technique for Emission Modelling (InTEM) has been developed that uses a non-negative least squares minimisation technique to determine the emission magnitude and distribution that most accurately reproduces the observations. By estimating the underlying </span><span><em>baseline</em></span><span> time series, atmospheric concentrations where the short-term impact of regional pollution has been removed, and by modelling where the air has passed over on route to the observation stations on a regional scale, estimates of UK emissions are made. </span>In this study we use an extensive network of observations with six stations across the UK and six more in neighbouring countries<span>. InTEM uses information from a</span> Lagrangian dispersion model NAME (Numerical Atmospheric dispersion Modelling Environment), driven by three-dimensional, modelled meteorology, to understand how the air mixes during transport from the emission sources to observation points. <span>The InTEM inversion results are submitted annually by the UK as part of their National Inventory Report to the UNFCCC. They are used within the UK inventory team to highlight areas for investigation and have led to significant improvements to the submitted UK inventory. The latest UK comparisons will be shown along with examples of how the inversion results have informed the inventory.</span></p>


2021 ◽  
Vol ahead-of-print (ahead-of-print) ◽  
Author(s):  
BinBin Zhang ◽  
Fumin Zhang ◽  
Xinghua Qu

Purpose Laser-based measurement techniques offer various advantages over conventional measurement techniques, such as no-destructive, no-contact, fast and long measuring distance. In cooperative laser ranging systems, it’s crucial to extract center coordinates of retroreflectors to accomplish automatic measurement. To solve this problem, this paper aims to propose a novel method. Design/methodology/approach We propose a method using Mask RCNN (Region Convolutional Neural Network), with ResNet101 (Residual Network 101) and FPN (Feature Pyramid Network) as the backbone, to localize retroreflectors, realizing automatic recognition in different backgrounds. Compared with two other deep learning algorithms, experiments show that the recognition rate of Mask RCNN is better especially for small-scale targets. Based on this, an ellipse detection algorithm is introduced to obtain the ellipses of retroreflectors from recognized target areas. The center coordinates of retroreflectors in the camera coordinate system are obtained by using a mathematics method. Findings To verify the accuracy of this method, an experiment was carried out: the distance between two retroreflectors with a known distance of 1,000.109 mm was measured, with 2.596 mm root-mean-squar error, meeting the requirements of the coarse location of retroreflectors. Research limitations/implications The research limitations/implications are as follows: (i) As the data set only has 200 pictures, although we have used some data augmentation methods such as rotating, mirroring and cropping, there is still room for improvement in the generalization ability of detection. (ii) The ellipse detection algorithm needs to work in relatively dark conditions, as the retroreflector is made of stainless steel, which easily reflects light. Originality/value The originality/value of the article lies in being able to obtain center coordinates of multiple retroreflectors automatically even in a cluttered background; being able to recognize retroreflectors with different sizes, especially for small targets; meeting the recognition requirement of multiple targets in a large field of view and obtaining 3 D centers of targets by monocular model-based vision.


2010 ◽  
Author(s):  
Mohamed Amin Anwar ◽  
Said Zaki ◽  
Dan Amin Johnson ◽  
Alfredo Mendez ◽  
Robert Kuchinski ◽  
...  

Author(s):  
James G. Droppo ◽  
Bruce A. Napier ◽  
Jeremy P. Rishel ◽  
Richard W. Bloom

The current cleanup of structures related to cold-war production of nuclear materials includes the need to demolish a number of highly alpha-contaminated structures. The process of planning for the demolition of such structures includes unique challenges related to ensuring the protection of both workers and the public. Pre-demolition modeling analyses were conducted to evaluate potential exposures resulting from the proposed demolition of a number of these structures. Estimated emission rates of transuranic materials during demolition are used as input to an air-dispersion model. The climatological frequencies of occurrence of peak air and surface exposures at locations of interest are estimated based on years of hourly meteorological records. The modeling results indicate that downwind deposition is the main operational limitation for demolition of a highly alpha-contaminated building. The pre-demolition modeling directed the need for better contamination characterization and/or different demolition methods—and in the end, provided a basis for proceeding with the planned demolition activities. Post-demolition modeling was also conducted for several contaminated structures, based on the actual demolition schedule and conditions. Comparisons of modeled and monitoring results are shown. Recent monitoring data from the demolition of a UO3 plant shows increments in concentrations that were previously identified in the pre-demolition modeling predictions; these comparisons confirm the validity and value of the pre-demolition source-term and air dispersion computations for planning demolition activities for other buildings with high levels of radioactive contamination.


2017 ◽  
Vol 54 (5) ◽  
pp. 655-669 ◽  
Author(s):  
MARIKO INGOLD ◽  
SASKIA SCHMIDT ◽  
HERBERT DIETZ ◽  
RAINER GEORG JOERGENSEN ◽  
EVA SCHLECHT ◽  
...  

SUMMARYQuality of animal manure as a nutrient source for crops and as a soil conditioner depends on how fast the organic matter is decomposed, releasing plant nutrients or building up the soil organic matter (SOM) pool. This turnover process is governed by manure composition, soil temperature, soil moisture and secondary metabolites in the manure such as tannins. To investigate the turnover and nutrient release from tannin-containing manure, a litterbag experiment was conducted in an irrigated lowland soil of northern Oman. A standardized quebracho tannin extract (QT) was either added to the goats’ diet and defecated with manure (QTf), or added to manure in a QT water suspension (QTc) prior to field application. Litterbags were installed within a two-year field experiment at 10-cm depth at the beginning of a consecutive sweet corn and radish cultivation, followed by their recovery every 2-–6 weeks until crop harvests. The litterbags contained pure goat manure (control) and the two types of QT-amended goat manure. Generally, QT increased OM remaining in litterbags at sampling by up to 22% compared with the control. QT reduced relative C, N, P and K release by 10% to 63% compared with the control, but effects were contradictory under sweet corn and radish. While under radish, both QT treatments reduced or tended to reduce C, N, P and K release from manure, QTc even increased N and P release under sweet corn. QTf, on the other hand, did not affect C, P and K release under sweet corn, whereas N release was reduced by 36–63% under both crops. As quebracho tannins in goat manure slowed down organic matter decomposition and reduced nutrient release, they may be useful agents in manure application to increase SOM pools and soil nutrient pools. However, the immobilization particularly of N by tannins can reduce the availability of this nutrient to crops.


2010 ◽  
Vol 49 (2) ◽  
pp. 221-233 ◽  
Author(s):  
M. Sofiev ◽  
E. Genikhovich ◽  
P. Keronen ◽  
T. Vesala

Abstract The problem of providing dispersion models with meteorological information from general atmospheric models used, for example, for weather forecasting is considered. As part of a generalized meteorological-to-dispersion model interface, a noniterative scheme diagnosing the surface layer characteristics from wind, temperature, and humidity profiles was developed. The scheme verification included long-term comparison with data of meteorological masts at Cabauw, the Netherlands, and Hyytiälä, Finland. The algorithm compatibility and consistency with the High-Resolution Limited-Area Model (HIRLAM) was also checked, as this model is routinely used as a meteorological driver for the Air Quality and Emergency Modeling System (SILAM). The comparison with Cabauw mast data showed a good quantitative agreement between observed and diagnosed heat and momentum fluxes: the temporal correlation coefficient was ∼0.8, bias was less than 10% of the absolute flux levels, regression slope deviated from unity for less than 20% with the intercept being less than 10% of the absolute flux values, and so on. In the case of complex surface features (Hyytiälä mast in forest) the scheme proved to be robust with large deviations appearing only if the input profile data were taken outside the constant-flux layer. Comparison with the HIRLAM model showed qualitatively good agreement but also highlighted several differences between the goals, standards, and methodologies of meteorological and dispersion models. The scheme was implemented in SILAM, which served as the development platform.


2021 ◽  
Vol 14 (9) ◽  
pp. 5987-6003
Author(s):  
Pramod Kumar ◽  
Grégoire Broquet ◽  
Camille Yver-Kwok ◽  
Olivier Laurent ◽  
Susan Gichuki ◽  
...  

Abstract. We present a local-scale atmospheric inversion framework to estimate the location and rate of methane (CH4) and carbon dioxide (CO2) releases from point sources. It relies on mobile near-ground atmospheric CH4 and CO2 mole fraction measurements across the corresponding atmospheric plumes downwind of these sources, on high-frequency meteorological measurements, and on a Gaussian plume dispersion model. The framework exploits the scatter of the positions of the individual plume cross sections, the integrals of the gas mole fractions above the background within these plume cross sections, and the variations of these integrals from one cross section to the other to infer the position and rate of the releases. It has been developed and applied to provide estimates of brief controlled CH4 and CO2 point source releases during a 1-week campaign in October 2018 at the TOTAL experimental platform TADI in Lacq, France. These releases typically lasted 4 to 8 min and covered a wide range of rates (0.3 to 200 g CH4/s and 0.2 to 150 g CO2/s) to test the capability of atmospheric monitoring systems to react fast to emergency situations in industrial facilities. It also allowed testing of their capability to provide precise emission estimates for the application of climate change mitigation strategies. However, the low and highly varying wind conditions during the releases added difficulties to the challenge of characterizing the atmospheric transport over the very short duration of the releases. We present our series of CH4 and CO2 mole fraction measurements using instruments on board a car that drove along roads ∼50 to 150 m downwind of the 40 m × 60 m area for controlled releases along with the estimates of the release locations and rates. The comparisons of these results to the actual position and rate of the controlled releases indicate ∼10 %–40 % average errors (depending on the inversion configuration or on the series of tests) in the estimates of the release rates and ∼30–40 m errors in the estimates of the release locations. These results are shown to be promising, especially since better results could be expected for longer releases and under meteorological conditions more favorable to local-scale dispersion modeling. However, the analysis also highlights the need for methodological improvements to increase the skill for estimating the source locations.


2020 ◽  
Author(s):  
Pramod Kumar ◽  
Grégoire Broquet ◽  
Camille Yver-Kwok ◽  
Olivier Laurent ◽  
Susan Gichuki ◽  
...  

Abstract. We present a local-scale atmospheric inversion framework to estimate the location and rate of methane (CH4) and carbon dioxide (CO2) releases from point sources. It relies on mobile near-ground atmospheric CH4 and CO2 mole fraction measurements across the corresponding atmospheric plumes downwind the sources, on high-frequency meteorological measurements, and a Gaussian plume dispersion model. It exploits the spread of the positions of individual plume cross-sections and the integrals of the gas mole fractions above the background within these plume cross-sections to infer the position and rate of the releases. It has been developed and applied to provide estimates of brief controlled CH4 and CO2 point source releases during a one-week campaign in October 2018 at the TOTAL's experimental platform TADI in Lacq, France. These releases lasted typically 4 to 8 minutes and covered a wide range of rates (0.3 to 200 gCH4/s and 0.2 to 150 gCO2/s) to test the capability of atmospheric monitoring systems to react fast to emergency situations in industrial facilities. It also allowed testing their capability to provide precise emission estimates for the application of climate change mitigation strategies. However, the low and highly varying wind conditions during the releases added difficulties to the challenge of characterizing the atmospheric transport over the very short duration of the releases. We present our series of measurements of CH4 and CO2 mole fractions using instruments onboard a car that drives along the roads ~50 to 150 m downwind the 40 m × 60 m area of controlled releases for each of the releases and the results from the inversions of the release locations and rates. The comparisons of these results to the actual position and rate of the controlled release indicate a 20 %–30 % average error on the release rates and a ~30–40 m errors in the estimates of the release locations. These results are shown to be promising especially since better results could be expected for longer releases and under meteorological conditions more favorable to local scale dispersion modeling.


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